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Journal of Earth Science 2024年第3期35卷 786-796页

作者： Zhengqin Gan Qinglai Feng yuehua wei Guichun Liu Xiaomei Nie Tianyu Zhao State Key Laboratory of Geological Processes and Mineral Resources China University of GeosciencesWuhan 430078China School of Earth Sciences China University of GeosciencesWuhan 430074China

The Changning-Menglian suture zone is a critical tectonic belt pivotal to the evolution of the *** Wenquan Formation,characterized as turbidite deposited on the western side of the Changning-Menglian suture zone as well as the eastern edge of the Baoshan *** of detrital zircons from the Wenquan Formation reveals two significant age peaks approximately at 440 and 980 Ma,with additional age populations around 600,780,and 2500 *** major age peak at about 440 Ma is come from the andesitic-dominant volcanic arc within the Lancang Block and the western Simao Block,corroborated by the presence of andesite fragments in thin section ***,the zircons that form the secondary age peak at~980 Ma and other older age groups probably originate from the Baoshan *** on the western side of the Paleo-Tethyan ophiolites,the Wenquan Formation received detrital materials from the continental margin on the opposite ***,the main Paleo-Tethyan Ocean basin was not sufficiently broad enough to cut off the transference of detrital *** was a relatively narrow basin in the Early Devonian.

关键词： Changning-Menglian suture zone sandstone zircon Paleo-Tethys Devonian tectonics.

哀牢山构造带新元古代双峰式岩浆岩的锆石U-Pb年代学、元素-同位素地球化学特征及构造意义

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大地构造与成矿学 2024年第5期48卷 1148-1166页

作者：苏路路魏月华杨朝刘桂春刘嵘訾建威中国地质大学(武汉)地质过程与矿产资源国家重点实验室湖北武汉430074 云南省地质调查院云南昆明650216 中国地质大学(武汉)地球科学学院湖北武汉430074 John de Laeter Centre Curtin UniversityBentley WA 6102Australia

分布于扬子克拉通西缘的新元古代岩浆岩对研究华南陆块的前寒武纪演化及其与Rodinia超大陆的关系意义重大,但由于该区域后期构造-热历史的复杂性,关于一些重要岩石单元的时代、属性和构造背景仍存在诸多争议。本文聚焦哀牢山构造带南段... 详细信息

分布于扬子克拉通西缘的新元古代岩浆岩对研究华南陆块的前寒武纪演化及其与Rodinia超大陆的关系意义重大,但由于该区域后期构造-热历史的复杂性,关于一些重要岩石单元的时代、属性和构造背景仍存在诸多争议。本文聚焦哀牢山构造带南段的桃家寨岩体,报道了来自该岩体的一套变基性岩和钠长花岗岩组合的年代学和地球化学组成,以期为解决现存争议提供新的证据和约束。SHRIMP原位锆石U-Pb同位素测年表明变基性岩和钠长花岗岩的结晶年龄分别为756±9 Ma和763±23 Ma,表明二者为同期岩浆作用的产物,其合并加权平均年龄759±7 Ma(MSWD=0.88,n=8)代表了岩浆事件年龄;同时,来自两件样品的锆石都记录了~730 Ma的岩浆后热扰动事件。变基性岩具有低碱(Na2O+K2O=0.17%~0.36%),高Mg#(76~79)的地球化学特征,略富集轻稀土元素(LREEs),并具有弱的Nb-Ta负异常和正的ε_(Nd)(t)值(+2.67~+3.10),表明其来自E-MORB型富集地幔岩浆源区,可能经历了俯冲板片流体或者熔体的改造。钠长花岗岩显示高碱(Na_(2)O+K_(2)O=6.70%~8.30%)、富集LREEs和大离子亲石元素(LILEs)、亏损重稀土元素(HREEs)等特点,具有负的ε_(Nd)(t)值(-2.43~-1.26),表明其母岩浆可能源自下地壳物质部分熔融与基性熔体的混合。综合前人研究,发现桃家寨岩体的岩石组合具有双峰式特点,并在地球化学特征上显示典型的弧-弧后盆地属性;岩浆作用峰期~760 Ma,指示其为新元古代扬子克拉通西缘的洋陆俯冲构造体系的一部分,从而为将华南陆块置于Rodinia外围的超大陆重建模式提供了新的证据。

