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Exploring the Roles of Single Atom in Hydrogen Peroxide Photosynthesis

Nano-Micro Letters 2024年第2期16卷 32-67页

作者： Kelin He Zimo Huang Chao Chen Chuntian Qiu Yu Lin Zhong Qitao Zhang International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518000China Queensland Micro‑and Nanotechnology Centre School of Environment and ScienceGriffith UniversityNathanQLD 4222Australia Institute for Sustainable Transformation School of Chemical Engineering and Light IndustryGuangdong University of TechnologyGuangzhou 51006China ZJU‑Hangzhou Global Scientific and Technological Innovation Center Zhejiang UniversityHangzhou 311215China

This comprehensive review provides a deep exploration of the unique roles of single atom catalysts(SACs)in photocatalytic hydrogen peroxide(H_(2)O_(2))*** offer multiple benefits over traditional catalysts such as improved efficiency,selectivity,and flexibility due to their distinct electronic structure and unique *** review discusses the critical elements in the design of SACs,including the choice of metal atom,host material,and coordination environment,and how these elements impact the catalytic *** role of single atoms in photocatalytic H_(2)O_(2)production is also analysed,focusing on enhancing light absorption and charge generation,improving the migration and separation of charge carriers,and lowering the energy barrier of adsorption and activation of *** these advantages,several challenges,including H_(2)O_(2)decomposition,stability of SACs,unclear mechanism,and low selectivity,need to be *** towards the future,the review suggests promising research directions such as direct utilization of H_(2)O_(2),high-throughput synthesis and screening,the creation of dual active sites,and employing density functional theory for investigating the mechanisms of SACs in H_(2)O_(2)*** review provides valuable insights into the potential of single atom catalysts for advancing the field of photocatalytic H_(2)O_(2)production.

关键词： Single atom catalysts H_(2)O_(2)photosynthesis Catalyst design and optimization

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LP modes exchange based on multiplane light conversion

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Chinese Optics Letters 2024年第3期22卷 14-18页

作者：钟亚楠林楚璇方浚丞雷霆袁小聪 Nanophotonics Research Centre Shenzhen Key Laboratory of Micro-Scale Optical Information Technology&Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China

Data exchange between different mode channels is essential in the optical communication network with mode-division multiplexing(MDM).However,there are challenges in realizing mode exchange with low insert loss,low mode crosstalk,and high ***,we designed and fabricated a mode exchange device based on multiplane light conversion(MPLC),which supports the transmission of LP01,LP11a,LP11b,and LP21 modes in the C-band and *** simulated exchanged mode purities are greater than 85%.The phase masks were fabricated on a silicon substrate to facilitate the integration with optical systems,with an insert loss of less than 2.2 dB and mode crosstalk below-21 dB due primarily to machining inaccuracies and alignment *** carried out an optical communication experiment with 10 Gbit/s OOK and QPSK data transmission at the wavelength of 1550 nm and obtained excellent performance with the *** paves the way for flexible data exchange as a building block in MDM optical communication networks.

关键词： mode exchange mode-division multiplexing multiplane light conversion

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Filterless narrowband photodetectors enabled by controllable band modulation through ion migration: The case of halide perovskites

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InfoMat 2024年第1期6卷 123-138页

作者： Yu Li Shanshan Yu Junjie Yang Kai Zhang Mingyu Hu Weitao Qiu Fumin Guo Wei Qian Sean Reinecke Tao Chen Makhsud I.Saidaminov Jian Wang Shihe Yang Guangdong Provincial Key Lab of Nano-Micro Materials Research School of Chemical Biology and BiotechnologyShenzhen Graduate SchoolPeking UniversityShenzhenGuangdongthe People's Republic of China shenzhen Bay Laboratory Institute of Biomedical EngineeringShenzhenGuangdongthe People's Republic of China School of Advanced Materials Shenzhen Graduate SchoolPeking UniversityShenzhenGuangdongthe People's Republic of China Department of Chemistry The University of Hong KongHong Kong SARthe People's Republic of China Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy ConversionDepartment of Materials Science and EngineeringSchool of Chemistry and Materials ScienceUniversity of Science and Technology of ChinaHefeiAnhuithe People's Republic of China College of Materials and Energy South China Agricultural UniversityGuangzhouGuangdongthe People's Republic of China Department of Chemistry University of VictoriaVictoriaBritish ColumbiaCanada

