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Role of inflammatory lipid and fatty acid metabolic abnormalities induced by plastic additives exposure in childhood asthma

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Journal of Environmental Sciences 2024年第3期137卷 172-180页

作者： Zhiyu Chen Fang Li Lei Fu Yu Xia Ying luo Ang Guo Xiaona Zhu Huifang Zhong Qian luo Institute of Biomedical and Health Engineering Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China University of Chinese Academy of Sciences Beijing 100049China Rheumatology&Immunology Depa.tment of Shenzhen Children’s Hospital Shenzhen 518038China Hubei Key Laboratory of Environmental and Health Effects of Persistent Toxic Substances Institute of Environment and HealthJianghan UniversityWuhan 430056China

Lipid metabolism play an essential role in occurrence and development of asthma,and it can be disturbed by phthalate esters(pa.s)and organophosphate fame retardants(OPFRs).As a chronic infammatory respiratory disease,the occurrence risk of childhood asthma is increased by pa.s and OPFRs exposure,but it remains not entirely clear how pa.s and OPFRs contribute the onset and progress of the *** have profiled the serum levels of pa.s and OPFRs congeners by liquid chromatography coupled with mass spectrometry,and its relationships with the dysregulation of lipid metabolism in asthmatic,bronchitic(acute infammation)and healthy(non-infammation)*** pa.s and nine OPFRs congeners were found in the serum of children(1–5 years old)from Shenzhen,and their total median levels were 615.16 ng/m L and 17.06 ng/m L,***,the serum levels of mono-methyl phthalate(MMP),tri-propyl phosphate(TPP)and tri-n-butyl phosphate(TNBP)were significant higher in asthmatic children than in healthy and bronchitic children as ***-one characteristic lipids and fatty acids of asthma were screened by machine-learning random forest model based on serum lipidome data,and the alterations of infammatory characteristic lipids and fatty acids including pa.mitic acids,12,13-Di HODE,14,21-Di HDHA,prostaglandin D2 and Lyso pa.18:2)showed significant correlated with high serum levels of MMP,TPP and *** results imply pa.s and OPFRs promote the occurrence of childhood asthma via disrupting infammatory lipid and fatty acid metabolism,and provide a novel sight for better understanding the effects of plastic additives on childhood asthma.

关键词： Phthalate esters Organophosphate fame retardants Childhood asthma Lipid and fatty acid metabolism Machine-learning random forest model Chronic airway infammation

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In situ modification of heavy oil catalyzed by nanosized metal-organic framework at mild temperature and its mechanism

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Chinese Journal of Chemical Engineering 2024年第3期67卷 166-173页

作者： Li Wang Ji-Xiang Guo Rui-Ying Xiong Chen-Hao Gao Xiao-Jun Zhang Dan luo The Unconventional Oil and Gas Institute China University of Petroleum-BeijingBeijing 102200China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China

Two catalysts, nano-sized cobalt-metal-organic framework(Co-MOF) and nickel(Ni)-MOF, were successfully prepa.ed by the modification method. Tetralin(C10H12) was used as the hydrogen donor for the catalytic cracking and hydrogenation modification study of the dehydrated crude oil from the Shengli Oilfield. The optimal reaction conditions were determined through orthogonal experiments, and the components of the crude oil and modified oil samples were analyzed. The results revealed that the nanoMOF catalysts were successfully prepa.ed and exhibited high catalytic activity. They could catalyze the cracking of large molecules in heavy oil at mild temperatures(pa.s to 1266.2 m pa.s,with a viscosity reduction rate of 91.97%. The modification effect of Co-MOF was the next best, which could reduce the viscosity of heavy oil to 2500.1 m pa.s with a viscosity reduction rate of 84.14%. Molecular dynamics simulations revealed a strong interaction force between the MOF surface and asphaltene molecules. In the process of heavy-oil catalytic hydrogenation, the nano-MOF catalyst exhibited high catalytic activity. On the one hand, the empty d orbitals outside the metal atoms in the catalyst could polarize the carbon atoms in the organic matter, accelerating the breaking of long chains. On the other hand, the metal atoms in the catalyst could bond with the carbon σ bonds, breaking the carbon-carbon bonds. This disrupted the structure of the recombined components in the crude oil, irreversibly reducing the viscosity of the heavy oil and improving its fluidity.

