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Advances in self-assembly-based circularly polarized luminescent materials

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Science China Chemistry 2024年第10期67卷 3247-3257页

作者： Bing-Hao liu Yang Zong na liu Zong-Quan Wu State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin University The School of Pharmaceutical Sciences Jilin University

Circularly polarized luminescent(CPL) materials have garnered attention for their diverse applications, including three-dimensional(3D) imaging, bio-imaging, chiral sensing, and other emerging fields. Traditionally, the fabrication of CPL-activated materials required the use of chiral luminescent small molecules. The introduction of the idea of self-assembly has transformed the production of CPL-activated materials, providing new and promising opportunities for their advancement. Through utilizing self-assembly, it is now feasible to produce chiral nano-assemblies with CPL activity not only from chiral molecules but also from non-chiral substances and inorganic nanoparticles. In addition, self-assembly routes provide a way to increase the asymmetry factor, creating possibilities for additional refinement and adjustment of CPL material characteristics. This review offers a summary of the current progress and developments in the self-assembly of small molecules and polymers, with a specific emphasis on their capacity to create or enhance CPL in different contexts. The aim of this review is to inspire interest in optical materials that are based on the principles of self-assembly.

关键词： circularly polarized luminescence photochemistry self-assembly chiral materials

Emerging clinical relevance of microbiome in cancer:promising biomarkers and therapeutic targets

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Protein & Cell 2024年第4期15卷 239-260页

作者： Jia-Hao Dai Xi-Rong Tan Han Qiao na liu State Key Laboratory of Oncology in South China Guangdong Key Laboratory of Nasopharyngeal Carcinoma Diagnosis and TherapyGuangdong Provincial Clinical Research Center for CancerSun Yat-sen University Cancer CenterGuangzhou 510050China

The profound influence of microbiota in cancer initiation and progression has been under the spotlight for years,leading to numerous researches on cancer microbiome entering clinical *** promising biomarkers and therapeutic targets,the critical involvement of microbiota in cancer clinical practice has been increasingly ***,recent progress in this field is *** describe the potential of tumor-associated microbiota as effective diagnostic and prognostic biomarkers,*** addition,we highlight the relationship between microbiota and the therapeutic efficacy,toxicity,or side effects of commonly utilized treatments for cancer,including chemotherapy,radiotherapy,and *** that microbial factors influence the cancer treatment outcome,we further summarize some dominating microbial interventions and discuss the hidden risks of these *** review aims to provide an overview of the applications and advancements of microbes in cancer clinical relevance.

关键词： microbiome cancer diagnosis prognosis therapy

Mapping the intellectual structure and emerging trends for the application of nanomaterials in gastric cancer:A bibliometric study

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World Journal of Gastrointestinal Oncology 2024年第5期16卷 2181-2199页

作者： Bo-na liu Xiao-Li Gao Ying Piao Department of Oncology General Hospital of Northern Theater CommandShenyang 110015Liaoning ProvinceChina

BACKGROUND Recent reviews have outlined the main nanomaterials used in relation to gastrointestinal tumors and described the basic properties of these ***,the research hotspots and trends in the application of nanomaterials in gastric cancer(GC)remain *** To demonstrate the knowledge structure and evolutionary trends of research into the application of nanomaterials in *** Publications related to the application of nanomaterials in GC were retrieved from the Web of Science Core Collection for this systematic review and bibliometric *** and CiteSpace were used for bibliometric and visualization *** From 2000 to 2022,the application of nanomaterials in GC developed *** keyword co-occurrence analysis showed that the related research topics were divided into three clusters:(1)The application of nanomaterials in GC treatment;(2)The application and toxicity of nanomaterials in GC diagnosis;and(3)The effects of nanomaterials on the biological behavior of GC ***,silver nanoparticles,and green synthesis are the latest high-frequency keywords that represent promising future research *** The application of nanomaterials in GC diagnosis and treatment and the mechanisms of their effects on GC cells have been major themes in this field over the past 23 years.

关键词： nanomaterials Gastric cancer Bibliometrics Drug delivery VOSviewer CiteSpace Systematic review

Discovery of GluN2A subtype-selective N-methyl-d-aspartate(NMDA)receptor ligands

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Acta Pharmaceutica Sinica B 2024年第5期14卷 1987-2005页

作者： Liyang Jiang na liu Fabao Zhao Boshi Huang Dongwei Kang Peng Zhan Xinyong liu Department of Medicinal Chemistry Key Laboratory of Chemical Biology(Ministry of Education)School of Pharmaceutical SciencesCheeloo College of MedicineShandong UniversityJinan 250012China

The N-methyl-d-aspartate(NMDA)receptors,which belong to the ionotropic Glutamate receptors,constitute a family of ligand-gated ion *** the various subtypes of NMDA receptors,the GluN1/2A subtype plays a significant role in central nervous system(CNS)*** present article aims to provide a comprehensive review of ligands targeting GluN2A-containing NMDA receptors,encompassing negative allosteric modulators(naMs),positive allosteric modulators(PAMs)and competitive ***,the ligands’structure–activity relationships(SARs)and the binding models of representative ligands are also discussed,providing valuable insights for the clinical rational design of effective drugs targeting CNS diseases.