Narrowband photodetectors conventionally rely on optical structure design orbandpass filters to achieve the narrowband regime. Recently, a strategy forfilterless narrowband photoresponse based on the charge collection narrowing(CCN) mechanism was reported. However, the CCN strategy requires an electrically and optically “thick” photoactive layer, which poses challenges in controlling the narrowband photoresponse. Here we propose a novel strategy forconstructing narrowband photodetectors by leveraging the inherent ion migration in perovskites, which we term “band modulation narrowing” (BMN). Bymanipulating the ion migration with external stimuli such as illumination,temperature, and bias voltage, we can regulate in situ the energy-band structure of perovskite photodetectors (PPDs) and hence their spectral *** the Fermi energy levels obtained by the Kelvin probe force microscopy, the internal potential profiles from solar cell capacitance simulator simulation, and the anion accumulation revealed by the transient ion-drifttechnique, we discover two critical mechanisms behind our BMN strategy: theextension of an optically active but electronically dead region proximal to the top electrode and the down-bending energy bands near the electron transportlayer. Our findings offer a case for harnessing the often-annoying ionmigration for developing advanced narrowband PPDs.

关键词： band structure ion migration narrowband detection perovskite spatial distribution of charge carriers

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Generation and observation of multiple solitons from a mid-infrared ultrafast fiber laser

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Chinese Optics Letters 2024年第3期22卷 83-88页

作者：李梦媛宋宇锋张春香王振洪刘军 Institute of Microscale Optoelectronics College of Electronics and Information EngineeringShenzhen UniversityShenzhen 518060China shenzhen Key Laboratory of Ultraintense Laser and Advanced Material Technology Center for Advanced Material Diagnostic TechnologyCollege of Engineering PhysicsShenzhen Technology UniversityShenzhen 518118China

We demonstrate the generation of a unique regime of multiple solitons in a Tm-doped ultrafast fiber laser at~1938.72 *** temporal pulse-to-pulse separation among the multiple solitons,10 in a single-pulse bunch,increases from 0.89 ns to1.85 ns per round *** addition,with the increasing pump power,the number of bunched solitons increases from 3 up to 24linearly,while the average time separation in the soliton bunch varies irregularly between~0.80 and~1.52 *** results contribute to a more profound comprehension of nonlinear pulse dynamics in ultrafast fiber lasers.

关键词： mode-locked fiber laser multiple solitons pump hysteresis pulse-to-pulse interval

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A vectorial model for the nonlinear gradient force exerted on metallic Rayleigh nanoparticles

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Chinese Optics Letters 2024年第2期22卷 207-213页

作者：朱政张聿全闵长俊 Aurèle J.LAdam H.Paul Urbach 袁小聪 Research Center for Humanoid Sensing Research Institute of Intelligent SensingZhejiang LabHangzhou 311100China Nanophotonics Research Center Institute of Microscale Optoelectronics&State Key Laboratory of Radio Frequency Heterogeneous IntegrationShenzhen UniversityShenzhen 518060China Optics Research Group ImPhys DepartmentFaculty of Applied SciencesDelft University of TechnologyDelft 2628 CJThe Netherlands

Optical tweezers have proved to be a powerful tool with a wide range of *** gradient force plays a vital role in the stable optical trapping of *** scalar method is convenient and effective for analyzing the gradient force in traditional optical ***,when the third-order nonlinear effect of the nano-object is stimulated,the scalar method cannot adequately present the optical response of the metal nanoparticle to the external optical ***,we propose a theoretical model to interpret the nonlinear gradient force using the vector *** combining the optical Kerr effect,the polarizability vector of the metallic nanoparticle is derived.A quantitative analysis is obtained for the gradient force as well as for the optical potential *** vector method yields better agreement with reported experimental *** suggest that this method could lead to a deeper understanding of the physics relevant to nonlinear optical trapping and binding phenomena.