关键词： Nano-sized MOF Petroleum Viscosity reduction Catalyst Nanomaterials

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Single-ended Time Domain Fault Location Based on Transient Signal Measurements of Transmission Lines

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Protection and Control of Modern Power Systems 2024年第2期9卷 61-74页

作者： Jian luo Yao Liu Qiushi Cui Jiayong Zhong Lin Zhang Chongqing University ChongqingChina Taiyuan University of Technology TaiyuanChina School of Electrical Engineering and with the Liyang Smart City Research Institute Chongqing UniversityChongqing 400044China Electrical Engineering from chongqing University ChongqingChina State Grid Chongqing Electric Power Compa.y Research Institute ChongqingChina

Precise fault location plays an important role in the reliability of modern power *** the in-creasing penetration of renewable energy sources,the power system experiences a decrease in system inertia and alterations in steady-state characteristics following a fault *** existing single-ended phasor domain methods assume a certain impedance of the remote-end system or consistent current phases at both *** problems present challenges to the applicability of con-ventional phasor-domain location *** pa.er presents a novel single-ended time domain fault location method for single-phase-to-ground faults,one which fully considers the distributed pa.ameters of the line *** fitting of transient signals in the time domain is real-ized to extract the instantaneous amplitude and ***,to eliminate the error caused by assumptions of lumped series resistance in the Bergeron model,an im-proved numerical derivation is presented for the distrib-uted pa.ameter line *** instantaneous symmet-rical components are extracted for decoupling and inverse transformation of three-phase recording *** on the above,the equation of instantaneous phase constraint is established to effectively identify the fault *** proposed location method reduces the negative effects of fault resistance and the uncertainty of remote end pa.rameters when relying on one-terminal data for ***,the proposed fault analysis methods have the ability to adapt to transient processes in power *** compa.isons with existing methods in three different systems,the fault position is correctly identified within an error of 1%.Also,the results are not affected by sampling rates,data windows,fault inception angles,and load conditions. Index Terms—Fault location,distributed pa.ameter line model,transient signal,renewable energy,instantaneous phase.

关键词： Fault location distributed pa.ameter line model transient signal renewable energy instantaneous phase

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Activatable fluorescent probes for imaging and diagnosis of rheumatoid arthritis

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Military Medical Research 2024年第2期11卷 287-307页

作者： pa. luo Fu-Qiang Gao Wei Sun Jun-You Li Cheng Wang Qing-Yu Zhang Zhi-Zhuo Li Peng Xu Depa.tment of Joint Surgery Honghui HospitalXi'an Jiaotong UniversityXi'an 710054China Depa.tment of Orthopedics China-Japan Friendship HospitalBeijing 100029China Depa.tment of Orthopa.dic Surgery of the Perelman School of Medicine University of PennsylvaniaPhiladelphiaPA 19104USA School of Mechanical Engineering Sungkyunkwan UniversitySuwon 16419South Korea Depa.tment of Orthopa.dic Surgery Peking University Third HospitalPeking UniversityBeijing 100191China Depa.tment of Orthopedics Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinan 250021China State Key Laboratory of Pharmaceutical Biotechnology Division of Sports Medicine and Adult Reconstructive SurgeryDepartment of Orthopedic SurgeryNanjing Drum Tower Hospitalthe Affiliated Hospital of Nanjing University Medical SchoolNanjing 210008China

Rheumatoid arthritis(RA)is a systemic autoimmune disease that is primarily manifested as synovitis and polyarticular opa.ity and typically leads to serious joint damage and irreversible disability,thus adversely affecting locomotion ability and life ***,good prognosis heavily relies on the early diagnosis and effective therapeutic monitoring of *** fluorescent probes play vital roles in the detection and imaging of biomarkers for disease diagnosis and in vivo ***,we review the fluorescent probes developed for the detection and imaging of RA biomarkers,namely reactive oxygen/nitrogen species(hypochlorous acid,peroxynitrite,hydroxyl radical,nitroxyl),pH,and cysteine,and address the related challenges and prospects to inspire the design of novel fluorescent probes and the improvement of their performance in RA studies.

