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Synthesis of tetraphenylene derivatives and their recent advances

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national Science Review 2017年第6期4卷 892-916页

作者： Jian-Wei Han Xiao-Shui Peng Henry n.c.wong Shanghai-Hong Kong Joint Laboratory in chemical Synthesis Shanghai Institute of Organic ChemistryChinese Academy of Sciences Key Laboratory for Advanced Materials Institute of Fine Chemicals School of Chemistry & Molecular Engineering East China University of Science and Technology Department of chemistry Center of Novel Functional Molecules Institute of Molecular Functional Materials and State Key Laboratory of Synthetic ChemistryThe Chinese University of Hong Kong

The synthetic strategies towards tetraphenylene derivatives are comprehensively summarized in this *** advances in the functionalized tetraphenylene skeleton for research into their structurally unique properties are ... 详细信息

关键词： tetraphenylene aromatic chiral carbocycles eight-membered rings

Recent advances on iron-catalyzed coupling reactions involving organolithium reagents

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chinese chemical Letters 2019年第8期30卷 1463-1467页

作者： Zhuliang Zhong Xiao-Shui Peng Henry n.c.wong Department of chemistry and State Key Laboratory of Synthetic Chemistry The Chinese University of Hong Kong

Owing to their inexpensive and environmentally friendly properties,iron-based catalysts have been actively investigated for new organic *** this account,we summarized our recent results on iron-catalyzed cross-coupling reactions and homo-coupling *** iron-based catalysts,we constructed diverse carbon-carbon bonds,i.e.,c(sp^2)-c(sp^3),c(sp^3)-c(sp^3),c(sp^3)-c(sp^2)and c(sp^2)-c(sp^2)*** order to demonstrate the usefulness of our iron protocol,we also carried out these reactions on gram-scale reactions,leading to good yields.

关键词： Iron-catalyzed cross-coupling Homo-coupling Organolithium Gram-scale

Organic Synthesis:A Plea for Pure Science

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The Innovation 2021年第1期2卷 135-136页

作者： Henry n.c.wong School of Science and Engineering The Chinese University of Hong KongShenzhen2001 Longxiang Boulevard.Longgang DistrictShenzhen 518172China Department of chemistry The Chinese University of Hong KongShatinNew TerritoriesHong Kong SARChina

In 1883,Henry ***,the first President of the American Physical Society and Professor of Physics at Johns Hopkins University,published an essay entitled“A Plea for Pure Science”in Popular Science *** took the development of gunpowder as an example to emphasize that ScIEncE itself must be sought in the applications of science.“They(chinese)have known the application of gunpowder for centuries;and yet the reasons for its peculiar action,if sought in the proper manner,would have developed the science of chemistry,and even of physics,with all their numerous applications.”

关键词： Popular sought Hopkins

Spectral control of nonclassical light pulses using an integrated thin-film lithium niobate modulator

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Light(Science & Applications) 2022年第12期11卷 2922-2930页

作者： Di Zhu changchen chen Mengjie Yu Linbo Shao Yaowen Hu cJXin Matthew Yeh Soumya Ghosh Lingyan He christian Reimer neil Sinclair Franco n.c.wong Mian Zhang Marko Loncar John A.Paulson School of Engineering and Applied Sciences Harvard UniversityCambridgeMA 02138USA Institute of Materials Research and Engineering Agency for ScienceTechnology and Research(A*STAR)Singapore 138634Singapore Research Laboratory of Electronics Massachusetts Institute of TechnologyCambridgeMA 02139USA HyperLight corporation 1 Bow StreetSuite 420CambridgeMA 02139USA Division of Physics Mathematics and Astronomyand Alliance for Quantum Technologies(AQT)California Institute of TechnologyPasadenaCA 91125USA

Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation,communication,and networking protocols,and for bridging spectral mismatch among various quantum ***,quantum spectral control requires a strong nonlinearity mediated by light,microwave,or acoustics,which is challenging to realize with high efficiency,low noise,and on an integrated ***,we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate(TFLn)phase *** achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range(±641 GHz or±5.2 nm),enabling high visibility quantum interference between frequency-nondegenerate photon *** further operate the modulator as a time lens and demonstrate over eighteen-fold(6.55 nm to 0.35 nm)bandwidth compression of single *** results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.

关键词： quantum lithium film

Artificial intelligence analysis of videos to augment clinical assessment:an overview

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neural Regeneration Research 2024年第4期19卷 717-718页

作者： David c.wong Stefan Williams University of Leeds Leeds Teaching Hospitals Trust LeedsUK

Observation is a fundamental part of the practice of clinical *** of movement is particularly important for the *** such as Parkinson’s disease,multiple sclerosis,stroke,epilepsy,and many others affect a person’s movement in characteristic *** some conditions,changes in the patient’s voice can be included in this-changes in sound caused by changes in the movements of *** clinician’s detection of a characteristic abnormality,and their judgment of its severity,plays a central role in both diagnosis and the assessment of prognosis or response to ***,that practice depends upon a limited resource of experienced *** addition,these experts are limited by human visual judgment,which cannot reliably or precisely detect and measure small or subtle changes in movement(Williams et al.,2023).

