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A mixed-coordination electron trapping-enabled high-precision touch-sensitive screen for wearable devices

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Bio-Design and Manufacturing 2024年第4期7卷 413-427页

作者： Xi Zhang Junchi Ma Hualin deng Jinming Zhong Kaichen Xu Qiang Wu Bo wen Dongfeng Diao Guangdong Provincial Key Laboratory of Micro/Nano Optomechatronics Engineering College of Mechatronics and Control EngineeringShenzhen UniversityShenzhen 518060China State Key Laboratory of Fluid Power and Mechatronic Systems School of Mechanical EngineeringZhejiang UniversityHangzhou 310058China Shenzhen University General Hospital Shenzhen 518055China Research Center of Medical Plasma Technology Shenzhen UniversityShenzhen 518060China

Touch-sensitive screens are crucial components of wearable *** such as reduced graphene oxide(rGO),carbon nanotubes(CNTs),and graphene offer promising solutions for flexible touch-sensitive ***,when stacked with flexible substrates to form multilayered capacitive touching sensors,these materials often suffer from substrate delamination in response to deformation;this is due to the materials having different Young’s modulus *** results in failure to offer accurate touch screen *** this work,we demonstrate an induced charge-based mutual capacitive touching sensor capable of high-precision touch *** is enabled by electron trapping and polarization effects related to mixed-coordinated bonding between copper nanoparticles and vertically grown graphene ***,we used an electron cyclotron resonance system to directly fabricate graphene-metal nanofilms(GMNFs)using carbon and copper,which are firmly adhered to flexible *** being subjected to 3000 bending actions,we observed almost no change in touch *** screen interaction system,which has a signal-to-noise ratio of 41.16 dB and resolution of 650 dpi,was tested using a handwritten Chinese character recognition trial and achieved an accuracy of 94.82%.Taken together,these results show the promise of touch-sensitive screens that use directly fabricated GMNFs for wearable devices.

关键词： Flexible touch-sensitive screen Graphene-metal nanofilms Mixed coordination Wearable device

Numerical simulation of water-slag elbow erosion-inhibiting by regulating the slag injection position with a novel preceding rotating sheet structure

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Particuology 2024年第7期90卷 323-339页

作者： Fopeng wen Liuyun Xu yixiang Chen Zhaofu deng Shen Zhang wenming Song Yuge Li Liping Wei School of Chemical Engineering Northwest UniversityXi’an710069China School of Chemistry and Chemical Engineering Yan'an UniversityYan'an716000China Machinery Industry Shanghai Lanya Petrochemical Equipment Inspection Institute Co. Ltd.Shanghai201518China The Research Center of Chemical Engineering Applying Technology for Resource of Shaanxi Xi’an710069China

The elbow erosion seriously jeopardizes the safe and stable operation of water–slag discharge pipeline of the coal gasification *** work simulated water–slag elbow characteristics with various slag injection positions by simulating five simplified and representative erosion categories,including A-type horizontal-vertical elbow with an upstream flow,B-type horizontal-vertical elbow with a downstream flow,C-type vertical-horizontal elbow with an upstream flow,D-type vertical-horizontal elbow with a downstream flow and E-type horizontal-horizontal *** with the C/D-type elbow,where particles were injected uniformly,the A-type elbow and E-type elbow were found to increase erosion rate,while the B-type elbow decreases erosion *** interesting discovery is that the elbow erosion rate is relatively low for small particles when particles are injected from the middle and bottom positions of the inlet section of the *** on the observation,a novel preceding rotating sheet structure was developed to regulate the particle injection *** shows an excellent anti-erosion performance by reducing the maximum erosion rate of particles with diameters of 50,100,and 200μm by 23%,35%,and 43%,respectively.

关键词： Erosion Slag-water Uneven particles Elbow pipe Erosion inhibition Preceding rotating sheet structure

Application of in-situ characterization techniques in modern aqueous batteries

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Rare Metals 2024年第8期43卷 3553-3575页

作者： Jia-Hao Wu Hong-Wei Cai Zhao-Hui deng Jean-Jacques Gaumet Yu Bao wen Luo Department of Physics State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingSchool of Materials Science and EngineeringWuhan University of TechnologyWuhan430070China Laboratoire de Chimie Et Physique:Approche Multi-Echelles Des Milieux Complexes(LCP-A2MC)Institut Jean BarriolUniversitéde Lorraine57070MetzFrance Department of Medicinal Chemistry Hubei College of Chinese MedicineJingzhou 434020China

