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Low-Temperature Fabrication of Stable Black-Phase CsPbI₃ Perovskite Flexible Photodetectors Toward Wearable Health Monitoring

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NANO-MICRO LETTERS 2025年第1期17卷 1-14页

作者： Zhao, Yingjie Sun, Yicheng Pei, Chaoxin Yin, Xing Li, Xinyi Hao, Yi Zhang, Mengru Yuan, Meng Zhou, Jinglin Chen, Yu song, Yanlin Zhengzhou Univ Coll Chem Zhengzhou 450001 Peoples R China Zhengzhou Univ Pingyuan Lab Zhengzhou 450001 Peoples R China Chinese Acad Sci Inst Chem Key Lab Green Printing Beijing 100190 Peoples R China Chinese Acad Sci Tech Inst Phys & Chem Key Lab Bioinspired Mat & Interfacial Sci Beijing 100190 Peoples R China Chinese Acad Sci Inst High Energy Phys Beijing 100049 Peoples R China

Low-temperature fabrication of black-phase CsPbI3 perovskite films is first demonstrated by using diphenylphosphinic chloride additive under 30-50 degrees C, arising from the steric effect and chloride insertion ***-area high-quality all-inorganic perovskite films with fewer defects enhanced crystallographic orientation, and excellent environmental stability is *** record performances are demonstrated for flexible wearable photodetectors with a responsivity of 42.1 A W-1, a detectivity of 1.3 x 1014 Jones, high-fidelity image, photoplethysmography sensor functions, and high mechanical stability. Flexible wearable optoelectronic devices fabricated from organic-inorganic hybrid perovskites significantly accelerate the development of portable energy, biomedicine, and sensing fields, but their poor thermal stability hinders further applications. Conversely, all-inorganic perovskites possess excellent thermal stability, but black-phase all-inorganic perovskite film usually requires high-temperature annealing steps, which increases energy consumption and is not conducive to the fabrication of flexible wearable devices. In this work, an unprecedented low-temperature fabrication of stable black-phase CsPbI3 perovskite films is demonstrated by the in situ hydrolysis reaction of diphenylphosphinic chloride additive. The released diphenyl phosphate and chloride ions during the hydrolysis reaction significantly lower the phase transition temperature and effectively passivate the defects in the perovskite films, yielding high-performance photodetectors with a responsivity of 42.1 A W-1 and a detectivity of 1.3 x 1014 Jones. Furthermore, high-fidelity image and photoplethysmography sensors are demonstrated based on the fabricated flexible wearable photodetectors. This work provides a new perspective for the low-temperature fabrication of large-area all-inorganic perovskite flexible optoelectronic devices.

关键词： In situ hydrolyzation Low-temperature processing All-inorganic perovskite Flexible photodetectors Health monitoring

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A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three‑Dimensionally Conductive MOF Network for Gas and Pressure Sensing

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Nano-Micro Letters 2025年第2期17卷 601-620页

作者： Qingqing Zhou Qihang Ding Zixun Geng Chencheng Hu Long Yang Zitong Kan Biao Dong Miae Won Hongwei song Lin Xu Jong Seung Kim State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012People’s Republic of China Department of Chemistry Korea UniversitySeoul 02841Republic of Korea TheranoChem Incorporation Seoul 02856Republic of Korea

