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Diclofenac sodium aqueous systems at low concentrations: Interconnection between physicochemical properties and action on hydrobionts

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Journal of Environmental Sciences 2020年第2期32卷 177-186页

作者： Irina S.Ryzhkina Yuliya V.Kiseleva Lyaisan I.murtazina Tatyana V.Kuznetsova Erik R.Zainulgabidinov Igor V.Knyazev Andrew m.Petrov sergey E.Kondakov Alexander I.Konovalov Arbuzov Institute of Organic and Physical Chemistry FRC Kazan Scientific CenterRussian Academy of Sciences8 Arbuzov str.Kazan 420088Russia Institute for Problems of Ecology and mineral Wealth Use of Tatarstan Academy of Sciences 28 Daurskaya Str.Kazan 420087Russia Lomonosov moscow State University Chemistry Dept.1/3 Lenin HillsMoscow 119899Russia

Diclofenac sodium(DS) is a widely used nonsteroidal anti-inflammatory drug(NSAIDs).NSAIDs are poorly removed during standard wastewater *** consequences of the presence of NSAIDs in rivers and lakes at 10-11–10-8 mol/L are not yet established;therefore, ecotoxicologists have focused their efforts on studying the effect of lowconcentration NSAIDs on fish and hydrobionts, and also on predicting the potential risks to *** provides some information about the bioeffects of some NSAID solutions in low concentrations but there is no physicochemical explanation for these *** the physicochemical patterns of DS solutions in the low range of concentrations and establishing an interconnection between the solutions’ physicochemical properties and bioeffects can provide a conceptually new and important source of information regarding the unknown effects of *** physicochemical properties and action of DS solutions on Ceriodaphnia affinis cladocerans,Paramecium caudatum infusoria, Chlorella vulgaris unicellular green algae, as well as on the growth of the roots of Triticum vulgare wheat seeds, were studied in the calculated concentration range of 1 × 10-3–1 × 10-18 mol/*** relationship between these phenomena was established using the certified procedures for monitoring the toxicity of natural water and *** was shown for the first time that water solutions of DS are dispersed systems in which the dispersed phase undergoes a rearrangement with dilution, accompanied by changes in its size and properties, which affects the nonmonotonic dependences of the system’s physicochemical properties and could cause nonmonotonic changes in action on hydrobionts in the low concentration range.

关键词： Diclofenac sodium Low concentration Aqueous solutions Physicochemical properties Hydrobionts Toxicity

Non-Local and memory Character of Frictional Energy Dissipation on Atomic Scale

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Engineering（科研） 2017年第1期9卷 14-21页

作者： sergey Yu. Krylov Joost W. m. Frenken Frumkin Institute of Physical Chemistry and Electrochemistry Russian Academy of Sciences Moscow Russia Advanced Research Center for Nanolithography Amsterdam The Netherlands

The traditional description of atomic-scale friction, as investigated in Friction force microscopy, in terms of mechanical stick-slip instabilities appears so successful that it obscures the actual mechanisms of frictional energy dissipation. more sophisticated theoretical approach, which takes into account damping explicitly, reveals the existence of some hidden, unexplained problems, like the universal nearly-critical damping and unexpectedly high value of the dissipation rate. In this paper, we combine analysis in the framework of nonequilibrium statistical mechanics with simple atomistic modeling to show that the hidden problems of atomic scale friction find their origin in the nontrivial character of energy dissipation that is non-local and dominated by memory effects, which have not been addressed before in the context of dry, atomic-scale friction.

关键词： Nanotribology Atomic Scale Friction Dissipation Non-Locality memory

Resolution and contrast enhancement of laser-scanning multiphoton microscopy using thulium-doped upconversion nanoparticles

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Nano Research 2019年第12期12卷 2933-2940页

作者： Alexey B.Kostyuk Artem D.Vorotnov Andrey V.Ivanov Arthur B.Volovetskiy Aleksandr V.Kruglov Lyudmila m.Sencha Liuen Liang Evgenii L.Guryev Vladimir A.Vodeneev sergey m.Deyev Yiqing Lu Andrei V.Zvyagin Lobachevsky State University of Nizhny Novgorod Nizhny Novgorod 603950Russia Center of Biomedical Engineering Institute of Molecular MedicineSechenov UniversityMoscow 119991Russia ARC Centre of Excellence"Nanoscale BioPhotonics" Department of Physics and AstronomyMacquarie UniversitySydney 2109Australia Institute ofBioorganic Chemistry Russian Academy of SciencesMoscow 117997Russia