The development of high-performance aqueous batteries calls for an in-depth knowledge of their chargedischarge redox and failure mechanism,as well as a systematic understanding of the dynamic evolution of microstructure,phase composition,chemical composition,and local chemical environment of the materials for ***-situ characterization technology is expected to understand and reveal the problems faced by aqueous rechargeable batteries,such as the dissolution of electrode materials,the growth of metal negative electrode dendrites,passivation,corrosion,side reactions and a series of *** on this,typical in-situ characterization techniques and their basic mechanisms are summarized,including in-situ optical visualization,in-situ microscopy techniques(in-situ scanning electron microscopy(SEM),in-situ transmission electron microscopy(TEM)),in-situ X-ray techniques(in-situ X-ray diffraction(XRD),in-situ X-ray photoelectron spectroscopy(XPS),in-situ near-edge structural X-ray absorption spectroscopy(XANES)),and in-situ spectroscopy techniques(in-situ Raman spectroscopy,in-situ Fourier transform infrared(FTIR)).Moreover,some emerging techniques concerning aqueous battery research,especially gas evolution and materials dissolution issues,such as in-situ electrochemical quartz crystal microbalance(EQCM).in-situ fiber-optic sensing,in-situ gas chromatography(GC) are *** last,the applications of advanced in-situ characterizations in future research of aqueous batteries are emphasized and discussed,along with some of the remaining challenges and possible solutions.

关键词： Aqueous battery In-situ characterization Phase transformation Solid electrolyte interphase Zinc dendrite growth

Transition-metal free trifluoromethylimination of alkenes enabled by direct activation of N-unprotected ketimines

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Chinese Chemical Letters 2024年第9期35卷 155-159页

作者： Boqiang Wang Yongzhuo Xu Jiajia Wang Muyang Yang Guo-Jun deng wen Shao Key Laboratory for Green Organic Synthesis and Application of Hunan Province Key Laboratory of Environmentally Friendly Chemistry and Application of Ministry of EducationCollege of ChemistryXiangtan UniversityXiangtan 411105China Department School of Chemistry and Chemical Engineering Henan Normal UniversityXinxiang 453007China

A highly site-selective intermolecular trifluoromethylimination of activated and unactivated olefins was reported under transition-metal-and photosensitizer-free *** newly developed strategy provides straightforward and efficient access to diverse value-added vicinal trifluoromethyl amines without resorting to the pre-functionalized *** experiments demonstrate that the approach proceeded through CF_(3)and iminyl two-radicals process,which were generated directly from commercially available benzophenone imine in a novel electron-donor mode via a SET process activated by the bifunctional hypervalent iodine *** synthetic potential of the protocols was further showcased via the condensation/amination sequential cascade,and transformations to accessβ-CF_(3)primary amines.

关键词： Transition-metal free Alkenes difunctionalization Amination Trifluoromethylation Single-electron transfer

Exploring deep learning for landslide mapping:A comprehensive review

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China Geology 2024年第2期7卷 330-350页

作者： Zhi-qiang Yang wen-wen Qi Chong Xu Xiao-yi Shao College of Surveying and Geo-Informatics Tongji UniversityShanghai 200092China National Institute of Natural Hazards Ministry of Emergency ManagementBeijing 100085China Key Laboratory of Compound and Chained Natural Hazards Dynamics Ministry of Emergency Management of ChinaBeijing 100085China

A detailed and accurate inventory map of landslides is crucial for quantitative hazard assessment and land *** methods relying on change detection and object-oriented approaches have been criticized for their dependence on expert knowledge and subjective *** advancements in highresolution satellite imagery,coupled with the rapid development of artificial intelligence,particularly datadriven deep learning algorithms(DL)such as convolutional neural networks(CNN),have provided rich feature indicators for landslide mapping,overcoming previous *** this review paper,77representative DL-based landslide detection methods applied in various environments over the past seven years were *** study analyzed the structures of different DL networks,discussed five main application scenarios,and assessed both the advancements and limitations of DL in geological hazard *** results indicated that the increasing number of articles per year reflects growing interest in landslide mapping by artificial intelligence,with U-Net-based structures gaining prominence due to their flexibility in feature extraction and ***,we explored the hindrances of DL in landslide hazard research based on the above research *** such as black-box operations and sample dependence persist,warranting further theoretical research and future application of DL in landslide detection.

关键词： Landslide Mapping Quantitative hazard assessment Deep learning Artificial intelligence Neural network Big data Geological hazard survery engineering

Asymptotic Inference in the Random Coefficient Autoregressive Model with Time-functional Variance Noises

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 320-346页

作者： En-wen ZHU Zi-wei deng Han-jun ZHANG Jun CAO Xiao-hui LIU Department of Mathematics and Statistics Changsha University of Science and TechnologyChangsha 410114China School of Mathematics and Computational Science Xiangtan UniversityXiangtan 411105China School of Statistics and Data Science and Key Laboratory of Data Science in Finance and EconomicsJiangxi University of Finance and EconomicsNanchang 330013China

This paper considers the random coefficient autoregressive model with time-functional variance noises,hereafter the RCA-TFV *** first establish the consistency and asymptotic normality of the conditional least squares estimator for the constant *** semiparametric least squares estimator for the variance of the random coefficient and the nonparametric estimator for the variance function are constructed,and their asymptotic results are reported.A simulation study is presented along with an analysis of real data to assess the performance of our method in finite samples.