The rising flexible and intelligent electronics greatly facilitate the noninvasive and timely tracking of physiological information in telemedicine *** building bionic-sensitive moieties is vital for designing efficient electronic skin with advanced cognitive functionalities to pluralistically capture external ***,realistic mimesis,both in the skin’s three-dimensional interlocked hierarchical structures and synchronous encoding multistimuli information capacities,remains a challenging yet vital need for simplifying the design of flexible logic ***,we construct an artificial epidermal device by in situ growing Cu_(3)(HHTP)_(2) particles onto the hollow spherical Ti_(3)C_(2)T_(x) surface,aiming to concurrently emulate the spinous and granular layers of the skin’s *** bionic Ti_(3)C_(2)T_(x)@Cu_(3)(HHTP)_(2) exhibits independent NO_(2) and pressure response,as well as novel functionalities such as acoustic signature perception and Morse code-encrypted message ***,a wearable alarming system with a mobile application terminal is self-developed by integrating the bimodular senor into flexible printed *** system can assess risk factors related with asthmatic,such as stimulation of external NO_(2) gas,abnormal expiratory behavior and exertion degrees of fingers,achieving a recognition accuracy of 97.6%as assisted by a machine learning *** work provides a feasible routine to develop intelligent multifunctional healthcare equipment for burgeoning transformative telemedicine diagnosis.

关键词： Ti_(3)C_(2)T_(x)@Cu_(3)(HHTP)_(2)composites NO_(2)/pressure flexible sensors Health-monitoring Machine learning

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De novo synthesis of atropisomeric benzofurans via Cu/SPDO complex catalyzed asymmetric formal [3 + 2] annulation

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Science China Chemistry 2025年第1期 174-180页

作者： Fan-Xiao Meng Xing-Yu Wang Ka Lu Ju-song Yang Fu-Min Zhang Ai-Jun Ma Bao Du Yong-Qiang Tu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical Engineering Lanzhou University School of Chemistry and Chemical Engineering Shanghai Jiao Tong University School of Biotechnology and Health Sciences Wuyi University

Herein, the de novo synthesis of atropisomeric benzofurans through the Cu/spirocyclic-pyrrolidine-oxazoline(SPDO) complex catalyze asymmetric formal [3 + 2] cycloaddition between quinones and ynamides is explored, producing a range of structurally diverse axially chiral benzofurans in satisfactory yields with good to excellent enantioselectivities. Furthermore, density functional theory calculations were applied to explain the possible reaction mechanism.

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Multi-Task Learning Using Attention-Based Convolutional Encoder-Decoder for Dilated Cardiomyopathy CMR Segmentation and Classification

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Computers, Materials & Continua 2020年第5期63卷 995-1012页

作者： Chao Luo Canghong Shi Xiaojie Li Xin Wang yucheng Chen Dongrui Gao Youbing Yin Qi song Xi Wu Jiliu Zhou 无 College of Computer Science Chengdu University of Information TechnologyChengdu610000China College of Information Science and Technology Southwest Jiaotong UniversityChengdu610000China West China Hospital Sichuan UniversityChengdu610000China AI Institute CuraCloud CorporationSeattle98101USA

Myocardial segmentation and classification play a major role in the diagnosis of cardiovascular *** Cardiomyopathy(DCM)is a kind of common chronic and life-threatening *** diagnostics significantly increases the chances of correct treatment and ***,accurate and rapid diagnosis of DCM is still challenge due to high variability of cardiac structure,low contrast cardiac magnetic resonance(CMR)images,and intrinsic noise in synthetic CMR images caused by motion artifact and cardiac ***,visual assessment and empirical evaluation are widely used in routine clinical diagnosis,but they are subject to high inter-observer variability and are both subjective and *** solve this problem,we proposed an effective unified multi-task framework for dilated cardiomyopathy CMR segmentation and classification simultaneously,and we firstly update one independent encoder from both recovery decoder and parallel attention path sharing some partial *** can encode both task choices into good embedding,but each one can achieve significant improvements respectively from the given *** consists of three branches:extraction path,attention path,and recovery path,which allows the model to learn more higher-level intermediate representations and makes a more accurate *** validated our approach on a DCM dataset,which contains 1155 CMR LGE *** results show that our multi-task network has achieved accuracy of 97.63%,AUC of 98.32%,demonstrating effectively segmenting the myocardium,quickly and accurately diagnosing the presence or absence of dilation.

