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Analyze the Performance of Electroactive Anticorrosion Coating of Medical Magnesium Alloy Using Deep Learning

Computers, Materials & Continua 2024年第4期79卷 263-278页

作者： Yashan Feng Yafang Tian Yongxin Yang Yufang Zhang Haiwei Guo Jing’an Li Advanced Functional Materials Laboratory Zhengzhou Railway Vocational and Technical CollegeZhengzhou450000China School of Materials science and Engineering Zhengzhou UniversityZhengzhou450000China

Electroactive anticorrosion coatings are specialized surface treatments that prevent or minimize corrosion. Thestudy employs strategic thermodynamic equilibriumcalculations to pioneer a novel factor in corrosion protection.A first-time proposal, the total acidity (TA) potential of the hydrogen (pH) concept significantly shapes medicalmagnesium alloys. These coatings are meticulously designed for robust corrosion resistance, blending theoreticalinsights and practical applications to enhance our grasp of corrosion prevention mechanisms and establisha systematic approach to coating design. The groundbreaking significance of this study lies in its innovativeintegration of the TA/pH concept,which encompasses the TA/pH ratio of the chemical environment. This approachsurpasses convention by acknowledging the intricate interplay between the acidity and pH levels within thecoating formulation, thereby optimizing metal-phosphate-based conversion coatings and transforming corrosionmitigation strategies. To authenticate the TA/pH concept, the study comprehensively compares its findings withexisting research, rigorously validating the theoretical framework and reinforcing the correlates among TA/pHvalues and observed corrosion resistance in the coatings. The influence of mutations that occur naturally inthe detergent solution on persistent phosphorus changes is shown by empirical confirmation, which improvescorrosion resistance. This realization advances the field ofmaterials and the field’s knowledge of coated generation,particularly anticorrosion converter layers.

关键词： Medical magnesium alloys hydrogen gas anticorrosion total acidity potential of the hydrogen(pH)

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Primitive functional groups directed distinct photocatalytic performance of imine-linked donor-acceptor covalent organic frameworks

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Nano Research 2024年第6期17卷 4994-5001页

作者： Xitong Ren Jiajie Sun Yusen Li Feng Bai Key Laboratory for Special Functional Materials of Ministry of Education National and Local Joint Engineering Research Center for High-Efficiency Display and Lighting TechnologySchool of Materials Science and Engineeringand Collaborative Innovation Center of Nano Functional Materials and ApplicationsHenan UniversityKaifeng 475004China School of Physics and Electronics Henan UniversityKaifeng 475004China

The combination of donor-acceptor(D-A)structures presents a viable strategy for fabricating covalent organic frameworks(COFs)with exceptional photocatalytic ***,the selection of functional groups on donor or acceptor building blocks and their effect on the macroscopic properties of COFs are *** this study,we tactfully synthesized a pair of Py-DBT-COFs from the same pyrene(Py)donor and 4,7-diphenylbenzo[c][1,2,5]thiadiazole(DBT)acceptor cores with distinct primitive functional *** primitive functional groups of building units determine the photocatalytic properties of corresponding ***,Py-C-DBT-COF synthesized from Py-4CHO and DBT-2NH_(2)showcases a splendid H_(2)evolution rate as high as 21,377.7μmol/(g·h)(with 5 wt.%Pt)originating from better charge transfer capacity,which is significantly superior to that of Py-N-DBT-COF constructed from Py-4NH_(2)and *** distinct photocatalytic performances of the two COFs are demonstrated to originate from the different charge separation and transfer *** work supplies a new avenue for optimizing the photocatalytic performance of D-A COFs from the perspective of primitive functional group selections.

关键词： covalent organic frameworks functional group donor-acceptor photocatalysis

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A coupled Legendre-Laguerre polynomial method with analytical integration for the Rayleigh waves in a quasicrystal layered half-space with an imperfect interface

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Applied Mathematics and Mechanics(English Edition) 2024年第9期45卷 1539-1556页

作者： Bo ZHANG Honghang TU Weiqiu CHEN Jiangong YU L.ELMAIMOUNI School of Mechanical and Power Engineering Henan Polytechnic UniversityJiaozuo 454000Henan ProvinceChina henan International Joint Laboratory of Advanced Electronic Packaging Materials Precision Forming Henan Polytechnic UniversityJiaozuo 454000Henan ProvinceChina Department of Engineering Mechanics Zhejiang UniversityHangzhou 310027China Polydisciplinary Faculty of Ouarzazate Ibnou Zohr UniversityOuarzazate 45000Morocco