关键词： NMDA receptors GluN2A subtype Subtype-selective ligands SARs Protein ligand interactions

Structure characterization of the oxide film on FGH96 superalloy powders with various oxidation degrees

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International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 2037-2047页

作者： Yang liu Yufeng liu Sha Zhang Lin Zhang Peng Zhang Shaorong Zhang na liu Zhou Li Xuanhui Qu Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China Science and Technology on Advanced High Temperature Structural Materials Laboratory AECC Beijing Institute of Aeronautical MaterialsBeijing 100095China

The structure of the oxide film on FGH96 alloy powders significantly influences the mechanical properties of *** this study,FGH96 alloy powders with various oxygen contents were investigated using high-resolution transmission electron microscopy and atomic probe technology to elucidate the structure evolution of the oxide *** dispersive spectrometer analysis revealed the presence of two distinct components in the oxide film of the alloy powders:amorphous oxide layer covering the γ matrix and amorphous oxide particles above the *** alloying elements within the oxide layer showed a laminated distribution,with Ni,Co,Cr,and Al/Ti,which was attributed to the decreasing oxygen equilibrium pressure as oxygen diffused from the surface into the γ *** the other hand,Ti enrichment was observed in the oxide particles caused by the oxidation and decomposition of the carbide *** analysis of the oxide film with oxygen contents of 140,280,and 340 ppm showed similar element distributions,while the thickness of the oxide film varies approximately at 9,14,and 30 nm,*** findings provide valuable insights into the structural analysis of the oxide film on FGH96 alloy powders.

关键词： Ni-based superalloys surface structure oxide layer thickness oxidation behavior element distribution

Efficient and selective upcycling of waste polylactic acid into acetate using nickel selenide

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Journal of Energy Chemistry 2024年第10期97卷 575-584页

作者： Bing Lan Yinfang Chen nantian Xiao na liu Chao Juan Chuan Xia Fan Zhang national Engineering Laboratory of Eco-Friendly Polymeric Materials College of Chemistry Sichuan University School of Materials and Energy University of Electronic Science and Technology of China

The conversion of waste polylactic acid（PLA） plastics into high-value-added chemicals through electrochemical methods is a promising and sustainable ***,developing efficient and highly selective catalysts for lactic acid oxidation reaction（LAOR） and understanding the reaction process are ***,we report the electrooxidation of waste PLA to acetate at a high current density of 100 mA cm-2 with high Faraday efficiency（～95%） and excellent stability（>100 h） over a nickel selenide nanosheet *** addition,a total Faraday efficiency of up to 190% was achieved for carboxylic acids,including acetic acid and formic acid,by coupling with the cathodic CO2reduction *** situ experimental results and theoretical simulations revealed that the catalytic activity center of LAOR was dynamically formed NiOOH species,and the surface-adsorbed SeOxspecies accelerated the formation of Ni3+species,thus promoting catalytic *** mechanism of lactic acid electrooxidation was further *** acid was dehydrogenated to produce pyruvate first and then formed CH3CO due to preferential C-C bond cleavage,resulting in the presence of *** work demonstrated a sustainable method for recycling waste PLA and CO2into high-value-added products.

关键词： Acetic acid Lactic acid electro-oxidation Poly (lactic acid) Waste plastic upcycling

The Impact of Sleep Determination on Procrastination before Bedtime:The Role of Anxiety

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International Journal of Mental Health Promotion 2024年第5期26卷 377-387页

作者： na liu Junxiu Wang Wanli Zang School of Sociology and Ethnology University of Chinese Academy of Social SciencesBeijing102488China School of Mental Health Wenzhou Medical UniversityWenzhou325000China Institute of Psychosocial Services Kangning Hospital of Wenzhou Medical UniversityWenzhou325000China Postgraduate School Harbin Sport UniversityHarbin150008China