关键词： Dilated cardiomyopathy multitasking network attention classification segmentation

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Infiltration by monocytes of the central nervous system and its role in multiple sclerosis: reflections on therapeutic strategies

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Neural Regeneration Research 2025年第3期20卷 779-793页

作者： Guangyong Zhang Qing Yao Chubing Long Pengcheng Yi Jiali song Luojia Wu Wei Wan Xiuqin Rao Yue Lin Gen Wei Jun Ying Fuzhou Hua Department of Anesthesiology the Second Affiliated Hospital of Nanchang UniversityNanchangJiangxi ProvinceChina Key Laboratory of Anesthesiology of Jiangxi Province NanchangJiangxi ProvinceChina

Mononuclear macrophage infiltration in the central nervous system is a prominent feature of neuroinflammation. Recent studies on the pathogenesis and progression of multiple sclerosis have highlighted the multiple roles of mononuclear macrophages in the neuroinflammatory process. Monocytes play a significant role in neuroinflammation, and managing neuroinflammation by manipulating peripheral monocytes stands out as an effective strategy for the treatment of multiple sclerosis, leading to improved patient outcomes. This review outlines the steps involved in the entry of myeloid monocytes into the central nervous system that are targets for effective intervention: the activation of bone marrow hematopoiesis, migration of monocytes in the blood, and penetration of the blood–brain barrier by monocytes. Finally, we summarize the different monocyte subpopulations and their effects on the central nervous system based on phenotypic differences. As activated microglia resemble monocyte-derived macrophages, it is important to accurately identify the role of monocyte-derived macrophages in disease. Depending on the roles played by monocyte-derived macrophages at different stages of the disease, several of these processes can be interrupted to limit neuroinflammation and improve patient prognosis. Here, we discuss possible strategies to target monocytes in neurological diseases, focusing on three key aspects of monocyte infiltration into the central nervous system, to provide new ideas for the treatment of neurodegenerative diseases.

关键词： blood–brain barrier macrophages monocytes multiple sclerosis neuroinflammation review therapy

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3WF-1300型悬挂式喷杆喷雾机的设计与试验

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农机化研究 2025年第3期47卷 77-81页

作者：李存斌梁玉成张庆柱陈宝昌谢宇峰吕海杰宋秋梅黑龙江省农业机械工程科学研究院哈尔滨150081

针对我国目前大田喷雾机仍以中小型机具为主,产品技术含量相对较低,使用可靠性差,施药过程存在雾滴飘移、喷洒不均匀、农药有效利用率低等问题,在分析悬挂式喷杆喷雾机工作原理的基础上设计并研制了一种高效、安全的3WF-1300型悬挂式喷... 详细信息

针对我国目前大田喷雾机仍以中小型机具为主,产品技术含量相对较低,使用可靠性差,施药过程存在雾滴飘移、喷洒不均匀、农药有效利用率低等问题,在分析悬挂式喷杆喷雾机工作原理的基础上设计并研制了一种高效、安全的3WF-1300型悬挂式喷杆喷雾机。该机配套动力为88.2~117.6 kW,药箱容量1 300 L,喷幅18 m,可液压控制喷杆折叠、展开和升降,有效降低了驾驶人员的操控难度,能够实现舒适、精准、高效的农药喷施作业,提高了农药有效利用率、降低了农药施用量、减少了环境污染,极大地保护了操控人员的身体健康。田间试验结果表明:喷雾机结构参数设计合理,喷杆的折叠、展开和升降过程平稳顺滑,无卡顿现象;喷雾均匀,作业效率高,达到了设计指标的要求;田间试验中,沿喷杆方向喷雾分布变异系数为5.3%,结果优于国家标准。

关键词：喷杆式喷雾机折叠喷杆悬挂机构升降机构

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Staphylococcus aureus and biofilms:transmission, threats, and promising strategies in animal husbandry

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Journal of Animal Science and Biotechnology 2024年第4期15卷 1408-1423页

