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Special Issue: Functional Polymer Materials

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Chinese Journal of Polymer Science 2024年第7期42卷 895-896,I0004页

作者： Gu, Jun-Wei Wang, Du-Jin Shaanxi Key laboratory of Macromolecular Science and Technology School of Chemistry and Chemical Engineering Northwestern Polytechnical University Xi’an China beijing national laboratory for molecular sciences CAS Key Laboratory of Engineering Plastics Institute of Chemistry Chinese Academy of Sciences Beijing China

The rapid development of science has led to a significant role for polymer materials in multitude fields,including industry,medicine,energy,and the environment,*** a leading academic journal in the field of polymer,Chinese Journal of Polymer Science has been dedicated to fostering the advancement and utilization of polymer science.

关键词： polymer Polymer Functional

Deep learning-based optical aberration estimation enables offline digital adaptive optics and super-resolution imaging

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Photonics Research 2024年第3期12卷 474-484页

作者： CHANG QIAO HAOYU CHEN RUN WANG TAO JIANG YUWANG WANG DONG LI Department of Automation Tsinghua UniversityBeijing 100084China Institute for Brain and Cognitive sciences Tsinghua UniversityBeijing 100084China national laboratory of Biomacromolecules New Cornerstone Science LaboratoryCAS Center for Excellence in BiomacromoleculesInstitute of BiophysicsChinese Academy of SciencesBeijing 100101China College of Life sciences University of Chinese Academy of SciencesBeijing 100049China beijing national Research Center for Information Science and Technology Tsinghua UniversityBeijing 100084China

Optical aberrations degrade the performance of fluorescence *** adaptive optics(AO)leverages specific devices,such as the Shack–Hartmann wavefront sensor and deformable mirror,to measure and correct optical ***,conventional AO requires either additional hardware or a more complicated imaging procedure,resulting in higher cost or a lower acquisition *** this study,we proposed a novel space-frequency encoding network(SFE-Net)that can directly estimate the aberrated point spread functions(PSFs)from biological images,enabling fast optical aberration estimation with high accuracy without engaging extra optics and image *** showed that with the estimated PSFs,the optical aberration can be computationally removed by the deconvolution ***,to fully exploit the benefits of SFE-Net,we incorporated the estimated PSF with neural network architecture design to devise an aberration-aware deeplearning super-resolution model,dubbed *** demonstrated that the combination of SFE-Net and SFT-DFCAN enables instant digital AO and optical aberration-aware super-resolution reconstruction for live-cell imaging.

关键词： optics resolution enable

Tailoring-compensated ferrimagnetic state and anomalous Hall effect in quaternary Mn–Ru–V–Ga Heusler compounds

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Chinese Physics B 2024年第7期33卷 595-603页

作者：梁瑾静郗学奎王文洪刘永昌 beijing national laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China University of Chinese Academy of sciences Beijing 100049China Tiangong University Tianjin 300387China

Cubic Mn_(2)Ru_(x)Ga Heusler compound is a typical example of compensated ferrimagnet with attractive potential for high-density,ultrafast,and low-power spintronic *** the form of epitaxial thin films,Mn_(2)Ru_(x)Ga exhibits high spin polarization and high tunability of compensation temperature by freely changing the Ru content x in a broad range(0.31.0).Herein Mn-Ru-Ga-based polycrystalline bulk buttons prepared by arc melting are systematically studied and it is found that in equilibrium bulk form,the cubic structure is unstable when x1.8).

关键词： compensated ferrimagnet anomalous Hall effect residual resistivity ratio

Preface:special topic on rechargeable battery technology

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Science China Chemistry 2024年第1期67卷 1-3页

作者： Yu-Guo Guo Qiang Zhang Jun Chen Li-Jun Wan CAS Key laboratory of molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of sciences Beijing 100049China beijing Key laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China Frontiers Science Center for New Organic Matter Renewable Energy Conversion and Storage Center(RECAST)Haihe Laboratory of Sustainable Chemical TransformationsKey Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China

Rechargeable batteries play a major role in the transition from fossil energy to renewable energy and are considered the key-enabling decarbonization technology for several industries,including electronics,transportat... 详细信息

