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Amorphous electrocatalysts for urea oxidation reaction

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Progress in Natural Science:Materials International 2024年第2期34卷 362-375页

作者： Fenghui Guo Dongle Cheng Qian Chen Hao Liu Zhiliang Wu Ning Han Bing-Jie Ni Zhijie Chen School of Materials Science and Technology China University of Geosciences Shenzhen Academy of Metrology and Quality Inspection Centre for Technology in Water and Wastewater School of Civil and Environmental Engineering University of Technology Sydney College of Safety and Environmental Engineering Shandong University of Science and Technology Institute of Yellow River Delta Earth Surface Processes and Ecological Integrity Shandong University of Science and Technology Discipline of Chemical Engineering Western Australian School of Mines: Minerals Energy and Chemical Engineering Curtin University Department of Materials Engineering School of Civil and Environmental Engineering The University of New South Wales

Electrochemical urea oxidation reaction(UOR) is a promising alternative to oxygen evolution reaction(OER) for realizing energy-saving hydrogen production. Developing efficient electrocatalysts for UOR becomes a central challenge. Recently, amorphous materials have been extensively used as UOR catalysts because of their numerous defective sites and flexible electronic properties. In this review, recent advancements in the development of amorphous UOR electrocatalysts are analyzed. The UOR mechanism is discussed, and the design of amorphous catalysts is then analyzed. The main catalyst design strategies are illustrated, including nanostructure control,heteroatom doping, composition regulation, and heterostructure construction. Also, electrocatalysts' structureperformance correlation is interpreted. Perspectives in this field are proposed for guiding future studies on the development of high-performance amorphous catalysts towards energy sustainability.

关键词： Catalyst design Hydrogen energy Heterostructures Heteroatom doping Component regulation

Influence of laser parameters on the microstructures and surface properties in laser surface modification of biomedical magnesium alloys

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Journal of Magnesium and Alloys 2024年第1期12卷 72-97页

作者： Chee Ying Tan Cuie Wen Hua Qian Ang School of Engineering RMIT UniversityMelbourneVictoria 3001Australia

Biodegradable implants from magnesium(Mg)alloys have emerged in the biomedical field especially in the orthopedic and cardiovascular stent applications owing to their low density,high specific strength,excellent machinability,good biocompatibility,and *** primary shortcoming of Mg-based implants is their low corrosion resistance in the physiological environment,which results in premature mechanical integrity loss before adequate healing and the production of excessive hydrogen gas,which is harmful to the body tissues and negatively affects the biocompatibility of the *** surface modification has recently received attention because it can improve the surface properties such as surface chemistry,roughness,topography,corrosion resistance,wear resistance,hydrophilicity,and thus cell response to the surface of the *** composition and microstructures including textures and phases of laser-treated surfaces depend largely on the laser processing parameters(input laser power,laser scan velocity,frequency,pulse duration,pressure,gas circulation,working time,spot size,beam focal position,and laser track overlap)and the thermophysical properties of the substrate(solubility,melting point,and boiling point).This review investigates the impacts of various laser surface modification techniques including laser surface melting,laser surface alloying,laser cladding,laser surface texturing,and laser shock peening,and highlights their significance in improving the surface properties of biodegradable Mg alloys for implant ***,we explore how different laser process parameters affect its composition,microstructure,and surface properties in each laser surface modification technique.

关键词： Biocompatibility Biodegradability Corrosion Implant applications Laser surface modification Magnesium alloys

Triphenylphosphine-Assisted Exsolution Engineering on Ruddlesden-Popper Perovskites for Promoting Oxygen Evolution

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Energy & Environmental Materials 2024年第4期7卷 433-441页

作者： Juan Bai Jing Shang Jun Mei Dongchen Qi Ting Liao Ziqi Sun School of Chemistry and Physics Queensland University of Technology Centre for Materials Science Queensland University of Technology School of Materials Science and Engineering Shaanxi University of Science and Technology School of Mechanical Medical and Process Engineering Queensland University of Technology

Metal exsolution engineering has been regarded as a promising strategy for activating intrinsically inert perovskite oxide catalysts toward efficient oxygen evolution *** metal exsolution processes on perovskites are often achieved by using the reducing hydrogen gas; however,this is not effective for the relatively stable phase,such as Ruddlesden-Popper perovskite oxides.

关键词： exsolution oxygen evolution perovskite reconstruction Ruddlesden–Popper

Communication Resource-Efficient Vehicle Platooning Control With Various Spacing Policies

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 362-376页

作者： Xiaohua Ge Qing-Long Han Xian-Ming Zhang Derui Ding IEEE School of Science Computing and Engineering TechnologiesSwinburne University of TechnologyMelbourne VIC 3122Australia

Platooning represents one of the key features that connected automated vehicles may possess as it allows multiple automated vehicles to be maneuvered cooperatively with small headways on roads. However, a critical challenge in accomplishing automated vehicle platoons is to deal with the effects of intermittent and sporadic vehicle-to-vehicle data transmissions caused by limited wireless communication resources. This paper addresses the co-design problem of dynamic event-triggered communication scheduling and cooperative adaptive cruise control for a convoy of automated vehicles with diverse spacing policies. The central aim is to achieve automated vehicle platooning under various gap references with desired platoon stability and spacing performance requirements, while simultaneously improving communication efficiency. Toward this aim, a dynamic event-triggered scheduling mechanism is developed such that the intervehicle data transmissions are scheduled dynamically and efficiently over time. Then, a tractable co-design criterion on the existence of both the admissible event-driven cooperative adaptive cruise control law and the desired scheduling mechanism is derived. Finally, comparative simulation results are presented to substantiate the effectiveness and merits of the obtained results.

