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Recent advances in highly integrated energy conversion and storage system

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SusMat 2022年第2期2卷 142-160页

作者： Changxiang Shao Yang Zhao Liangti Qu School of Chemistry and Pharmaceutical Engineering Shandong First Medical University&Shandong Academy of Medical SciencesTaianShandongP.-R.China Key Laboratory of Photoelectronic/Electrophotonic conversion Materials Key Laboratory of Cluster ScienceMinistry of Education of ChinaSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijingP.R.China Key Lab of Organic Optoelectronics and Molecular Engineering of Ministry of Education Department of ChemistryTsinghua UniversityBeijingP.R.China

The vigorous development in the field of energy conversion and storage devices directly contributes to the full utilization and convenient use of clean energy.However,some drawbacks of independent energy conversion and storage devices,including unstable,insufficient energy output and dependence on external power supply,are difficult to overcome by self-optimization,thus,hindering their further development and direct application.Coincidentally,the combination of above two devices can solve these problems,which conforms to their intrinsic needs for development.At the same time,the pursuit of portability and miniaturization also promotes the development of the power system toward a highly integrated direction.Therefore,we introduce several integration modes of energy conversion and storage systems,with emphasis on all-in-one power system,possessing the highest integration in this review.From the aspect of device configuration,working mechanisms and their performances,the all-inone power systems based on different energy sources(e.g.,mechanical,solar,thermal,and chemical energy)are discussed and analyzed.Finally,the design strategies are summarized and the potential development directions in the future are proposed.This review aims to provide a comprehensive overview of highly integrated energy conversion and storage system,and seeks to point out the opportunities and orientations of future research in this field.

关键词： all-in-one energy conversion energy storage high integration power system

The energy conversion rates from eddies and mean fl ow into internal lee waves in the global ocean

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Journal of Oceanology and Limnology 2022年第4期40卷 1304-1313页

作者： Bing HAN Laboratory for Coastal Ocean Variation and Disaster Prediction College of Ocean and MeteorologyGuangdong Ocean UniversityZhanjiang 524088China State Key Laboratory of Tropical Oceanography South China Sea Institute of OceanologyChinese Academy of SciencesGuangzhou 510301China Institut für Meereskunde Universität HamburgHamburg 20146Germany Key Laboratory of Climate Resources and Environment in Continental Shelf Sea and Deep Sea of Department of Education of Guangdong ProvinceGuangdong Ocean UniversityZhanjiang 524088China

Internal lee waves play an important role in transferring energy from eddies to small scale mixing.However,the energy conversion from eddies into lee waves in the global ocean remains poorly understood.conversion rates from eddies and from mean fl ow in the global ocean were diff erentiated using single beam sounding data,stratifi cation from climatology,eddy velocity,and mean fl ow from a global ocean model.The global integral energy conversion from eddies is estimated to be 0.083 TW and is almost twice as that from the mean fl ow.A new method was developed to study the uncertainties of energy conversion caused by dealing with the topographic data.Results show that diff erent data processing procedures,and the resolution and accuracy of topographic data have a signifi cant impact on the estimated global energy conversion.

关键词： internal lee waves eddies mean flow energy conversion topography

Tree Ring‑Inspired Fibrous Helix for UV Shielding and Warning Based on Photo‑electricity‑Acoustic energy conversion

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Advanced Fiber Materials 2023年第2期5卷 681-693页