关键词：哀牢山构造带桃家寨岩体新元古代双峰式岩浆岩 SHRIMP锆石U-Pb年代学地球化学

Tethyan evolution from early Paleozoic to early Mesozoic in southwest Yunnan

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Science China Earth Sciences 2023年第12期66卷 2728-2750页

作者： Qinglai FENG Guichun LIU Zhengqin GAN Tianyu ZHAO Jianwei ZI yuehua wei State Key Laboratory of Geological Processes and Mineral Resources China University of GeosciencesWuhan 430074China School of Earth Science China University of GeosciencesWuhan 430074China Yunnan Institute of Geological Survey Kunming 650216China John de Laeter Centre Curtin UniversityPerth WA 6102Australia

The Tethys orogenic belt in SW Yunnan constitutes a critical part of the expansive Tethys-Himalayan tectonic *** abundant,well-preserved geologic records make it an ideal area for studying the tectonic evolution of Proto-and *** this paper,we focus on several major tectonic units in SW Yunnan and reconstruct the Tethyan evolution from the early Paleozoic to the early Mesozoic,based on stratigraphic,sedimentologic,and magmatic *** recently discovered early Paleozoic Yunxian-Menghai ophiolitic belt in the Lincang Terrane situated east of the Changning-Menglian Belt represents the suture zone of the *** oceanic basin of Proto-Tehtys opened in the latest Neoproterozoic and subsequently began subducting in the late Miaolingian of the Cambrian(about 505 Ma).From the late Late Ordovician to the ealiest Silurian(about 450–442 Ma),the Proto-Tethys basin gradually closed resulting in the collision of the continental plates on both sides of the Proto-Tethyan *** main collision stage occurred in the early Silurian(about 442–430 Ma)and the postcollision stage lasted from the mid-Silurian to the early Carboniferous(430–355 Ma).The earliest record of Paleo-Tethyan oceanic crust was generated in the late Devonian,and the ocean was then subducted in an eastward direction in the middle Late Carboniferous(about 310 Ma).The initial collision stage in the Paleo-Tethys took place at the end of the Permian(about 253Ma),and the main stage of the collision persisted into the early Ladinian(about 253–238 Ma).This was followed by postcollision extension from the late Ladinian to the early Jurassic(ca.238–196 Ma).We suggest that the opening of Paleo-Tethyan Ocean in SW Yunnan was a result of the extensional rift basin of the ***,the activity of the Manxin mantle plume was likely a crucial factor in the rapid expansion of the Paleo-Tethyan Ocean.

关键词： Historical tectonics Stratigraphic sequence Proto-Tethys Paleo-Tethys Tectonic evolution SW Yunnan

Highly anisotropic thermal conductivity of few-layer CrOCl for efficient heat dissipation in graphene device

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Nano Research 2022年第10期15卷 9377-9385页

作者： Xiaoming Zheng yuehua wei Zhenhua wei wei Luo Xiao Guo Xiangzhe Zhang Jinxin Liu Yangbo Chen Gang Peng weiwei Cai Shiqiao Qin Han Huang Chuyun Deng Xueao Zhang College of Physical Science and Technology Xiamen UniversityXiamen 361005China College of Advanced Interdisciplinary Studies National University of Defense TechnologyChangsha 410073China College of Arts and Sciences National University of Defense TechnologyChangsha 410073China Hunan Key Laboratory of Super-microstructure and Ultrafast Process School of Physics and ElectronicsCentral South UniversityChangsha 410083China Jiujiang Research Institute of Xiamen University Jiujiang 332105China

