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Boost VS_(2) electrochemical reactive kinetics by regulating crystallographic planes and coupling carbon matrix for high performance sodium-ion storage

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Rare Metals 2024年第1期43卷 98-112页

作者： Min Zeng Ming-Shan Wang Lin Chen En-zhi Li Zhen-Liang Yang dan Zhou Hai-Jiao Xie Jun-Chen Chen zhi-Yuan Ma Bing-Shu Guo Bo Yu Xing Li School of New Energy and Materials Southwest Petroleum UniversityChengdu 610500China Energy Storage Research Institute Southwest Petroleum UniversityChengdu 610500China Institute of Materials China Academy of Engineering PhysicsMianyang 621908China Beijing Advanced Innovation Center for Materials Genome Engineering University of Science and TechnologyBeijingBeijing 100083China Hangzhou Yanqu Information Technology Co. Ltd.Hangzhou 310003China

Vanadium disulfide(VS_(2)) as a typical two-dimensional transition metal chalcogenide has excellent competitiveness for sodium-ion storage due to its wide layer spacing(0.575 nm),high theoretical capacity of 932mAh·g^(-1) originating from multi-electron electrochemical ***,continuous sodiation process accompanied by crystal structural evolution and collapse cause rapid capacity ***,novel few-layer VS_(2)nanosheets with open(001) crystal planes are in-situ constructed on reduced graphene oxide to solve these issues mentioned *** indicates that few-layer VS_(2)provides more Na^(+) storage activity due to the low Na^(+)surface migration energy barrier on exposed crystal(001)*** flexible and high electronic conductivity of carbon matrix also effectively builds multi-level buffer structure and electron transport kinetics to boost the Na^(+)insertion/conversion reactive activity on VS_(2) as well as Na^(+) pseudocapacitance storage kinetics on edges and defects of nano *** coupling effects result in high rate capability and long cycling stability as a battery/capacitor *** delivers conspicuous high energy density of 81 and 40 Wh·kg^(-1) at power density of 118 and 10,286W·kg^(-1),as well as 80% energy retention rate after 5000cycles,confirming its great application potential in sodiumbased storage devices.

关键词： Vanadium disulfide Reduced graphene oxide Anode Sodium-ion battery Sodium-ion capacitor

An arch-shape wood evaporator decorated by metal-organic framework for solar interface evaporation

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Nano Research 2024年第7期17卷 6661-6672页

作者： Tiantian Wu Liming Zhao Yaning xu Ziwei Cui Lixing Kang Yahui Cai Zupeng Chen dan Tian Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037China Key Laboratory of Multifunctional Nanomaterials and Smart Systems Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China College of Materials Science and Engineering Nanjing Forestry UniversityNanjing 210037China

To achieve sustainable desalination and water purification,solar interface evaporation technology is an effective means due to its high energy *** photothermal conversion materials and surface design are crucial for the interfacial solar evaporation *** to design water transport routes and thermal insulating layers simultaneously is one of the major challenges to solar interface evaporation technology ***,this work reports an arch-shaped wood evaporator(pine@carbon black(CB)-metal-organic framework-801(MOF-801)-36%)for efficient,fast and continuous interfacial solar evaporation,which is composed of an arch-shaped wood substrate,MOF-801,and CB as a light absorption *** archshaped structure has a double-sided evaporation effect,which has a synergistic effect on augmenting solar evaporation *** addition,the in-situ growth of MOF-801 in pretreated wood microchannels renders the wood evaporator a significant function of reducing the equivalent enthalpy of evaporation due to the reduction of the hydrogen bonding density of water molecules as they pass through the wood *** best evaporation rate of the arch-shaped wood evaporator can reach 2.535 kg·m^(−2)·h−1,and the efficiency reaches 93.7%under the irradiation of 1 sun ***,it could be used for desalination and wastewater treatment to collect fresh water that meets drinking requirements set by the World Health Organization(WHO).This integrated evaporator provides an efficient way for commercial portable photothermal conversion and new ideas for advanced solar-driven water treatment technology.

