Recent progress in electrolyte design for advanced lithium metal batteries
作者机构：School of Chemical Engineering&Advanced MaterialsThe University of AdelaideAdelaideAustralia
出 版 物：《SmartMat》 (智能材料（英文）)
年 卷 期：2023年第4卷第5期
页 面：1-29页
核心收录：
基 金：Financial support provided by the Australian Research Council(ARC)(Nos.FL210100050,LP160101629,and DP210101486)is gratefully acknowledged Mingnan Li acknowledges the Chinese Sponsorship Council for scholarship support(No.202106130006)
主 题：anion-derived SEI fast charge liquid electrolyte design lithium metal batteries safe electrolytes wide working temperature
摘 要：Lithium metal batteries(LMBs)have attracted considerable interest for use in electric vehicles and as next-generation energy storage devices because of their high energy ***,a significant practical drawback with LMBs is the instability of the Li metal/electrolyte interface,with concurrent parasitic reactions and dendrite growth,that leads to low Coulombic efficiency and poor cycle *** to the significant role of electrolytes in batteries,rationally designed electrolytes can improve the electrochemical performance of LMBs and possibly achieve fast charge and a wide range of working temperatures to meet various requirements of the market in the *** there are some review papers about electrolytes for LMBs,the focus has been on a single parameter or single performance separately and,therefore,not sufficient for the design of electrolytes for advanced LMBs for a wide range of working *** review presents a systematic summary of recent progress made in terms of electrolytes,covering the fundamental understanding of the mechanism,scientific challenges,and strategies to address drawbacks of electrolytes for high-performance *** advantages and disadvantages of various electrolyte strategies are also analyzed,yielding suggestions for optimum properties of electrolytes for advanced LMBs ***,the most promising research directions for electrolytes are discussed briefly.
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