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Weathering and accumulation of trace elements in the soils of the Porali Plain, Balochistan: repercussions in agriculture

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Acta Geochimica 2024年第2期43卷 214-234页

作者： Maria Kaleem Erum Bashir Shahid Naseem Tahir Rafique Bushra Shahab Department of Geology University of KarachiKarachi 75270Pakistan Applied Chemistry Research Centre PCSIR Laboratories ComplexKarachi 75280Pakistan

This study is theﬁrst attempt to assess the nature of the soil,especially on the western side of the Porali Plain in Balochistan;a new emerging agriculture hub,using weathering and pollution indices supplemented by multi-variate analysis based on geochemical data.The outcomes of this study are expected to help farmers in soil manage-ment and selecting suitable crops for the region.Twenty-ﬁve soil samples were collected,mainly from the arable land of the Porali Plain.After drying and coning-quarter-ing,soil samples were analyzed for major and trace ele-ments using the XRF technique;sieving and hydrometric methods were employed for granulometric analysis.Esti-mated data were analyzed using Excel,SPSS,and Surfer software to calculate various indices,correlation matrix,and spatial distribution.The granulometric analysis showed that 76%of the samples belonged to loam types of soil,12%to sand type,and 8%to silt type.Weathering indices:CIA,CIW,PIA,PWI,WIP,CIX,and ICV were calculated to infer the level of alteration.These indices reﬂect mod-erate to intense weathering;supported by K_(2)O/AI_(2)O_(3),Rb/K_(2)O,Rb/Ti,and Rb/Sr ratios.Assessment of the geo-ac-cumulation and Nemerow Pollution indices pinpoint rela-tively high concentrations of Pb,Ni,and Cr concentration in the soils.The correlation matrix and Principal Compo-nent Analysis show that the soil in this study area is mainly derived from the weathering of igneous rocks of Bela Ophiolite(Cretaceous age)and Jurassic sedimentary rocks of Mor Range having SEDEX/MVT type mineralization.Weathering may result in the undesirable accumulation of certain trace elements which adversely affects crops.

关键词： Weathering indices Pollution indices accumulation Repercussions Trace elements Multivariate analyses Porali Plain Balochistan

accumulation of Heavy Metals in Maga-Pouss Rice Fields (Far-North Region, Cameroon) and Transfer to Rice Grains

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Agricultural Sciences 2024年第3期15卷 311-326页

作者： Diane Madomguia Gilbert Bello Basokdou Kalieu W. Appoline Isabelle Patrice Kuitekam Dongo Edouard Nya Serge Hubert Zebaze Togouet Department of Hydraulics and Water Management National Advanced School of Engineering University of Maroua Maroua Cameroon Research Center of Global Studies with Multidisciplinary Units (CREGUM) Maroua Cameroon National Laboratory of Analysis of Agricultural Inputs and Products Ministry of Agriculture and Rural Development Messa-Yaoundé Cameroon Department of Animal Physiology and Biology Faculty of Sciences University of Yaoundé I Yaoundé Cameroon

Monitoring of heavy metals contamination of agricultural products and their transfer and bioaccumulation in crops like rice has become a hot topic worldwide over the last two decades. The present study was carried out to determine the accumulation of heavy metals in rice fields and their transfer to rice grains. Soil, irrigation water and rice grains samples were gathered in Maga-Pouss, Far-North, Cameroon. Concentrations of six heavy metals (lead, cadmium, zinc, copper, iron and mercury) were evaluated by Atomic Absorption Spectrophotometer (AAS). Mercury was not detected in this study. Average concentrations of metals were in this order (in mg/kg): Fe (188.60 ± 97.06) > Pb (63.63 ± 7.11) > Cd (2.59 ± 0.29) > Zn (1.10 ± 1.05) > Cu (0.80 ± 0.73) in water and Pb (105.50 ± 31.11) > Fe (105.50 ± 31.11) > Cu (45.93 ± 14.39) > Zn (22.52 ± 6.40) > Cd (3.15 ± 0.49) in soil. Water in Maga-Pouss rice fields appears to be more harmful than the soil, notably for lead, cadmium and copper. In rice grains, heavy metals were found in this order (mg/kg): Fe (188.01 ± 82.62) > Cu (27.20 ± 0.00) > Zn (23.61 ± 12.42) > Pb (19.50 ± 19.91) > Cd (2.02 ± 1.05). The mean bioconcentration factor (BCF) of metals from soil to rice grains was in the following order: Fe (2.60) > Zn (1.05) > Cd (0.64) > Cu (0.59) > Pb (0.18). From water to rice grains, the order is: Cu (37.26) > Zn (22.49) > Cd (6.97) > Pb (2.74) > Fe (1.94). Rice field pH and electrical conductivity favored the uptake of lead, copper and cadmium by rice grains. The findings of this study will be good documentation for risk assessment, and decision-making by environmental managers in this region.

