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Engineering hierarchical quaternary superstructure of an integrated MOF-derived electrode for boosting urea electrooxidation assisted water electrolysis

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Green Energy & Environment 2024年第4期9卷 695-701页

作者： Jianjun Tian Changsheng Cao Yingchun He Muhammad Imran Khan Xin-Tao Wu Qi-long zhu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of Sciences(CAS)Fuzhou350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou350108China University of Chinese Academy of Sciences Beijing100049China Research Institute of Sciences and Engineering(RISE) University of SharjahSharjah27272United Arab Emirates

Controllable design of the catalytic electrodes with hierarchical superstructures is expected to improve their electrochemical ***,a self-supported integrated electrode(NiCo-ZLDH/NF)with a unique hierarchical quaternary superstructure was fabricated through a self-sacrificing template strategy from the metal–organic framework(Co-ZIF-67)nanoplate arrays,which features an intriguing well-defined hierarchy when taking the unit cells of the NiCo-based layered double hydroxide(NiCo-LDH)as the primary structure,the ultrathin LDH nanoneedles as the secondary structure,the mesoscale hollow plates of the LDH nanoneedle arrays as the tertiary structure,and the macroscale three-dimensional frames of the plate arrays as the quaternary ***,the distinctive structure of NiCo-ZLDH/NF can not only accelerate both mass and charge transfer,but also expose plentiful accessible active sites with high intrinsic activity,endowing it with an excellent electrochemical performance for urea oxidation reaction(UOR).Specially,it only required the low potentials of 1.335,1.368 and 1.388 V to deliver the current densities of 10,100 and 200 mA cm^(-2),respectively,much superior to those for typical *** NiCo-ZLDH/NF as the bifunctional electrode for both anodic UOR and cathodic HER,an energy-saving electrolysis system was further explored which can greatly reduce the needed voltage of 213 mV to deliver the current density of 100 mA cm^(-2),as compared to the conventional water electrolysis system composed of *** work manifests that it is prospective to explore the hierarchically nanostructured electrodes and the innovative electrolytic technologies for high-efficiency electrocatalysis.

关键词： Hierarchical superstructures Metal–organic frameworks Layered double hydroxides Urea oxidation reaction Hydrogen evolution reaction

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Deep-learning architecture for PM_(2.5) concentration prediction: A review

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Environmental Science and Ecotechnology 2024年第5期21卷 17-33页

作者： Shiyun Zhou Wei Wang long zhu Qi Qiao Yulin Kang Institute of Environmental Information Chinese Research Academy of Environmental SciencesBeijing 100012China School of Optics and Photonics Beijing Institute of TechnologyBeijing 100081China College of Water Sciences Beijing Normal UniversityBeijing 100875China

Accurately predicting the concentration of fine particulate matter(PM_(2.5))is crucial for evaluating air pollution levels and public *** advancements have seen a significant rise in using deep learning(DL)models for forecasting PM_(2.5) ***,there is a lack of unified and standardized frameworks for assessing the performance of DL-based PM_(2.5) prediction *** we extensively reviewed those DL-based hybrid models for forecasting PM_(2.5) levels according to the Preferred Reporting Items for Systematic Reviews and Meta-Analyses(PRISMA)*** examined the similarities and differences among various DL models in predicting PM_(2.5) by comparing their complexity and *** categorized PM_(2.5) DL methodologies into seven types based on performance and application conditions,including four types of DL-based models and three types of hybrid learning *** research indicates that established deep learning architectures are commonly used and respected for their ***,many of these models often fall short in terms of innovation and ***,models hybrid with traditional approaches,like deterministic and statistical models,exhibit high interpretability but compromise on accuracy and ***,hybrid DL models,representing the pinnacle of innovation among the studied models,encounter issues with *** introduce a novel three-dimensional evaluation framework,i.e.,Dataset-MethodExperiment Standard(DMES)to unify and standardize the evaluation for PM_(2.5) predictions using DL *** review provides a framework for future evaluations of DL-based models,which could inspire researchers to standardize DL model usage in PM_(2.5) prediction and improve the quality of related studies.