关键词： gradient forces nonlinear effect metallic nanoparticles

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Photothermal properties of Cu@polycarbonate composites with strong localized surface plasmon resonances

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Nano Research 2024年第9期17卷 8513-8520页

作者： Fengyi Wang Jiangling He Junshan Hu Zhihui Chen Yumeng Shi Qing-Hua Xu SZU-NUS Collaborative Innovation Center for Optoelectronic Science and Technology International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of EducationInstitute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China Department of Chemistry National University of Singapore3 Science Drive 3Singapore 117543Singapore College of Materials Science and Engineering Sichuan UniversityChengdu 610065China

Copper is relatively low cost and highly abundant compared with the well-studied noble metals such as gold and ***,the poor plasmonic and high susceptibility towards oxidation limit the study of its optical properties and applications as ***,copper nanoparticles@polycarbonate(Cu@PC)composites were prepared by using a facile one-step solvothermal *** Cu@PC composites have strong localized surface plasmon resonances(LSPR)due to that the PC shell can induce the particles to form many-particles system with different particle numbers,which not only lead to overlap and hybridize of the LSPR modes,but also shift the LSPR away from the interband transitions,and the PC layer also prevents the oxidation of Cu *** photothermal conversion efficiency of Cu@PC composites reaches 41.1%under 808 nm continuous wave(CW)laser irradiation which is higher than previously reported Cu nanomaterials that have been ***,the composites also have high photothermal ***,interfacial evaporator is prepared by assembling the Cu@PC composites on scouring sponge as light absorption layer which has>92.8%absorption in entire solar spectrum *** seawater evaporation rate is 3.177 kg·m-2·h^(-1)with a E_(evaporator)/E_(water)of *** high evaporation rate interfacial evaporator with low cost,simple,and scalable approach shows great application value in the field of photothermal evaporation.

关键词： Cu nanoparticles localized surface plasmon resonances(LSPR) photothermal interfacial evaporation

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Bandgap engineering of high mobility two-dimensional semiconductors toward optoelectronic devices

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Journal of Materiomics 2023年第3期9卷 527-540页

作者： Qiaoyan Hao Peng Li Jidong Liu Jiarui Huang Wenjing Zhang International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen518060China shenzhen Institute of Advanced Electronic Materials Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen518103China

Over the last few years,great advances have been achieved in exploration of high-mobility two-dimensional(2D)semiconductors such as metal chalcogenide InSe and noble-transition-metal dichal-cogenide PdSe_(2).These materials are competitive candidates for constructing next-generation optoelec-tronic devices owing to their unique crystalline and electronic ***,the optical and electronic properties of 2D materials can be efficiently modified via precisely engineering their band structures,which is critical for widening specific applications ranging from high-performance opto-electronics to catalysis and energy *** this review,we focus on the progress in bandgaps engineering of newly emerging high-mobility 2D semiconductors and their applications in optoelec-tronic devices,incorporating our recent study in the InSe and PdSe_(2)*** of all,we discuss the structure-property relationship of typical high-mobility 2D semiconductors(InSe and PdSe 2).Next,we analyze several viable strategies for bandgap engineering,including thickness,strain or pressure,alloying,heterostructure,surface modification,intercalation,and so ***,we summarize the optoelectronic devices fabricated with such high-mobility 2D *** conclusion and outlook in this topic are finally *** review aims to provide valuable insights in bandgap engineering of newly emerging 2D semiconductors and explore their potential in future optoelectronic applications.

关键词： High mobility 2D semiconductors Bandgap engineering Alloying Heterostructure

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Q[8]/SC[6]A-based framework constructed via OSIQ for metal ion capture

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Chinese Chemical Letters 2022年第3期33卷 1524-1528页

作者： Li-Fei Tian Ming Liu Li-Xia Chen Chao Huang Qian-Jiang Zhu Kai Chen Jiang-Lin Zhao Zhu Tao Key Laboratory of Macrocyclic and Supramolecular Chemistry of Guizhou Province Guizhou UniversityGuiyang 550025China Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlSchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044China Institute of Biomedical&Health Engineering Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen518055 China

Since the outer surface interaction of Q[n]s (OSIQ, including self-, anion- and aromatic-induced OSIQs) was proposed in 2014, it has become the most important research area in our group to construct various Q[n]-based supramolecular frameworks via the OSIQ strategy. Herein, we report a novel supramolecular framework constructed using cucurbit[8]uril (Q[8]) and 4-sulfocalix[6]arene (SC[6]A). This Q[8]/SC[6]A-based supramolecular framework is a product via the perfect combination of self-, anion- and aromatic-induced OSIQs. This framework has the characteristics of easy preparation and high stability with the most important feature being the sequence selective capture of specific metal cations, such as common alkali- and alkaline earth metal ions, and renewability. Thus, this framework may be used in seawater desalination, potassium ion enrichment, radioactive cesium ion pollution source treatment, Gruinard's treatment or water softening and other applications.