The Laguerre polynomial method has been successfully used to investigate the dynamic responses of a ***,it fails to obtain the correct stress at the interfaces in a layered half-space,especially when there are significant differences in material ***,a coupled Legendre-Laguerre polynomial method with analytical integration is *** Rayleigh waves in a one-dimensional(1D)hexagonal quasicrystal(QC)layered half-space with an imperfect interface are *** correctness is validated by comparison with available *** computation efficiency is *** dispersion curves of the phase velocity,displacement distributions,and stress distributions are *** effects of the phonon-phason coupling and imperfect interface coefficients on the wave characteristics are *** novel findings reveal that the proposed method is highly efficient for addressing the Rayleigh waves in a QC layered *** can save over 99%of the computation *** method can be expanded to investigate waves in various layered half-spaces,including earth-layered media and surface acoustic wave(SAW)devices.

关键词： coupled Legendre-Laguerre polynomial method analytical integration Rayleigh wave quasicrystal(QC)layered half-space imperfect interface

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Tumor microenvironment of cancer stem cells:Perspectives on cancer stem cell targeting

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Genes & Diseases 2024年第3期11卷 275-302页

作者： Qianqian Guo Yi Zhou Tianyuan Xie Yin Yuan Huilong Li Wanjin Shi Lufeng Zheng Xiaoman Li Wenzhou Zhang Department of Pharmacy The Affiliated Cancer Hospital of Zhengzhou University&Henan Cancer HospitalZhengzhouHenan 450003China Jiangsu Key Laboratory for Pharmacology and Safety Evaluation of Chinese Materia Medica School of PharmacyNanjing University of Chinese MedicineNanjingJiangsu 210023China School of Life science and technology Jiangsu Key Laboratory of Carcinogenesis and InterventionChina Pharmaceutical UniversityNanjingJiangsu 211198China

There are few tumor cell subpopulations with stem cell characteristics in tumor tis-sue,defined as cancer stem cells(CSCs)or cancer stem-like cells(CSLCs),which can recon-struct neoplasms with malignant biological behaviors such as invasiveness via self-renewal and unlimited *** microenvironment that CsCs depend on consists of various cellular components and corresponding medium *** these factors existing at a variety of levels and forms,cytokine networks and numerous signal pathways play an important role in signaling *** factors promote or maintain cancer cell stem-ness,and participate in cancer recurrence,metastasis,and *** review aims to summarize the recent molecular data concerning the multilayered relationship between CsCs and CsC-favorable *** also discuss the therapeutic implications of target-ing this synergistic interplay,hoping to give an insight into targeting cancer cell stemness for tumortherapyandprognosis.

关键词： Cancer stem cells Cancerstem-like cells Cellular factors Non-cellularfactors Tumor microenvironment

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Formatted PVDF in lamellar composite solid electrolyte for solidstate lithium metal battery

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Nano Research 2024年第6期17卷 5159-5167页

作者： Xinji Zhang Yafang Zhang Shiyue Zhou Jingchuan Dang Chenye Wang Wenjia Wu Jingtao Wang School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China

Solid polymer electrolytes(SPEs)hold great application potential for solid-state lithium metal battery because of the excellent interfacial contact and processibility,but being hampered by the poor room-temperature conductivity(~10^(−7)S·cm^(−1))and low lithium-ion transference number(tLi+).Here,a lamellar composite solid electrolyte(Vr-NH_(2)@polyvinylidene fluoride(PVDF)LCSE)withβ-conformation PVDF is fabricated by confining PVDF in the interlayer channel of-NH_(2)modified vermiculite lamellar *** demonstrate that the conformation of PVDF can be manipulated by the nanoconfinement effect and the interaction from channel *** presence of-NH_(2)groups could induce the formation ofβ-conformation PVDF through electrostatic interaction,which serves as continuous and rapid lithium-ion transfer *** a result,a high room-temperature ionic conductivity of 1.77×10^(−4)S·cm^(−1)is achieved,1-2 orders of magnitude higher than most ***,Vr-NH_(2)@PVDF LCSE shows a high tLi+of 0.68 because of the high dielectric constant,~3 times of that of PVDF SPE,and surpassing most of reported *** LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)||Li cell assembled by Vr-NH_(2)@PVDF LCSE obtains a discharge specific capacity of 137.1 mAh·g^(−1)after 150 cycles with a capacity retention rate of 93%at 1 C and 25℃.This study may pave a new avenue for high-performance SPEs.

