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Production of biomass-derived monomers through catalytic conversion of furfural and hydroxymethylfurfural

Green Chemical Engineering 2021年第2期2卷 158-173页

作者： hirong Yang Jing Zhang Gang Qian Xuezhi Duan Xinggui Zhou State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai200237China

The synthesis of biomass-derived monomers has received great attention in recent years,motivated by the depletion of fossil fuels and environmental ***,the intrinsic functionality within the biomass or biomass-derived chemicals has great potential to produce new types of monomers containing multiple acid or alcohol groups,thereby leading to materials with novel *** their versatile functional groups and easy production from cellulose/hemicellulose,furfural and hydroxymethylfurfural were regarded as very important biomass-derived platform chemicals through which multiple monomers can be produced via heterogeneous *** the current review,recent development in heterogeneous catalysis for the production of 6 bio-based monomers,furfuryl alcohol,2,5-bis(hydroxymethyl)furan,2,5-bis-(hydroxymethyl)tetrahydrofuran,1,5-pentanediol,1,6-hexanediol,and 2,5-furandicarboxylic acid,from furfural and hydroxymethylfurfural is reviewed and *** major challenge is how to efficiently and selectively convert specific functional group(s)in furfural and hydroxymethylfurfural during the production of these ***,catalyst stability issues need to be addressed due to necessity of using hot water as reaction medium and high tendency of carbonaceous deposit formation on catalyst *** current review mainly focuses on efforts of catalytic site design and modification,including selection of metal/support,use of synergy between metal and support,tuning metal size,use of inverse catalysts,adding catalytic promoters,constructing bimetallic sites,etc.,to realize efficient,selective and stable production of bio-based monomers from furfural and hydroxymethylfurfural.

关键词： biomass-derived monomers Catalyst design Furfural Hydroxymethylfurfural Heterogeneous catalysis

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