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Low-temperature chlorination roasting technology for the simultaneous recovery of valuable metals from spent LiCoO_(2)cathode material

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 80-91页

作者： Junjie Shi Changle Hou Jingjing Dong Dong Chen Jianzhong Li key Laboratory for Ecological Metallurgy of Multimetallic Mineral(ministry of Education) Northeastern UniversityShenyang 110819China School of Metallurgy Northeastern UniversityShenyang 110819China

With the continuous increase in the disposal volume of spent lithium-ion batteries(LIBs),properly recycling spent LIBs has become essential for the advancement of the circular *** study presents a systematic analysis of the chlorination roasting kinetics and proposes a new two-step chlorination roasting process that integrates thermodynamics for the recycling of LIB cathode *** activation energy for the chloride reaction was 88.41 kJ/mol according to thermogravimetric analysis–derivative thermogravimetry data obtained by using model-free,model-fitting,and Z(α)function(αis conversion rate).Results indicated that the reaction was dominated by the first-order(F1)model when the conversion rate was less than or equal to 0.5 and shifted to the second-order(F2)model when the conversion rate exceeded *** conditions were determined by thoroughly investigating the effects of roasting temperature,roasting time,and the mass ratio of NH_(4)Cl to LiCoO_(2).Under the optimal conditions,namely 400℃,20 min,and NH_(4)Cl/LiCoO_(2)mass ratio of 3:1,the leaching efficiency of Li and Co reached 99.43% and 99.05%,*** of the roasted products revealed that valuable metals in LiCoO_(2)transformed into CoCl_(2) and ***,the reaction mechanism was elucidated,providing insights for the establishment of a novel low-temperature chlorination roasting technology based on a crystal structure *** technology can guide the development of LIB recycling processes with low energy consumption,low secondary pollution,high recovery efficiency,and high added value.

关键词： spent lithium-ion battery thermodynamics chlorination roasting kinetics circular economy

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Single-cell omics: experimental workflow, data analyses and applications

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Science china Life Sciences 2025年第1期68卷 5-102页

作者： Fengying Sun Haoyan Li Dongqing Sun Shaliu Fu Lei Gu Xin Shao Qinqin Wang Xin Dong Bin Duan Feiyang Xing Jun Wu Minmin Xiao Fangqing Zhao Jing-Dong J.Han Qi Liu Xiaohui Fan Chen Li Chenfei Wang Tieliu Shi Department of Clinical Laboratory the Affiliated Wuhu Hospital of East China Normal University (The Second People's Hospital of Wuhu City) Pharmaceutical Informatics Institute College of Pharmaceutical SciencesZhejiang University key Laboratory of Spine and Spinal Cord Injury Repair and Regeneration (Tongji University) Ministry of EducationOrthopaedic DepartmentTongji HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Frontier Science Center for Stem Cells School of Life Sciences and TechnologyTongji University Translational Medical Center for Stem Cell Therapy and Institute for Regenerative Medicine Shanghai East HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University research Institute of Intelligent Computing Zhejiang Lab Shanghai research Institute for Intelligent Autonomous Systems Center for Single-cell Omics School of Public HealthShanghai Jiao Tong University School of Medicine National key Laboratory of Chinese Medicine Modernization Innovation Center of Yangtze River DeltaZhejiang University Center for Bioinformatics and Computational Biology Shanghai Key Laboratory of Regulatory Biologythe Institute of Biomedical Sciences and School of Life SciencesEast China Normal University Beijing Institutes of Life Science Chinese Academy of Sciences Peking-Tsinghua Center for Life Sciences Academy for Advanced Interdisciplinary StudiesCenter for Quantitative Biology (CQB)Peking University Zhejiang key Laboratory of Precision Diagnosis and Therapy for Major Gynecological Diseases Women's HospitalZhejiang University School of Medicine key Laboratory of Advanced Theory and Application in Statistics and Data Science-MOE School of StatisticsEast China Normal University

Cells are the fundamental units of biological systems and exhibit unique development trajectories and molecular features. Our exploration of how the genomes orchestrate the formation and maintenance of each cell, and control the cellular phenotypes of various organismsis, is both captivating and intricate. Since the inception of the first single-cell RNA technology, technologies related to single-cell sequencing have experienced rapid advancements in recent years. These technologies have expanded horizontally to include single-cell genome, epigenome,proteome, and metabolome, while vertically, they have progressed to integrate multiple omics data and incorporate additional information such as spatial sc RNA-seq and CRISPR screening. Single-cell omics represent a groundbreaking advancement in the biomedical field,offering profound insights into the understanding of complex diseases, including cancers. Here, we comprehensively summarize recent advances in single-cell omics technologies, with a specific focus on the methodology section. This overview aims to guide researchers in selecting appropriate methods for single-cell sequencing and related data analysis.