With the packing density growing continuously in integrated electronic devices,sufficient heat dissipation becomes a serious ***,dielectric materials with high thermal conductivity have brought insight into effective dissipation of waste heat in electronic devices to prevent them from overheating and guarantee the performance *** CrOCl,an antiferromagnetic insulator with low-symmetry crystal structure and atomic level flatness,might be a promising solution to the thermal ***,we have systematically studied the thermal transport of suspended few-layer CrOCl flakes by microRaman *** CrOCl flakes exhibit high thermal conductivities along zigzag direction,from~392±33 to~1,017±46 W·m^(−1)·K^(−1) with flake thickness from 2 to 50 ***,pronounced thickness-dependent thermal conductivity ratio(/from~2.8±0.24 to~4.3±0.25)has been observed in the CrOCl flakes,attributed to the discrepancy of phonon dispersion and phonon surface *** a demonstration to the heat sink application of layered CrOCl,we then investigate the energy dissipation in graphene devices on CrOCl,SiO_(2) and hexagonal boron nitride(h-BN)substrates,*** graphene device temperature rise on CrOCl is only 15.4%of that on SiO_(2) and 30%on h-BN upon the same electric power density,indicating the efficient heat dissipation of graphene device on *** study provides new insights into two-dimentional(2D)dielectric material with high thermal conductivity and strong anisotropy for the application of thermal management in electronic devices.

关键词： CrOCl High thermal conductivity strong anisotropy efficient heat dissipation heat sink graphene devices

Highly in-plane anisotropy of thermal transport in suspended ternary chalcogenide Ta_(2)NiS_(5)

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Nano Research 2022年第7期15卷 6601-6606页

作者： Yue Su Chuyun Deng Jinxin Liu Xiaoming Zheng yuehua wei Yangbo Chen wei Yu Xiao Guo weiwei Cai Gang Peng Han Huang Xueao Zhang College of Physical Science and Technology Xiamen UniversityXiamen 361005China College of Arts and Sciences National University of Defense TechnologyChangsha 410073China College of Advanced Interdisciplinary Studies National University of Defense TechnologyChangsha 410073China Jiujiang Research Institute of Xiamen University Jiujiang 332105China Hunan Key Laboratory of Super-microstructure and Ultrafast Process School of Physics and ElectronicsCentral South UniversityChangsha 410083China Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of SciencesBeijing 100190China

Energy dissipation has always been an attention-getting issue in modern electronics and the emerging low-symmetry two-dimensional(2D)materials are considered to have broad prospects in solving the energy dissipation *** the thermal transport of a typical 2D ternary chalcogenide Ta_(2)NiS_(5) is *** the first time we have observed strongly anisotropic in-plane thermal conductivity towards armchair and zigzag axes of suspended few-layer Ta_(2)NiS_(5) flakes through Raman *** 7-nm-thick Ta_(2)NiS_(5) flakes,theκz i g z a g is 4.76 W·m^(−1)·K^(−1) andκa r m c h a i r is 7.79 W·m^(−1)·K^(−1),with a large anisotropic ratio(κa r m c h a i r/κz i g z a g)of 1.64 mainly ascribed to different phonon mean-free-paths along armchair and zigzag ***,the thickness dependence of thermal anisotropy is also *** the flake thickness increases,theκa r m c h a i r/κz i g z a g reduces sharply from 1.64 to *** could be attributed to the diversity in phonon boundary scattering,which decreases faster in zigzag direction than in armchair *** anisotropic property enables heat flow manipulation in Ta_(2)NiS_(5) based devices to improve thermal management and device *** work helps reveal the anisotropy physics of ternary transition metal chalcogenides,along with significant guidance to develop energy-efficient next generation nanodevices.