High-contrast optical imagi ng is achievable using phosphoresce nt labels to suppress the short-lived background due to the optical backscatterand autofluoresce ***,the long-lived phosphorescence is generally incompatible with high-speed laser-scan ning imaging ***,we show that upc on versi on nan oparticles of structure NaYF4:Yb co-doped with 8%Tm(8T-UCNP)in combi nation with a commerciallaser-scanning multiphoton microscopy are uniquely suited for labeling biological systems to acquire high-resolution images with the enhancedcon *** comparison with many phosphoresce nt labels,the 8T-UCNP emission lifetime of-15μs affords rapid image ***-order optical nonlinearity of the 8T-UCNP(n=4,as confirmed experimentally and theoretically)afforded pushing the resolution limitattain able with UCNPs to the *** contrast enha nceme nt was achieved by suppressing the backgro und using(i)ban dpassspectral filtering of the narrow emission peak of 8T-UCNP at 455-nm,and(ii)time-gating implemented with a time-correlated single-photon counting system that demonstrated the contrast enhancement of>2.5-fold of polyethyle neimine-coated 8T-UCNPs take n up by huma nbreast adeno carcinoma cells *** a result,discrete 8T-UCNP nan oparticles became clearly observable in the freshly excised splee ntissue of laboratory mice 15-min post in trave nous injectio n of an 8T-UCNP *** dem on strated approach paves the way forhigh-contrast,high-resoluti on,and high-speed multiphot on microscopy in challe nging envir onments of i ntense autofluorescence,exogenous staining,and turbidity,as typically occur in intravital imaging.

关键词： upconversion nanoparticles autofluorescence time-gated imaging scanning microscopy time-correlated single photon counting

multiscale wood micromechanics and size effects study via nanoindentation

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生物质资源与工程(英文) 2023年第3期8卷 246-264页

作者： Yuri I.Golovin Alexander A.Gusev Dmitry Yu.Golovin sergey m.matveev Alexander I.Tyrin Alexander A.Samodurov Viktor V.Korenkov Inna A.Vasyukova maria A.Yunack Institute“Nanotechnology and Nanomaterials” G.R.Derzhavin Tambov State University392000 TambovRussia Department of Chemical Enzymology School of ChemistryLomonosov Moscow State University119991 MoscowRussia Research and Educational Center«Sustainable Development of the Forest Complex» Voronezh State Forestry University Named after G.F.Morozov394087 VoronezhRussia Department of Functional Nanosystems and High-Temperature materials National University of Science and Technology“MISIS”119991 MoscowRussia

Wood as a material is a natural composite with a complex hierarchically arranged *** scale levels of wood structure contribute to its macroscopic mechanical *** nature of such characteristics and deformation modes differs radically at different scale *** macroscopic properties are well studied,and the relevant information can be easily found in the ***,the knowledge of the deformation mechanisms at the mesoscopic level corresponding to the cellular structure of early and late wood layers of annual growth rings is *** hinders building the comprehensive multiscale model of how wood mechanical properties are *** paper described the results of scanning of mechanical properties of softwood and hardwood samples,such as common pine,small-leaf lime,and pedunculate oak,by means of nanoindentation(NI).The NI technique allows varying the size of deformed region within a wide range by altering maximal load(P max)applied to the indenter so that one can re-peatedly and non-destructively test wood structural components at different scale levels on the same sample without changing the technique or *** was discovered that the effective microhardness(H eff)and Young’s modulus(E eff)decreased manifold with P max growing from 0.2 to 2000 *** drop in H effwas observed when the locally deformed region grew,and re-sulting from P max increase generally follows the rule similar to the Hall-Petch relation for yield stress,strength,and hardness initially established for metals and alloys,though obviously in those cases the underlying internal mechanisms are quite *** nature and micromechanisms of such size effect(SE)in wood revealed using NI were discussed in this *** P maxmN,the deformed area under the pyramidal Berckovich indenter was much smaller than the cell wall ***,in this case,NI measured the internal mechanical properties of the cell wall material as long as free boundaries impact