作者： Mengda song Qi Tang Yakun Ding Peng Tan yucheng Zhang Tao Wang Chenlong Zhou Shenrui Xu Mengwei Lyu Yueyu Bai Xi Ma State Key Laboratory of Animal Nutrition and Feeding College of Animal Science and TechnologyChina Agricultural UniversityBeijing 100193China Key Laboratory of Innovative Utilization of Local Cattle and Sheep Germplasm Resources(Co‑Construction by Ministry and Province) Ministry of Agriculture and Rural AffairsSchool of Agricultural SciencesZhengzhou UniversityZhengzhou 450001China

Staphylococcus aureus(S. aureus) is a common pathogenic bacterium in animal husbandry that can cause diseases such as mastitis, skin infections, arthritis, and other ailments. The formation of biofilms threatens and exacerbates S. aureus infection by allowing the bacteria to adhere to pathological areas and livestock product surfaces, thus triggering animal health crises and safety issues with livestock products. To solve this problem, in this review, we provide a brief overview of the harm caused by S. aureus and its biofilms on livestock and animal byproducts(meat and dairy products). We also describe the ways in which S. aureus spreads in animals and the threats it poses to the livestock industry. The processes and molecular mechanisms involved in biofilm formation are then explained. Finally, we discuss strategies for the removal and eradication of S. aureus and biofilms in animal husbandry, including the use of antimicrobial peptides, plant extracts, nanoparticles, phages, and antibodies. These strategies to reduce the spread of S. aureus in animal husbandry help maintain livestock health and improve productivity to ensure the ecologically sustainable development of animal husbandry and the safety of livestock products.

关键词： Animal husbandry Biofilm Mastitis Mitigation strategies Staphylococcus aureus

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Transcranial electrical stimulation motor-evoked potentials in a spinal cord ischaemia rabbit model

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Chinese Neurosurgical Journal 2019年第4期5卷 203-210页

作者： yucheng Lu Baotao Lv Qimin song Central Laboratory Linyi People's HospitalShandong ProvinceLinyi 276000China Department of Radiology Linyi People's HospitalShandong ProvinceLinyi 276000China Department of Neurosurgery Linyi People's HospitalShandong ProvinceLinyi 276000China

Background:Spinal cord ischaemia animal models were established by selective ligation of the lumbar artery in a craniocaudal direction between the renal artery and the aortic *** electrical stimulation motor-evoked potentials were measured to enable their use in future studies on spinal cord ischaemia ***:Thirty-three New Zealand rabbits were randomly divided into 6 *** electrical stimulation motor-evoked potentials were recorded before vascular ligation,30 min after vascular ligation,and 2days after vascular *** functions were assessed after surgery and 2 days after vascular *** specimens were taken 2 days after ligation for histopathologic ***:With increased numbers of ligations,a transient extension of the latency became clear,but there were no significant differences in the statistical *** of variance after ligation at the same time in each group and t tests before and after ligation(P>0.05)were not *** or 2 ligations did not cause spinal cord ischaemic *** were no significant differences before and after ligation for the amplitude(P>0.05).With increased numbers of ligations,the amplitude before and after ligation was gradually reduced in the 3-5 ligation groups(P<0.05).Conclusions:Ligation of segmental spinal cord vessels on 1 or 2 levels did not cause ischaemic *** cord ischaemia was observed after 3,4,or 5 *** amplitude was more sensitive to spinal cord ischaemia than *** cord function can be predicted by early changes in the amplitude.