关键词： PM_(2.5)concentration prediction Deep-learning based model Bibliometrics analysis Evaluation framework

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Elemene Antitumor Drugs Development Based on "Molecular Compatibility Theory" and Clinical Application: A Retrospective and Prospective Outlook

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Chinese Journal of Integrative Medicine 2024年第1期30卷 62-74页

作者： JIANG Xiao-ying SHI Li-ping zhu Jun-long BAI Ren-ren XIE Tian School of Pharmacy Hangzhou Normal UniversityHangzhou(311121)China Key Laboratory of Elemene Class Anti-cancer Chinese Medicines Engineering Laboratory of Development and Application of Traditional Chinese MedicinesCollaborative Innovation Center of Traditional Chinese Medicines of Zhejiang ProvinceHangzhou Normal UniversityHangzhou(311121)China Good Clinical Practice Center Affliliated Hospital of Nanjing University of Chinese MedicineNanjing(210000)China

Elemene, derived from Curcuma wenyujin, one of the "8 famous genuine medicinal materials of Zhejiang province," exhibits remarkable antitumor activity. It has gained wide recognition in clinical practice for effectiveness on tumors. Dr. XIE Tian introduced the innovative concept of "molecular compatibility theory" by combining Chinese medicine principles, specifically the "monarch, minister, assistant, and envoy" theory, with modern biomedical technology. This groundbreaking approach, along with a systematic analysis of Chinese medicine and modern biomedical knowledge, led to the development of elemene nanoliposome formulations. These novel formulations offer numerous advantages, including low toxicity, well-defined composition, synergistic effects on multiple targets, and excellent biocompatibility. Following the principles of the "molecular compatibility theory", further exploration of cancer treatment strategies and methods based on elemene was undertaken. This comprehensive review consolidates the current understanding of elemene's potential antitumor mechanisms, recent clinical investigations, advancements in drug delivery systems, and structural modifications. The ultimate goal of this review is to establish a solid theoretical foundation for researchers, empowering them to develop more effective antitumor drugs based on the principles of "molecular compatibility theory".

关键词： molecular compatibility theory Chinese integrative medicine elemene antitumor activity drug delivery structural modification

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Effectiveness of urban distributed runoff model for discharge and water depth calculation in urban drainage pipe networks

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Journal of Hydrodynamics 2024年第3期36卷 582-591页

作者： Yang Zhou Yi-ling Leng Peng-yu Wang Shang-hong Zhang Yu-long zhu Yu-jun Yi School of Water Resources and Hydropower Engineering North China Electric Power UniversityBeijing102206China State Key Laboratory of Water Environment Simulation School of EnvironmentBeijing Normal UniversityBeijing100875China

Effective urban land-use re-planning and the strategic arrangement of drainage pipe networks can significantly enhance urban flood defense *** at reducing the potential risks of urban flooding,this paper presents a straightforward and efficient approach to an urban distributed runoff model(UDRM).The model is developed to quantify the discharge and water depth within urban drainage pipe networks under varying rainfall intensities and land-use *** Nash efficiency coefficient of UDRM exceeds 0.9,which indicates its high computational efficiency and potential benefit in predicting urban *** prediction of drainage conditions under both current and re-planned land-use types is achieved by adopting different flood recurrence *** findings reveal that the re-planned land-use strategies could effectively diminish flood risk upstream of the drainage pipe network across 20-year and 50-year flood recurrence ***,in the case of extreme rainfall events(a 100-year flood recurrence),the re-planned land-use approach fell short of fulfilling the requirements necessary for flood disaster *** these instances,the adoption of larger-diameter drainage pipes becomes an essential requisite to satisfy drainage ***,the proposed UDRM effectively combines land-use information with pipeline data to give practical suggestions for pipeline modification and land-use optimization to combat urban ***,this methodology warrants further promotion in the field of urban re-planning.

关键词： Stormwater runoff water depth urban distributed runoff model urban drainage pipe networks urban land-use re-planning

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Regulating the key performance parameters for Hg-based IR NLO chalcogenides via bandgap engineering strategy

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Chinese Chemical Letters 2024年第10期35卷 490-494页

作者： A-Yang Wang Sheng-Hua Zhou Mao-Yin Ran Xin-Tao Wu Hua Lin Qi-long zhu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of Sciences(CAS)Fuzhou 350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China College of Chemistry Fuzhou UniversityFuzhou 350108China University of Chinese Academy of Sciences Bejing 100049China

