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A critical review on nickel-based cathodes in rechargeable batteries

International Journal of Minerals,Metallurgy and Materials 2022年第5期29卷 925-941页

作者： Lifan Wang Jingyue Wang Leiying Wang Mingjun Zhang Rui Wang Chun Zhan State Key Laboratory of Advanced Metallurgy School of Metallurgical and Ecological EngineeringUniversity of Science and Technology BeijingBeijing 100083China

The 3d transition-metal nickel(Ni)-based cathodes have long been widely used in rechargeable batteries for over 100 years,from Ni-based alkaline rechargeable batteries,such as nickel-cadmium(Ni-Cd)and nickel-metal hydride(Ni-MH)batteries,to the Ni-rich cathode featured in lithium-ion batteries(LIBs).Ni-based alkaline batteries were first invented in the 1900s,and the well-developed Ni-MH batteries were used on a large scale in Toyota Prius vehicles in the *** the same time,however,Sony Corporation commercialized the first LIBs in *** temporally fading as LiCoO_(2) dominated the cathode in LIBs,nickel oxide-based cathodes eventually found their way back to the mainstreaming battery *** uniqueness of Ni in batteries is that it helps to deliver high energy density and great storage capacity at a low *** review mainly provides a comprehensive overview of the key role of Ni-based cathodes in rechargeable *** presenting the physical and chemical properties of the 3d transition-metal Ni,which make it an optimal cationic redox center in the cathode of batteries,we introduce the structure,reaction mechanism,and modification of nickel hydroxide electrode in Ni-Cd and Ni-MH rechargeable *** then move on to the Ni-based layered oxide cathode in LIBs,with a focus on the structure,issues,and challenges of layered oxides,LiNiO_(2),and LiNi_(1−x−y)Co_(x)Mn_(y)O_(2).The role of Ni in the electrochemical performance and thermal stability of the Ni-rich cathode is *** bridging the“old”Ni-based batteries and the“modern”Ni-rich cathode in the LIBs,this review is committed to providing insights into the Ni-based electrochemistry and material design,which have been under research and development for over 100 *** overview would shed new light on the development of advanced Ni-containing batteries with high energy density and long cycle life.

关键词： nickel-based alkaline batteries nickel hydroxide electrodes lithium-ion battery Ni-rich layered oxide cathodes

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