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Spatially Bandgap-Graded Mo S2（1-x）Se2x Homojunctions for Self-Powered Visible–Near-Infrared phototransistors

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Nano-Micro Letters 2020年第2期12卷 185-198页

作者： Hao Xu Juntong Zhu Guifu Zou Wei Liu Xiao Li Caihong Li Gyeong Hee Ryu Wenshuo Xu Xiaoyu Han Zhengxiao Guo Jamie HWarner Jiang Wu Huiyun Liu Department of Electronic and Electrical Engineering University College LondonTorrington PlaceLondon WC1E 7JEUK School of Energy Soochow Institute for Energy and Materials Innovationsand Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceSoochow UniversitySuzhou 215006People’s Republic of China London Centre for Nanotechnology University College LondonLondon WC1H 0AHUK Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaChengdu 610054People’s Republic of China Department of Materials University of OxfordParks RoadOxford OX13PHUK Department of Chemistry University College London20 Gordon StBloomsburyLondon WC1H 0AJUK Department of Chemistry The University of Hong KongPokfulam RoadHong KongPeople’s Republic of China Zhejiang Institute of Research and Innovation The University of Hong KongQingshan Lake SciTech CityHangzhouPeople’s Republic of China

Ternary transition metal dichalcogenide alloys with spatially graded bandgaps are an emerging class of two-dimensional materials with unique features,which opens up new potential for device ***,visible–near-infrared and self-powered phototransistors based on spatially bandgap-graded MoS2(1−x)Se2x alloys,synthesized by a simple and controllable chemical solution deposition method,are *** graded bandgaps,arising from the spatial grading of Se composition and thickness within a single domain,are tuned from 1.83 to 1.73 eV,leading to the formation of a homojunction with a builtin electric ***,a strong and sensitive gate-modulated photovoltaic effect is demonstrated,enabling the homojunction phototransistors at zero bias to deliver a photoresponsivity of 311 mA W−1,a specific detectivity up to^10^11 Jones,and an on/off ratio up to^10^***,when illuminated by the lights ranging from 405 to 808 nm,the biased devices yield a champion photoresponsivity of 191.5 A W−1,a specific detectivity up to^1012 Jones,a photoconductive gain of 10^6–10^7,and a photoresponsive time in the order of^50 *** results provide a simple and competitive solution to the bandgap engineering of two-dimensional materials for device applications without the need for p–n junctions.

关键词： Transition metal dichalcogenides Graded bandgaps Homojunctions phototransistors Self-powered

High carrier mobility and strong fluorescence emission: Toward highly sensitive single-crystal organic phototransistors

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Aggregate 2023年第2期4卷 247-252页

作者： Jingwei Tao Zhaoyang Liu Dan Liu Huanli Dong Jiangbo Jing Jiaxing Song Leijing Liu Bin Xu Wenjing Tian State Key Laboratory of Supramolecular Structure and Materials Jilin UniversityChangchunChina State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchunChina Beijing National Laboratory for Molecular Sciences Key Laboratory of Organic SolidsInstitute of ChemistryChinese Academy of SciencesBeijingChina China–Australia Institute for Advanced Materials and Manufacturing Jiaxing UniversityJiaxingChina

Organic single crystals(OSCs)offer a unique combination of both individual and collective properties of the employed molecules,but it remains highly challenging to achieve OSCs with both high mobilities and strong fluorescence emissions for their potential applications in multifunctional ***,we demonstrate the design and synthesis of two novel triphenylamine-functionalized thienoacenes-based organic semiconductors,4,8-distriphenylamineethynylbenzo[1,2-b:4,5-b′]dithiophene(4,8-DTEBDT)and 2,6-distriphenylamineethynylbenzo[1,2-b:4,5-b′]dithiophene(2,6-DTEBDT),with high-mobility and strong fluorescence *** two compounds show the maximum mobilities up to 0.25 and 0.06 cm^(2) V^(-1) s^(-1),the photoluminescence quantum yields(PLQYs)of 51% and 45%,and the small binding energies down to 55.13 and 58.79 *** excellent electrical and optical properties ensured the application of 4,8-DTEBDT and 2,6-DTEBDT single crystals in ultrasensitive UV phototransistors,achieving high photoresponsivity of 9.60×105 and 6.43×10^(4) AW^(-1),and detectivity exceeding 5.68×10^(17) and 2.99×10^(16) Jones.

关键词： high mobility phototransistors single-crystal organic field-effect transistors strong fluorescence emission thienoacene derivatives

Theoretical modelling and experimental study of novel photothermal microactuators

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Chinese Optics Letters 2009年第8期7卷 694-698页

作者：马利红张冬仙刘超章海军 State Key Laboratory of Modern Optical Instrumentation Zhejiang University Information Optical Institute Zhejiang Normal University

We present a category of novel photothermal （PT） microactuators. Each microactuator consists of two PT arms that are jointed at the free end and connected to an anchor at the fixed end. When a laser beam irradiates one of the arms （called hot arm, and the other is cold arm）, light energy is absorbed and converted into heat. The asymmetric thermal expansion of the hot and cold arms results in lateral deflection. Based on conduction heat transfer theory and heat dissipation mechanism, we study the PT effects and establish the theoretical model of PT expansion for the microactuators. The temperature distribution and the linear thermal expansion can be numerically calculated. The analytical solution provides an insight into the operation of the actuators and predicts the performance of the actuators with new designs. A symmetry microactuator and a microswitch as the prototypes have been fabricated and tested. The experimental results are in good agreement with the theoretical predictions and prove the feasibility of the novel PT microactuators.