关键词： anisotropic thermal conductivity ternary transition metal chalcogenide Ta_(2)NiS_(5) energy dissipation phonon mode

Enormous enhancement in electrical performance of few-layered MoTe2 due to Schottky barrier reduction induced by ultraviolet ozone treatment

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Nano Research 2020年第4期13卷 952-958页

作者： Xiaoming Zheng Xueao Zhang yuehua wei Jinxin Liu Hang Yang Xiangzhe Zhang Shitan Wang Haipeng Xie Chuyun Deng Yongli Gao Han Huang Hunan Key Laboratory of Super-microstructure and Ultrafast Process School of Physics and ElectronicsCentral South UniversityChangsha 410083China College of Arts and Science National University of Defense TechnologyChangsha 410073China College of Physical Science and Technology Xiamen UniversityXiamen 361005China Department of Physics and Astronomy University of RochesterRochesterNY 14627USA

Doping can improve the band alignment at the metal-semiconductor interface to modify the corresponding Schottky barrier,which is crucial for the realization of high-performance logic ***,we systematically investigated a convenient and effective method,ultraviolet ozone treatment,for p-type doping of MoTe2 field-effect transistors to enormously enhance the corresponding electrical *** resulted hole concentration and mobility are near 100 times enhanced to be〜1.0×10^13 cm^-2 and 101.4 cm^2/(V·s),respectively,and the conductivity is improved by 5 orders of *** values are comparable to the highest ones ever obtained via annealing doping or non-lithographic fabrication methods at room *** with the pristine one,the photoresponsivity(522 mA/W)is enhanced approximately 100 *** excellent performances can be attributed to the sharply reduced Schottky barrier because of the surface charge transfer from MoTe2 to MoOx(x<3),as proved by photoemission ***,the p-doped devices exhibit excellent stability in ambient *** findings show significant potential in future nanoelectronic and optoelectronic applications.

关键词： MoTe2 ultraviolet ozone surface charge transfer Schottky barrier air stable hole doping

Non-radical activation of persulfate with Bi_(2)O_(3)/BiO_(1.3)I_(0.4)for efficient degradation of propranolol under visible light

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Journal of Environmental Sciences 2024年第8期142卷 57-68页

作者： yuehua Deng Qianqian Che Yani Li Jiating Luo Xiang Gao Yan He Yiling Liu Tong Liu Xiaolong Zhao Xiaobin Hu wei Zhao College of Geology and Environment Xi’an University of Science and TechnologyXi’an 710054China Shaanxi Provincial Key Laboratory of Geological Support for Coal Green Exploitation Xi’an 710054China Department of Mechanical Engineering The University of Hong KongHong Kong 999077China School of Life Science Huzhou UniversityHuzhou 313000China School of Materials Engineering Changshu Institute of TechnologyChangshu 215500China

Non-radical activation of persulfate(PS)by photocatalysts is an effective approach for removing organic pollutants from aqueous *** this study,a novel Bi_(2)O_(3)/BiO_(1.3)I_(0.4)heterojunction was synthesized using a facile solvothermal approach and used for the first time for non-radical activation of PS to degrade propranolol(PRO)in the presence of visible *** findings found that the degradation rate of PRO in the Bi_(2)O_(3)/BiO_(1.3)I_(0.4)/PS system was significantly increased from 19%to more than 90%within 90 min compared to the Bi_(2)O_(3)/BiO_(1.3)I_(0.4)*** indicated that the composite system exerted an excellent synergistic effect between the photocatalyst and the persulfate-based *** tests and electron paramagnetic resonance demonstrated that the non-radical pathway with singlet oxygen as the active species played a major role in the photocatalytic *** existence of photo-generated holes during the reaction could also be directly involved in the oxidation of ***,a possible PRO degradation pathway was also ***,the impacts of pH,humic acid and common anions on the PRO degradation by the Bi_(2)O_(3)/BiO_(1.3)I_(0.4)/PS were explored,and the system’s stability and reusability were also *** study exhibits a highly productive catalyst for PS activation via a non-radical pathway and provides a new idea for the degradation of PRO.

