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Efficient and Stable Photoassisted Lithium‑Ion Battery Enabled by Photocathode with Synergistically Boosted Carriers Dynamics

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Nano-Micro Letters 2025年第3期17卷 440-454页

作者： Zelin Ma Shiyao wang Zhuangzhuang Ma Juan Li Luomeng Zhao Zhihuan Li Shiyuan wang Yazhou Shuang Jiulong wang fang wang Weiwei Xia Jie Jian Yibo He Junjie wang Pengfei Guo Hongqiang wang State Key Laboratory of Solidification Processing Center for Nano Energy MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical University and Shaanxi Joint Laboratory of Graphene(NPU)Xi’an 710072People’s Republic of China State Key Laboratory of Solidification Processing School of Materials Science and Engineering DepartmentNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China Research and Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518063People’s Republic of China Key Laboratory of Applied Surface and Colloid Chemistry Shaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringNational Ministry of EducationShaanxi Normal UniversityXi’an 710119People’s Republic of China

Efficient and stable photocathodes with versatility are of significance in photoassisted lithium-ion batteries(PLIBs),while there is always a request on fast carrier transport in electrochemical active *** work proposes a general approach of creating bulk heterojunction to boost the carrier mobility of photocathodes by simply laser assisted embedding of plasmonic *** employed in PLIBs,it was found effective for synchronously enhanced photocharge separation and transport in light charging ***,experimental photon spectroscopy,finite difference time domain method simulation and theoretical analyses demonstrate that the improved carrier dynamics are driven by the plasmonic-induced hot electron injection from metal to TiO_(2),as well as the enhanced conductivity in TiO2 matrix due to the formation of oxygen vacancies after Schottky *** from these merits,several benchmark values in performance of TiO2-based photocathode applied in PLIBs are set,including the capacity of 276 mAh g^(−1)at 0.2 A g^(−1)under illumination,photoconversion efficiency of 1.276%at 3 A g^(−1),less capacity and Columbic efficiency loss even through 200 *** results exemplify the potential of the bulk heterojunction strategy in developing highly efficient and stable photoassisted energy storage systems.

关键词： Photoassisted lithium-ion batteries Bulk heterojunction Carrier dynamics TiO2 nanofiber Plasmonic metal nanocrystals

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Small modifications of endo-functionalized cavities lead to large changes in molecular interaction in water

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Science China Chemistry 2025年第1期 369-376页

作者： Song-Meng wang Hao Nian Yan-fang wang Li-Shuo Zheng Yu-Tao Zheng Yi-Wei Dong Liping Huang Xiaoping wang Wei Jiang Liu-Pan Yang Department of Chemistry Southern University of Science and Technology School of Chemistry and Pharmaceutical Sciences State Key Laboratory for Chemistry and Molecular Engineering of Medicinal ResourcesGuangxi Normal University School of Pharmaceutical Science Hengyang Medical School University of South China

Studying molecular recognition in aqueous environments is crucial for understanding biological processes. Herein, we present a series of N-doped endo-functionalized anthracene-based cavities by introducing inward-directed pyridine units. The subtle modifications can significantly affect the binding properties of these receptors, which is similar to the mutations in biological systems. Combining theoretical calculations and molecular recognition experiments demonstrated that these “mutations” have an impact on the hydrophobicity and charge distribution of the hosts, consequently significantly influencing molecular *** is crucial for understanding the intricate mechanisms of molecular-level interactions in biological receptors.

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控制方向未知的受限多智能体系统的预设时间模糊控制

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工程科学学报 2025年第1期47卷 121-129页

作者：李菲周超范利蓉王芳燕山大学理学院秦皇岛066004 河北农业大学海洋学院秦皇岛066003

综合考虑受控制方向未知、输入受限和状态时延影响的有领导者多智能体系统的编队控制问题,设计基于模糊逻辑系统的预设时间一致性控制策略.为了保证编队输出误差在预设时间内满足预定的约束范围要求,引入预设时间性能函数,构造Lyapunov-... 详细信息

综合考虑受控制方向未知、输入受限和状态时延影响的有领导者多智能体系统的编队控制问题,设计基于模糊逻辑系统的预设时间一致性控制策略.为了保证编队输出误差在预设时间内满足预定的约束范围要求,引入预设时间性能函数,构造Lyapunov-Krasovskii(L-K)泛函解决状态时延问题,将外界干扰和L-K泛函的导数中的部分项定义为未知非线性函数,并利用模糊逻辑系统对其进行估计,利用Nussbaum函数和均值定理分别处理控制方向未知和输入受限问题,基于以上设计,提出预设时间模糊控制策略,并通过Lyapunov稳定性理论,分析闭环系统的有界稳定性,数值对比仿真和两级化学反应器应用仿真说明控制方法的有效性.