关键词： arch-shaped solar evaporation wood metal-organic frameworks(MOFs) double-sided evaporation

Optimized Auxiliary Frequency Control of Wind Farm Based on Piecewise Reduced-order Frequency Response Model

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Journal of Modern Power Systems and Clean Energy 2024年第3期12卷 791-802页

作者： xu Zhang Chen Zhao Junchao Ma Long Zhang dan Sun Chenxu Wang Yan Peng Heng Nian the School of Electrical Engineering Zhejiang UniversityHangzhou 310058China Electric Power Research Institute of State Grid Zhejiang Electric Power Corporation Hangzhou 310014China

With the increasing wind power penetration in the power system,the auxiliary frequency control(AFC)of wind farm(WF)has been widely *** traditional system frequency response(SFR)model is not suitable for the wind power generation system due to its poor accuracy and *** this paper,a piecewise reduced-order frequency response(PROFR)model is proposed,and an optimized auxiliary frequency control(O-AFC)scheme of WF based on the P-ROFR model is ***,a full-order frequency response model considering the change in operating point of wind turbine is established to improve the *** order to simplify the fullorder model,a P-ROFR model with second-order structure and high accuracy at each frequency response stage is *** on the proposed P-ROFR model,the relationship between the frequency response indexes and the auxiliary frequency controller coefficients is expressed ***,an OAFC scheme with the derived explicit expression as the optimization objective is proposed in order to improve the frequency support capability on the premise of ensuring the full release of the rotor kinetic energy and the full use of the effect of time delay on frequency ***,the effectiveness of the proposed P-ROFR model and the performance of the proposed OAFC scheme are verified by simulation studies.

关键词： Frequency response piecewise reduced-order wind farm auxiliary frequency control

Immune states:integrated views of immunity by combining traditional Chinese medicine and modern medicine

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Science China Life Sciences 2024年

作者： Anlong xu Yuxing zhi School of Life Sciences and Qi-Huang School of Chinese Medicine Beijing University of Chinese Medicine School of Life Sciences Sun Yat-sen University

Human immune system is an extraordinarily complex physiological system composed of multiple anatomical systems,diverse tissues and molecules from macroscopic to microscopic level. Numerous cells and molecules collectively participate in immune defense and immune surveillance to maintain homeostasis. More than two thousand years ago, the traditional Chinese medicine(TCM) practitioner has recognized that there are factors in the human body responsible for resisting various exogenous and endogenous pathogens, and referred these factors as“Zheng Qi”(healthy Qi), but referred various pathogenic factors as “Xie Qi”(un-healthy Qi).

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Silencing of peroxiredoxin 2 suppresses proliferation and Wnt/β-catenin pathway,and induces senescence in hepatocellular carcinoma

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Oncology Research 2024年第1期32卷 213-226页

作者： xuEGANG YANG XIANHONG XIANG GUOHUI xu SHI ZHOU TIANzhi AN zhi HUANG Department of Interventional Radiology Sichuan Cancer Hospital and InstituteSichuan Cancer CenterSchool of MedicineUniversity of Electronic Science and Technology of ChinaRadiation Oncology Key Laboratory of Sichuan ProvinceChengdu610041China Department of Interventional Radiology The First Affiliated Hospital of Sun Yat-sen UniversityGuangzhou510080China Department of Interventional Radiology Affiliated Hospital of Guizhou Medical UniversityGuiyang550004China School of Basic Medical Science Guizhou Medical UniversityGuiyang550002China

Hepatocellular carcinoma(HCC),a common malignancy worldwide,still lacks effective clinical *** study aimed to investigate the oncogenes that affect the progression of HCC and their possible *** our study,we initially confirmed a higher level of PRDX2 in the bile of HCC patients compared to those with choledocholithiasis by 2-DE,LC-MS,and ***,we demonstrated the high expression of peroxiredoxin 2(PRDX2)in HCC based on the TCGA database and clinical sample ***,PRDX2 overexpression enhanced the viability of HCC *** PRDX2 silencing induced senescence of HCC *** vivo,knockdown of PRDX2 significantly reduced the weight of xenograft ***2 also was found to activate the Wnt/β-catenin pathway by inducingβ-catenin nuclear ***,we proved that silencing PRDX2 could inhibit proliferation and Wnt/β-catenin pathway while promoting senescence in HCC cells.

