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Intensified warming suppressed the snowmelt in the Tibetan Plateau

Advances in Climate Change Research 2024年第3期15卷 452-463页

作者： Xiang li Peng CUI Xue-Qin ZHANG fang ZHANG Key Lab of Land Surface Pattern and Simulation Institute of Geographic Sciences and Natural Resources ResearchBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China China‒Pakistan Joint Research Center on Earth Sciences Chinese Academy of Sciences and Higher Education CommissionIslamabad 45320Pakistan

Understanding how hydrological factors interrelate is crucial when examining the impact of climate warming on ***,these connections are often overlooked,leading to an unclear relationship between temperature and *** study investigates the complex interplay between temperature and snowmelt in the Tibetan Plateau from 1961 to 2020,focusing on how extreme high-temperature events affect the frequency of extreme *** a structural equation model,we detected three temperature-related factors that predominantly influenced snowmelt and extreme *** annual average temperature was found to have a significant indirect impact on snowmelt,mediated by changes in snowfall,snow depth and snow *** contrast,high-temperature days(daily maximum temperatures exceeding the 90th percentile)and heat waves(at least three consecutive high-temperature days)negatively affected extreme snowmelt directly or *** direct effect of increasing extreme temperature events was associated with an earlier onset of high-temperature periods,which accelerated snowmelt and shortened the duration of extreme snowmelt ***,the reduction in snow cover owing to warming emerged as a main factor suppressing snowmelt and extreme snowmelt *** also revealed spatiotemporal variations in the temperature‒snowmelt relationship that highly depended on changes in snowmelt *** study elucidated why warming suppresses snowmelt and extreme snowmelt events in the Tibetan Plateau,highlighting the mediating roles of snow-related and phenological *** findings will provide scientific support for climate simulation and water management policymaking in alpine regions worldwide.

关键词： Climate change Extreme temperature Snowmelt Structural equation model Tibetan Plateau

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Theoretical and experimental investigations on single-atom catalysis:Pt_(1)/FeO_(x) for water-gas shift reaction

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Nano Research 2024年第9期17卷 8627-8637页

作者： Shan-Fei Wang Yangyang li Haiyan Wang Jin-Xia liang Chun Zhu Botao qiao School of Chemistry and Chemical Engineering Guizhou UniversityGuiyang 550025China CAS Key Laboratory of Science and Technology on Applied Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China University of Chinese Academy of Sciences Beijing 100049China

Oxide-supported metal single-atom catalysts(SACs)have exhibited excellent catalytic performance for water-gas shift(WGS)***,we report the single-atom catalyst Pt1/FeOx exhibits excellent medium temperature catalytic performance for WGS reactions by the density functional theory(DFT)calculations and experimental *** calculations indicate that H_(2)O molecules are easily dissociated at oxygen vacancies,and the formed*OH and*O are adsorbed on Pt1 single atoms and the adjacent O atoms,*** studying four possible reaction mechanisms,it is found that the optimal WGS reaction pathway is proceeded along the carboxyl mechanism(pathway III),in which the formation of*COOH intermediates can promote the stability of Pt_(1)/FeO_(x) SAC and the easier occurrence of WGS *** energy barrier of the rate-determining step during the entire reaction cycle is only 1.16 eV,showing the high activity for the medium temperature WGS reaction on Pt_(1)/FeO_(x) SAC,which was verified by experimental ***,the calculated turnover frequencies(TOFs)of CO_(2)and H_(2)formation on Pt1/FeOx at 610 K(337℃)can reach up to 1.14×10^(-3)s^(-1)·site^(-1)through carboxyl *** this work,we further expand the application potential of Pt1/FeOx SAC in WGS reaction.

