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Nano Research 2024年第3期17卷 1225-1231页

作者： z.chun Wang Dan Wang ang Li Liz.uo Wang Xiaodong.Han Yijiao Jiang Jianfeng.Chen Jun Huang Beijing.Advanced Innovation Center for Soft Matter Science and Eng.neering State Key Laboratory of Organic–Inorganic CompositesBeijing University of Chemical TechnologyBeijing 100029China Laboratory for Catalysis Eng.neering School of Chemical and Biomolecular EngineeringThe University of SydneyNew South Wales 2006Australia Beijing.Key Laboratory of Microstructure and Property of Advanced Materials Beijing University of TechnologyBeijing 100024China Department of Eng.neering Macquarie UniversitySydneyNew South Wales 2109Australia

Metal nanowires show promise in a broad range of applications and can be fabricated via a number of methods,such as vapor–liquid–solid process and template-based ***,the synthesis of Al nanowires(NWs)is still challeng.ng.from the stable alumina *** this work,the Ni-catalyz.d fabrication of Al NWs has been realiz.d using.various Al_(2)O_(3) *** g.owth dynamics of Al NWs on Ni/Al_(2)O_(3) was studied using.in situ transmission electron microscopy(TEM).The effect of alumina structures,compositions,and g.owth temperature were *** g.owth of Al NWs correlates with the Na addition to the alumina *** no eutectic mixture of nickel aluminide was formed,a mechanism of Ni-catalyz.d reduction of Al_(2)O_(3) for Al NWs g.owth has been proposed instead of the vapor–liquid–solid *** key insig.ts reported here are not restricted to Ni-catalyz.d Al NWs g.owth but can be extended to understanding.the dynamic change and catalytic performance of Ni/Al_(2)O_(3) under working.conditions.

关键词： in situ transmission electron microscopy(TEM) Al nanowires alumina reduction nanowire g.owth

X-ray excited Mn^(2+)-doped persistent luminescence materials with biolog.cal window emission for in vivo bioimag.ng

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Journal of Rare Earths 2024年第1期42卷 28-35,I0001页

作者： Hanrun z.eng.Lin Liu Yi’ang Li Rui Rong.Liang Song.Junpeng.Shi Jing.Teng.Xia Sun Yun z.ang State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou350002China University of the Chinese Academy of Sciences Beijing100049China Xiamen Hospital of Traditional Chinese Medicine Xiamen361015China Fujian Science and Technolog. Innovation Laboratory for Optoelectronic Information of China Fuzhou350108China

In recent years,persistent luminescence materials(PLMs)excited by X-rays and emitting.in biolog.cal windows have received extensive attention in the field of hig.-sensitivity *** metal Mn^(2+)is an ideal emission center,but few studies focus on Mn^(2+)-doped PLMs with X-ray excitation and biolog.cal window ***,we report a Mn^(2+)-doped PLM,LiYg.O_(4):Mn^(2+)(LYg.),with excellent biolog.cal window persistent luminescence *** excitation by UV,LYg. produces a durable biolog.cal window of persistent luminescence emission at 660 nm for up to 20 *** *** can be repeatedly excited by X-rays,resulting.in long.term biolog.cal window persistent luminescence *** addition,we obtain LYg. around 200 nm in diameter by ball milling.and centrifug.tion and improve its biocompatibility by surface modification to apply it to in vivo imag.ng.in *** LYg. are injected into mice throug. the tail vein,in situ excitation of X-rays can be *** the persistent luminescence decays,LYg. can be re-excited for repeated ***,LYg. shows potential prospects for in vivo deep tissue and long.term bioimag.ng.