Recently,non-centrosymmetric(NCS)Hg-based chalcogenides have garnered significant interest due to their strong second-harmonic-generation intensities(deff),making them attractive candidates for infrared nonlinear optical(IR-NLO)***,achieving both wide band gaps(Eg)and large phasematched deffsimultaneously in these materials remains a challenge due to their inherent constraints on each *** this research,we have successfully obtained two quaternary NCS Hg-based chalcogenides,Rb2HgGe_(3)S_(8)and Cs_(2)HgGe_(3)S_(8),by implementing a bandgap engineering strategy that involves alkali metal introduction and Hg/Ge ratio *** compounds consist of 2D[Hg Ge_(3)S_(8)]_(2)–anionic layers made of 1D[HgGeS_(6)]^(6–)chains and dimeric[Ge_(2)S_(6)]_(4–)polyhedra arranged alternately,and the charge-balanced Rb+/Cs+cations located between these ***,Rb_(2)HgGe_(3)S_(8)and Cs_(2)HgGe_(3)S_(8)exhibit overall properties required for promising IR-NLO materials,including sufficient PM deff(0.55–0.70×AgGaS_(2)@20_(5)0 nm),large Eg(3.27–3.41 e V),giant laser-induced damage thresholds(17.4–19.7×AgGaS_(2)@1064 nm),broad optical transmission intervals(0.32–17.5μm),and suitable theoretical birefringence(0.069–0.086@2050 nm).Furthermore,in-depth theoretical analysis reveals that the exceptional IRNLO performance is attributed to the synergy effects of distorted[HgS_(4)]and[GeS_(4)]*** study provides a useful strategy for enhancing the Eg and advancing Hg-based IR-NLO materials,which is expected to extended and implemented in other chalcogenide systems.

关键词： Hg-based chalcogenides IR nonlinear material Structure-activity relationship Wide energy gap Bandgap engineering strategy

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Hydrogen bond producers in powerful protic ionic liquids for enhancing dissolution of natural cellulose

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SusMat 2024年第5期4卷 189-201页

作者： Shi-Peng Chen Dan-Yang Zhao Jin-long zhu Jing Wang Gan-Ji Zhong Hua-Dong Huang Zhong-Ming Li College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengduChina

The manipulation of hydrogen bonding within protic ionic liquids is conducive to conquering the robust hydrogen bonding interactions in cellulose for its effective dissolution,but it is a great challenge to establish the delicate bal-ance of hydrogen bonding network between solvent and ***,we proposed the concept of“hydrogen bond producers”for urea molecules in 1,1,3,3-tetramethylguanidinium methoxyacetate acid([TMGH][MAA])to enhance the dissolution of *** optimization of physicochemical properties for[TMGH][MAA]solvent as a function of urea concentration revealed a remark-able increase in cellulose solubility from 13%to 17%(w/w)by adding only 0.25 wt%urea,highlighting the efficiency of[TMGH][MAA]as a power-ful solvent for the dissolution of *** experimental and simulation results verified that the significant improvement on dissolution of cellulose was attributed to the hydrogen bonding interaction of urea molecules with ion pairs and part of free ions,reducing the interference with the active ions bonded to ***,the considerable enhancement on compre-hensive properties of regenerated cellulose films demonstrated the effectiveness of[TMGH][MAA]/urea *** concept of“hydrogen bond producers”presented here opens a new avenue for significantly enhancing the dissolu-tion of natural cellulose,promoting the sustainable development in large-scale processing of cellulose.

关键词： cellulose dissolution hydrogen bond producers protic ionic liquids

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Prediction of (n, 2n) reaction cross-sections of long-lived fission products based on tensor model

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NUCLEAR SCIENCE AND TECHNIQUES 2024年第10期35卷 1-14页

作者： Huang, Jia-Li Wang, Hui Huang, Ying-Ge Xiao, Er-Xi Feng, Yu-Jie Lei, Xin Gu, Fu-Chang zhu, long Chen, Yong-Jing Su, Jun Sun Yat Sen Univ Sino French Inst Nucl Engn & Technol Zhuhai 519082 Peoples R China China Inst Atom Energy Key Lab Nucl Data Beijing 102413 Peoples R China China Inst Atom Energy China Nucl Data Ctr Beijing 102413 Peoples R China

Interest has recently emerged in potential applications of (n, 2n) reactions of unstable nuclei. Challenges have arisen because of the scarcity of experimental cross-sectional data. This study aims to predict the (n, 2n) reaction cross-section of long-lived fission products based on a tensor model. This tensor model is an extension of the collaborative filtering algorithm used for nuclear data. It is based on tensor decomposition and completion to predict (n, 2n) reaction cross-sections; the corresponding EXFOR data are applied as training data. The reliability of the proposed tensor model was validated by comparing the calculations with data from EXFOR and different databases. Predictions were made for long-lived fission products such as 60Co, 79Se\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{79}} {\mathrm{Se}}$$\end{document}, 93Zr\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{93}}\mathrm{Zr}$$\end{document}, 107P\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{107}}\mathrm{P}$$\end{document}, 126Sn\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{126}}\mathrm{Sn}$$\end{document}, and 137Cs\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepack

关键词： (n, 2n) Reaction cross-section Tensor model Machine learning Collaborative filtering algorithm Selective transmutation NUCLEAR-DATA TRANSMUTATION N,2N

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Progress in biological research on Tupaia belangeri

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Life Research 2024年第4期7卷 1-8页

作者： Di Zhang Yan Geng Wan-long zhu Department of Pharmacy Yunnan College of Business ManagementKunming 650000China School of Life Sciences Yunnan Normal UniversityKunming 650500China.