关键词： solid-state lithium metal battery lamellar composite solid electrolyte β-conformation polyvinylidene fluoride(PVDF) room-temperature ionic conductivity lithium-ion transference number

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Extraction and recycling technologies of cobalt from primary and secondary resources:A comprehensive review

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International Journal of Minerals,Metallurgy and Materials 2024年第4期31卷 628-649页

作者： Yukun Huang Pengxu Chen Xuanzhao Shu Biao Fu Weijun Peng Jiang Liu Yijun Cao Xiaofeng Zhu ZhongYuan Critical Metals Laboratory Zhengzhou UniversityZhengzhou 450001China State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of TechnologyLanzhou 730050China

Cobalt has excellent electrochemical,magnetic,and heat *** a strategic resource,it has been applied in many hightech ***,the recent rapid growth of the battery industry has substantially depleted cobalt resources,leading to a crisis of cobalt resource *** paper examines cobalt ore reserves and distribution,and the recent development and consumption of cobalt resources are summarized as *** addition,the principles,advantages and disadvantages,and research status of various methods are discussed *** can be concluded that the use of diverse sources(Cu-Co ores,Ni-Co ores,zinc plant residues,and waste cobalt products)for cobalt production should be enhanced to meet developmental ***,in recovery technology,the pyro-hydrometallurgical process employs pyrometallurgy as the pretreatment to modify the phase structure of cobalt minerals,enhancing its recovery in the hydrometallurgical stage and facilitating high-purity cobalt ***,it represents a promising technology for future cobalt ***,based on the above conclusions,the prospects for cobalt are assessed regarding cobalt ore processing and sustainable cobalt recycling,for which further study should be conducted.

关键词： cobalt recovery copper-cobalt ore nickel-cobalt ore zinc plant residue waste cobalt products

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Lamellar quasi-solid electrolyte with nanoconfined deep eutectic solvent for high-performance lithium battery

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Nano Research 2024年第7期17卷 6176-6183页

作者： Shiwei Liu Jing Wang Keqi Wu Zhirong Yang Yan Dai Junmei Zhang Wenjia Wu Jingtao Wang School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China

Electrolytes with high-efficiency lithium-ion transfer and reliable safety are of great importance for lithium *** having superior ionic conductivity(10^(−3)–10^(−2) S·cm^(−1)),traditional liquid-state electrolytes ... 详细信息

关键词： quasi-solid electrolyte deep eutectic solvent lamellar structure lithium-ion transference number solvation shell

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An anonymous authentication and secure data transmission scheme for the Internet of Things based on blockchain

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Frontiers of Computer science 2024年第3期18卷 183-197页

作者： Xingxing CHEN Qingfeng CHENG Weidong YANG Xiangyang LUO State Key Laboratory of Mathematical Engineering and Advanced Computing Zhengzhou Institute of Information Science and TechnologyZhengzhou 450001China henan Key Laboratory of Grain Photoelectric Detection and Control Henan University of TechnologyZhengzhou 450001China henan Province Key Laboratory of Cyberspace Situation Awareness Zhengzhou Institute of Information Science and TechnologyZhengzhou 450001China

With the widespread use of network infrastructures such as 5G and low-power wide-area networks,a large number of the Internet of Things(IoT)device nodes are connected to the network,generating massive amounts of ***,it is a great challenge to achieve anonymous authentication of IoT nodes and secure data *** present,blockchain technology is widely used in authentication and s data storage due to its decentralization and ***,Fan et *** a secure and efficient blockchain-based IoT authentication and data sharing *** studied it as one of the state-of-the-art protocols and found that this scheme does not consider the resistance to ephemeral secret compromise attacks and the anonymity of IoT *** overcome these security flaws,this paper proposes an enhanced authentication and data transmission scheme,which is verified by formal security proofs and informal security ***,Scyther is applied to prove the security of the proposed ***,it is demonstrated that the proposed scheme achieves better performance in terms of communication and computational cost compared to other related schemes.