关键词： clinical epilepsy diagnosis

Langmuir-Schaefer Film Investigation and Density Functional Theory Band Gap calculations of calix[n]arene-Para-Aminobenzoic Acid for Drug nanosensor Application

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1311-1318页

作者： wong Yeong Yi F L Supian A Radzwan M Musa n F n Abd Karim Department of Physics Sultan Idris Education UniversityTanjong Malim 35900Malaysia Department of chemistry Sultan Idris Education UniversityTanjong Malim 35900Malaysia

calix[n]arenes was utilized to detect PABA,the primary sunscreen *** study investigates the interaction of calix[4]arene(c4),calix[6]arene(c6),and PABA using the Langmuir method and first-principle density functional theory(DFT).Using the Langmuir-Schaefer(LS)technique,an ultrathin film composed of calix[n]arenes and their complexes with PABA was deposited on various *** on the Langmuir study,the PABA molecule was bonded to the lower rims of both c4 and c6 with the host-guest ratio of 1:*** of the LS films formed were then characterized by ultravioletvisible spectroscopy(UV-Vis),Fourier-transform infrared spectroscopy(FTIR)and carbon,hydrogen,nitrogen,sulfur elemental analyzer(cHnS).The band gap reduction obtained in the DFT study denotes the charge transfer interaction with promising reactivity between the calix[n]arenes and *** sensing of PABA by c4 and c6 is successful based on the formation of bonding between them due to the hosts’effective trapping *** outcomes of this study could be applied to drug delivery systems for future pharmaceutical and medical applications.

关键词： calix[n]arenes band gap density functional theory Langmuir-Schaefer PABA sensor

cRYSTAL STRUcTURES OF 1,2-BEnZO[2.2]PARAcYcLOPHAnE AnD 1,2-BEnZO[2.2]PARAcYcLOPHAnE-1,7-DIEnE

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结构化学 1985年第3期 214-217页

作者：黄乃正陈展榮麥松威 Department of chemistry The chinese University of Hong Kong Shatin new Territories Hong Kong

c20H16 (1) Mr = 256.34 and c20H14 (2), Mr = 254.32 are isomorphous, orthorhombic, P212121, Z = 4. For (?), ?a= 7.116(1), b =7.874(2), c = 24.564(4) A, V = 1376.4(3) A3, Dx = 1.237 g cm-3, μ(Mo-K α) =0.65 cm-1 , final R = 0.047 for 1152 observed reflections; for 2, a=6.963(2), b = 7.985(4), c = 24.315(8) A, V = 1351.9(8) A3, Dx = 1.250 g cm-3,μ(Mo-Kα) = 0.66 cm-1 , final R = 0.076 for 886 observed data. Structuralfeatures are similar to those of the parent [2.2]paracyclophane and related derivatives.

关键词： parent orthorhombic fused substitution benzene morethan bonds diene adequately allowed

Synthetic brochosomes:Design,synthesis,and applications

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nano Research 2024年第2期17卷 734-742页

作者： Lin Wang Jinsol choi Tak-Sing wong Department of Mechanical Engineering The Pennsylvania State UniversityUniversity ParkPA 16802USA Materials Research Institute The Pennsylvania State UniversityUniversity ParkPA 16802USA Department of Biomedical Engineering The Pennsylvania State UniversityUniversity ParkPA 16802USA

Brochosomes,which are nanoscopic buckyball-shaped granules produced by leafhoppers,are one of the most intricate structures discovered in *** functions of brochosomes have been proposed but only a few have been experimentally validated due to the challenge of fabricating their synthetic *** in micro-and nanofabrication have recently led to the emergence of synthetic brochosomes,opening up new possibilities for innovative *** review explores the early discovery of natural brochosomes and their geometrical features,followed by the recent progress in fabricating synthetic brochosomes and their *** on future applications and challenges in the scalable manufacturing of synthetic brochosomes are discussed.

关键词： synthetic brochosomes leafhopper antireflection superhydrophobicity surface-enhanced Raman scattering photocatalyst energy harvesting

Early Phases of Star Formation: Testing chemical Tools

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Research in Astronomy and Astrophysics 2024年第1期24卷 96-118页

作者： n.c.Martinez S.Paron cOnIcET-Universidad de Buenos Aires.Instituto de Astronomía y Física del Espacio Ciudad Universitaria(C1428EGA)Ciudad Autónoma de Buenos AiresArgentina

Star-forming processes strongly influence the ISM ***,many high-quality databases are available at millimeter *** them,it is possible to carry out studies that review and deepen previous *** these studies involve large samples of sources,it is preferred to use direct tools to study the molecular *** the aim of testing these tools such as the use of the Hcn/Hnc ratio as a thermometer,and the use of H^(13)cO^(+),Hc_(3)n,n_(2)H^(+) and c_(2)H as "chemical clocks," we present a molecular line study toward 55 sources representing massive young stellar objects at different evolutionary stages:infrared dark clouds(IRDcs),highmass protostellar objects(HMPOs),hot molecular cores(HMcs) and ultracompact H II *** found that the use of the Hcn/Hnc ratio as a universal thermometer in the ISM should be taken with care because the Hcn optical depth is a big issue that can affect the ***,this tool should be utilized only after a careful analysis of the Hcn spectrum,checking that no line,neither the main nor the hyperfine ones,presents absorption *** point out that the analysis of the emission of H^(13)cO^(+),Hc_(3)n,n_(2)H^(+) and c_(2)H could be useful to trace and distinguish regions among IRDcs,HMPOs and *** molecular line widths of these four species increase from the IRDc to the HMc stage,which can be a consequence of the gas dynamics related to the starforming processes taking place in the molecular *** results not only contribute with more statistics,acting as a probe of such chemical tools,useful to obtain information in large samples of sources,but also complement previous works through the analysis of other types of sources.

关键词： stars:formation ISM:molecules ISM:clouds