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Nanoengineering Metal–Organic Frameworks and Derivatives for Electrosynthesis of Ammonia

Nano-Micro Letters 2023年第11期15卷 205-240页

作者： Daming Feng Lixue Zhou timothy j.white Anthony K.Cheetham Tianyi Ma Fengxia Wei College of Chemistry Liaoning UniversityShenyang 110036People’s Republic of China School of Materials Science and Engineering Nanyang Technological University50 Nanyang AvenueSingapore 639798Singapore Materials Research Laboratory University of CaliforniaSanta BarbaraCA 93106USA School of Science RMIT UniversityMelbourneVIC 3000Australia Institute of Materials Research and Engineering(IMRE) Agency for ScienceTechnology and Research(A^(*)STAR)2 Fusionopolis WayInnovis 08‑03Singapore 138634Singapore

Electrocatalytic synthesis under mild conditions has become increasingly important as one of the practical alternatives for industrial applications,especially for the green ammonia(NH_(3))industry.A properly engineered electrocatalyst plays a vital role in the realization of superior catalytic *** various types of promising nanomaterials,metal–organic frameworks(MOFs)are competitive candidates for developing efficient electrocatalytic NH_(3) synthesis from simple nitrogen-containing molecules or ions,such as N_(2) and NO_(3)^(−).In this review,recent advances in the development of electrocatalysts derived from MOFs for the electrosynthesis of NH_(3) are collected,categorized,and discussed,including their application in the N_(2) reduction reaction(NRR)and the NO_(3)^(−)reduction reaction(NO3RR).Firstly,the fundamental principles are illustrated,such as plausible mechanisms of NH_(3) generation from N_(2) and NO_(3)^(−),the apparatus of corresponding electrocatalysis,parameters for evaluation of reaction efficiency,and detection methods of yielding NH_(3).Then,the electrocatalysts for NRR processes are discussed in detail,including pristine MOFs,MOF-hybrids,MOF-derived N-doped porous carbons,single atomic catalysts from pyrolysis of MOFs,and other MOF-related ***,MOF-related NO3RR processes are also listed and ***,the existing challenges and prospects for the rational design and fabrication of electrocatalysts from MOFs for electrochemical NH_(3) synthesis are presented,such as the evolution of investigation methods with artificial intelligence,innovation in synthetic methods of MOF-related catalysts,advancement of characterization techniques,and extended electrocatalytic reactions.

关键词： Metal–organic frameworks Electrosynthesis of ammonia Nitrogen reduction reactions Nitrate reduction reactions

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Hydrothermal base catalyzed depolymerization and conversion of technical lignin-An introductory review

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Carbon Resources Conversion 2019年第1期2卷 59-71页

作者： Malte Otromke Robin j.white jorg Sauer Institute of Catalysis Research and Technology(IKFT) Karlsruhe Institute of Technology(KIT)Eggenstein-LeopoldshafenGermany Sustainable Catalytic Materials Group Division Hydrogen TechnologiesFraunhofer Institute for Solar Energy Systems ISEHeidenhofstr.279110 FreiburgGermany GmbH Group Process TechnologyFrankfurt am MainGermany

Lignin represents the most significant potential source of sustainable aromatic ***,the vast majority of technical lignin could be sourced from industrial paper production and in particular the Kraft process,where it is conventionally combusted for chemicals recovery and heat generation(*** plant operation).While in recent years several efforts have concerned the conversion of native lignin(*** found in nature)during biomass processing,there has also been significant focus on the“Base Catalyzed”conversion of technical *** process is of significant interest,since it could be potentially integrated into existing Kraft mill *** following review paper focuses on the development of the hydrothermal base catalyzed depolymerization(HBCD)of lignin,as a basis to produce valuable chemical *** will be placed on NaOH catalyzed reactions in the aqueous phase,as this approach is considered the most *** is placed on reaction conditions and characterization of monomeric aromatic compounds from the HBCD ***,as largest product fraction,is also considered,however,these are seldom analyzed in detail in the literature and ideas on further use are *** review also addresses findings in literature concerning the assessment of the solid,liquid,and gas product streams arising from *** this paper,process conditions for HBCD reactions can be derived and it is shown that the solid phase has a high potential for further valorization and downstream processing.

关键词： catalyzed polymerization lignin

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Evaluation of alternative surface runoff accounting procedures using SWAT model

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International journal of Agricultural and Biological Engineering 2015年第3期8卷 54-68页

作者： Haw Yen Michael j.white jaehak jeong Mazdak Arabi jeffrey G.Arnold Department of Civil and Environmental Engineering Colorado State UniversityFort Coll insColorado 80523USA Blackland Research&Extension Center Texas A&M Agrilife ResearchTempleTexas 76502USA Grassland Soil&Water Research LaboratoryUSDA-ARSTempleTexas 76502USA