关键词： Heavy Metals Rice Field Bioconcenration Factor Maga-Pouss accumulation

accumulation, transportation, and distribution of tetracycline and cadmium in rice

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Journal of Environmental Sciences 2023年第4期126卷 58-69页

作者： Chunfeng He Jini Zhou Chen Yang Zhiyi Song Junheng He Ziqing Huang Yurong Deng Jinling Wang Yu Xiong Zhi Dang College of Environment and Energy South China University of TechnologyGuangzhou 510006China The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationGuangzhou 510006China Department of Environmental Sciences The State University of New JerseyRutgers UniversityNew BrunswickNJ 08901USA Guangdong Institute of Ecological Environment and Soil Guangzhou 510650China

Co-exposure to heavy metal and antibiotic pollution might result in complexation and synergistic interactions,affecting rice growth and further exacerbating pollutant enrichment.Therefore,our study sought to clarify the influence of different Tetracycline (TC) and Cadmium(Cd) concentration ratios (both alone and combined) on rice growth,pollutant accumulation,and transportation during the tillering stage in hydroponic system.Surprisingly,our findings indicated that the interaction between TC and Cd could alleviate the toxic effects of TC/Cd on aerial rice structures and decrease pollutant burdens during root elongation.In contrast,TC and Cd synergistically promoted the accumulation of TC/Cd in rice roots.However,their interaction increased the accumulation of TC in roots while decreasing the accumulation of Cd when the toxicant doses increased.The strong affinity of rice to Cd promoted its upward transport from the roots,whereas the toxic effects of TC reduced TC transport.Therefore,the combined toxicity of the two pollutants inhibited their upward transport.Additionally,a low concentration of TC promoted the accumulation of Cd in rice mainly in the root tip.Furthermore,a certain dose of TC promoted the upward migration of Cd from the root tip.Laser ablation-inductively coupled plasma mass spectrometry demonstrated that Cd mainly accumulated in the epidermis and stele of the root,whereas Fe mainly accumulated in the epidermis,which inhibited the absorption and accumulation of Cd by the rice roots through the generation of a Fe plaque.Our findings thus provide insights into the effects of TC and Cd co-exposure on rice growth.

关键词： Laser ablation-inductively coupled plasma mass spectrometry Tetracycline Cadmium accumulation Distribution

The risks of sulfur addition on cadmium accumulation in paddy rice under different water-management conditions

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Journal of Environmental Sciences 2022年第8期34卷 101-111页

作者： Zhe Liu Qi-qi Wang Si-yu Huang Ling-xuan Kong Zhong Zhuang Qi Wang Hua-fen Li Ya-nan Wan Beijing Key Laboratory of Farmland Soil Pollution Prevention and Remediation Key Laboratory of Plant-Soil Interactions of the Ministry of EducationCollege of Resources and Environmental SciencesChina Agricultural UniversityBeijing 100193China

Recently, the application of sulfur(S) has been recommended to control the accumulation of cadmium(Cd) in rice in contaminated paddy soil. However, the effects of exogenous S on Cd transfer in paddy rice systems under different water-management practices have not been systematically investigated. Pot experiments were performed to monitor the composition of soil pore water and the Cd accumulation in iron plaque and rice tissue were compared under different S(0 and 200 mg/kg Na_(2)SO_(4)) and water(continuous and discontinuous flooding) treatments. Sulfur application significantly increased Cd concentrations in soil pore water under discontinuous flooding conditions, but slightly reduced them under continuous flooding. Moreover, the oxidation/reduction potential(Eh) was the most critical factor that affected the Cd levels. When the Eh exceeded-42.5 mV, S became the second critical factor, and excessive S application promoted Cd dissolution. In addition, S addition elevated the Cd levels in iron plaque and reduced the Cd transfer from the iron plaque to rice roots. In rice, S addition inhibited Cd transfer from the rice roots to the straw;thus, more Cd was stored in the rice roots. Nevertheless, additional S application increased the Cd content in the rice grains by 72% under discontinuous flooding, although this effect was mitigated by continued flooding. Under simulated practical water management conditions, S addition increased the risk of Cd contamination in rice, suggesting that S application should be reconsidered as a paddy fertilization strategy.