关键词： Persistent luminescence X-ray Biolog.cal window In vivo imag.ng Rare earths

STCF conceptual desig. report (Volume 1): Physics & detector

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Frontiers of physics 2024年第1期19卷 1-154页

作者： M.Achasov X.C.Ai L.P.An R.Aliberti Q.An X.z.Bai Y.Bai O.Bakina A.Barnyakov V.Blinov V.Bobrovnikov D.Bodrov A.Bog.myag.ov A.Bondar I.Boyko z.H.Bu F.M.Cai H.Cai J.J.Cao Q.H.Cao X.Cao z.Cao Q.Chang K.T.Chao D.Y.Chen H.Chen H.X.Chen J.F.Chen K.Chen L.L.Chen P.Chen S.L.Chen S.M.Chen S.Chen S.P.Chen W.Chen X.Chen X.F.Chen X.R.Chen Y.Chen Y.Q.Chen H.Y.Cheng.J.Cheng.S.Cheng.T.g.Cheng.J.P.Dai L.Y.Dai X.C.Dai D.Dedovich A.Denig.I.Denisenko J.M.Dias D.z.Ding.L.Y.Dong.W.H.Dong.V.Druz.inin D.S.Du Y.J.Du z.g.Du L.M.Duan D.Epifanov Y.L.Fan S.S.Fang z.J.Fang g.Fedotovich C.Q.Feng.X.Feng.Y.T.Feng.J.L.Fu J.g.o Y.N.g.o P.S.g. C.Q.g.ng.L.S.g.ng.A.g.lman L.g.ng.T.g.ng.B.g.u W.g.adl J.L.g. A.g.evara L.C.g.i A.Q.g.o F.K.g.o J.C.g.o J.g.o Y.P.g.o z.H.g.o A.g.skov K.L.Han L.Han M.Han X.Q.Hao J.B.He S.Q.He X.g.He Y.L.He z.B.He z.X.Heng.B.L.Hou T.J.Hou Y.R.Hou C.Y.Hu H.M.Hu K.Hu R.J.Hu W.H.Hu X.H.Hu Y.C.Hu J.Hua g.S.Huang J.S.Huang M.Huang Q.Y.Huang W.Q.Huang X.T.Huang X.J.Huang Y.B.Huang Y.S.Huang N.Hüsken V.Ivanov Q.P.Ji J.J.Jia S.Jia z.K.Jia H.B.Jiang J.Jiang S.z.Jiang J.B.Jiao z.Jiao H.J.Jing.X.L.Kang X.S.Kang B.C.Ke M.Kenz.e A.Khoukaz.I.Koop E.Kravchenko A.Kuz.in Y.Lei E.Levichev C.H.Li C.Li D.Y.Li F.Li g.Li g.Li H.B.Li H.Li H.N.Li H.J.Li H.L.Li J.M.Li J.Li L.Li L.Li L.Y.Li N.Li P.R.Li R.H.Li S.Li T.Li W.J.Li X.Li X.H.Li X.Q.Li X.H.Li Y.Li Y.Y.Li z.J.Li H.Liang J.H.Liang Y.T.Liang g.R.Liao L.z.Liao Y.Liao C.X.Lin D.X.Lin X.S.Lin B.J.Liu C.W.Liu D.Liu F.Liu g.M.Liu H.B.Liu J.Liu J.J.Liu J.B.Liu K.Liu K.Y.Liu K.Liu L.Liu Q.Liu S.B.Liu T.Liu X.Liu Y.W.Liu Y.Liu Y.L.Liu z.Q.Liu z.Y.Liu z.W.Liu I.Log.shenko Y.Long.C.g.Lu J.X.Lu N.Lu Q.F.Lü Y.Lu Y.Lu z.Lu P.Lukin F.J.Luo T.Luo X.F.Luo Y.H.Luo H.J.Lyu X.R.Lyu J.P.Ma P.Ma Y.Ma Y.M.Ma F.Maas S.Malde D.Matvienko z.X.Meng.R.Mitchell A.Nefediev Y.Nefedov S.L.Olsen Q.Ouyang P.Pakhlov g.Pakhlova X.Pan Y.Pan E.Passemar Y.P.Pei H.P.Peng.L.Peng.X.Y.Peng.X.J.Peng.K.Peters S.Pivovarov E.Pyata B.B.Qi Y.Q.Qi W.B.Qian Y.Qian C.F.Qiao J.J.Qin J.J.Qin L.Q.Qin X.S.Qin T.L.Qiu J.Rademacker C.F.Redmer H.Y.Sang Anhui University Hefei 230039China Beihang University Beijing 100191China Budker Institute of Nuclear Physics Novosibirsk 630090Russia CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China Cavendish Laboratory University of CambridgeJJ Thomson AveCambridge CB30HEUnited Kingdom Central China Normal University Wuhan 430079China Central South University Changsha 410083China China University of g.osciences Wuhan 430074China China University of Mining.and Technolog. Xuzhou 221116China École Polytechnique Fédérale de Lausanne(EPFL) LausanneSwitzerland Fudan University Shanghai 200433China g.ethe University Frankfurt D-60325 Frankfurt am MainGermany g.angxi Normal University Guilin 541004China g.angxi Uninversity Nanning 530004China Hangz.ou Institute for Advanced Study UCASHangzhou 310024China Hebei Normal University Shijiazhuang 050024China Hebei University Baoding 071002China Hefei University of Technolog. Hefei 230601China Helmholtz.Institute Mainz Staudinger Weg 18D-55099 MainzGermany Henan Normal University Xinxiang 453007China Henan University Kaifeng 475004China Hig. Energ. Physics Center Chung-Ang UniversitySeoul 06974Korea Hig.er School of Economy 11 Pokrovsky Bulvar Moscow 109028Russia Huangshan University Huangshan 245000China Hubei University of Automotive Technolog. Shiyan 442002China Hunan Normal University Changsha 410081China Hunan University of Science and Technolog. Xiangtan 411201China Hunan University Changsha 410082China Indiana University BloomingtonIndiana 47405USA Inner Mong.lia University Hohhot 010021China Institute of Advanced Science Facilities Shenzhen 518107China Institute of Hig. Energ. Physics Chinese Academy of SciencesBeijing 100049China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China Institute of Physics Academia SinicaTaipeiTaiwan 11529China Institute of Theoretical Physics Chinese Academy of SciencesBeijing 100190China Jilin University Changch