关键词： Automated vehicles constant time headway spacing constant spacing cooperative adaptive cruise control event-triggered communication vehicle platooning

Finite dimensional irreducible representations of Lie superalgebra D(2,1;α)

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Communications in Theoretical Physics 2024年第2期76卷 14-28页

作者：陈曦杨文力丁祥茂张耀中 College of Intelligent Systems Science and Engineering Hubei Minzu University 445000China Institute of Modern Physics Northwest UniversityXian 710069China Institute of Applied Mathematics Academy of Mathematics and Systems ScienceChinese Academy of SciencesBeijing 100080China School of Mathematics and Physics The University of QueenslandBrisbaneQLD 4072Australia

This paper focuses on the finite dimensional irreducible representations of Lie superalgebra D(2,1;α).We explicitly construct the finite dimensional representations of the superalgebra D(2,1;α)by using the shift operator and differential operator *** ordinary Lie algebra representation,there are typical and atypical representations for most ***,its typical and atypical representation conditions are also *** results are expected to be useful for the construction of primary fields of the corresponding current superalgebra of D(2,1;α).

关键词： superalgebra representations shift operator conformal field theory

Managing underground legal boundaries in 3D-extending the CityGML standard

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Underground Space 2024年第1期14卷 239-262页

作者： Bahram Saeidian Abbas Rajabifard Behnam Atazadeh Mohsen Kalantari The Centre for Spatial Data Infrastructures and Land Administration Department of Infrastructure EngineeringThe University of MelbourneParkvilleVIC 3010Australia School of Civil and Environmental Engineering University of New South WalesSydneyNSW 2052Australia

Legal boundaries are used for delineating the spatial extent of ownership property’s *** underground environments,these boundaries are defined by referencing physical objects,surveying measurements,or ***,there is a gap in connecting and managing these boundaries and underground legal spaces,due to a lack of data model.A 3D data model supporting underground land administration(ULA)should define and model these boundaries and the relationships between them and underground ownership *** 3D data models can be enriched to model underground legal *** research aims to propose a new taxonomy of underground legal boundaries and model them by extending CityGML,which is a widely used 3D data model in the geospatial science *** developed,implemented,and tested the model for different types of underground legal *** implemented prototype showcased the potential benefits of CityGML for managing underground legal boundaries in *** proposed 3D underground model can be used to address current challenges associated with communicating and managing legal boundaries in underground *** this data model was specifically developed for Victoria,Australia,the proposed model and approach can be used and replicated in other jurisdictions by adjusting the data requirements for underground legal boundaries.

关键词： Underground Legal boundaries Land administration 3D data model City model

Flow structure and shear stress in the presence of both ice cover on water surface and leafless vegetation in channel bed

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Journal of Hydrodynamics 2024年第2期36卷 340-354页

作者： Mahboubeh Barahimi Jueyi Sui School of Engineering University of Northern British ColumbiaPrince GeorgeCanada

This study aimed to investigate the previously unexplored effects of ice cover and submerged vegetation on flow *** were undertaken under both open channel and ice-covered flow *** bed material consisted of three non-uniform *** findings revealed that when vegetation patches were present on the bed and an ice cover was present,the velocity profiles exhibited a distinctive pattern with two peak *** kinetic energy(TKE)also exhibited two peaks,one above the vegetation bending height and another at the sheath section,with a decreasing trend towards the ice ***,quadrant analysis showed that when the flow surface is covered by an ice cover,the contributions of inward and outward events increased compared with those observed in an open channel *** most cases,these contributions surpassed the sweep and ejection *** findings enhance our understanding of vegetation’s response to diverse surface conditions and have practical implications for river management and environmental engineering.

关键词： Ice cover vegetation flow structure Reynolds shear stress turbulent kinetic energy(TKE) quadrant analysis

Character Sheaves for Classical Graded Lie Algebras

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Acta Mathematica Sinica,English Series 2024年第3期40卷 870-884页

作者： Ting XUE School of Mathematics and Statistics University of MelbourneVIC 3010Australia Department of Mathematics and Statistics University of HelsinkiHelsinki 00014Finland

In this note we study character sheaves for graded Lie algebras arising from inner automorphisms of special linear groups and Vinberg’s type Ⅱ classical graded Lie algebras.

关键词： Graded Lie algebras character sheaves Fourier transform nilpotent orbits

Cooperative control for heterogeneous multi-agent systems: progress, applications, and challenges

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Science China(Information Sciences) 2024年第5期67卷 318-320页

作者： Bing YAN Peng SHI Jonathon CHAMBERS School of Electrical and Mechanical Engineering Faculty of Science Engineering and TechnologyThe University of Adelaide School of Engineering College of Science and Engineering University of Leicester

Cooperative control for heterogeneous multi-agent systems(MASs) is a critical and rapidly evolving field in modern automation and robotics. Characterized by the integration of agents with diverse capabilities and func... 详细信息

关键词： Multi agent systems