For surface runoff estimation in the Soil and Water Assessment Tool(SWAT)model,the curve number(CN)procedure is commonly adopted to calculate surface runoff by dynamically updating CN values based on antecedent soil moisture condition(SCSI)in *** SWAT2005 and onward,an alternative approach has become available to apply the CN method by relating the runoff potential to daily evapotranspiration(SCSII).While improved runoff prediction with SCSII has been reported in several case studies,few investigations have been made on its influence to water quality output or on the model uncertainty associated with the SCSII *** objectives of the research were:(1)to quantify the improvements in hydrologic and water quality predictions obtained through different surface runoff estimation techniques;and(2)to examine how model uncertainty is affected by combining different surface runoff estimation techniques within SWAT using Bayesian model averaging(BMA).Applications of BMA provide an alternative approach to investigate the nature of structural uncertainty associated with both CN *** showed that SCSII and BMA associated approaches exhibit improved performance in both discharge and total NO3 predictions compared to *** addition,the application of BMA has a positive effect on finding well performed solutions in the multi-dimensional parameter space,but the predictive uncertainty is not evidently reduced or ***,we recommend additional future SWAT calibration/validation research with an emphasis on the impact of SCSII on the prediction of other pollutants.

关键词： Soil and Water Assessment Tool(SWAT),curve number method,Bayesian model averaging,uncertainty analysis hydrology,water quality

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Ammonium Improves Corn Phosphorus Acquisition Through Changes in the Rhizosphere Processes and Root Morphology

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Pedosphere 2019年第4期29卷 534-539页

作者： Elialdo Alves DE SOUZA Natália Rodrigues FERREIRA-ELOY Camila da Silva GRASSMANN Ciro Antonio ROSOLEM Philip j.white School of Agronomic Sciences Sao Paulo State University The james Hutton Institute

Dear Editor, Phosphorus (P) deficiency is the most limiting factor in tropical agriculture since most soils in this region are predominantly acids with high-energy P-binding compounds. Therefore, up to 90% of the P applied becomes fixed in soils, which raises environmental concerns and production costs (Syers et al., 2008). Thus, developing strategies to imptove P use efficiency (PUE) is essential to mitigate environmental problems and improve profits. These strategies should consider the soil-root-rhizosphere system because it is the most biochemical active site where nutrient uptake occurs (Hinsinger, 2011).

关键词： Root Morphology Rhizosphere Processes Dear Editor

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Targeted protein delivery:carbodiimide crosslinking influences protein release from microparticles incorporated within collagen scaffolds

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Regenerative Biomaterials 2019年第5期6卷 279-287页

作者： Constantin Edi Tanase Omar Qutachi Lisa j.white Kevin M.Shakesheff Andrew W.McCaskie Serena M.Best Ruth E.Cameron Department of Materials Science and Metallurgy University of CambridgeCambridge Centre for Medical MaterialsCambridge27Charles Babbage RoadCB30FSUK Centre for Biomolecular Sciences School of PharmacyUniversity of NottinghamUniversity ParkNottingham NG72RDUK Division of Trauma&Orthopaedic Surgery Department of SurgeryUniversity of CambridgeBox 180Addenbrooke’s HospitalHills RoadCambridge CB20QQUK Present address:School of Pharmacy De Montforte UniversityLeicester LE19BHUK

Tissue engineering response may be tailored via controlled,sustained release of active agents from protein-loaded degradable microparticles incorporated directly within three-dimensional(3D)ice-templated collagen ***,the effects of covalent crosslinking during scaffold preparation on the availability and release of protein from the incorporated microparticles have not been ***,we load 3D ice-templated collagen scaffolds with controlled additions of poly-(DL-lactide-co-glycolide)*** probe the effects of subsequent N-(3-dimethylaminopropyl)-N0-ethylcarbodiimide hydrochloride crosslinking on protein release,using microparticles with different internal protein *** isothiocyanate labelled bovine serum albumin is used as a model protein *** scaffolds display a homogeneous microparticle distribution,and a reduction in pore size and percolation diameter with increased microparticle addition,although these values did not fall below those reported as necessary for cell *** protein distribution within the microparticles,near the surface or more deeply located within the microparticles,was important in determining the release profile and effect of crosslinking,as the surface was affected by the carbodiimide crosslinking reaction applied to the *** of microparticles with a high proportion of protein at the surface caused both a reduction and delay in protein *** located within the bulk of the microparticles,was protected from the crosslinking reaction and no delay in the overall release profile was seen.

关键词： collagen scaffolds PLGA microparticles FITC-BSA EDC crosslinking pore size percolation diameter

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Apples to oranges:environmentally derived,dynamic regulation of serotonin neuron subpopulations in adulthood?

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Neural Regeneration Research 2025年第9期20卷 2596-2597页

作者： Christopher j.O’Connell Matthew j.Robson Department of Genetics College of MedicineHarvard UniversityBostonMAUSA james L.Winkle College of Pharmacy Division of Pharmaceutical SciencesUniversity of CincinnatiCincinnatiOHUSA Neuroscience Graduate Program College of MedicineUniversity of CincinnatiCincinnatiOHUSA

Traumatic brain injury(TBI)is a public health problem with an undue economic burden that impacts nearly every age,ethnic,and gender group across the globe(Capizzi et al.,2020).TBIs are often sustained during a dynamic range of exposures to energetic environmental forces and as such outcomes are typically heterogeneous regarding severity and pathology(Capizzi et al.,2020).