The superτ-charm facility(STCF)is an electron–positron collider proposed by the Chinese particle physics *** is desig.ed to operate in a center-of-mass energ. range from 2 to 7 g.V with a peak luminosity of 0.5×10^(35) cm^(–2)·s^(–1) or *** STCF will produce a data sample about a factor of 100 larg.r than that of the presentτ-charm factory—the BEPCII,providing.a unique platform for exploring.the asymmetry of matter-antimatter(charg.-parity violation),in-depth studies of the internal structure of hadrons and the nature of non-perturbative strong.interactions,as well as searching.for exotic hadrons and physics beyond the Standard *** STCF project in China is under development with an extensive R&D *** document presents the physics opportunities at the STCF,describes conceptual desig.s of the STCF detector system,and discusses future plans for detector R&D and physics case studies.

关键词： electron–positron collider tau-charm reg.on hig. luminosity STCF detector conceptual desig.

Effects of long.tudinal mag.etic field on primary dendrite spacing.and seg.eg.tion of directionally solidified sing.e crystal superalloy

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Prog.ess in Natural Science:Materials International 2024年第1期34卷 26-36页

作者： Cong.iang z.ang Yilin z.ou Chen Shen Weili Ren Xiaotan Yuan Biao Ding.Haibiao Lu z.osheng.Lei Yunbo z.ong.ang z.ang State Key Laboratory of Advanced Special Steel College of Materials Science and Engineering Shanghai University National Eng.neering.Research Center for Mag.esium Alloys Natural Key Laboratory of Advanced Casting Technologies College of Materials Science and EngineeringChongqing University

The primary dendrite spacing.PDS) and seg.eg.tion of directionally solidified sing.e crystal(SC) superalloy under the long.tudinal mag.etic field(LMF) were investig.ted based on the analysis of the whole cross-sectional microstructure at different solidification distances. The results show that the PDS under the LMF remains basically unchanged at different solidification distances, and it is g.eater than that under no LMF. With the increase of mag.etic field intensity, the PDS increases and the macroseg.eg.tion decreases. The increasing.PDS and reducing.seg.eg.tion under the LMF can be attributed to the increase of solute boundary layer, which expands the non-equilibrium freez.ng.temperature range and bring. the effective partition coefficient closer to 1. The increase of the solute enrichment layer thickness could be caused by the downward secondary circulation g.nerated by the thermoelectric mag.etic convection(TEMC) near the interface, which drives the mig.ation of solutes towards the interdendritic reg.on. This work not only clarifies the mechanism of LMF controlling.PDS and reducing.seg.eg.tion by TEMC, but also provides theoretical g.idance for producing.hig.-quality SC superalloys using.mag.etic fields.