关键词： single-cell sequencing genome epigenome proteomics metabolomics multimodal spatial transcriptomics CRISPR screening

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Identification and spatial patterns of coastal water pollution sources based on GIS and chemometric approach

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Journal of Environmental Sciences 2007年第7期19卷 805-810页

作者： ZHOU Feng GUO Huai-cheng LIU Yong HAO Ze-jia College of Environmental Sciences Peking University Beijing 100871 China.

Comprehensive and joint applications of GIS and chemometric approach were applied in identification and spatial patterns of coastal water pollution sources with a large data set （5 years （2000-2004）, 17 parameters） obtained through coastal water monitoring of Southern Water Control Zone in Hong Kong. According to cluster analysis the pollution degree was significantly different between September-next May （the 1st period） and June-August （the 2nd period）. Based on these results, four potential pollution sources, such as organic/eutrophication pollution, natural pollution, mineral/anthropic pollution and fecal pollution were identified by factor analysis/principal component analysis. Then the factor scores of each monitoring site were analyzed using inverse distance weighting method, and the results indicated degree of the influence by various potential pollution sources differed among the monitoring sites. This study indicated that hybrid approach was useful and effective for identification of coastal water pollution source and spatial patterns.

关键词： source identification spatial pattern cluster analysis (CA) principal component analysis (PCA) inverse distance weighting (IDW) Hong Kong

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Experimental study on co-pyrolysis characteristics of typical medical waste compositions

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Journal of Central South University 2014年第12期21卷 4613-4622页

作者：邓娜崔文谦王维维张强张于峰马洪亭 School of Environmental Science and Engineering Tianjin University key Laboratory of Efficient Utilization of Low and Medium Grade Energy of ministry of Education(Tianjin University)

Thermal decomposition of 21 kinds of binary mixtures between typical medical compositions was investigated under nitrogen conditions by dynamic thermogravimetric analysis(TGA) at 25–800 °C. The weighed sum method(WSM) coupled with thermal analysis was applied to study the interaction between components. Then, co-pyrolysis kinetic model of the binary mixtures(tube for transfusion(TFT) and gauze) was established to verify the reliability of conclusions. The results show the follows. 1) Strong or weak interactions are shown between binary mixtures containing polyvinyl chloride(PVC), the main ingredient of TFT. The addition of other medical waste could enhance first stage decomposition of TFT. While, the secondary stage pyrolysis may be suppressed or enhanced or not affected by the addition. 2) There exists no interaction between catheter and other component, the DTG peak temperature representing Ca CO3 decomposition in catheter fraction is obviously lower than that of pure catheter; while,the shape of DTG peak keeps unchanged. 3) No evident reaction occurs between the other mix-samples, it is considered that their co-pyrolysis characteristics are linear superposition of mono-component pyrolysis characteristics.

关键词： co-pyrolysis medical waste tube for transfusion(TFT) catheter interaction

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TiO_2-modified nano-egg-shell Pd catalyst for selective hydrogenation of acetylene

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Particuology 2010年第3期8卷 251-256页

作者： Jin Gao Qiufeng Zhu Lixiong Wen key Lab for Nanomaterials Ministry of Education Beijing University of Chemical Technology Beijing 100029 China research Center of the ministry of Education for High Gravity Engineering and Technology Beijing University of Chemical Technology Beijing 100029 China

Pd-based egg-shell nano-catalysts were prepared using porous hollow silica nanoparticles （PHSNs） as support, and the as-prepared catalysts were modified with TiO2 to promote their selectivity for hydro-genation of acetylene. Pd nanoparticles were loaded evenly on PHSNs and TiO2 was loaded on the active Pd particles. The effects of reduction time and temperature and the amount of TiO2 added on catalytic per-formances were investigated by using a fixed-bed micro-reactor. It was found that the catalysts showed better performance when reduced at 300 ℃ than at 500℃, and if reduced for 1 h than 3 h. When the amount of Ti added was 6 times that of Pd, the catalyst showed the highest ethylene selectivity.