关键词： water-gas shift(WGS)reaction single-atom catalyst(SAC) density functional theory(DFT) thermocatalysis

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Temperature-adaptive metasurface radiative cooling device with excellent emittance and low solar absorptance for dynamic thermal regulation

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Advanced Photonics 2024年第4期6卷 70-82页

作者： Junlin Yang Qianyi li Shiqiao liu Debao fang Jingyao Zhang Haibo Jin Jingbo li Beijing Institute of Technology School of Materials Science and Engineering Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications

Passive radiative cooling is a promising passive cooling technology that emits heat to deep space without energy consumption. Nevertheless, the persistent challenge of overcooling in static radiative techniques has raised concerns. Although a desirable solution is suggested based on vanadium dioxide（VO2）in the form of a Fabry–Perot（F–P） resonant cavity, the inherent contradiction between desired high emissivity（ε） and low solar absorptance(αsol) remains a notable limitation. Here, we employed a simple mask-filling technique to develop a temperature-adaptive metasurface radiative cooling device（ATMRD） for dynamic thermal regulation. Simulation and experimental results substantially evidenced that multiple localized polariton resonances were induced by the VO2metasurface, significantly enhancing the thermal emittance of the ATMRDs. The engineered ATMRD achieved an amazing switch of the atmospheric window emittance from 0.13 to 0.85 when the surface temperature exceeds a pre-set transition temperature, accompanied by a commendable αsolof 27.71%. The mechanism of multiple localized polariton resonances is discussed in detail to understand the enhanced performance based on the investigation of the relationship between the metasurface structure and multiple localized polariton resonances. We demonstrate an efficient smart radiative technique achieved by a simple micro/nanoprocess and, most importantly, contribute a valuable reference for the design of radiative devices, which is crucial in various areas such as passive cooling,smart windows, multifunctional electromagnetic response, and space application technologies.

关键词： dynamic radiative cooling emittance metasurface plasmon resonance vanadium dioxide

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Tuberculosis Prevalence Trends from a Predictive Modelling Study-10 High-Burden Countries,1980-2035

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China CDC weekly 2024年第12期6卷 225-229,I0001,I0002页

作者： Qiuping Chen qiao liu Kangguo li Laurent Gavotte Roger Frutos Tianmu Chen CIRAD IntertrypMontpellierFrance Universitéde Montpellier MontpellierFrance State Key Laboratory of Molecular Vaccinology and Molecular Diagnostics National Innovation Platform for Industry-Education Integration in Vaccine ResearchXiamen UniversityXiamen CityFujian ProvinceChina State Key Laboratory of Vaccines for Infectious Diseases Xiang An Biomedicine LaboratorySchool of Public HealthXiamen UniversityXiamen CityFujian ProvinceChina Espace-Dev Universitéde MontpellierMontpellierFrance

What is already known about this topic?Given the challenges presented by drug-resistant strains of tuberculosis(TB)and the rising mobility of the population,achieving the objective of eradicating TB appears *** is added by this report?The examination of TB incidence trends in 10 highburden countries(HBCs)indicated a steady rise in cases,with India and China jointly accounting for nearly 70%of the *** for the future show diverse trajectories in these countries,with potential difficulties in reaching the TB elimination target,especially in Nigeria,Congo,and South *** are the implications for public health practice?The number of TB cases is on the *** is crucial to learn from successful strategies to improve TB prevention and control worldwide through collaborative efforts.

关键词： tuberculosis uncertain Tuberculosis

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CdTe QDs@SiO2 composite material for efficient photocatalytic degradation of tetracycline composites

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Green Chemical Engineering 2024年第4期5卷 533-542页

作者： Taihang Zhou Fen qiao Sen Qian Shoaib Muhammad Haitao li Yanzhen liu School of Energy & Power Engineering Jiangsu University Institute for Energy Research Jiangsu University

In the contemporary context,tetracycline is widely utilized as a prevalent antibiotic in various facets of ***,the excessive use of antibiotics has caused visible environmental ***,the scientific community has increasingly focused on developing catalysts that exhibit exceptional efficacy in the proficient degradation of *** this study,a novel nanomaterial was developed to encapsulate Cd Te quantum dots （QDs） with a *** distinct synthesis approach generated a composite material that showed heterogeneity and considerably increased the contact area with ***,the transfer of photoelectron to the SiO2spheres was significantly improved,leading to a more efficient separation during the catalytic *** study investigated how different factors,such as the loading of the catalyst,the initial concentration of tetracycline,p H levels,and the wight ratio of Cd Te QDs （SiO2+Cd Te QDs） affected the effectiveness of photocatalytic tetracycline *** findings indicated that the optimal degradation efficiency was observed at a catalyst concentration of 0.25 g/L and a solution p H of 9,leading to an impressive degradation rate of 96%within a mere 2 h timeframe.