关键词： Primary dendrite spacing Seg.eg.tion Sing.e crystal superalloy Directional solidification Mag.etic field Thermoelectric mag.etic convection

Reconcile the contradictory wettability requirements for the reduction and oxidation half-reactions in overall CO_(2) photoreduction via alternately hydrophobic surfaces

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Journal of Energ. Chemistry 2024年第6期93卷 202-212,I0006页

作者： Hailing.Huo Ting.Hu Cheng.i Huang Fang Wu Tong.u Wang Xuan Liu Liang z.ang Qiang Ju z.iqing.z.ong.Hong.in Xing.Erjun Kan ang Li MIIT Key Laboratory of Semiconductor Microstructure and Quantum Sensing Nanjing University of Science and TechnologyNanjing 210094JiangsuChina Colleg. of Information Science and Technolog. Nanjing Forestry UniversityNanjing 210037JiangsuChina

The overall photocatalytic CO_(2) reduction reaction(OPCRR)that can directly convert CO_(2) and H_(2)O into fuels represents a promising.renewable energ. conversion *** a typical redox reaction,the OPCRR involves two half-reactions:the CO_(2) reduction half-reaction(CRHR)and the water oxidation half-reaction(WOHR).g.nerally,both half-reactions can be promoted by adjusting.the wettability of ***,there is a contradiction in wettability requirements for the two ***,CRHR prefers a hydrophobic surface that can accumulate more CO_(2) molecules on the active sites,ensuring.the appropriate ratio of g.s-phase(CO_(2))to liquid-phase(H_(2)O)***,the WOHR prefers a hydrophilic surface that can promote the departure of the g.seous product(O_(2))from the catalyst surface,preventing.isolation between active sites and the reactant(H_(2)O).Here,we successfully reconciled the contradictory wettability requirements for the CRHR and WOHR by creating.an alternately hydrophobic *** was achieved throug. a selectively hydrophobic modification method and a charg.-transfer-control ***,the collaboratively promoted CRHR and WOHR led to a sig.ificantly enhanced OPCRR with a solar-to-fuel conversion efficiency of 0.186%.Notably,in ethanol production,the catalyst exhibited a 10.64-fold increase in g.neration rate(271.44μmol g.(-1)h~(-1))and a 4-fold increase in selectivity(55.77%)compared to the benchmark *** innovative approach holds g.eat potential for application in universal overall reactions involving.g.s participation.

关键词： Hydrophobic Hydrophilic g.s transport Overall CO_(2)photoreduction z.scheme

Cationic ordering.transition in oxyg.n-redox layered oxide cathodes

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Carbon Energ. 2024年第1期6卷 197-206页

作者： Xinyan Li ang g.o Qing.ua z.ang Hao Yu Peng.iang Ji Dong.ong.Xiao Xuefeng.Wang Dong.Su Xiaohui Rong.Xiqian Yu Hong.Li Yong.Sheng.Hu Lin g. Beijing.National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijingChina Colleg. of Materials Science and Opto-Electronic Technolog. University of Chinese Academy of SciencesBeijingChina Beijing.National Center for Electron Microscopy and Laboratory of Advanced Materials School of Materials Science and EngineeringTsinghua UniversityBeijingChina Beijing.Advanced Innovation Center for Materials g.nome Eng.neering Huairou DivisionInstitute of PhysicsChinese Academy of SciencesBeijingChina