关键词： Egg-shell nano-catalyst Porous hollow silica nanoparticles Modification Selective hydrogenation Acetylene

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Design and Implementation of a Network Management System Based on Mobile RMON Agent

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Journal of china University of Mining and Technology 2006年第3期16卷 325-329页

作者： SHAN Xin LIU Peng WU Lin LIU Ying GUO Jun School of Information Engineering Beijing University of Posts ＆ Telecommunications Beijing 100876 China

To improve the scalability of RMON-based network management, the concept of Mobile RMON Agent (MRA) was presented by combining the mobile agent technology with RMON. Then an MRA-based Network Management System (MRANMS) was designed and implemented. RMON functions were achieved by programming the mobile agent to make it capture and analyze packets locally. The experimental result on the Grasshopper platform indicates that MRA as a mobile agent can migrate to another subnet and calculate a RMON MIB value and TrafficMatrix in a subnet with 29 hosts. Furthermore, the behavior of MRA can be customized to achieve new RMON functions, such as the statistics of hostTable in RMON MIB. It can be concluded that MRANMS is based on the mode of distribution, and besides the compatibility with standard RMON, the system possesses scalability of management function.

关键词： network management RMON mobile agent MRA scalability

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Sorption and Fractionation of a Peat Derived Humic Acid by Kaolinite, Montmorillonite, and Goethite

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Pedosphere 2009年第1期19卷 21-30页

作者： S. GHOSH WANG Zhen-Yu S. KANG P. C. BHOWMIK B. S. XING Department of Plant Soil and Insect Sciences University of Massachusetts Amherst MA 01003 （USA）. College of Environmental Science and Engineering Ocean University of China Qingdao 266100 （China）

Sorption of humic acid （HA） on mineral surfaces has a profound interest regarding the fate of hydrophobic organic contaminants （HOCs） and carbon sequestration in soils. The objective of our study is to determine the fractionation behavior of HA upon sorption on mineral surfaces with varying surface properties. HA was coated sequentially on kaolinite （1：1 clay）, montmorillonite （2：1 clay）, and goethite （iron oxide） for four times. The unadsorbed HA fractions were characterized by elemental analysis, diffuse reflectance infrared Fourier transform spectroscopy （DRIFT）, and solid state 13C nuclear magnetic resonance spectroscopy （NMR）. The mineral-HA complexes were characterized by DRIFT. Polarity index [（N＋O）/C] revealed higher polarity of the unadsorbed HA fractions after coating on kaolinite, reflecting that relatively higher polarity fractions of HA remain unadsorbed. Sorption of aiiphatic alcohol fraction along with carbohydrate was prominent on kaolinite surface. DRIFT results of the unadsorbed HA fractions indicated more sorption of aiiphatic moieties on both kaolinite and montmorillonite. DRIFT results of the unadsorbed HA fractions after sorption on kaolinite and goethite showed the sorption of the proteinaceons fractions of HA. The HA fractions obtained after coating on goethite showed significant sorption of carboxylic moieties. The results mentioned above comply reasonably well with the DRIFT spectra of the minerai-HA complexes. ^13C NMR results showed higher sorption of anomeric C on kaolinite surface. Higher sorption of paraffinic fraction waS observed on montmorillonite. NMR data inferred the sorption of carboxylic moieties on goethite surface. Overall, this study showed that aliphatic moieties of HA preferentially sorbed on kaolinite and montmorillonite, while carboxylic functional groups play a significant role in sorption of HA on goethite. The sorbed fractions of HA may modify the mineral surface properties, and thus, the interaction with organic cont

关键词： carboxylic group DRIFT hydrophobic NMR sequential coating

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Form transition of sodium during combustion of black liquor coal slurry

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Journal of china University of Mining and Technology 2008年第1期18卷 6-12页

作者： LAN Ze-quan CAO Xin-yu ZHOU Jun-hu LIU Jian-zhong2, CHENG Jun CEN Ke-fa North china Institute of Science and Technology Yanjiao Hebei 065201 China State key Laboratory of Clean Energy Utilization Zhejiang University Hangzhou Zhejiang 31.0027 China