关键词： Photocatalysis Silica-based catalyst Photocatalytic degradation Photocatalytic mechanism

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内波吸引子的数值模拟

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海洋学报 2010年第6期32卷 25-34页

作者：王刚乔方利国家海洋局第一海洋研究所山东青岛266061 海洋环境科学和数值模拟国家海洋局重点实验室山东青岛266061

密度稳定层结的流体中产生的内波沿着由内波固有频率、流体浮力频率等因素所确定的特征线(或内波射线)传播。边界上的反射不改变内波的频率,从而也不改变反射后的内波特征线与重力方向所成的夹角。侧边界倾斜的封闭容器内,内波能量沿特... 详细信息

密度稳定层结的流体中产生的内波沿着由内波固有频率、流体浮力频率等因素所确定的特征线(或内波射线)传播。边界上的反射不改变内波的频率,从而也不改变反射后的内波特征线与重力方向所成的夹角。侧边界倾斜的封闭容器内,内波能量沿特征线传播的过程中经侧壁、表面和底面的反射可能会集中在一个封闭的轨道上,形成内波吸引子。该现象已经得到水槽试验、线性理论和数值试验的验证。本文利用非线性非静压的环流模式MITgcm,模拟了二维封闭区域中(1,1)-吸引子和(2,1)-吸引子的形成过程,并讨论初值条件对它们的影响。稳定的(1,1)-吸引子其极限环两侧流速出现很强的剪切流。当减小地形的坡度时,由于线性因素的增加,吸引子的结构不变,但吸引子厚度在相空间中的收缩速度加快。对于(2,1)-吸引子,由于轨道所成的两个环中间的节点耗散了部分能量,吸引子的收敛速度较慢。节点处,流体速度始终为0,但存在强烈混合,流体浮力频率呈现振幅较大的周期变化。

关键词：内波吸引子 MITgcm 非静压内波特征线均匀层结

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Biobased Furfurylated Poplar Wood for Flame-Retardant Modification with Boric Acid and Ammonium Dihydrogen Phosphate

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Journal of Renewable Materials 2024年第8期12卷 1355-1368页

作者： Ming Ni Lei li Yiqiang Wu Jianzheng qiao Yan Qing Ping li Yingfeng Zuo College of Materials Science and Engineering Central South University of Forestry and TechnologyChangsha410004China College of Furniture and Art Design Central South University of Forestry and TechnologyChangsha410004China

Furfurylated wood exhibits excellent dimensional stability and corrosion resistance,making it a promising material for constructing buildings,but it is highly ***,flame-retardant furfurylated poplar wood was produced via a two-step process utilizing boric acid(BA)and ammonium dihydrogen phosphate(ADP)as flame-retardant components,and biomass-derived furfuryl alcohol(FA)as a *** acidity of BA and ADP allowed them to catalyze the polymerization of FA,which formed a cross-linked network that immobilized BA and ADP inside the *** addition of BA/ADP substantially delayed the time to ignition from 10 to 385 s and reduced the total heat release and total smoke release by 58.75%and 77.31%,*** of the pyrolysis process showed that the decomposition products of BA and ADP protected the underlying furfurylated wood and diluted combustible *** method significantly improved the fire retardancy and smokeless properties of furfurylated wood,providing promising prospects for its application as an engineering material.

关键词： Poplar wood furfuryl alcohol furfurylated wood flame retardancy boric acid ammonium dihydrogen phosphate

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Fake News Detection Based on Text-Modal Dominance and Fusing Multiple Multi-Model Clues

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Computers, Materials & Continua 2024年第3期78卷 4399-4416页

作者： li fang Fu Huanxin Peng Changjin Ma Yuhan liu College of Arts and Sciences Northeast Agricultural UniversityHarbin150030China College of Engineering Northeast Agricultural UniversityHarbin150030China