关键词： Heat conduction Microactuators phototransistors Thermal stress

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Organic optocouplers

Science China Chemistry 2011年第7期54卷 1017-1026页

作者： SUN QiuJian DONG GuiFang WANG LiDuo QIU Yong Key Laboratory of Organic Optoelectronics & Molecular Engineering of Ministry of Education Department of ChemistryTsinghua UniversityBeijing 100084China

Organic optocoupler(OOC) or organic photocoupler,optical coupler is a novel and one of the most promising organic optoelectronic devices for its well electrical isolation and anti-jamming ability in long-distance and real-time digital *** performance parameters of OOC were greatly raised during the past decade,and its development was strongly associated with basic organic devices such as organic light emitting diodes(OLED),organic photodiodes(OPD) and organic phototransistors(OPT) *** we describe the principles of OOC,review recent breakthroughs in this field,and summarize the photosensor and light emitting parts which could be used in the *** technical points,such as current transfer ratio,frequency,matching and stability were also discussed in this paper.

关键词： organic optocoupler organic photocoupler photodiodes phototransistors light emitting diode current transfer ratio cut-off frequency

Surface doping effect on the optoelectronic performance of 2D organic crystals based on cyano-substituted perylene diimides

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Chinese Chemical Letters 2024年第9期35卷 193-197页

作者： Jaeyong Ahn Zhenping Li Zhiwei Wang Ke Gao Huagui Zhuo Wanuk Choi Gang Chang Xiaobo Shang Joon Hak Oh School of Chemical and Biological Engineering Institute of Chemical ProcessesSeoul National UniversitySeoul 08826South Korea State Key Laboratory for Mechanical Behavior of Materials Shaanxi International Research Center for Soft MatterSchool of Materials Science and EngineeringXi’an Jiaotong UniversityXi’an 710049China Center for Ordered Nanoporous Materials Synthesis School of Environmental Science and EngineeringPohang University of Science and TechnologyGyeongbuk 37673South Korea Instrumental Analysis Center of Xi’an Jiaotong University Xi’an 710049China

Compared to organic thin films,organic single crystals offer significant potential in organic phototransistors(OPTs)due to their enhanced charge transport,large surface area,and defect-free ***,the development of n-type semiconductors has lagged behind p-type *** enhance semiconductor device performance,a doping process can be employed,which typically involves the introduction of charged impurities into the crystalline semiconducting *** aim is to reduce the Ohmic losses,increase carrier density,improve transport capabilities,and facilitate effective carrier injection,ultimately enhancing the electrical properties of the *** doping processes,however,often pose a risk of damaging the structure of single *** this study,we have synthesized novel cyanosubstituted chiral perylene diimides,which self-assemble into two-dimensional single crystals that can be used for n-type semiconductor *** have employed a surface doping strategy using diethylamine vapor without disrupting the crystal *** fabricated devices exhibit significantly higher charge transport properties after doping,achieving a maximum electron mobility of 0.14 cm^(2)V^(-1)s^(-1),representing an improvement of over ***,the optoelectronic performance of the doped devices has significantly improved,with the external quantum efficiency increased by over 9 times and the significantly improved response *** results suggest that our surface doping technology is a promising way for enhancing the performance of 2D organic single-crystal OPTs.

关键词： Doping effect phototransistors Perylene diimides Organic crystals Cyano substitution

Active pixel image sensor array for dual vision using large-area bilayer WS_(2)

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InfoMat 2024年第4期6卷 68-82页

作者： Arindam Bala Mayuri Sritharan Na Liu Muhammad Naqi Anamika Sen Gyuchull Han Hyun Yeol Rho Youngki Yoon Sunkook Kim School of Advanced Materials Science and Engineering Sungkyunkwan UniversitySuwonRepublic of Korea Waterloo Institute for Nanotechnology(WIN) University of WaterlooWaterlooOntarioCanada Department of Electrical and Computer Engineering University of WaterlooWaterlooOntarioCanada

Transition metal dichalcogenides(TMDs)are a promising candidate for developing advanced sensors,particularly for day and night vision systems in vehicles,drones,and security *** traditional systems rely on separate sensors for different lighting conditions,TMDs can absorb light across a broad-spectrum *** this study,a dual vision active pixel image sensor array based on bilayer WS2 phototransistors was *** bilayer WS2 film was synthesized using a combined process of radio-frequency sputtering and chemical vapor *** WS2-based thin-film transistors(TFTs)exhibit high average mobility,excellent Ion/Ioff,and uniform electrical *** optoelectronic properties of the TFTs array exhibited consistent behavior and can detect visible to near-infrared light with the highest responsivity of 1821 A W1(at a wavelength of 405 nm)owing to the photogating ***,red,green,blue,and near-infrared image sensing capabilities of active pixel image sensor array utilizing light stencil projection were *** proposed image sensor array utilizing WS2 phototransistors has the potential to revolutionize the field of vision sensing,which could lead to a range of new opportunities in various applications,including night vision,pedestrian detection,various surveillance,and security systems.

关键词： dual vision image sensors infrared wavelength detection phototransistors thin-film transistor arrays transition metal dichalcogenides