关键词： Rheumatoid arthritis Fluorescent probe Imaging Diagnosis Biomarker

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An underwater vest containing an antioxidant MXene hydrogel for sensitive recognition of fish locomotion

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Microsystems & Nanoengineering 2024年第2期10卷 115-131页

作者： Chengxiu Yang Jiafei Hu Lihui Liu Shaowei Wu Mengchun pa. Yan Liu Haomiao Wang Peisen Li Qi Zhang Weicheng Qiu Huihui luo College of Intelligence Science and Technology National University of Defense TechnologyChangsha410073China

The perception of fish locomotion is important for understanding their adaptive behaviors and ethological ***,the main strategy used for extracting fish attitudes involves the use of a vision-based monitoring system,which is limited in its range of observation and cannot perform tracking for long ***,we report the use of a wearable tagging electronic device,referred to as an underwater vest,to capture the surrounding flow field disturbances triggered by swimming or momentary postural *** of these goals were achieved by integrating a pa.r of pseudocapa.itive pressure-sensing units and a flexible circuit ***,additional conditions,such as variable hydraulic pressures and minimal changes in fish posture,require high stability and sensitivity of the sensing ***,hybrid hydrogel electrodes were developed through cross-linking MXene with holey-reduced graphene oxide nanosheets and further modification with 1-ethyl-3-methylimidazolium dicyanamide ionic liquids,which increased the interfacial capa.itance and long-term interfacial activity of the ***,the sensing unit exhibited ultrahigh sensitivity(S_(max)~136,207 kpa.(−1))in an aquatic environment for 60 days and superior high-pressure resolution(10 pa.within a wide working range of 1 ***,an underwater vest integrated with such sensing units clearly distinguished and recorded fish *** believe that the designed device may open avenues in flow field monitoring and ocean current detection and provide new insights into the development of sensitive underwater tagging.

关键词： underwater fish linking

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Deep insight of unique phase transition behaviors and mechanism in Zr_(2)Co-H isotope system with ultra-low equilibrium pressure

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Rare Metals 2024年第1期43卷 212-224页

作者： Yang Liu pa.-pa. Zhou Xue-Zhang Xiao Jia-Cheng Qi Jia-Peng Bi Tiao Ying Xing-Wen Feng Yan Shi Wen-Hua luo Li-Xin Chen State Key Laboratory of Silicon Materials School of Materials Science and EngineeringZhejiang UniversityHangzhou 310027China Institute of Materials China Academy of Engineering PhysicsMianyang 621907China Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province Hangzhou 310013China

Efficient capture,safe storage and release of tritium from the international thermonuclear experimental reactor(ITER) reaction exhaust gas is a perplexing problem,and the development of an efficient tritium-getter material with ultra-low hydrogenation equilibrium pressure is considered as a reliable *** this work,Zr_(2)Co alloy was selected as a tritium-getter material and prepa.ed through induction levitation *** performance test results show that Zr_(2)Co exhibits an ultra-low hydrogenation equilibrium pressure of 3.22 × 10^(-6) pa.at 25℃ and excellent hydriding kinetics under a low hydrogen pressure of 0.005 ***,unique phase transition behaviors were presented in Zr_(2)Co-H ***,Zr_(2)CoH_(5) formed by Zr_(2)Co hydrogenated at room temperature is initially decomposed into ZrH_(2) and ZrCoH_(3) at200 ℃.With the temperature increasing to 350 ℃,ZrCoH_(3)is dehydrogenated to ZrCo,and then ZrCo further reacts with ZrH_(2) at 650 ℃ to reform Zr_(2)Co and *** the staged phase transition pa.hways during dehydrogenation,the decomposition of Zr_(2)CoH_(5) occurs preferentially,which is well accordance with both the smallest reaction energy barrier and the maximum reaction spontaneity that are determined respectively from kinetics activation energy and thermodynamics Gibbs free ***,first principles calculation results indicate that the stronger binding of hydrogen in interstitial environments of ZrCoH_(3)and ZrH_(2) triggers the hydrogen-stabilized phase transformation of Zr_(2)CoH_(5).The unique phase transition mechanisms in Zr_(2)Co-H system can shed light on the further exploration and regulation of analogous staged phase transition of hydrogen storage materials.

关键词： Zr_(2)Co alloy Tritium-getter materials Ultralow equilibrium hydrogen pressure Phase transition mechanism

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Leisure-time physical activity and all-cause mortality and cardiovascular disease in adults with type 2 diabetes:Cross-country compa.ison of cohort studies

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Journal of Sport and Health Science 2024年第2期13卷 212-221页