Several typical ash samples from a 0.25 MW test furnace fired black liquor coal slurry were selected for investigation. The phases and compounds containing sodium in ash samples were acquired from X-ray diffraction analyses. As well, detailed analyses of the amounts of major mineral elements along thickness gradients of representative ash samples were carried out. The elements, including Na, Si, A1, S and C1 were analyzed by the advanced electron probe microanalyzer equipment, which provid evidence and interpretation for the analytical results of XRD. The findings indicate that the occurrence form of sodium has experi- enced important changes during the combustion of black liquor coal slurry, which translated into nepheline, thenardite, sodium sulfate, sodium chloride, sodium silicoaluminate, hanyne and other phases containing sodium, from NaOH, Na2CO3 and Na2S in raw fuel. Of all the sodium compounds, nepheline, thenardite and sodium sulfate are the most important forms of Na in solid com- bustion residues. Such a transformation of Na during the combustion of black liquor coal slurry resulted in a considerable impact on ash deposition and is not only different from the raw coal and papermaldng black liquors, but is also affected by local circum- stances in the combustion furnace. Amounts of Na, S and C1 in ash deposits from low temperature zones were larger than those from high temperature zones. Our findings should provide important theoretical instructions for industrial applications of black liquor coal slurry.

关键词： black liquor coal slurry sodium form transition ash deposition

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Characteristics of emissive spectrum and the removal of nitric oxide in N_2/O_2/NO plasma with argon additive

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Journal of Environmental Sciences 2009年第6期21卷 790-794页

作者： LIN Wenfeng,ZHANG Bin,HOU Wenhui,LI Dawei,YANG Hongmin School of Power Engineering,Nanjing Normal University,Nanjing 210042,china School of Power Engineering Nanjing Normal University Nanjing 210042 China. E-mail: booboo.ai@***

Although the approach using non-thermal plasma（NTP） for deNOx has been studied for over 15 years,how to achieve higher removal effciency with lower cost is still a barrier for its industrial *** order to investigate the impact of the argon additive on electron density,energy and nitric oxide reduction process in plasma,the spectrum of the dielectric barrier discharge at atmospheric pressure in a coaxial reactor was measured using the monochromater with high *** comparative experiments for NO reduction were carried out simultaneously in N2/O2/NO plasma stream with and without argon,*** nitrogen molecular spectrum which is attributed to the energy level transition（C^3πu→ B^3πg） was compared in the wavelength range 300-480 nm and the electron density and temperature were determined based on the relative intensities and Stark broadening width of spectral *** spectrum results indicated that the argon additive could enhance the intensity of emissive spectrum of plasma,thus the electron concentration as well as the energy was increased,and finally prompted the ionization rate to produce active N,O and *** results of NO reduction showed that NO conversion effciency increased in the range of 10%-30% with 5% addition of argon in stream comparing with the condition without argon *** study will play a positive role in the industrial application of dielectric barrier discharge deNOx reactor.

关键词： argon emissive spectrum nitric oxide non-thermal plasma

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Mechanism of inflammatory response and therapeutic effects of stem cells in ischemic stroke:current evidence and future perspectives

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Neural Regeneration research 2025年第1期20卷 67-81页

作者： Yubo Wang Tingli Yuan Tianjie Lyu Ling Zhang Meng Wang Zhiying He Yongjun Wang Zixiao Li Vascular Neurology Department of NeurologyBeijing Tiantan HospitalCapital Medical UniversityBeijingChina china National Clinical research Center for Neurological Diseases Beijing Tiantan HospitalCapital Medical UniversityBeijingChina Shanghai Engineering research Center of Stem Cells Translational Medicine ShanghaiChina National Center for Healthcare Quality Management in Neurological Diseases Beijing Tiantan HospitalCapital Medical UniversityBeijingChina Institute for Regenerative Medicine Shanghai East HospitalSchool of Life Sciences and TechnologyTongji UniversityShanghaiChina Chinese Institute for Brain research BeijingChina research Unit of Artificial Intelligence in Cerebrovascular Disease Chinese Academy of Medical SciencesBeijingChina Beijing Engineering research Center of Digital Healthcare for Neurological Diseases BeijingChina

Ischemic stroke is a leading cause of death and disability worldwide,with an increasing trend and tendency for onset at a younger ***,in particular,bears a high burden of stroke *** recent years,the inflammatory response after stroke has become a research hotspot:understanding the role of inflammatory response in tissue damage and repair following ischemic stroke is an important direction for its *** review summarizes several major cells involved in the inflammatory response following ischemic stroke,including microglia,neutrophils,monocytes,lymphocytes,and ***,we have also highlighted the recent progress in various treatments for ischemic stroke,particularly in the field of stem cell ***,understanding the complex interactions between inflammation and ischemic stroke can provide valuable insights for developing treatment strategies and improving patient *** cell therapy may potentially become an important component of ischemic stroke treatment.

关键词： cell therapy immune cell inflammatory ischemic stroke stem cell

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