关键词： Internet of Things blockchain authentication data transmission

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High-lattice-adapted surface modifying Na_(4)MnV(PO_(4))_(3) for better sodium storage

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Nano Research 2024年第4期17卷 2728-2735页

作者： Chongran Song Shiyu Li Ying Bai International Joint Research Laboratory of New Energy Materials and Devices of henan Province School of Physics and ElectronicsAcademy for Advanced Interdisciplinary StudiesHenan UniversityKaifeng 475004China

Sodium-ion batteries(SIBs)are required to possess long cycle life when used for large-scale energy *** polyanionic Na_(4)MnV(PO_(4))_(3)(NMVP)reveals good cyclic stability due to its unique three-dimensional(3D)frame structure,but it still faces the challenge of interfacial degradation in practical *** this work,NASICON-type Na_(1.3)Al_(0.7)Ti_(1.3)(PO_(4))_(3)(NATP)was deposited on the surface of NMVP to promote interface stability by surface modification and gradient *** a result,the optimized NMVP@2%NATP released a capacity retention of 44.8%after 1000 cycles at 5 C,much higher than that of the initial NMVP(28.9%).The enhanced electrochemical performance was mainly attributed to NATP coating acting as a fast ion transport carrier and physical barrier,significantly facilitating the Na^(+)diffusion and isolating side reaction at the electrode/electrolyte *** the other hand,Ti_(4)^(+)and Al^(3+)cations from the NATP were partially doped inside the NMVP surface to boost the transport of Na^(+),and the perfect lattice matching of NVMP and NATP improved the interface and structural stability accompanying long *** work demonstrated the effectiveness of surface modification with high lattice match material and provided new perspectives for high energy density solid-state SIBs.

关键词： high-lattice-adapted cathode surface modification sodium-ion batteries

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Deletion of a 1,049 bp sequence from the 5′UTR upstream of the SiHEC3 gene induces a seed non-shattering mutation in sesame

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Journal of Integrative Agriculture 2024年第8期23卷 2589-2604页

作者： Ming Ju Guiting Li Qiuzhen Tian Hengchun Cao Qin Ma Yinghui Duan Hui Guo Zhanyou Zhang Yingying Huang Huili Wang Haiyang Zhang Hongmei Miao The Shennong Laboratory Zhengzhou 450002China henan Sesame Research Center Henan Academy of Agricultural SciencesZhengzhou 450002China Key Laboratory of Specific Oilseed Crops Genomics of henan Province Henan Sesame Research CenterHenan Academy of Agricultural SciencesZhengzhou 450002China

Sesame is a labor intensive crop with limited mechanized harvesting mainly due to the seed shattering(SS)*** this study,we performed a genetic analysis of the seed-shattering resistance(SR)trait with a SR sesame mutant *** the SS type,the parenchyma cells in the abscission zone of the 12M07 mutant are arranged loosely but adhere to the seed *** analysis of six generations derived from 12M07(SR)×Xiangcheng Dazibai(SS)showed that the SR trait is recessive and controlled by a single gene *** mapping of the F2population with 888,619 variants(single-nucleotide polymorphisms(SNPs)and insertion-deletion(InDels))and 31,884 structural variations(SVs)determined that only SV12002 in the 5′upstream region of gene Sindi0765000(named SiHEC3)in Chr.3 was significantly associated with the SR ***3 encodes the bHLH transcription factor.A 1,049 bp deletion occurred in the 5′UTR of Sihec3 in ***3 is mainly expressed in developing placental tissues,with the expression peaking in capsules at 45 days after pollination.A dual-luciferase reporter assay in tobacco confirmed that the promoter activity of Sihec3 was reduced because of the deletion of the 1,049 bp promoter ***–protein interaction network analysis showed that HEC3 is co-expressed with nine key proteins,such as SHATTERPROOF1(SHP1)and SEEDSTICK(STK)which participate in the secondary wall biosynthesis of the abscission layer in *** findings of this study show the important function of Sihec3corresponding with the SR trait and supply the genetic information for breeding new varieties that are amenable to mechanized harvesting in sesame and other crops.

关键词： sesame(Sesamum indicum L.) association mapping seed shattering structure variation bHLH transcription factor

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