关键词： battery artificial technology

Electronic transport evolution across the successive structural transitions in Ni_(50-x)Fe_xTi_(50) shape memory alloys

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Chinese Physics B 2024年第7期33卷 529-536页

作者：何萍杨金颖任秋飒王彬彬吴光恒刘恩克 beijing national laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical sciences University of Chinese Academy of SciencesBeijing 100049China School of Materials Science and Engineering University of Science and Technology of BeijingBeijing 100083China

TiNi-based shape memory alloys have been extensively investigated due to their significant applications,but a comprehensive understanding of the evolution of electronic structure and electrical transport in a system with martensitic transformations(MT) is still *** this work,we focused on the electronic transport behavior of three phases in Ni_(50-x)Fe_xTi_(50)across the MT.A phase diagram of Ni_(50-x)Fe_xTi_(50) was established based on x-ray diffraction,calorimetric,magnetic,and electrical *** reveal the driving force of MT,phonon softening was revealed using first-principles ***,the transverse and longitudinal transport behavior changed significantly across the phase transition,which can be attributed to the reconstruction of electronic *** work promotes the understanding of phase transitions and demonstrates the sensitivity of electron transport to phase transition.

关键词： martensitic transformation electronic behavior transport properties first-principles calculations

Absence of BCS–BEC crossover in FeSe0.45Te0.55 superconductor

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Chinese Physics B 2024年第7期33卷 89-96页

作者：贾俊杰谷亚东殷超辉束英杰陈逸雯史聚民张杏陈浩苗泰民任晓琳梁波朱文培蔡能张丰丰张申金杨峰王志敏彭钦军许祖彦毛寒青刘国东任治安赵林周兴江 national laboratory for Superconductivity Beijing National Laboratory for Condensed Matter PhysicsInstitute of Physics Chinese Academy of Sciences University of Chinese Academy of sciences Technical Institute of Physics and Chemistry Chinese Academy of Sciences Songshan Lake Materials laboratory

In iron-based superconductor Fe（Se,Te）, a flat band-like feature near the Fermi level was observed around the Brillouin zone center in the superconducting state. It is under debate whether this is the evidence on the presence of the BCS–BEC[Bardeen–Cooper–Schrieffer（BCS）, Bose–Einstein condensation（BEC）] crossover in the superconductor. High-resolution laser-based angle-resolved photoemission measurements are carried out on high quality single crystals of FeSe0.45Te0.55superconductor to address the issue. By employing different polarization geometries, we have resolved and isolated the dyz band and the topological surface band, making it possible to study their superconducting behaviors separately. The dyz band alone does not form a flat band-like feature in the superconducting state and the measured dispersion can be well described by the BCS picture. We find that the flat band-like feature is formed from the combination of the dyz band and the topological surface state band in the superconducting state. These results reveal the origin of the flat band-like feature and rule out the presence of BCS-BEC crossover in Fe（Se,Te） superconductor.

关键词： ARPES BCS-BEC crossover electronic structure FeSe0.45Te0.55 superconducting gap

Four Late-type Galaxies with Double Radio Lobes and Properties of Such Galaxies

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Research in Astronomy and Astrophysics 2024年第4期24卷 84-90页

作者： Z.S.Yuan X.Y.Gao Z.L.Wen J.L.Han national Astronomical Observatories Chinese Academy of SciencesBeijing 100101China CAS Key laboratory of FAST National Astronomical ObservatoriesChinese Academy of SciencesBeijing 100101China School of Astronomy and Space sciences University of Chinese Academy of SciencesBeijing 100049China

The triggering mechanism for radio lobes from late-type galaxies is not fully *** samples are desired for a thorough investigation and *** utilizing the optical data from the newly released Dark Energy Spectroscopic Instrument imaging surveys and the radio sources from the NRAO VLA Sky Survey and the Faint Images of the Radio Sky at Twenty-centimeter,we identify four Late-type Galaxies with double Radio Lobes(La GRLs):J0217-3645,J0947+6220,J1412+3723 and J1736+*** previously known La GRLs,we confirm the correlation between radio power P_(1.4GHz)and stellar mass M_(*)of host ***(25/35)La GRLs belong to the blue cloud galaxies,while the newly identified cases in this work are located within the region of the red *** find a clear correlation between the differential radio power,i.e.,the offset from the P_(1.4GHz)-M_(*)relation,and the galaxy color,indicating that bluer galaxies at a fixed M_(*)tend to host more powerful radio ***,the majority(31/36)of La GRLs are either located in a galaxy group or displaying a disturbed *** suggest that all of the galaxy mass,color and surrounding environment could play important roles in triggering radio lobes in late-type galaxies.

