Towards catalytic reactions of Cu single-atom catalysts:Recent progress and future perspective

作     者：Yitao Zhao Lei Tao Yitao Zhao;Lei Tao

作者机构：Jiangsu Province Engineering Research Center of Special Functional Textile MaterialsChangzhou Vocational Institute of Textile and GarmentChangzhou 213164China Jiangsu Key Laboratory of Advanced Catalytic Materials and TechnologyAdvanced Catalysis and Green Manufacturing Collaborative Innovation CenterSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China 

出 版 物：《Chinese Chemical Letters》 (中国化学快报（英文版）)

年 卷 期：2024年第35卷第2期

页      面：197-207页

核心收录：

学科分类：081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）] 0703[理学-化学] 

基　　金：financially supported by the Postgraduate Research&Practice Innovation Program of Jiangsu Province(No.KYCX21_2795) the Basic Science(Natural Science)Research Project of Colleges and Universities of Jiangsu Province(No.21KJB540001) Changzhou Sci&Tech Program(Nos.CJ20220180,CJ20210042),China 

主　　题：Cu SACs Energy conversion Catalysis Coordination environment 

摘      要：One of the urgent and challenging topics in diversified sustainable energy conversion is the development of high-performance,low-cost,and well durable *** single-atom catalysts(SACs)have become promising catalysts for diversified sustainable energy conversion due to their capability to maximize the utilization efficiency,acquire modulated electronic structure and optimized binding strength with *** this review,we have provided an interview of the recent progress achieved in the field of electrocatalysis,photocatalysis,and heterogeneous reaction based on Cu *** by this review,we have summarized some advanced synthetic strategies for the construction of Cu ***,the performance-improving strategies are discussed in terms of the coordination environments of the reaction center,reaction mechanism and selectivity,based on free energy diagram and electron structure ***,the remaining issues,challenges,and opportunities of Cu SACs are also provided,affording a perspective for future *** review not only offers us a deep understanding on the catalytic mechanism of Cu SACs for energy conversion,but also encourages more endeavors in prompting their practical application.