关键词： Peroxiredoxin 2 Hepatocellular carcinoma Wnt/β-catenin pathway Senescence Proliferation

Mirizzi syndrome:Problems and strategies

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Hepatobiliary & Pancreatic Diseases International 2024年第3期23卷 234-240页

作者： Jun Wu Shuang-Yong Cai xu-Liang Chen zhi-Tao Chen Shao-Hua Shi Department of Hepatobiliary and Pancreatic Surgery People’s Hospital of Jiulongpo DistrictChongqing 400050China Department of Hepatobiliary and Pancreatic Surgery Shulan(Hangzhou)Hospital Affiliated to Zhejiang Shuren University Shulan International Medical CollegeHangzhou 310003China

Mirizzi syndrome is a serious complication of gallstone *** is caused by the impacted stones in the gallbladder neck or cystic *** of the features of Mirizzi syndrome is severe inflammation or dense fibrosis at the Calot’s *** our clinical practice,bile duct,branches of right hepatic artery and right portal vein clinging to gallbladder infundibulum are often observed due to gallbladder infundibulum adhered to right hepatic *** intraoperative damage of branches of right hepatic artery occurs more easily than that of bile duct,all of which are hidden pitfalls for *** resonance cholangiopancreatography(MRCP)and endoscopic retrograde cholangiopancreatography(ERCP)are the preferable tools for the diagnosis of Mirizzi *** cholecystectomy in Mirizzi syndrome is easy to damage branches of right hepatic artery and bile duct due to gallbladder infundibulum adhered to right hepatic *** cholecystectomy is an easy,safe and definitive approach to Mirizzi *** combined with the application of ERCP,a laparoscopic management of Mirizzi syndrome by well-trained surgeons is feasible and *** objective of this review was to highlight its existing problems:(1)low preoperative diagnostic rate,(2)easy to damage bile duct and branches of right hepatic artery,and(3)high concomitant gallbladder ***,the review aimed to discuss the possible therapeutic strategies:(1)to enhance its preoperative recognition by imaging findings,and(2)to avoid potential pitfalls during surgery.

关键词： Mirizzi syndrome Bile duct injury Artery injury Surgical treatment Subtotal cholecystectomy

Delving into the dissimilarities in electrochemical performance and underlying mechanisms for sodium and potassium ion storage in N-doped carbon-encapsulated metallic Cu_(2)Se nanocubes

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Journal of Energy Chemistry 2024年第8期95卷 336-347,I0008页

作者： Xinyu Wang Yanan xu Xiaofeng Liu Lei Tan Huaiqiang Gu Xin Du dan Li College of Chemistry Zhengzhou UniversityZhengzhou 450001HenanChina Green Catalysis Center College of ChemistryZhengzhou UniversityZhengzhou 450001HenanChina Institute of Theoretical Physics Lanzhou UniversityLanzhou 730000GansuChina School of Nuclear Science and Technology Lanzhou UniversityLanzhou 730000GansuChina Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) College of ChemistryNankai UniversityTianjin 300071China State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046XinjiangChina

The large volumetric variations experienced by metal selenides within conversion reaction result in inferior rate capability and cycling stability,ultimately hindering the achievement of superior electrochemical ***,metallic Cu_(2)Se encapsulated with N-doped carbon(Cu_(2)Se@NC)was prepared using Cu_(2)O nanocubes as templates through a combination of dopamine polymerization and hightemperature *** unique nanocubic structure and uniform N-doped carbon coating could shorten the ion transport distance,accelerate electron/charge diffusion,and suppress volume variation,ultimately ensuring Cu_(2)Se@NC with excellent electrochemical performance in sodium ion batteries(SIBs)and potassium ion batteries(PIBs).The composite exhibited excellent rate performance(187.7 mA h g^(-1)at 50 A g^(-1)in SIBs and 179.4 mA h g^(-1)at 5 A g^(-1)in PIBs)and cyclic stability(246,8 mA h g^(-1)at 10 A g^(-1)in SIBs over 2500 cycles).The reaction mechanism of intercalation combined with conversion in both SIBs and PIBs was disclosed by in situ X-ray diffraction(XRD)and ex situ transmission electron microscope(TEM).In particular,the final products in PIBs of K_(2)Se and K_(2)Se_(3)species were determined after discharging,which is different from that in SIBs with the final species of Na_(2)*** density functional theory calculation showed that carbon induces strong coupling and charge interactions with Cu_(2)Se,leading to the introduction of built-in electric field on heterojunction to improve electron ***,the theoretical calculations discovered that the underlying cause for the relatively superior rate capability in SIBs to that in PIBs is the agile Na~+diffusion with low energy barrier and moderate adsorption *** findings offer theoretical support for in-depth understanding of the performance differences of Cu-based materials in different ion storage systems.