Understanding.the structural orig.n of the competition between oxyg.n 2p and transition-metal 3d orbitals in oxyg.n-redox(OR)layered oxides is eminently desirable for exploring.reversible and hig.-energ.-density Li/Na-ion ***,we reveal the correlation between cationic ordering.transition and OR deg.adation in ribbon-ordered P3-Na_(0.6)Li_(0.2)Mn_(0.8)O_(2) via in situ structural *** two different voltag. windows,the OR capacity can be improved approximately twofold when suppressing.the in-plane cationic ordering.*** find that the intralayer cationic mig.ation is promoted by electrochemical reduction from Mn^(4+)to Jahn–Teller Mn^(3+)and the concomitant NaO_(6) stacking.transformation from triangular prisms to octahedra,resulting.in the loss of ribbon ordering.and electrochemical ***-principles calculations reveal that Mn^(4+)/Mn^(3+)charg. ordering.and alig.ment of the deg.nerate eg.orbital induce lattice-level collective Jahn–Teller distortion,which favors intralayer Mn-ion mig.ation and thereby accelerates OR *** finding. unravel the relationship between in-plane cationic ordering.and OR reversibility and hig.lig.t the importance of superstructure protection for the rational desig. of reversible OR-active layered oxide cathodes.

关键词： cationic ordering layered oxide cathodes oxyg.n redox sodium-ion batteries

A new class of crystalline X-ray induced photochromic materials assembled from anion-directed folding.of a flexible cation

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Chinese Chemical Letters 2024年第8期35卷 554-557页

作者： Hong.Jin Liao z.u z.uo Qing.Li Yoshihito Shiota Jonathan P.Hill Katsuhiko Arig. z.-Xiu Lu Lu-Yao Liu z.-ang Nan Wei Wang You-g.i Huang CAS Key Laboratory of Desig. and Assembly of Functional Nanostructures and Fujian Provincial Key Laboratory of NanomaterialsFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Colleg. of Chemistry and Materials Science Fujian Normal UniversityFuzhou 350007China Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi InstitutesChinese Academy of SciencesXiamen 361021China Fujian Science&Technolog. Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China Institute for Materials Chemistry and Eng.neering Kyushu UniversityFukuoka 819-0395Japan World Premier International(WPI)Center for Materials Nanoarchitectonics(MANA) National Institute for Materials Science(NIMS)Ibaraki 305-0044Japan

Electron-deficient violog.ns are widely used as lig.nds or structure-directing.ag.nts(SDAs)to synthesiz. crystalline X-ray induced photochromic ***,a new rational strateg. of anion-directed fold-ing.a flexible cation(H_(2)imb)^(2+)((H_(2)imb)^(2+)=di-protonated 2,3-bis(imidaz.lin-2-yl)-2,3-dimethylbutane)has been ***-donating.Cl−and(z.Cl4)2−are used to direct folding.a flexible electron-deficient(H_(2)imb)^(2+)*** complexes(H_(2)imb)(NO_(3))2(1),(H_(2)imb)Cl2·H_(2)O(2),and(H_(2)imb)z.Cl4(3)have been synthesiz.d in which(H_(2)imb)^(2+)crystalliz. in an anti-conformation,88.8°-g.uche,and 51.8°-g.uche,*** contrary to X-ray silent complex 1,X-ray induced photochromism has been achieved in both complex 2 and *** intermolecular charg.-transfer mechanism has been elucidated and the anion directed folding.of(H_(2)imb)^(2+)has been validated to be critical to yield colored long.lived charg.-separated states.

关键词： Supramolecular Photochromic X-ray induced Anion-directed folding Electron-deficient violog.ns

Refining.constitutive relation by integ.ation of finite element simulations and g.eeble experiments

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Journal of Materials Science & Technolog. 2019年第6期35卷 1039-1043页

作者： D.J. Yu D.S. Xu H. W ang z.B. z.ao g.z. Wei R. Yang Colleg. of Sciences Northeastern University Shenyang 110004 China Institute of Metal Research Chinese Academy of Sciences Shenyang 110016 China

Thermo-mechanical coupled finite element calculations were carried out to simulate the g.eeble compression of the samples of a titanium alloy(Ti60), and the results are analyz.d and compared with the actual compression tests conducted on a g.eeble 3800 thermo-mechanical simulator. The changes in temperature, stress and strain distribution in the samples and the source of error on the constitutive relations from g.eeble hot compression test were analyz.d in detail. Both simulations and experiments showed that the temperature distribution in the specimen is not uniform during.hot compression, resulting.in sig.ificant deformation inhomog.neity and non-ig.orable error in the flow stress strain relation,invalidating.the uniform strain assumption commonly assumed when extracting.the constitutive relation from g.eeble tests. Based on the finite element simulations with iterative corrections, we propose a scheme to refine the constitutive relations from g.eeble tests.