Tupaia belangeri,as a typical tropical species,has high value in biological *** has the characteristics of small body size,high brain to body mass ratio,short reproductive cycle,short lifespan,and low maintenance *** biomedical research,experimental animals considered as substitutes for *** review discusses the systematic classification,distribution,and research progress of *** was focus on the research progress,developmental status,and basic biological research in *** that the ***,as the closest species to humans,has many advantages as an experimental animal,and it can be further widely applied in human disease ***,how to create a clear and stable strain of *** with a clear genetic background is crucial for the development of the national economy and scientific research.

关键词： Tupaia belangeri animal models research progress systemic development

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大气压微波放电CO_(2)等离子体温度的发射光谱诊断

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光谱学与光谱分析 2024年第3期44卷 688-692页

作者：李容毅朱海龙山西大学物理电子工程学院山西太原030006

大气压微波等离子体因具有活性粒子密度高、气体温度高、能量转换效率高、可控性好等独特优势,在分解和转化二氧化碳治理环境领域展现出重要的应用价值。以大气压微波等离子体的二氧化碳分解与转化为应用背景,开展了大气压微波等离子体... 详细信息

大气压微波等离子体因具有活性粒子密度高、气体温度高、能量转换效率高、可控性好等独特优势,在分解和转化二氧化碳治理环境领域展现出重要的应用价值。以大气压微波等离子体的二氧化碳分解与转化为应用背景,开展了大气压微波等离子体的放电特性与温度参数的测量和诊断研究。通过研究等离子体炬的放电形态的变化规律,分析了大气压二氧化碳等离子体的放电特点;利用发射光谱的诊断方法,分析了二氧化碳放电区内产生的C_(2)分子的转动温度,得到了二氧化碳等离子体内不同位置在不同功率和不同气体流量下的放电形态以及温度的变化规律。研究结果表明,这种大气压微波等离子体的放电形态呈现明亮的中心放电区和外围的余辉区,且这两个区域存在清晰的边界;放电区的长度随微波功率增加接近线性增长,受送气流量大小的影响微弱。等离子体发射光谱诊断结果显示,大气压微波等离子体放电过程中,主放电区中除了化学荧光连续谱外还存在很强的C_(2)分子的Swan谱带;基于这一谱带计算得到的主放电区等离子体温度约为6 000 K,且这一温度几乎不随功率和气流的变化;不同中心放电区位置,温度略有变化(±100 K)。

关键词：大气压微波放电等离子体转动温度二氧化碳

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高性能内燃机用滤纸的制备及其对性能的影响

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材料导报 2024年第6期38卷 261-266页

作者：马锐金圣楠龙柱朱瑞丰孙昌江南大学造纸研究室江苏无锡214122 江南大学短纤维功能材料研究室江苏无锡214122

采用高强高模聚乙烯(UHMWPE)纤维与针叶木浆混抄,制备具有力学性能高、疏水性好和透气性适当的内燃机用滤纸。通过探讨原纸制备工艺、树脂浸渍和热压工艺对滤纸性能的影响,确定试验条件下的最佳参数,并采用相关手段表征了滤纸的力学性... 详细信息

采用高强高模聚乙烯(UHMWPE)纤维与针叶木浆混抄,制备具有力学性能高、疏水性好和透气性适当的内燃机用滤纸。通过探讨原纸制备工艺、树脂浸渍和热压工艺对滤纸性能的影响,确定试验条件下的最佳参数,并采用相关手段表征了滤纸的力学性能、热稳定性能、孔径大小以及疏水性能。结果表明:在试验条件下,当UHMWPE纤维与针叶木浆的质量比为8∶2、针叶木浆打浆度为22°SR、分散剂PEO和增强剂CPAM相对于绝干浆的质量分数分别为0.5%和0.1%、热压时间为15 min、热压压力为10 MPa、热压温度为140℃时,制备的内燃机用UHMWPE滤纸性能最佳,其中,滤纸抗张指数为50.28 N·m/g,耐破度为503.55 kPa,接触角为123.52°且1 min内不渗透,熔点提高至155℃。

关键词：高强高模聚乙烯(UHMWPE)纤维酚醛树脂热压耐破度滤纸

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