作者： Yan Wang Ziyi Guo Jie Xiong Jingchong Liu Yong Zhao Fengyun Guo Key Laboratory of Intelligent Textile and Flexible Interconnection of Zhejiang Province School of Textile Science and Engineering(International Silk Institute)Zhejiang Sci-Tech UniversityHangzhou 310018China Key Laboratory of Bioinspired Intelligent Interface Science and Technology Ministry of Education School of Chemistry Beihang UniversityBeijing 100191China Beijing Key Laboratory for Bioengineering and Sensing Technology Daxing Research InstituteSchool of Chemistry and Biological EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Flexible wearable ultraviolet(UV)shielding,monitoring and warning devices have important applications in civil and mili-tary fields.However,most flexible wearable UV devices show unsatisfactory performance due to their poor stability and easy failure at large strains.Herein,inspired by tree rings,we engineered a hierarchical composite nanofibrous helix with an alternately stacked Archimedes spiral structure via a cost-effective strategy.Based on a photo-electricity-acoustic energy conversion system,we fabricated an all-in-one device exhibiting strain-insensitive UV protection at 0–500%strain for UV shielding as well as strain-sensitive UV monitoring at 500–1500%strain for UV early warning.Compared with previously reported common nanofibrous membrane devices,the as-prepared composite nanofibrous helix shows great advantages in terms of stability and UV protection,especially at large strains.Furthermore,the helix demonstrates multiple functions of wear resistance,antibacterial properties,biodegradation and knittability.This versatile strategy holds great promise for wearable electronics and multifunctional devices.

关键词： Electrospinning Nanofibrous helix energy conversion UV shielding and warning Multifunction Flexible electronics

Revitalizing osmium-based catalysts for energy conversion

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energy Reviews 2023年第4期2卷 81-88页

作者： Ding Chen Shichun Mu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070China

Designing high cost-effective catalysts has been one of the core topics in energy conversion and storage.Due to unique electronic structure and excellent comprehensive properties,Pt-group metal(PGM)based-materials occupy the top region of numerous volcanic curves and are currently difficult to be replaced by abundant tran-sition metal catalysts.Herein,we pay attention to the osmium(Os),as the cheapest and the least noticed PGM in the field of electrocatalysis,with promising application prospects.Specifically,the three main modification strategies(anion modulation,heterostructure construction,substrate engineering)of Os-based catalysts in hydrogen evolution reaction(HER),the structural advantages provided in oxygen evolution reaction(OER),and other energy-related electrocatalysis applications are discussed one by one.In addition,we discuss the key problems and countermeasures faced in their further breakthroughs,and look forward to future development trends and prospects.Undoubtedly,the insights in this work will promote the understanding and designation of Os-based catalysts.

关键词： energy conversion Electrocatalysis Pt-group metals Os-based catalysts

energy conversion and deposition behaviour in gravitational collapse of granular columns

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Journal of Mountain Science 2020年第1期17卷 216-229页

作者： HUANG Bo-lin WANG Jian ZHANG Quan LUO Chao-lin CHEN Xiao-ting Hubei Key Laboratory of Disaster Prevention and Mitigation China Three Gorges UniversityYichang 443002China National Observatory of the Three Gorges Landslide Yangtze RiverHubei ProvinceChina Three Gorges UniversityYichang 443002China Pearl River Water Resources Research Institute Pearl River Water Resources Research InstituteGuangzhou 510611China

The high-density gravitational collapse of granular columns is very similar to the movements of large collapsing columns in nature. Based on the development of dangerous columnar rock mass in fields, granular column collapse boundary condition in the physical experiments of this study is a new type of boundary conditions with a single free face and a three-dimensional deposit. Physical experiments have shown that the mobility of small particles during the collapse of granular columns was greater than that of large particles. For example, when particle size was increased from 5 to 15 mm, deposit runout was decreased by about 16.4%. When a column consisted of two particle types with different sizes, these particles could mix in the vicinity of layer interfaces and small particles might increase the mobility of large particles. In the process of collapse, potential and kinetic energy conversion rate is fluctuated. By increasing initial aspect ratio a, the ratio of the initial height of column to its length along flow direction,potential and kinetic energy conversion rate is decreased. For example, as a was increased from 0.5 to 4, the ratio of maximum kinetic energy obtained and total potential energy loss was decreased from47.6% to 7.4%. After movement stopped, an almost trapezoidal body remained in the column and a fanlike or fan-shaped accumulation was formed on the periphery of column. Using multiple exponential functions of the aspect ratio a, the planar morphology of the collapse deposit of granular columns could be quantitatively characterized. The movement of pillar dangerous rock masses with collapse failure mode could be evaluated using this granular column experimental results.