关键词：多智能体系统状态时延输出误差约束输入受限控制方向未知

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基于小尺寸模型分析氢氧旋转爆轰波传播的不稳定性机制

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爆炸与冲击 2025年第1期45卷 28-40页

作者：徐鸿飞王放武郁文翁春生南京理工大学瞬态物理全国重点实验室江苏南京210094

氢氧的高反应活性给旋转爆轰波的稳定传播带来了巨大的挑战,为研究氢氧旋转爆轰波传播不稳定性,通过改变当量比对小尺寸模型下二维氢氧旋转爆轰波进行数值模拟研究,揭示了氢氧旋转爆轰波复杂多变的传播特性,并分析了典型流场结构,探讨... 详细信息

氢氧的高反应活性给旋转爆轰波的稳定传播带来了巨大的挑战,为研究氢氧旋转爆轰波传播不稳定性,通过改变当量比对小尺寸模型下二维氢氧旋转爆轰波进行数值模拟研究,揭示了氢氧旋转爆轰波复杂多变的传播特性,并分析了典型流场结构,探讨了传播模态的不稳定性以及爆轰波湮灭和再起爆机制。结果表明:随着当量比的提高,流场内分别呈现熄爆、单波、单双波混合3种传播模态,且爆轰波的传播速度随当量比的增大几乎呈线性提高,速度亏损为5%~8%。激波的扰动使得爆燃面失稳产生明显的扭曲和褶皱,氢氧的高反应活性让爆燃面明显分层且在2个分界面上呈现不同的不稳定性,上分界面为Kelvin-Helmholtz(K-H)不稳定性,下分界面为Rayleigh-Taylor(R-T)不稳定性。单双波混合模态下爆轰波极不稳定,保持湮灭、单波、双波对撞3种状态之间循环。爆轰波有2种湮灭方式:一是双波对撞导致爆轰波湮灭,二是爆燃面燃烧加剧使得爆燃面下移导致爆轰波湮灭。再起爆的主要原因是:R-T不稳定性诱导爆轰产物与新鲜预混气在爆燃面上相互挤压产生尖峰和气泡结构,增强爆燃面上的反应放热,产生了局部热点并逐渐增强为爆轰波,实现爆燃转爆轰。

关键词：旋转爆轰波传播特性当量比不稳定性湮灭再起爆

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Leader-following coordination of multi-agent systems with information feedback

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Journal of Systems Engineering and Electronics 2009年第4期20卷 823-828页

作者： wang Dongmei fang Huajing Dept. of Control Science and Engineering Huazhong Univ of Science and Technology Wuhan 430074 P. R. China

Based on the strategy of information feedback from followers to the leader, flocking control of a group of agents with a leader is studied. The leader tracks a pre-defined trajectory and at the same time the leader uses the feedback information from followers to the leader to modify its motion. The advantage of this control scheme is that it reduces the tracking errors and improves the robustness of the team cohesion to followers＇ faults. The results of simulation are provided to illustrate that information feedback can improve the performance of the system.

关键词： multi-agent system leader-following flocking control information feedback.

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Effect of three dimensional stress state on unstable fracture condition and crack opening level in a new crack growth model

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Acta Metallurgica Sinica(English Letters) 2010年第1期23卷 41-49页

作者： fang wang Weicheng CUI China Ship Scientific Research Center Wuxi 214082 China

A new model for the analysis of fatigue crack growth in the metal structures was proposed. This model shows a promising capability of explaining various fatigue phenomena. The new crack growth model is further completed by a continuous empirical formula for estimating the value of variable fracture toughness during crack propagation and a modified continuous equation for the crack tip stress/strain constraint factor used to calculate the stress intensity factor at the opening level. The prediction results are proved to agree well with the observed phenomena in test.

关键词： Marine structures Crack growth rate Three dimensional stress state Fracture toughness Crack tip stress/strain constraint factor

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Novel method for hybrid multiple attribute decision making based on TODIM method

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Journal of Systems Engineering and Electronics 2015年第5期26卷 1023-1031页

作者： fang wang Hua Li School of Economics and Management Xidian University

The TODIM(an acronym in Portuguese for interactive and multiple attribute decision making) method is a valuable tool to solve the multiple attribute decision making(MADM) problems considering the behavior of the decision maker(DM), while it cannot be used to handle the problem with unknown weight information on attributes. In this paper, a novel method based on the classical TODIM method is proposed to solve the hybrid MADM problems with unknown weight information on attributes,in which attribute values are represented in four different formats:crisp numbers, interval numbers, triangular fuzzy numbers and trapezoidal fuzzy numbers. Firstly, the positive-ideal alternative and negative-ideal alternative are determined, and the gain and loss matrices are constructed by calculating the gain and loss of each alternative relatived to the ideal alternatives concerning each attribute based on different distance calculation formulas, which may avoid the information missing or information distortion in the process of unifying multiform attribute values into a certain representation form. Secondly, an optimization model based on the maximizing deviation(MD) method, by which the attribute weights can be determined, is established for the TODIM method. Further, the calculation steps to solve the hybrid MADM problems are given. Finally, two numerical examples are presented to illustrate the usefulness of the proposed method, and the results show that the DM’s psychological behavior, attribute weights and the transformed information would highly affect the ranking orders of alternatives.