In recent years,how to efficiently and accurately identify multi-model fake news has become more ***,multi-model data provides more evidence but not all are equally ***,social structure information has proven to be effective in fake news detection and how to combine it while reducing the noise information is ***,existing approaches fail to handle these *** paper proposes a multi-model fake news detection framework based on Tex-modal Dominance and fusing Multiple Multi-model Cues(TD-MMC),which utilizes three valuable multi-model clues:text-model importance,text-image complementary,and text-image ***-MMC is dominated by textural content and assisted by image information while using social network information to enhance text *** reduce the irrelevant social structure’s information interference,we use a unidirectional cross-modal attention mechanism to selectively learn the social structure’s features.A cross-modal attention mechanism is adopted to obtain text-image cross-modal features while retaining textual features to reduce the loss of important *** addition,TD-MMC employs a new multi-model loss to improve the model’s generalization *** experiments have been conducted on two public real-world English and Chinese datasets,and the results show that our proposed model outperforms the state-of-the-art methods on classification evaluation metrics.

关键词： Fake news detection cross-modal attention mechanism multi-modal fusion social network transfer learning

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Large-scale spatial data visualization method based on augmented reality

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虚拟现实与智能硬件（中英文） 2024年第2期6卷 132-147页

作者： Xiaoning qiao Wenming XIE Xiaodong PENG Guangyun li Dalin li Yingyi GUO Jingyi REN Key Laboratory of Electronics and Information Technology for Space Systems National Space Science CenterChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China Ordnance Science and Research Academy of China Beijing 100089China

Background A task assigned to space exploration satellites involves detecting the physical environment within a certain ***,space detection data are complex and *** data are not conducive for researchers'visual perceptions of the evolution and interaction of events in the space *** A time-series dynamic data sampling method for large-scale space was proposed for sample detection data in space and time,and the corresponding relationships between data location features and other attribute features were established.A tone-mapping method based on statistical histogram equalization was proposed and applied to the final attribute feature *** visualization process is optimized for rendering by merging materials,reducing the number of patches,and performing other *** The results of sampling,feature extraction,and uniform visualization of the detection data of complex types,long duration spans,and uneven spatial distributions were *** real-time visualization of large-scale spatial structures using augmented reality devices,particularly low-performance devices,was also *** The proposed visualization system can reconstruct the three-dimensional structure of a large-scale space,express the structure and changes in the spatial environment using augmented reality,and assist in intuitively discovering spatial environmental events and evolutionary rules.

关键词： Large-scale spatial data analysis Visual analysis technology Augmented reality 3D reconstruction Space environment

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Tissue adhesive,ROS scavenging and injectable PRP-based‘plasticine’for promoting cartilage repair

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Regenerative Biomaterials 2024年第1期3卷 94-107页

作者： Shiao li Dawei Niu Haowei fang Yancheng Chen Jinyan li Kunxi Zhang Jingbo Yin Peiliang Fu Department of Orthopedics Shanghai Changzheng HospitalNaval Medical UniversityShanghai 200003P.R.China Department of Polymer Materials School of Materials Science and EngineeringShanghai UniversityShanghai 200444P.R.China

Platelet-rich plasma(PRP)that has various growth factors has been used clinically in cartilage ***,the short residence time and release time at the injury site limit its therapeutic *** present study fabricated a granular hydrogel that was assembled from gelatin microspheres and tannic acid through their abundant hydrogen *** microspheres with the gelatin concentration of 10wt%and the diameter distribution of 1-10 lm were used to assemble by tannic acid to form the granular hydrogel,which exhibited elasticity under low shear strain,but flowability under higher shear *** viscosity decreased with the increase in shear ***,the granular hydrogel exhibited self-healing feature during rheology ***,granular hydrogel carrying PRP not only exhibited well-performed injectability but also performed like a‘plasticine’that possessed good *** granular hydrogel showed tissue adhesion ability and reactive oxygen species scavenging *** hydrogel carrying PRP transplanted to full-thickness articular cartilage defects could integrate well with native cartilage,resulting in newly formed cartilage articular fully filled in defects and well-integrated with the native cartilage and subchondral *** unique features of the present granular hydrogel,including injectability,plasticity,porous structure,tissue adhesion and reactive oxygen species scavenging provided an ideal PRP carrier toward cartilage tissue engineering.

关键词： cartilage regeneration granular hydrogel gelatin tannic acid PRP

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