关键词： Spinal cord ischaemic injury Motor-evoked potential Amplitude Rabbits

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电解水制氢技术:进展、挑战与未来展望

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工程科学学报 2025年第2期47卷 282-295页

作者：张正宋凌珺北京航空航天大学交通科学与工程学院北京102200

实现全球碳中和是各国在2050年制定的重要目标之一,旨在减缓气候变化的不良影响.氢能作为一种极具潜力的清洁能源,凭借其高能量密度、零碳排放、可再生性强等特性,被视为实现能源转型与应对气候变化的重要载体.为了实现这些目标,利用电... 详细信息

实现全球碳中和是各国在2050年制定的重要目标之一,旨在减缓气候变化的不良影响.氢能作为一种极具潜力的清洁能源,凭借其高能量密度、零碳排放、可再生性强等特性,被视为实现能源转型与应对气候变化的重要载体.为了实现这些目标,利用电解水制取氢气已经成为解决全球碳中和问题的重要关键方案之一.本文综述了碱性电解水、质子交换膜电解水、阴离子交换膜电解水和固体氧化物电解水制氢技术的最新进展,并对这四种电解水技术的工作原理、结构特点以及优缺点进行了详尽比较.此外,总结了电解水制氢催化剂材料的研究进展,尤其是新型材料的开发与结构优化,旨在提升材料的催化活性与稳定性.讨论了海水电解制氢和耦合制氢等新兴技术,强调通过电解质组成优化、高效双功能催化剂开发及利用小分子氧化反应热力学优势,可有效提升电解水制氢效率和系统稳定性.最后,提出了电解水制氢技术的发展趋势与未来研究方向,包括提升催化剂性能、降低电解过程能耗、开发新型电解设备等,旨在促进电解水制氢技术的进步,助力全球碳中和目标的实现,并为未来的研究提供参考与指导.

关键词：碳中和氢能电解水制氢催化剂电极材料

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Biological function of miRNA-145-5p in angiotensin II induced renal inflammation

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BIOCELL 2024年第4期48卷 601-611页

作者： BIN LI yucheng SHENG XIAOYING XU SHENGCUN WANG HONGYAN song JINGYUAN LI HAONAN JI QINGHUA WANG XIAODI ZHOU LONGJU QI Department of Pediatrics Affiliated Hospital of Nantong UniversityNantong226001China Department of Science and Education Affiliated Nantong Hospitalof Nantong UniversityNantong226001China Laboratory Animal Center Nantong UniversityNantong226001China Department of Gynecology and Obstetrics and Department of Oncology Hai’an Hospital Affiliated to Nantong UniversityNantong226600China

Objective:Chronic kidney disease(CKD)is a progressive disorder characterized by intricate structural and functional alterations in the kidneys,attributable to diverse causative ***,the therapeutic promise of miR-145-5p in addressing renal pathologies has been *** investigation seeks to elucidate the functional role of miR-145-5p in injured kidneys by subjecting human glomerular mesangial cells(HGMCs)to stimulation with Angiotensin II(AngII).Materials and Methods:Cellular viability and the levels of inﬂammatory mediators were evaluated utilizing Cell Counting Kit-8(CCK-8),quantitative real-time polymerase chain reaction(qRT-PCR),and western blot methodologies,both in the presence of AngII incubation and in scenarios of miR-145p overexpression and ***,the cell cycle dynamics were elucidated through Fluorescence-activated Cell Sorting(FACS)***:AngII incubation induced an upregulation of miR-145-5p and inﬂammatory factors including Intercellular Adhesion Molecule 1(ICAM-1),Interleukin 6(IL-6),Interleukin 8(IL-8),and Interleukin 1β(IL-1β).Additionally,it elevated the expression of Cyclin A2,Cyclin D1,and the G2/M cell cycle ***,inhibition of miR-145-5p heightened the levels of inﬂammatory factors and cell cycle regulators induced by AngII *** expression of miR-145-5p correlated with a downregulation of Interleukin 10(IL-10)expression,concurrently promoting HGMC proliferation under AngII ***,ectopic miR-145-5p expression demonstrated a reduction in inﬂammatory factors,cell cyclin regulators,G2/M cell cycle ratio,and overall ***:MiR-145-5p exhibited inhibitory effects on the inﬂammatory response and proliferation induced by Angiotensin II in HGMCs,showcasing its potential as a therapeutic avenue for the treatment of kidney injury.

关键词： miR-145-5p Kidney Angiotensin II Cell cycle Inflammation

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