Objective:The importance of good sleep for energy recovery and overall physical and mental health cannot be ***,the increasing competitiveness of society,diversifying lifestyles,and the rapid spread of the internet and electronic devices have significantly impacted people’s sleep patterns,particularly through bedtime ***,this study aims to investigate the relationship and underlying mechanisms between sleep determination,anxiety,and bedtime procrastination among the Chinese ***:The study utilized data from a national survey—the China Residents’Sleep Condition Survey(November 2021,with 6,037 participants).By constructing mediation and moderation models,it analyzed the relationship and mechanisms between sleep determination and bedtime procrastination,highlighting the dual role of anxiety:as a mediator between sleep determination and bedtime procrastination,and as a moderator of their ***:There was a negative correlation between sleep determination and bedtime procrastination;anxiety was related to an increase in bedtime procrastination behaviors;In the interplay between sleep determination and pre-bedtime procrastination,the regulatory effect of anxiety is found to be more pronounced than its intermediary role,with anxiety significantly diminishing the inverse relationship between sleep determination and procrastination before ***:Bedtime procrastination can lead to sleep issues,thus reducing sleep *** sleep determination or alleviating pre-sleep anxiety can help inhibit bedtime procrastination *** and reducing bedtime procrastination is one of the effective measures to improve sleep quality.

关键词： Sleep determination bedtime procrastination anxiety mediation moderation

Superwetting Ag/α-Fe_(2)O_(3) anchored mesh with enhanced photocatalytic and antibacterial activities for efficient water purification

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Green Energy & Environment 2024年第1期9卷 89-103页

作者： Jiakai Li Changpeng Lv Jiajia Song Xiaoling Zhang Xizhen Huang Yingzhuo Ma Haijie Cao na liu Department of Chemistry Tsinghua UniversityBeijing100084China Anhui Provincial Engineering Laboratory of Silicon-based Materials Engineering Technology Research Center of Silicon-based Materials(Anhui)School of Material and Chemical EngineeringBengbu UniversityBengbu233030China Institute of Materials for Energy and Environment College of Materials Science and EngineeringQingdao UniversityQingdao266071China

Superwetting materials have drawn unprecedented attention in the treatment of oily wastewater due to their preferable anti-fouling property and selective oil/water ***,it is still a challenge to fabricate multifunctional and environmentally friendly materials,which can be stably applied to purify the actual complicated ***,a Ag/Ag/α-Fe_(2)O_(3) heterostructure anchored copper mesh was intentionally synthesized using a facile two-step hydrothermal *** resultant mesh with superhydrophilicity and underwater superoleophobicity was capable of separating various oil/water mixtures with superior separation efﬁciency and high permeationﬂux driven by ***ﬁting from the joint effects of the smaller band gap of Ag/α-Fe_(2)O_(3) heterojunction,inherent antibacterial capacity of Ag/α-Fe_(2)O_(3) and Ag nanoparticles,favorable conductive substrate,as well as the hierarchical structure with superwettability,such mesh presented remarkably enhanced degradation capability toward organic dyes under visible light irradiation and antibacterial activity against both Escherichia coli(***)and Staphylococcus aureus(***)compared with the pure Ag/α-Fe_(2)O_(3) coated ***,the mesh exhibited bifunctional water puriﬁcation performance,in which organic dyes were eliminated simultaneously from water during oil/water separation in oneﬁltration *** importantly,this mesh behaved exceptional chemical resistance,mechanical stability and long-term ***,this material with multifunctional integration may hold promising potential for steady water puriﬁcation in practice.

关键词： Superwetting Ag/α-Fe_(2)O_(3)heterostructure Enhanced photocatalytic and antibacterial activities Water purification Long-term reusability

Optical trapping capability of tornado circular Pearcey beams

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Chinese Physics B 2024年第5期33卷 401-407页

作者：刘娜娜唐晓莹刘舜禹梁毅 Guangxi Key Laboratory for Relativistic Astrophysics Center on Nanoenergy ResearchGuangxi Colleges and Universities Key Laboratory of Blue Energy and Systems IntegrationSchool of Physical Science and TechnologyGuangxi UniversityNanning 530004China State Key Laboratory of Featured Metal Materials and Lifecycle Safety for Composite Structures Nanning 530004China

We systemically investigate optical trapping capability of a kind of tornado waves on Rayleigh *** tornado waves are named as tornado circular Pearcey beams(TCPBs)and produced by combining two circular Pearcey beams with different *** theoretical exploration delves into various aspects,including the propagation dynamics,energy flux,orbital angular momentum,trapping force,and torque characteristics of *** results reveal that the orbital angular momentum,trapping force,and torque of these beams can be finely tuned through the judicious manipulation of their topological charges(l_(1)and l_(2)).Notably,we observe a precise control mechanism wherein the force diminishes with|l_(1)+l_(2)|and|l_(1)-l_(2)|,while the torque exhibits enhancement by decreasing solely with|l_(1)+l_(2)|or increasing with|l_(1)-l_(2)|.These results not only provide quantitative insights into the optical trapping performance of TCPBs but also serve as a valuable reference for the ongoing development of innovative photonic tools.

关键词： trapping capability tornado beams autofocusing