关键词： Rice Cadmium Sulfur Water management Iron plaque accumulation

Effects of fulvic acid and humic acid from different sources on Hg methylation in soil and accumulation in rice

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Journal of Environmental Sciences 2022年第9期34卷 93-105页

作者： Shu Ran Tianrong He Xian Zhou Deliang Yin Key Laboratory of Karst Georesources and Environment(Guizhou University) Ministry of EducationGuiyang 550025China College of Resources and Environmental Engineering Guizhou UniversityGuiyang 550025China Guizhou Karst Environmental Ecosystems Observation and Research Station Ministry of EducationGuiyang 550025China

Humus is often used as an organic modifier to reduce the bioaccumulation of heavy metals in plants, but the effects of different humus components from different sources on the fate of mercury(Hg) in paddy fields are still unclear. Here, fulvic acid(FA) and humic acid(HA) extracted from composted straw(CS), composted cow dung(CCD), peat soil(PM) and lignite coal(LC) were used to understand their effects on the methylation and bioaccumulation of Hg in paddy soil by pot experiments. Amendments of both FA and HA largely increased the abundance of Hg-methylating microbes and low-molecular-weight organic matters(e.g, cysteine) in paddy soil. They were also found to change the aromaticity, molecular size and Chromophoric DOM concentration of DOM, and resulted in heterogeneous effects on migration and transformation of Hg. All the FA-amended treatments increased the mobility and methylation of Hg in soil and its absorption in roots. Nevertheless, FA from different sources have heterogeneous effects on transport of Hg between rice tissues. FA-CCD and FA-PM promoted the translocation of Me Hg from roots to rice grains by 32.95% and 41.12%, while FA-CS and FA-LC significantly inhibited the translocation of inorganic Hg(IHg) by 52.65% and 66.06% and of Me Hg by 46.65% and 36.23%, respectively. In contrast, all HA-amended treatments reduced the mobility of soil Hg, but promoted Hg methylation in soil. Among which, HA-CCD and HA-PM promoted the translocation of Me Hg in rice tissues by 88.95% and 64.10%, while its accumulation in rice grains by 28.43% and 28.69%, respectively. In general, the application of some FA and HA as organic modifiers to reduce Hg bioaccumulation in rice is not feasible.

关键词： Humic acid Fulvic acid Methylmercury accumulation Rice

Effects of Environmental Cadmium on Cadmium accumulation, Oxidative Response, and Microelements Regulation in the Liver and Kidney of Hexagrammos otakii

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Journal of Ocean University of China 2022年第2期21卷 479-485页

作者： HU Fawen SUN Ming LI Li GAO Fengxiang JIAN Yuxia WANG Xue WANG Xiaolong GUO Wen Marine Biology Institute of Shandong Province Healthy Mariculture Engineering Research Center of Shandong ProvinceQingdao 266104China

The effects of cadmium(Cd)on metal accumulation,microelements contents,and antioxidant responses in Hexagram-mos otakii were studied.The fish were exposed to 0.2,2.5,or 10μg L−1 Cd for 12 or 24 days.Then,the concentration of Cd and mi-croelements(Ca,Fe,Zn,and Se)were determined in the liver and kidney.Moreover,the activities of antioxidant enzymes including superoxide dismutase(SOD),catalase(CAT),and glutathione-S-transferase(GST),and the content of malondialdehyde(MDA)in the liver and kidney were also measured.A continuous accumulation of Cd was observed throughout the experimental period.Cd accumulation was higher in liver than that in the kidney,while Ca and Fe contents were lower in liver than those in the kidney.Cd exposure resulted in a decrease of Ca and Fe concentrations in the kidney,while there was no effect on the liver.Zn and Se remained unaffected with exposure to Cd.Cd exposure induced severe oxidative stress in H.otakii,as indicated by significant induction of the activities of SOD,CAT,and GST,and a simultaneous increase of MDA content.These data show that antioxidant enzymes and mi-croelements contents can be used as potential biomarkers to monitor environmental health in fish.

关键词： accumulation oxidative response ionoregulatory toxicity waterborne cadmium Hexagrammos otakii

accumulation of cadmium and copper by female Oxya chinensis (Orthopera: Acridoidea) in soil-plant-insect system

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Journal of Environmental Sciences 2006年第2期18卷 341-346页

作者： LI Li-jun LIU Xue-mei DUAN Yi-hao GUO Ya-ping CHENG Bin GUO Jun XI Yu-ying MA En-bo Institution of Soil Science and Fertilizer Shanxi Academy of Agriculture Sciences Taiyuan 030031 China College of Life Science and Technology Shanxi University Taiyuan 030006 China School of Environmental Science and Resources Taiyuan 030006 China