关键词： galaxies:active galaxies:jets galaxies:spiral radio continuum:galaxies

Cationic ordering transition in oxygen-redox layered oxide cathodes

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Carbon Energy 2024年第1期6卷 197-206页

作者： Xinyan Li Ang Gao Qinghua Zhang Hao Yu Pengxiang Ji Dongdong Xiao Xuefeng Wang Dong Su Xiaohui Rong Xiqian Yu Hong Li Yong-Sheng Hu Lin Gu beijing national laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijingChina College of Materials Science and Opto-Electronic Technology University of Chinese Academy of SciencesBeijingChina beijing national Center for Electron Microscopy and laboratory of Advanced Materials School of Materials Science and EngineeringTsinghua UniversityBeijingChina beijing Advanced Innovation Center for Materials Genome Engineering Huairou DivisionInstitute of PhysicsChinese Academy of SciencesBeijingChina

Understanding the structural origin of the competition between oxygen 2p and transition-metal 3d orbitals in oxygen-redox(OR)layered oxides is eminently desirable for exploring reversible and high-energy-density Li/Na-ion ***,we reveal the correlation between cationic ordering transition and OR degradation in ribbon-ordered P3-Na_(0.6)Li_(0.2)Mn_(0.8)O_(2) via in situ structural *** two different voltage windows,the OR capacity can be improved approximately twofold when suppressing the in-plane cationic ordering *** find that the intralayer cationic migration is promoted by electrochemical reduction from Mn^(4+)to Jahn–Teller Mn^(3+)and the concomitant NaO_(6) stacking transformation from triangular prisms to octahedra,resulting in the loss of ribbon ordering and electrochemical ***-principles calculations reveal that Mn^(4+)/Mn^(3+)charge ordering and alignment of the degenerate eg orbital induce lattice-level collective Jahn–Teller distortion,which favors intralayer Mn-ion migration and thereby accelerates OR *** findings unravel the relationship between in-plane cationic ordering and OR reversibility and highlight the importance of superstructure protection for the rational design of reversible OR-active layered oxide cathodes.

关键词： cationic ordering layered oxide cathodes oxygen redox sodium-ion batteries

Databases of 2D material-substrate interfaces and 2D charged building blocks

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Chinese Physics B 2024年第2期33卷 34-38页

作者：邓俊潘金波杜世萱 beijing national laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physics University of Chinese Academy of SciencesBeijing 100049China Songshan Lake Materials laboratory Dongguan 523808China

Discovery of materials using“bottom-up”or“top-down”approach is of great interest in materials *** materials consisting of two-dimensional(2D)building blocks provide a good platform to explore new materials in this *** van der Waals(vdW)layered materials,these building blocks are charge neutral and can be isolated from their bulk phase(top-down),but usually grow on *** ionic layered materials,they are charged and usually cannot exist independently but can serve as motifs to construct new materials(bottom-up).In this paper,we introduce our recently constructed databases for 2D material-substrate interface(2DMSI),and 2D charged building *** 2DMSI database,we systematically build a workflow to predict appropriate substrates and their geometries at substrates,and construct the 2DMSI *** the 2D charged building block database,1208 entries from bulk material database are *** of crystal structure,valence state,source,dimension and so on is provided for each entry with a json *** also show its application in designing and searching for new functional layered *** 2DMSI database,building block database,and designed layered materials are available in Science Data Bank at https://***/10.57760/sciencedb.j00113.00188.

关键词： 2D material-substrate interfaces charged building block database functional-oriented materials design layered materials density functional theory