关键词： Nano/microhardness Scanning nanoindentation Annual growth ring Early and late wood Dendrochronology

Electrochemical performance of Klason lignin as a low-cost cathode-active material for primary lithium battery

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Journal of Energy Chemistry 2015年第3期24卷 346-352页

作者： sergey V Gnedenkov Denis P Opra Ludmila A Zemnukhova sergey L Sinebryukhov Iliya A Kedrinskii Olga V Patrusheva Valentin I Sergienko Institute of Chemistry Far Eastern BranchRussian Academy of Sciences Far Eastern Federal University Siberian State Technological University

A few classes of organic compounds are promising electrode-active materials due to their high power and energy densities,low cost,environmental friendliness,and *** the present work,the possibility of using Klason lignin extracted from buckwheat husks as a cathode-active material for a primary lithium battery has been investigated for the first *** reaction mechanism in the lithium/lignin electrochemical cell was suggested based on the deep galvanostatic discharge（up to 0.005 V） data and cyclic voltammetry *** dependence of the electrochemical behavior of the Klason lignin on the milling degree was *** maximum specific capacity of the lignin is equal to 600 m Ah g-1at a discharge current density of 75 μA *** effect of the thermal treatment of the Klason lignin cathode at250°C on the cell performance was *** was found that the discharge capacity of the cell increased by 30% in the range from 3.3 to0.9 V for the treated cathode *** results demonstrate the prospects of using Klason lignin-based electrochemical cells as low-rate primary power sources.

关键词： Klason lignin primary lithium battery organic electrode buckwheat husks

The Confirmed Validity of the Explanatory Aspect of the Thermohydrogravidynamic Theory Concerning the Evaluated maximal magnitude of the Strongest Earthquake of the Earth near the Predicted Date 2021.1 AD during the Range from October 27, 2020 to may 17, 2021 AD

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Journal of Geoscience and Environment Protection 2022年第7期10卷 319-330页

作者： sergey V. Simonenko V. I. Il’ichev Pacific Oceanological Institute Far Eastern Branch of Russian Academy of Sciences Vladivostok Russia

We present the explanation (in the frame of the established thermohydrogravidynamic technology) of the maximal magnitude m = 8.1 (according to the U.S. Geological Survey) of the strongest earthquake of the Earth occurred in Kermadec Islands, New Zealand on march 4, 2021 AD (during the considered range from October 27, 2020 to may 17, 2021 AD). This strongest earthquake occurred near the calculated date 2021.1 AD corresponding (in the frame of the thermohydrogravidynamic theory) to the local maximal combined planetary and solar integral energy gravitational influence on the internal rigid core of the Earth. To obtain this explanation, we have analyzed the strongest earthquakes of the Earth (according to the U.S. Geological Survey) occurred near the dates of the local maximal combined planetary and solar integral energy gravitational influences on the internal rigid core of the Earth.

关键词： Thermohydrogravidynamic Theory Non-Stationary Cosmic Gravitation Gen-eralized First Law of Thermodynamics Cosmic Geology Cosmic Geophysics Cosmic Seismology Global Seismotectonic Processes Global Prediction Thermohydrogravidynamic Principles Thermohydrogravidynamic Technology

A GIS-based modeling of snow accumulation and melt processes in the Votkinsk reservoir basin

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Journal of Geographical Sciences 2018年第2期28卷 221-237页

作者： sergey V. PYANKOV Andrey N. SHIKHOV Nikolay A. KALININ Eugene m. SVIYAZOV Department of Cartography and Geoinformatics Perm State University 15 Bukireva Street 614990 Perm Russia Department of meteorology and Atmosphere Protection Perm State University 15 Bukireva Street 614990 Perm Russia

