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Recent progress in electrolyte design for advanced lithium metal batteries

SmartMat 2023年第5期4卷 1-29页

作者： Mingnan Li Caoyu Wang Kenneth Davey Jingxi Li Guanjie Li Shilin Zhang Jianfeng Mao Zaiping Guo School of Chemical Engineering&Advanced Materials The University of AdelaideAdelaideAustralia

Lithium metal batteries(LMBs)have attracted considerable interest for use in electric vehicles and as next-generation energy storage devices because of their high energy ***,a significant practical drawback with LMBs is the instability of the Li metal/electrolyte interface,with concurrent parasitic reactions and dendrite growth,that leads to low Coulombic efficiency and poor cycle *** to the significant role of electrolytes in batteries,rationally designed electrolytes can improve the electrochemical performance of LMBs and possibly achieve fast charge and a wide range of working temperatures to meet various requirements of the market in the *** there are some review papers about electrolytes for LMBs,the focus has been on a single parameter or single performance separately and,therefore,not sufficient for the design of electrolytes for advanced LMBs for a wide range of working *** review presents a systematic summary of recent progress made in terms of electrolytes,covering the fundamental understanding of the mechanism,scientific challenges,and strategies to address drawbacks of electrolytes for high-performance *** advantages and disadvantages of various electrolyte strategies are also analyzed,yielding suggestions for optimum properties of electrolytes for advanced LMBs ***,the most promising research directions for electrolytes are discussed briefly.

关键词： anion-derived SEI fast charge liquid electrolyte design lithium metal batteries safe electrolytes wide working temperature

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