关键词： Granular columns Rock collapse Collapse experiments energy conversion Deposit sequence Deposit prediction

Current and further trajectories in designing functional materials for solid oxide electrochemical cells:A review of other reviews

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Journal of energy Chemistry 2024年第7期94卷 302-331页

作者： Stanislav Baratov Elena Filonova Anastasiya Ivanova Muhammad Bilal Hanif Muneeb Irshad Muhammad Zubair Khan Martin Motola Sajid Rauf Dmitry Medvedev Hydrogen energy Laboratory Ural Federal University620002 EkaterinburgRussia Institute of Natural Sciences and Mathematics Ural Federal University620002 EkaterinburgRussia Department of Inorganic Chemistry Faculty of Natural SciencesComenius University BratislavaIlkovicova 6Mlynska Dolina84215 BratislavaSlovakia State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and EngineeringXi'an Jiaotong UniversityXi'an 710049ShaanxiChina Department of Physics University of Engineering and TechnologyLahore 54890Pakistan Pak-Austria Fachhochschule:Institute of Applied Sciences and Technology Mang Haripur 22621Khyber PakhtunkhwaPakistan College of Mechatronics and Control Engineering Shenzhen UniversityShenzhen 518000GuangdongChina Laboratory of Electrochemical Devices Based on Solid Oxide Proton Electrolytes Institute of High Temperature Electrochemistry620066 EkaterinburgRussia

Complex oxides are an important class of materials with enormous potential for electrochemical appli-cations.Depending on their composition and structure,such complex oxides can exhibit either a single conductivity(oxygen-ionic or protonic,or n-type,or p-type electronic)or a combination thereof gener-ating distinct dual-conducting or even triple-conducting materials.These properties enable their use as diverse functional materials for solid oxide fuel cells,solid oxide electrolysis cells,permeable membranes,and gas sensors.The literature review shows that the field of solid oxide materials and related electro-chemical cells has a significant level of research engagement,with over 8,000 publications published since 2020.The manual analysis of such a large volume of material is challenging.However,by examining the review articles,it is possible to identify key patterns,recent achievements,prospects,and remaining obstacles.To perform such an analysis,the present article provides,for the first time,a comprehensive summary of previous review publications that have been published since 2020,with a special focus on solid oxide materials and electrochemical systems.Thus,this study provides an important reference for researchers specializing in the fields of solid state ionics,high-temperature electrochemistry,and energyconversiontechnologies.

关键词： SOFCs SOECs PCFCS Electrochemistry energy conversion Hydrogen energy,Carbon neutrality

Self-assembled aerogel sheet electrodes of thermocells for low-grade heat harvest

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Science China Chemistry 2024年第5期67卷 1672-1679页

作者： Ziwei Mo Shouhao Wei Daibin Xie Kaihua Zhu Hongxiong Li Xin Lu Lirong Liang Chunyu Du Zhuoxin Liu Guangming Chen College of Materials Science and Engineering Shenzhen UniversityShenzhen 518055China State Key Laboratory of Polymer Materials Engineering Sichuan UniversityChengdu 610065China

Efficiently harvesting low-grade heat is crucial for sustainable energy management. Thermocells(TECs), inducing heat-toelectricity conversion via the thermogalvanic effect, have thus drawn tremendous attention in recent years. This study introduces a self-assembly approach for fabricating aerogel sheet electrodes(ASEs) tailored for TECs. The crafted ASEs retain a remarkable porous architecture with approximately 95% porosity, even with their slimmed-down thickness. Results reveal that the electrode composition has minimal influence on the thermopower of TECs. Notably, the porous ASE with tunned composition demonstrates an optimal effective surface area for the thermogalvanic effect, resulting in enhanced output current density. This balances the desirable traits of electrode compactness with abundant redox active sites, positioning it favorably against conventional bulky electrode designs. The TECs utilizing the optimized ASE achieve a peak output power of 22.10 μW cm^(-2)under a temperature difference of 30 K. Furthermore, a tubular TEC device is readily assembled and specially designed for harvesting heat energy from hot fluids. These findings underscore the potential of composite electrodes in the realm of low-grade heat harvest, paving the way for broader applications in sustainable energy solutions.

