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High-Energy Batteries:Beyond Lithium-Ion and Their Long Road to Commercialisation

Nano-Micro Letters 2022年第6期14卷 116-164页

作者： Yulin Gao Zhenghui Pan Jianguo Sun Zhaolin Liu John Wang Department of materials Science and Engineering National University of SingaporeSingapore 117574Singapore ST Engineering Advanced Material Engineering Pte.Ltd. Singapore 619523Singapore Institute of materials Research and Engineering Agency for ScienceTechnology and Research(A*STAR)Singapore 138634Singapore School of materials Science and Engineering Tongji UniversityShanghai 201804China

Rechargeable batteries of high energy density and overall performance are becoming a critically important technology in the rapidly changing society of the twenty-first *** lithium-ion batteries have so far been the dominant choice,numerous emerging applications call for higher capacity,better safety and lower costs while maintaining sufficient *** design space for potentially better alternatives is extremely large,with numerous new chemistries and architectures being simultaneously *** include other insertion ions(*** and numerous multivalent ions),conversion electrode materials(***,metallic anodes,halides and chalcogens)and aqueous and solid ***,each of these potential“beyond lithium-ion”alternatives faces numerous challenges that often lead to very poor cyclability,especially at the commercial cell level,while lithium-ion batteries continue to improve in performance and decrease in *** review examines fundamental principles to rationalise these numerous developments,and in each case,a brief overview is given on the advantages,advances,remaining challenges preventing cell-level implementation and the state-of-the-art of the solutions to these ***,research and development results obtained in academia are compared to emerging commercial examples,as a commentary on the current and near-future viability of these“beyond lithium-ion”alternatives.

关键词： High energy density Beyond lithium-ion batteries Multivalent-ion batteries conversion electrode materials Electrolyte

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