作者： Jakob Tarp Mengyun luo Miguel Adriano Sanchez-Lastra Knut Eirik Dalene Borja del Pozo Cruz Mathias Ried-Larsen Reimar Wernich Thomsen Ulf Ekelund Ding Ding Depa.tment of Clinical Epidemiology Aarhus University&Aarhus University HospitalAarhus 8200Denmark Prevention Research Collaboration Sydney School of Public HealthThe University of SydneyCamperdownNSW 2006Australia Charles Perkins Centre the University of SydneyCamperdownNSW 2050Australia Depa.tment of Sports Medicine Norwegian School of Sports SciencesOslo 0806Norway Depa.tment of Special Didactics Faculty of Education and Sports SciencesUniversity of VigoPontevedra 36005Spain Well-Move Research Group Galicia Sur Health Research Institute(IIS Galicia Sur)SERGAS-UVIGOVigo 36213Spain Depa.tment of Chronic Diseases Norwegian Institute of Public HealthOslo 0473Norway Centre for Active and Healthy Ageing Department of Sports Science and Clinical BiomechanicsUniversity of Southern DenmarkOdense 5230Denmark Faculty of Education University of CadizCadiz 11519Spain Biomedical Research and Innovation Institute of Cadiz(INiBICA)Research Unit Puerta del Mar University HospitalUniversity of CadizCadiz 11009Spain The Centre of Inflammation and Metabolism&the Centre for Physical Activity Research RigshospitaletUniversity of CopenhagenCopenhagen 2100Denmark Depa.tment of Sports Science and Clinical Biomechanics University of Southern DenmarkOdense 5230Denmark

Purpose:This study aimed to quantify the dose-response association and the minimal effective dose of leisure-time physical activity(pa.to prevent mortality and cardiovascular disease in adults with type 2 ***:Cross-country compa.ison of 2 prospective cohort studies including 14,913 and 17,457 population-based adults with type 2 diabetes from the UK and *** leisure-time pa.was self-reported and categorized by metabolic equivalent hours per week(MET-h/week)according to World Health Organization recommendations:none,below recommendation(>0-7.49 MET-h/week);at recommended level(7.5-14.9 MET-h/week);above recommendation(>15 MET-h/week).Mortality and cardiovascular disease data were obtained from national ***:During a median follow-up of 12.4 and 9.7 years,in the UK and China cohorts,repectively,higher levels of leisure-time pa.were inversely associated with all-cause(1571 and 2351 events)and cardiovascular mortality(392 and 1060 events),mostly consistent with a linear dose-response *** below,at,and above recommendations,compa.ed with no activity,yielded all-cause mortality hazard ratios of0.94(95%confidence interval(95%CI):0.79-1.12),0.90(95%CI:0.74-1.10),and 0.85(95%CI:0.70-1.02)in British adults and 0.87(95%CI:0.68-1.10),0.88(95%CI:0.74-1.03),and 0.77(95%CI:0.70-0.85)in Chinese *** with cardiovascular mortality were more pronounced in British adults(0.80(95%CI:0.58-1.11),0.75(95%CI:0.52-1.09),and 0.69(95%CI:0.48-0.97))but less pronounced in Chinese adults(1.06(95%CI:0.76-1.47),1.01(95%CI:0.80-1.28),and 0.79(95%CI:0.69-0.92)).pa.at recommended levels was not associated with lower rates of major adverse cardiovascular events(2345 and 4458 events).Conclusion:Leisure-time pa.at the recommended levels was not convincingly associated with lower mortality and had no association with risk of major adverse cardiovascular events in British or Chinese adults with type 2 ***-time pa.above current recom

关键词： Complications Epidemiology Exercise Prevention

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Community structure and carbon metabolism functions of bacterioplankton in the Guangdong coastal zone

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Marine Life Science & Technology 2024年第3期6卷 547-561页

作者： Ziqi Peng pa.deng Wang Xiaoqing luo Qiqi Deng Ziwen Yang Jiaxue Wu Wendong Xian Weicong Yan Xiaozhen Mou Yang Yuan Wenjun Li Jialing Li State Key Laboratory of Biocontrol Guangdong Provincial Key Laboratory of Plant Stress BiologySchool of Marine SciencesSchool of EcologySchool of Life SciencesSun Yat-Sen UniversityGuangzhou 510275China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou 511458China Depa.tment of Biological Sciences Kent State UniversityKentOH 44242USA Marine Microorganism Ecological&Application Lab Marine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316000China