关键词： hybrid multiple attribute decision making TODIM ranking

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Stochastic averaging method for estimating first-passage statistics of stochastically excited Duffing-Rayleigh-Mathieu system

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Acta Mechanica Sinica 2008年第5期24卷 575-582页

作者： Yongjun Wu wang fang Institute of Automation School of Information Scienceand Engineering East China University of Science and TechnologyShanghai 200237 China Hangzhou Yiheng Technologies Co. Ltd 2F28 Wantang Road Hangzhou 310013 China

The first-passage statistics of Duffing-Rayleigh- Mathieu system under wide-band colored noise excitations is studied by using stochastic averaging method. The motion equation of the original system is transformed into two time homogeneous diffusion Markovian processes of amplitude and phase after stochastic averaging. The diffusion process method for first-passage problem is used and the corresponding backward Kolmogorov equation and Pontryagin equation are constructed and solved to yield the conditional reliability function and mean first-passage time with suitable initial and boundary conditions. The analytical results are confirmed by Monte Carlo simulation.

关键词： First-passage Colored noise Stochastic averaging Reliability Monte Carlo simulation

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Application of the Modified nverse Design Method in the Optimization of the Runner Blade of a Mixed-Flow Pump

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Chinese Journal of Mechanical Engineering 2018年第6期31卷 137-153页

作者： Ye-Ming Lu Xiao-fang wang Wei wang fang-Ming Zhou School of Energy and Power Engineering Dalian University of TechnologyDalian 116000China Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of TechnologyDalian 116000China Collaborative Innovation Center of Major Machine Manufacturing in Liaoning Province Dalian 116000China

To improve the design speed and reduce the design cost for the previous blade design method, a modified inverse design method is presented. In the new method, after a series of physical and mathematical simplifications, a sail?like constrained area is proposed, which can be used to configure di erent runner blade shapes. Then, the new method is applied to redesign and optimize the runner blade of the scale core component of the 1400?MW canned nuclear coolant pump in an established multi?optimization system compromising the Computational Fluid Dynamics(CFD) analysis, the Response Surface Methodology(RSM) and the Non?dominated Sorting Genetic Algorithm?II(NSGA?II). After the execution of the optimization procedure, three optimal samples were ultimately obtained. Then, through comparative analysis using the target runner blade, it was found that the maximum e ciency improvement reached 1.6%, while the head improvement was about 10%. Overall, a promising runner blade inverse design method which will benefit the hydraulic design of the mixed?flow pump has been proposed.

关键词： Optimization Mixed?flow pump Inverse design method Runner blade Nuclear coolant

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采用小波变换的空间外差干涉图误差分析方法

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光谱学与光谱分析 2025年第1期45卷 8-14页

作者：王方原李晓静叶松李树王新强桂林电子科技大学光电工程学院广西桂林541004 广西光电信息处理重点实验室广西桂林541004

空间外差光谱技术(SHS)是一种应用于微弱物质探测、行星勘探以及大气遥感等领域的超光谱分析技术。受实验环境复杂及被测目标信号微弱等因素的影响,空间外差光谱仪的测量结果易出现干涉条纹倾斜、干涉图有斑点噪声等情况,从而最终影响... 详细信息

空间外差光谱技术(SHS)是一种应用于微弱物质探测、行星勘探以及大气遥感等领域的超光谱分析技术。受实验环境复杂及被测目标信号微弱等因素的影响,空间外差光谱仪的测量结果易出现干涉条纹倾斜、干涉图有斑点噪声等情况,从而最终影响测量光谱的精度。为了尝试解决这些问题,提出了基于小波变换的干涉图误差分析方法,对干涉图的斑点噪声水平和条纹倾斜误差进行有效的评价,从而为后续误差校正提供理论基础。首先对无误差的钾灯仿真干涉图加入不同标准差的高斯噪声,利用小波分解提取复小波系数,采用三种噪声估计法对干涉图数据进行计算,结果表明空域相关小波变换法噪声估计结果与真实值偏差最小,而Donoho估计法在修正截距后与真实值具有更好的吻合度。随后采用Db2小波对噪声水平不同的仿真钾灯干涉图进行一层小波分解并提取水平、对角及垂直三个方向的细节系数,采用Donoho估计法对干涉图进行二维噪声分析,有效表征了三幅干涉图各方向上的噪声水平特征。最后对仿真连续光干涉图进行小波分解并提取系数分析,研究了干涉条纹倾斜角度与小波分解系数的关系。研究结果表明,三个方向的小波细节系数估值变化分别在分解到不同层数时具有相似的变化规律:小波细节系数估值与条纹倾斜方向和小波细节系数的所属方向的夹角成反比,条纹倾斜方向与该小波细节系数的方向夹角越小,估值越大,反之则越小,且水平方向分解到第一层、对角方向分解到第二层、垂直方向分解到第三层符合变化规律。该研究是利用小波分解进行空间外差光谱误差分析的有益尝试,也为后续干涉图条纹倾斜误差的校正提供了一种新途径。

关键词：空间外差光谱技术噪声标准差估计干涉图小波变换

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