关键词： Cu_(2)Se nanocubes DFT calculations Ion storage mechanism Potassium ion batteries Sodium ion batteries

3D-printed MoS_(2)/Ni electrodes with excellent electro-catalytic performance and long-term stability for dechlorination of florfenicol

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Journal of Environmental Sciences 2024年第3期137卷 420-431页

作者： Jianhui xu Pengxu Wang Shenggui Chen Lei Li dan Li Yunfei Zhang Qi Wu Jinhong Fan LumingMa School of Environment and Civil Engineering Dongguan University of TechnologyDongguan 523808China School of Art and Design Guangzhou Panyu PolytechnicGuangzhou 511483China National Engineering Research Center for Urban Pollution Control State Key Laboratory of Pollution Control and Resources ReuseCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Dongguan Institute of Science and Technology Innovation Dongguan University of TechnologyDongguan 523808China School of Mechanical Engineering Dongguan University of TechnologyDongguan 523808China

Here,we report the production of 3D-printed MoS_(2)/Ni electrodes(3D-MoS_(2)/Ni)with longterm stability and excellent performance by the selective laser melting(SLM)*** a cathode,the obtained 3D-MoS_(2)/Ni could maintain a degradation rate above 94.0%for forfenicol(FLO)when repeatedly used 50 times in *** also found that the removal rate of FLO by 3D-MoS_(2)/Ni was about 12 times higher than that of 3D-printed pure Ni(3D-Ni),attributed to the improved accessibility of H^(*).In addition,the electrochemical characterization results showed that the electrochemically active surface area of the 3D-MoS_(2)/Ni electrode is about 3-fold higher than that of the 3D-Ni electrode while the electrical resistance is 4 times *** on tert-butanol suppression,electron paramagnetic resonance and triple quadrupole mass spectrometer experiments,a“dual path”mechanism and possible degradation pathway for the dechlorination of FLO by 3D-MoS_(2)/Ni were ***,we also investigated the impacts of the cathode potential and the initial pH of the solution on the degradation of ***,this study reveals that the SLM 3D printing technique is a promising approach for the rapid fabrication of high-stability metal electrodes,which could have broad application in the control of water contaminants in the environmental field.

关键词： 3D-print Electroreduction MoS_(2)/Ni Antibiotic Florfenicol

Clinical efficacy of laparoscopic cholecystectomy combined with endoscopic papillary balloon dilation in treatment of gallbladder stones with common bile duct stones: A retrospective study

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World Journal of Gastrointestinal Surgery 2024年第6期16卷 1700-1708页

作者： Hong-dan Liu Qi Zhang Wen-Si xu Shuang Jin Department of Gastroenterology The Third Affiliated Hospital of Qiqihar Medical UniversityQiqihar 161000Heilongjiang ProvinceChina

BACKGROUND The incidence of cholelithiasis has been on the rise in recent years,but the choice of procedure is *** To investigate the efficacy of laparoscopic cholecystectomy(LC)combined with endoscopic papillary balloon dilation(EPBD)in patients with gallbladder stones(GS)with common bile duct stones(CBDS).METHODS The clinical data of 102 patients with GS combined with CBDS were selected for retrospective analysis and divided into either an LC+EPBD group(n=50)or an LC+endoscopic sphincterotomy(EST)group(n=52)according to surgical ***-related indexes,postoperative recovery,postoperative complications,and expression levels of inflammatory response indexes were compared between the two *** Total surgical time,stone free rate,rate of conversion to laparotomy,and successful stone extraction rate did not differ significantly between the LC+EPBD group and LC+EST *** hemorrhage,time to ambulation,and length of hospitalization in the LC+EPBD group were lower than those of the LC+EST group(P<0.05).The rate of total complications of the two groups was 9.80%and 17.65%,respectively,and the difference was not statistically *** serious complications occurred in either *** 48 h postoperatively,the expression levels of interleukin-6,tumor necrosis factor-α,high-sensitivity Creactive protein,and procalcitonin were lower in the LC+EPBD group than in the LC+EST group(P<0.05).At 3 d postoperatively,the expression levels of aspartate transaminase,alanine transaminase,and total bilirubin were lower in the LC+EPBD group than in the LC+EST group(P<0.05).CONCLUSION LC combined with EPBD and LC combined with EST are both effective procedures for the treatment of GS with CBDS,in which LC combined with EPBD is beneficial to shorten the patient’s hospitalization time,reduce the magnitude of elevated inflammatory response indexes,and promote postoperative recovery.

关键词： Gallbladder stone Common bile duct stone Endoscopic papillary balloon dilation Laparoscopic cholecystectomy Endoscopic sphincterotomy