关键词： random coefficient autoregressive model time-functional variance conditional least squares semiparametric least squares

A historical overview of nano-optics:From near-field optics to plasmonics

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Chinese Physics B 2024年第5期33卷 134-145页

作者：邓妙怡朱星 Department of History of Science Technology and MedicineAcademy for Advanced Interdisciplinary StudiesPeking UniversityBeijing 100871China School of Physics Peking UniversityBeijing 100871China

Nano-optics is an emergent research field in physics that appeared in the 1980s,which deals with light–matter optical interactions at the nanometer *** early studies of nano-optics,the main concern focus is to obtain higher optical resolution over the diffraction *** researches of near-field imaging and spectroscopy based on scanning near-field optical microscopy(SNOM)are *** exploration of improving SNOM probe for near-field detection leads to the emergence of surface *** the sense of resolution and wider application,there has been a significant transition from seeking higher resolution microscopy to plasmonic near-field modulations in the nano-optics community during the nano-optic ***,studies of nano-optics prefer the investigation of plasmonics in different material *** this article,the history of the development of near-field optics is briefly *** difficulties of conventional SNOM to achieve higher resolution are *** an alternative solution,surface plasmons have shown the advantages of higher resolution,wider application,and flexible nano-optical modulation for new *** typical studies in different periods are introduced and characteristics of nano-optics in each stage are *** this way,the evolution progress from near-field optics to plasmonics of nano-optics research is *** future development of nano-optics is discussed then.

关键词： nano-optics near-field optics surface plasmon plasmonic modulation

Construction of ZnO@CDs@Co_(3)O_(4) sandwich heterostructure with multi-interfacial electron-transfer toward enhanced photocatalytic CO_(2) reduction

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Chinese Chemical Letters 2024年第4期35卷 147-152页

作者： Xiuzheng deng yi Ke Jiawen Ding yingtang Zhou Hui Huang Qian Liang Zhenhui Kang Advanced Catalysis and Green Manufacturing Collaborative Innovation Center CNPC-CZU Innovation AllianceSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316004China

Photocatalytic conversion of CO_(2) into small-molecule chemical feedstocks can meet the growing demand for energy and alleviate the global warming. Herein, a p-n ZnO@CDs@Co_(3)O_(4) heterojunction with sandwich structure was constructed by calcination method of self-assembled ZIF-8@CDs@ZIF-67. The ZnO@CDs@Co_(3)O_(4) with well-defined interfacial structure exhibited the significantly enhanced photocatalytic CO_(2) reduction activity, and the optimal catalyst indicated the(CO + CH_(4)) evolution rate of 214.53μmol g^(-1)h^(-1) under simulated solar light, which was superior to ZnO, Co_(3)O_(4) and binary ZnO@Co_(3)O_(4).The internal cavity, exposed active sites, multiple interfaces and constructed p-n heterojunction can facilitate the light harvesting and photoexcited electron transfer. Besides, after introduction of CDs placed in the middle layer between ZnO and Co_(3)O_(4), CDs with excellent photoelectric property further promoted charge separation and migration. This work represents an appealing strategy to construct well-defined photocatalysts for boosting CO_(2) photoreduction.

关键词： Metal-organic framework Photocatalytic CO_(2) reduction Carbon dots p-n heterojunction Sandwich heterostructure

Cutting performance of saw blades with microtextured rougher and finisher sawteeth

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Advances in Manufacturing 2024年第2期12卷 317-334页

作者： Yang Lu Jian-Xin deng Zhi-Hui Zhang Jia-Xing Wu Ran Wang yi-Chen Bao Key Laboratory of High Efficiency and Clean Mechanical Manufacture of MOE School of Mechanical EngineeringShandong UniversityJinan250061People’s Republic of China

The problems of severe sawtooth wear,harsh sawing noise,and low surface quality during the processing of circular saw blades need to be *** improve the cutting performance of TiC-based cermet saw blades,microtextures parallel to the cutting edge were fabricated on rough and fine sawteeth by laser *** cutting tests were performed on a sawing platform under lubricated *** of the sawing arc length and working sawtooth cutting force variations were developed for sawing steel pipes,and the accuracy of the sawing force model was verified *** results indicate that the variations in the sawing force are proportional to the sawing arc *** circular saw blades with microtextures that did not penetrate the sawtooth rake face exhibited the lowest cutting force,sawing noise,and highest machined surface ***,the worn-out distance of the rougher and finisher sawteeth was reduced by approximately 7.4%and 44.1%,respectively,compared with conventional circular saw *** main failure modes of sawteeth were tip wear,rake face adhesion,and oxidative *** addition,the mechanism by which the textures improve the cutting and wear properties of TiC-based circular saw blades was *** study provided a significant concept for enhancing the cutting performance of circular saw blades and improving the machined surface quality.

关键词： Circular saw blades Micro textures Cutting performance Wear performance