关键词： Iodine deficiency Heterojunction Persulfate(PS) Propranolol(PRO) Photocatalytic degradation

Multiple-dimensioned defect engineering for graphite felt electrode of vanadium redox flow battery

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Carbon Energy 2024年第2期6卷 143-153页

作者： Yingqiao Jiang Yinhui Wang Gang Cheng yuehua Li Lei Dai Jing Zhu wei Meng Jingyu Xi Ling Wang Zhangxing He School of Chemical Engineering North China University of Science and TechnologyTangshanChina Tsinghua Shenzhen International Graduate School Institute of Materials ResearchTsinghua UniversityShenzhenChina

The scarcity of wettability,insufficient active sites,and low surface area of graphite felt(GF)have long been suppressing the performance of vanadium redox flow batteries(VRFBs).Herein,an ultra-homogeneous multipledimensioned defect,including nano-scale etching and atomic-scale N,O codoping,was used to modify GF by the molten salt ***_(4)Cl and KClO_(3) were added simultaneously to the system to obtain porous N/O co-doped electrode(GF/ON),where KClO_(3) was used to ultra-homogeneously etch,and O-functionalize electrode,and NH4Cl was used as N dopant,***/ON presents better electrochemical catalysis for VO_(2)+/VO_(2)+ and V3+/V2+ reactions than only O-functionalized electrodes(GF/O)and *** enhanced electrochemical properties are attributed to an increase in active sites,surface area,and wettability,as well as the synergistic effect of N and O,which is also supported by the density functional theory ***,the cell using GF/ON shows higher discharge capacity,energy efficiency,and stability for cycling performance than the pristine cell at 140 mA cm^(−2) for 200 ***,the energy efficiency of the modified cell is increased by 9.7% from 55.2% for the pristine cell at 260 mA cm^(−2).Such an ultra-homogeneous etching with N and O co-doping through“boiling”molten salt medium provides an effective and practical application potential way to prepare superior electrodes for VRFB.

关键词： graphite felt molten salt N O co-doping ultra-homogeneous etching vanadium redox flow battery

Bi_(2)O_(3)/g-C_(3)N_(4)hollow core–shell Z-scheme heterojunction for photocatalytic uranium extraction

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Nano Research 2024年第7期17卷 5845-5855页

作者： Hao Fu yuehua Pan Zhenyu Cai Yuxiang Deng Minchen Hou Yuezhou wei Toyohisa Fujita Shunyan Ning Youbin Wang Shaolong Zhang Xinpeng Wang School of Chemistry&Chemical Engineering Guangxi UniversityNanning 530004China School of Resources Environment and MaterialsGuangxi UniversityState Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite StructuresNanning 530004China College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060China School of Materials Sun Yat-sen UniversityShenzhen 518107China School of Nuclear Science and Technology University of South ChinaHengyang 421001China

Photocatalytic uranium extraction from radioactive nuclear wastewater and seawater is critical for promoting the sustainable advancement of nuclear industry,but the complexity of real-world environments,particularly the occurrence of anoxic and oxygen-enriched states,presents significant challenges to effective uranium ***,a layered hollow core–shell structure of Bi_(2)O_(3)/g-C_(3)N_(4)Z-scheme heterojunction photocatalyst has been designed and successfully applied for photocatalytic uranium extraction in both aerobic and oxygen-free conditions,and the extraction efficiency of uranium can reach 98.4%and 99.0%,***,the photocatalyst still has ultra-high extraction efficiency under the influence of pH,inorganic ions,and other *** exceptional capability for uranium extraction is on the one hand due to the distinctive hollow core–shell architecture,which furnishes an abundant quantity of active *** the other hand,benefiting from the suitable band gap structure brought by the construction of Z-scheme heterojunction,Bi_(2)O_(3)/g-C_(3)N_(4)exhibits current densities(1.00μA/cm^(2))that are 5.26 and 3.85 times greater than Bi_(2)O_(3)and g-C_(3)N_(4),respectively,and the directional migration mode of Z-scheme carriers significantly prolongs the lifetime of photogenerated charges(1.53 ns),which separately surpass the pure samples by factors of 5.10 and ***,the reaction mechanism and reaction process of photocatalytic uranium extraction are investigated in the presence and absence of oxygen,respectively.

关键词： Bi_(2)O_(3)/g-C_(3)N_(4) Z-scheme photocatalytic uranium extraction

Plasma microRNA-15a/16-1-based machine learning for early detection of hepatitis B virus-related hepatocellular carcinoma

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