Coastal ecosystems are an important region for biogeochemical cycling,are a hotspot of anthropogenic disturbance and play a crucial role in global carbon cycling through the metabolic activities of *** can be broadly classified into two lifestyles:free-living(FL)and pa.ticle-attached(pa..However,how coastal bacterioplankton the community structure,co-occurrence networks and carbon metabolic functions with different lifestyles are differentiated is still largely *** these processes is necessary to better determine the contributions of coastal bacterioplankton to carbon ***,the characteristics of community structure and carbon metabolism function of bacterioplankton with two lifestyles in the coastal areas of Guangdong Province were investigated using amplicon sequencing,metagenomic,and metatranscriptomic *** results show that the main bacterioplankton responsible for carbon metabolism were the Pseudomonadota,Bacteroidota,and *** microbial community structure,carbon metabolic function,and environmental preferences differ between different *** and pa.bacteria exhibited higher carbon fixation and degradation potentials,respectively.A range of environmental factors,such as dissolved oxygen,pH,and temperature,were associated with the community structure and carbon metabolic functions of the *** activities,such as nutrient discharge,may affect the distribution of functional genes and enhance the carbon degradation functions of *** conclusion,this study increased the understanding of the role of microorganisms in regulating carbon export in coastal ecosystems with intense human activity.

关键词： pa.ticle-attached and free-living bacterioplankton Community structure Carbon metabolism Coastal ecosystem

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农地撂荒与粮食生产——一个非线性关系的考察

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华中农业大学学报（社会科学版） 2024年第2期 58-68页

作者：庄健罗必良华南农业大学经济管理学院广东广州510642 华南农业大学国家农业制度与发展研究院广东广州510642

农地撂荒现象已经受到学界广泛关注,但关于农地撂荒对粮食生产的影响还缺乏有效的定量评估。通过将农地撂荒与粮食生产纳入统一分析框架,并使用2017年中国农村家庭追踪调查数据(CRHPS)进行实证检验。研究发现:(1)农地撂荒对粮食产出的... 详细信息

农地撂荒现象已经受到学界广泛关注,但关于农地撂荒对粮食生产的影响还缺乏有效的定量评估。通过将农地撂荒与粮食生产纳入统一分析框架,并使用2017年中国农村家庭追踪调查数据(CRHPS)进行实证检验。研究发现:(1)农地撂荒对粮食产出的影响存在门槛效应,即农地撂荒需要达到一定规模才会影响粮食产出。(2)机制分析表明,农地撂荒与粮食产出之间的非线性关系是由于撂荒地块的质量差异与剩余地块要素配置水平变化共同引起的。小规模的撂荒主要涉及劣等地块,造成的粮食损失相对较小;同时,撂荒劣等地块还会提升剩余地块上的要素配置水平,带来粮食增产的效果,从而部分抵消了粮食损失。然而,这种增产效果会随着非农就业规模的增加而逐渐减弱。(3)进一步分析表明,引进农业技术和提高人力资本水平可以有效削弱农地撂荒对粮食产量的不利影响。文章强调,当前阶段的农地撂荒主要以产粮率较低的劣等地为主,并未对粮食安全构成明显威胁。此外,是否有必要采用行政手段促使劣等地块复耕种粮,应予以审慎考虑。相比之下,退耕还林(草)或改种其他经济作物等措施可能更具可行性和潜在优势。

关键词：农地撂荒粮食生产非线性关系门槛效应

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迭代奇异值方法在机械结构模态分离重构中的应用

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振动工程学报 2024年第2期37卷 210-217页

作者：罗治军田桂阎绍泽清华大学机械工程系摩擦学国家重点实验室北京100084 中国人民解放军96963部队博士创新工作站北京100084 陆军航空兵学院航电和兵器工程系北京101123

通过时频分解技术,将复杂的多模态信号分解成单模态成分,从而可以采用比较简单可靠的单模态识别方法对机械结构复杂模态信号进行参数辨识。经验小波变换(EWT)算法能有效解决模态分离问题,一些改进型EWT算法能有效克服噪声干扰,但是在模... 详细信息

通过时频分解技术,将复杂的多模态信号分解成单模态成分,从而可以采用比较简单可靠的单模态识别方法对机械结构复杂模态信号进行参数辨识。经验小波变换(EWT)算法能有效解决模态分离问题,一些改进型EWT算法能有效克服噪声干扰,但是在模态重构时,滤波器彼此重叠、临近模态互相干扰,会不可避免地出现重构模态失真。本文针对模态分离重构问题展开研究,分析了EWT算法在模态分离重构中面临的重构失真问题,提出了基于迭代截断奇异值分解(ITSVD)方法的改进算法,并在仿真信号和含结合面机械结构模型振动响应信号上进行了应用。结果表明,所提ITSVD⁃EWT算法能够更好地实现机械结构模态分离重构。

关键词：参数辨识经验模态分解机械结构经验小波变换迭代截断奇异值分解

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