One purpose of this research is to present accumulation of cadmium （Cd） and copper （Cu） by female Oxya chinensis （Orthopera： Acridoidea） in a simulated soil-plant-insect ecosystem treated with Cd. Fourth-instar nymphs of O. chinensis had been fed on wheat （Triticurn aestivum） seedlings contaminated with Cd and Cu for one month. In the ecosystem, the Cd concentration in wheat seedlings rose greatly with the increasing of Cd in the soil, but the Cu concentration in wheat seedlings was not found elevated. There was a highly significant difference（P〈0.05） in Cd concentrations of wheat seedlings and not any significant difference（P〉0.05） in Cu concentrations of wheat seedlings. The Cd and Cu concentration in different body part-head, thorax, abdomen, and hind femur, varied under different Cd concentrations in soil. There were significant differences （P〈0.05） in the four parts of Cd and Cu accumulations with all treatments. The order of Cd accumulation was thorax 〉abdomen 〉head 〉hind femur and the Cu was abdomen 〉thorax 〉 head〉hind femur. The results indicated that Cd and Cu were accumulated from the soil to grasshoppers through the plant; that is to say, Cd and Cu in environment could be transported to animal or human via food chain.

关键词： accumulation cadmium（Cd） copper（Cu） grasshopper（Oxya chinensisi） soil-plant-insect ecosystem

accumulation over the Greenland Ice Sheet as Represented in Reanalysis Data

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Advances in Atmospheric Sciences 2011年第5期28卷 1030-1038页

作者：陈琳玲 Ola M.JOHANNESSEN 王会军 Atsumu OHMURA Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of Sciences Beijing 100029 Mohn-Sverdrup Center Nansen Environmental and Remote Sensing Center Bergen 5006 Norway Nansen Scientific Society Bergen 5006 Norway Mohn-Sverdrup Center Nansen Environmental and Remote Sensing CenterBergen 5006Norway Nansen Scientific Society Bergen 5006Norway Institute for Atmospheric and Climate Science Swiss Federal Institute of Technology(ETH)Zrich 8092Switzerland

Annual precipitation,evaporation,and calculated accumulation from reanalysis model outputs have been investigated for the Greenland Ice Sheet （GrIS）,based on the common period of 1989-2001.The ERA-40 and ERA-interim reanalysis data showed better agreement with observations than do NCEP-1 and NCEP-2 reanalyses.Further,ERA-interim showed the closest spatial distribution of accumulation to the observation.Concerning temporal variations,ERA-interim showed the best correlation with precipitation observations at five synoptic stations,and the best correlation with in situ measurements of accumulation at nine ice core sites.The mean annual precipitation averaged over the whole GrIS from ERA-interim （363 mm yr 1） and mean annual accumulation （319 mm yr 1） are very close to the observations.The validation of accumulation calculated from reanalysis data against ice-core measurements suggests that further improvements to reanalysis models are needed.

关键词： Greenland Ice Sheet reanalysis data precipitation accumulation

accumulation and Output of Heavy Metals by the Invasive Plant Spartina alterniflora in a Coastal Salt Marsh

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Pedosphere 2018年第6期28卷 884-894页

作者： CHEN Lian GAO Jianhua ZHU Qingguang WANG Yaping YANG Yang School of Geographic and Oceanographic Sciences Nanjing UniversityNanjing 210046(China) Key Laboratory of Marine Sedimentary and Environmental Geology State Oceanic AdministratzonQingdao 266061(China)

Spartina alterniflora is a foreign introduced species and has far-reaching effects on salt marsh ecosystems, particularly on the biogeochemical cycle of heavy metals. To ascertain whether the invasive plant Spartina alterniflora Loisel is a source of metals in the environment, we determined the bimonthly concentrations of heavy metals, chromium(Cr), lead(Pb), copper(Cu), zinc(Zn),and manganese(Mn), in the roots, stems, and leaves of S. alterniflora from a typical semidiurnal tidal zone in the coastal area of northern Jiangsu Province, China. Based on the measurements, we calculated annual metal primary accumulation and output. To calculate the annual output of heavy metals from S. alterniflora, a new method that calculates the annual rate of biomass loss and decomposition was developed. The annual primary accumulation of Cr, Pb, Cu, Zn, and Mn was 19.08, 84.19, 63.74, 442.58, and774.66 mg m^(-2), respectively, and the annual output from S. alterniflora to the surrounding environment was 4.01, 18.09, 14.00, 97.11,and 164.28 mg m^(-2), respectively. Spartina alterniflora only provides temporary storage, and its absorption of heavy metals could be used to remediate contaminated soil and for phytomining. The heavy metals released by S. alterniflora to the environment cannot be ignored; thus, S. alterniflora should be considered a source of metal contamination. Therefore, when we evaluate the remarkable ability of certain plant species to concentrate metals in their tissues, the balance between heavy metal accumulation and output should be considered.

关键词： biomass contaminated soil decomposition litter metal primary accumulation phytomining sediment temporary repository