关键词： thermocells low-grade heat harvest energy conversion composite electrodes

Large-Area Gravure-Printed AgNWs Electrode on Water/Oxygen Barrier Substrate for Long-Term Stable Large-Area Flexible Organic Solar Cells

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Chinese Journal of Chemistry 2024年第5期42卷 478-484页

作者： Hao Wang Yaqin Pan Yunfei Han Zhuo Chen Tianyu Liu Lianping Zhang Qun Luo Chang-Qi Ma Printable Electronics Research Center & i-Lab Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of Sciences (CAS)SuzhouJiangsu215123 China Nano Science and Technology Institute University of Science and Technology of China166 Ren Ai RoadSEID SIPSuzhouJiangsu215123 China

Large-area AgNWs electrodes(25 cm×10 cm)were fabricated through roll-to-roll printing on the polyvinyl alcohol(PVA)modified water and oxygen barrier substrate.The modification of the barrier film with PVA improved the wettability of silver nanowires on the barrier films and led to the formation of homogenous large-area AgNWs networks.The mechanical flexibility,especially the adhesion force between the silver electrode and the barrier film substrate was dramatically improved through PVA modification.The efficiency of 13.51%for the flexible OSCs with an area of 0.64 cm2 was achieved based on the PET/barrier film/PVA/AgNWs electrode.The long-term stability showed the flexible OSCs based on the PET/barrier film/PVA/AgNWs electrode have a significantly improved stability relative to the device on PET/AgNWs electrode,and comparable air stability as the rigid device with glass/ITO device.The unencapsulated devices maintained nearly 50%of the original efficiency after storage for 600 h in air.After a simple top encapsulation,the flexible devices remained at 60%of the initial efficiency after 2000 h in the air.Therefore,the flexible AgNWs electrode based on the barrier film would have the potential to improve the air storage stability of organic flexible solar cells.

关键词： Flexible organic solar cell AgNWs electrode Air storage stability Barrier films substrate energy conversion Flexible electronics Interface

Towards catalytic reactions of Cu single-atom catalysts:Recent progress and future perspective

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Chinese Chemical Letters 2024年第2期35卷 197-207页

作者： Yitao Zhao Lei Tao Jiangsu Province Engineering Research Center of Special Functional Textile Materials Changzhou Vocational Institute of Textile and GarmentChangzhou 213164China Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology Advanced Catalysis and Green Manufacturing Collaborative Innovation CenterSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China

One of the urgent and challenging topics in diversified sustainable energy conversion is the development of high-performance,low-cost,and well durable catalysts.Cu single-atom catalysts(SACs)have become promising catalysts for diversified sustainable energy conversion due to their capability to maximize the utilization efficiency,acquire modulated electronic structure and optimized binding strength with intermediates.In this review,we have provided an interview of the recent progress achieved in the field of electrocatalysis,photocatalysis,and heterogeneous reaction based on Cu SACs.Started by this review,we have summarized some advanced synthetic strategies for the construction of Cu SACs.Subsequently,the performance-improving strategies are discussed in terms of the coordination environments of the reaction center,reaction mechanism and selectivity,based on free energy diagram and electron structure analysis.Finally,the remaining issues,challenges,and opportunities of Cu SACs are also provided,affording a perspective for future studies.This review not only offers us a deep understanding on the catalytic mechanism of Cu SACs for energy conversion,but also encourages more endeavors in prompting their practical application.

关键词： Cu SACs energy conversion Catalysis Coordination environment