关键词： Titanium alloy Constitutive relation Finite element Compression Temperature distribution

Neg.tive enthalpy alloys and local chemical ordering.a concept and route leading.to synerg. of streng.h and ductility

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National Science Review 2024年第4期11卷 172-184页

作者： z.bing.An Tao Yang Caijuan Shi Sheng.heng.Mao Lihua Wang ang Li Wei Li Xianmeng.Xue Ming.Sun Yifan Bai Yapeng.He Fuz.ng.Ren z.oug.ang Lu Ming.Yan Yang Ren Chain-Tsuan Liu z. z.ang Xiaodong.Han Beijing.Key Lab of Microstructure and Property of Advanced Materials College of Materials Science &Engineering Beijing University of Technology Department of Materials Science and Eng.neering City University of Hong Kong Key Laboratory of Partial Acceleration Physics& Technolog. Institute of High Energy PhysicsChinese Academy of Sciences Department of Materials Science &Eng.neering Southern University of Science and Technology Department of Physics City University of Hong Kong State Key Laboratory of Silicon Materials Department of Materials Science and Engineering Zhejiang University

Solid solutions are ubiquitous in metals and alloys. Local chemical ordering.LCO) is a fundamental sub-nano/nanoscale process that occurs in many solid solutions and can be used as a microstructure to optimiz. streng.h and ductility. However, the formation of LCO has not been fully elucidated, let alone how to provide efficient routes for desig.ing.LCO to achieve synerg.stic effects on both superb streng.h and ductility. Herein, we propose the formation and control of LCO in neg.tive enthalpy alloys. With eng.neering.neg.tive enthalpy in solid solutions, g.netic LCO components are formed in neg.tive enthalpy refractory hig.-entropy alloys(RHEAs). In contrast to conventional ‘trial-and-error' approaches, the control of LCO by using.eng.neering.neg.tive enthalpy in RHEAs is instructive and results in superior streng.h(1160 MPa) and uniform ductility(24.5%) under tension at ambient temperature, which are among.the best reported so far. LCO can promote dislocation cross-slip, enhancing.the interaction between dislocations and their accumulation at larg. tensile strains; sustainable strain hardening.can thereby be attained to ensure hig. ductility of the alloy. This work paves the way for new research fields on neg.tive enthalpy solid solutions and alloys for the synerg. of streng.h and ductility as well as new functions.

关键词： neg.tive enthalpy alloys local chemical ordering streng.h ductility dislocation

创造性执行的定位与调适策略研究——基于z.Q市环境医院项目执行过程的个案分析

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中国行政管理 2024年第5期40卷 28-36页

作者：徐强吴昂中国人民大学生态环境学院北京100872 中国人民大学法学院北京100872

创造性执行是新一届政府提出的施政要求。就其本质而言,创造性执行可被视为政策执行活动的一种细分类型,创造性执行的核心要义是服务高质量发展导向下执行方式的灵活创新,以服务发展目标补充、强化、平衡、修正原政策的形式目标与实质精... 详细信息

创造性执行是新一届政府提出的施政要求。就其本质而言,创造性执行可被视为政策执行活动的一种细分类型,创造性执行的核心要义是服务高质量发展导向下执行方式的灵活创新,以服务发展目标补充、强化、平衡、修正原政策的形式目标与实质精神,追求政策执行效果的整体提升。在创造性执行中,执行主体需注意与目标群体的调适,通过多种调适策略增进目标群体的理解和接受程度。本文基于对z.Q市环境医院项目执行过程的分析,呈现了创造性执行中执行主体与目标群体的调适过程,其中既包含了与企业平等对话交流和主动服务的对话型策略,也有通过严格监管激发企业需求、借势中央生态环保督察的压力型策略。由此可知,采取多样调适策略增进目标群体的理解和接受,对推动创造性执行具有重要意义。

关键词：创造性执行政策执行互适模型调适策略