关键词： sustained orange dynamic

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居住隔离论:理论与方法的比较研究

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山东社会科学 2016年第1期 96-106页

作者： Michael j.white Rebecca Wang 朱格张月飞布朗大学社会学系中国人民大学人口学系

隔离是指不同类别的社会群体差异分布的程度;居住隔离关注人群在特定地域空间(如城市)中分布的不均衡。本文重点回顾美国居住隔离的研究理论和测量方法。文章首先探讨居住隔离研究中的几个主要理论问题;其次重点介绍几类广为人知的测量... 详细信息

隔离是指不同类别的社会群体差异分布的程度;居住隔离关注人群在特定地域空间(如城市)中分布的不均衡。本文重点回顾美国居住隔离的研究理论和测量方法。文章首先探讨居住隔离研究中的几个主要理论问题;其次重点介绍几类广为人知的测量指标,包括变异指数、暴露指数、熵指数、空间邻近指数等,分析各自的优势与局限,并简要介绍其他(如地理信息系统,GIS)新方法技术的运用。随后,文章讨论将西方式的隔离测量和分析方法应用于其他社会环境(尤其是中国)的前景和困难。我们认为,中等收入国家的居住隔离研究无需重走过去的路径;相反,转型时期的当代社会及不断涌现的数据或许能为未来相关研究指明方向。

关键词：隔离居住隔离隔离测量变异指数

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Déjàvu:Might Future Eruptions of Hunga Tonga-Hunga Ha'apai Volcano be a Repeat of the Devastating Eruption of Santorini,Greece(1650 BC)?

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journal of Earth Science 2022年第2期33卷 229-235页

作者： timothy M.Kusky Center for Global Tectonics Three Gorges Research Center for Geo-HazardsChina University of GeosciencesWuhan 430074China

The remote Pacific islands nation of Tonga(about 170 islands,with a population of 105000),and surrounding countries,are suffering from the damage from one of the largest,most explosive volcanic eruptions in at least several decades,at least since the 1991 eruption of Pinatubo in the *** data is still coming in from the jan.15,2022 *** reports show(remarkably)few casualties,but the islands are still(as of this writing)inaccessible because of thick volcanic ash coverings。

关键词： volcanic eruption thick

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Gene therapy for spinal muscular atrophy:perspectives on the possibility of optimizing SMN1 delivery to correct all neurological and systemic perturbations

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Neural Regeneration Research 2025年第7期20卷 2011-2012页

作者： Sharon j.Brown Rafael j.Yáñez-Muñoz Heidi R.Fuller School of Pharmacy and Bioengineering Keele UniversityKeeleUK Wolfson Center for Inherited Neuromuscular Disease TORCH BuildingRJAH Orthopaedic HospitalOswestryUK *** Center of Gene and Cell TherapyDepartment of Biological SciencesSchool of Life Sciences and the EnvironmentRoyal Holloway University of LondonEghamUK

Spinal muscular atrophy(SMA)is a genetic condition that results in selective lower motor neuron loss with concomitant muscle weakness and *** genetic cause of SMA was understood in 1995 when loss or impairment of the survival motor neuron 1(SMN1)gene was identified as the main contributing factor(Lefebvre et al.,1995).This,in combination with the discovery that humans have a“back-up”gene,SMN2,which can produce low levels(approximately 10%)of the full-length functional SMN protein,has led to the generation of SMA-specific gene *** was traditionally classified according to age of symptom onset and developmental milestones achieved,with life expectancy and severity varying between ***,SMN2 copy number is used as a proxy for the prediction of disease severity,with higher SMN2 copy number typically being associated with reduced severity of SMA,although this relationship is not absolute:some individuals with low SMN2 copy number have less severe SMA phenotypes and vice ***,the etiology of SMA is further complicated by other factors,such as non-typical nucleotide variants and SMN2-independent modifiers of disease severity.

关键词： atrophy traditionally absolute

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CD40 stimulation as a molecular adjuvant for cancer vaccines and other immunotherapies

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Cellular & Molecular Immunology 2022年第1期19卷 14-22页

作者： timothy N.j.Bullock Department of Pathology University of VirginiaCharlottesvilleVAUSA

The substantial advances attained by checkpoint blockade immunotherapies have driven an expansion in the approaches used to promote T cell access to the tumor microenvironment to provide targets for checkpoint *** in any T cell response to a tumor antigen is the capacity of dendritic cells to initiate and support such ***,the rationale and early immunobiology of CD40 as a master regulator of dendritic cell activation is reviewed,with further contextualization and appreciation for the role of CD40 stimulation not only in cancer vaccines but also in other contemporary immune-oncology approaches.

关键词： CD40 vaccine CD40L T cell dendritic cell

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