Coupled hydrological and atmospheric modeling is an efficient method for snowmelt runoff forecast in large basins. We use short-range precipitation forecasts of mesoscale at- mospheric Weather Research and Forecasting （WRF） model combining them with ground-based and satellite observations for modeling snow accumulation and snowmelt processes in the Votkinsk reservoir basin （184,319 km2）. The method is tested during three winter seasons （2012-2015）. The mODIS-based vegetation map and leaf area index data are used to calculate the snowmelt intensity and snow evaporation in the studied basin. The GIS-based snow accumulation and snowmelt modeling provides a reliable and highly detailed spatial distribution for snow water equivalent （SWE） and snow-covered areas （SCA）. The modelling results are validated by comparing actual and estimated SWE and SCA data. The actual SCA results are derived from mODIS satellite data. The algorithm for assessing the SCA by mODIS data （ATBD-mOD 10） has been adapted to a forest zone. In general, the proposed method provides satisfactory results for maximum SWE calculations. The calculation accuracy is slightly degraded during snowmelt periods. The SCA data is simulated with a higher reliability than the SWE data. The differences between the simulated and actual SWE may be explained by the overestimation of the WRF-simulated total precipitation and the unrepresentativeness of the SWE measurements （snow survey）.

关键词： snow accumulation and snowmelt processes snow water equivalent GIS-based modeling WRF-ARW model

Web service for biodiversity estimation using remote sensing data

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International Journal of Digital Earth 2008年第4期1卷 367-376页

作者： mikhail A.Popov Nataliia N.Kussul sergey A.Stankevich Anna A.Kozlova Andrii Yu.Shelestov Oleksii m.Kravchenko mykhailo B.Korbakov Serhiy V.Skakun Scientific Centre for Aerospace Research of the Earth KievUkraine Department of Space Information Technologies and Systems Space Research Institute NASU-NSAUKievUkraine

This paper presents a technique for the assessment and mapping of land biodiversity by using remote sensing *** proposed approach uses a fuzzy model that encapsulates different ecological factors influencing *** imple... 详细信息

关键词： potential biodiversity index remote sensing data product pre-Black Sea region of the Ukraine web service

Viscous creep of ice-rich permafrost debris in a recently uncovered proglacial area in the Tianshan mountains, China

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Advances in Climate Change Research 2022年第4期13卷 540-553页

作者： Yu ZHOU Guo-Yu LI Hui-Jun JIN sergey SmARCHENKO Wei mA Qing-Song DU Jin-ming LI Dun CHEN State Key Laboratory of Frozen Soils Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China Da Xing'anling Observation and Research Station of Frozen-ground Engineering and Environment Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesJagdaqi 165000China School of Civil Engineering and Institute of Cold Regions Science and Engineering Northeast Forestry UniversityHarbin 150040China Geophysical Institute University of Alaska FairbanksFairbanksAK 99775USA

Since the Little Ice Age and as a consequence of climate warming,many recently deglaciated forefields have become and will continue to evolve into large ice-debris complexes exposed to periglacial processes and *** transitional processes have significant implications for geomorphologic shaping and water supply for the downstream communities,especially in arid regions,but our understanding of their evolutionary processes and their potential geomorphic and hydrological impacts is stil limited.A landform transition from partly debris-covered glaciers to ice-rich permafrost debris undergoing slow viscous creep was revealed in the Aerzailaikunai Valley in the eastern Tianshan mountains in China based on the results of in-situ observations and measurements(boreholes,ground temperature monitoring,electrical resistivity tomography surveys,and continuous global positioning system measurements,among others).The internal structure of ice-tll mixture contains pure ice layers,supersaturated frozen sands with ice lenses,and ice-bearing blocks with maximum volumetric contents of heterogeneous ice at 35%-60%.Beneath an 1.5-m-thick active layer,permafrost reached far into the underlying bedrock with the mean annual ground temperature of-2.1℃ at the depth of 20 *** higher surface velocities(with an accumulative displacement of 65 mm from October 2019 to may 2020)and extremely high electrical resistivity(several million Ω m)of the debris-covered glacier margin were in sharp contrast to those of the progressively stabilizing ground surface(up to 16 mm)and the lower zones with relatively smaler electrical resistivity(several thousand Ω m).Combined with the borehole stratigraphy(higher rock content),monitored ground temperatures(permafrost environment),lower electrical resistance(ice-rich moraine),and continuous global positioning system results(viscous creeping),this study documents a transition from glacial to periglacial conditions,materials and processes characteristic

关键词： Alpine permafrost Viscous creep Debris-covered glacier margins Climate warming Landform transition Evolution of rock glacier