关键词： Cucurbituril 4-Sulfocalixarene Outer surface interaction of Q[n]s Supramolecular framework Metal ion capture

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Optical spiral vortex from azimuthally increasing/decreasing exponential phase gradients

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Chinese Optics Letters 2023年第11期21卷 123-127页

作者：介珮桦谢振威袁小聪 Nanophotonics Research Centre Institute of Microscale Optoelectronics&State Key Laboratory of Radio Frequency Heterogeneous IntegrationShenzhen UniversityShenzhen 518060China Research Center for Humanoid Sensing Zhejiang LaboratoryHangzhou 311100China

A new type of power-exponent-phase vortex-like beams with both quadratic and cubic azimuthal phase gradients is investigated in this *** intensity and orbital angular momentum(OAM)density distributions are noticeably different when the phase gradient increases or decreases along the azimuth angle,while the orthogonality and total OAM remain *** characteristics of the optical field undergo a significant change when the phase shifts from linear to nonlinear,with the variation of the power index having little impact on the beam characteristics under nonlinear phase *** characteristics provide new ideas for applications such as particle manipulation,optical communications,and OAM encryption.

关键词： optical vortex orbital angular momentum optical spiral azimuthally varying phase gradient

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The Relationship between Dimensions of Emerging Adulthood and Behavioral Problems among Chinese Emerging Adults: The Mediating Role of Physical Activity and Self- Control

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International Journal of Mental Health Promotion 2023年第8期25卷 937-948页

作者： Jin Kuang Jeffrey Jensen Arnett Erle Chen Zsolt Demetrovics Fabian Herold Rebecca Y.M.Cheung Daniel L.Hall Michaela Markwart Markus Gerber Sebastian Ludyga Arthur F.Kramer Liye Zou Body-Brain-Mind Laboratory School of PsychologyShenzhen UniversityShenzhen518060China Department of Psychology Clark UniversityWorcesterMA 01610USA shenzhen College of International Education Shenzhen518172China Centre of Excellence in Responsible Gaming University of GibraltarGX111AAGibraltar Institute of Psychology ELTE Eötvös Loránd UniversityBudapest1239Hungary Research Group Degenerative and Chronic Diseases MovementFaculty of Health Sciences BrandenburgUniversity of PotsdamPotsdam14476Germany School of Psychology and Clinical Language Sciences University of ReadingReadingRG1UK Massachusetts General Hospital and Harvard Medical School Boston02115USA Department of Sport Exercise&HealthUniversity of BaselBasel4091Switzerland Center for Cognitive&Brain Health Northeastern UniversityBoston02115USA Beckman Institute University of IllinoisIllinois60001USA

Emerging adulthood(EA)is a critical stage of life to develop and sustain a healthy lifestyle,which is also a time of vulnerability to poor physical and mental health *** this study,we conducted a path analysis(N=1326)to examine associations among four dimensions of EA,levels of regular physical activity(PA),self-control,MPA tendency and irrational *** found:1)higher levels of PA predicted both MPA tendency(β=−0.08,95%CI:−0.11 to−0.06,p<0.001)and irrational procrastination(β=−0.01,95%CI:−0.17 to−0.008,p<0.01)indirectly via self-control;2)Instability(β=0.13,95%CI:0.08 to 0.18,p<0.01)and Responsibility(β=−0.06,95%CI:−0.10 to−0.08,p=0.03)exerted direct effects on irrational procrastination and Instability also indirectly predicted irrational procrastination via MPA tendency(β=0.03,95%CI:0.02 to 0.05,p<0.01).These findings proved that perceived features of EA are linked to behavioral problems and supported that regular PA plays a crucial role to protect mental health.

关键词： Emerging adulthood Chinese culture physical activity mobile phone addiction irrational procrastination self-control

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