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Chinese Medical Journal 2024年第10期137卷 1255-1257页

作者： tan Li Guangxiao Li Yijun Wu Chao Yang Jun Yang Liping Sun Chunyan ma Department of Cardiovascular ultrasound The First Hospital of China Medical UniversityShenyangLiaoning 110001China Clinical Medical Research Center of Imaging in Liaoning Province The First Hospital of China Medical UniversityShenyangLiaoning 110001China Department of Medical Record management Center The First Hospital of China Medical UniversityShenyangLiaoning 110001China Tumor Etiology and Screening Department of Cancer Institute and General Surgery The First Hospital of China Medical UniversityShenyangLiaoning 110001China Trauma Center and Department of Burns The First Hospital of China Medical UniversityShenyangLiaoning 110001China

To the Editor:Abdominal aortic aneurysm(AAA)is a life-threatening vascular *** intervention is typically recommended when the maximum AAA diameter reaches a threshold of 5.5cm for men and 5.0cm for women,or when an AAA experiences a rapid expansion of greater than 1.0cm/year.[1]Survival after AAA repair is inuenced by various factors,and the identication of independent prognostic factors and the development of accurate prediction models are crucial for optimal treatment planning,counseling,and postoperative *** several scoring systems with varying degrees of accuracy have been developed to predict the risk of mortality after intervention for patients with ruptured AAA.

关键词： patients mortality aneurysm

Single atom doping induced charge-specific distribution of Cu1-TiO_(2)for selective aniline oxidation via a new mechanism

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Chinese Journal of Catalysis 2024年第9期64卷 98-111页

作者： Jiaheng Qin Wantong Zhao Jie Song Nan Luo Zheng-Lan ma Baojun Wang Jiantai ma Riguang Zhang Yu Long State Key Laboratory of Applied Organic Chemistry(SKLAOC) the Key Laboratory of Catalytic Engineering of Gansu ProvinceCollege of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou 730000GansuChina State Key Laboratory of Clean and Efficient Coal utilization College of Chemical Engineering and TechnologyTaiyuan University of TechnologyTaiyuan 030024ShanxiChina

utilizing single atom sites doping into metal oxides to modulate their intrinsic active sites,achieving precise selectivity control in complex organic reactions,is a highly desirable yet challenging ***,identifying the active site also represents a significant obstacle,primarily due to the intricate electronic environment of single atom site doped metal ***,a single atom Cu doped TiO_(2)catalyst(Cu_(1)-TiO_(2))is prepared via a simple“colloid-acid treatment”strategy,which switches aniline oxidation selectivity of TiO_(2)from azoxybenzene to nitrosobenzene,without using additives or changing solvent,while other metal or nonmetal doped TiO_(2)did not *** mechanistic investigations and DFT calculations unveil that Ti-O active site is responsible for triggering the aniline to form a new PhNOH intermediate,two PhNOH condense to azoxybenzene over TiO_(2)*** for Cu_(1)-TiO_(2),the charge-specific distribution between the isolated Cu and TiO_(2)generates unique Cu_(1)-O-Ti hybridization structure with nine catalytic active sites,eight of them make PhNOH take place spontaneous dissociation to produce *** work not only unveils a new mechanistic pathway featuring the PhNOH intermediate in aniline oxidation for the first time but also presents a novel approach for constructing single-atom doped metal oxides and exploring their intricate active sites.

关键词： Single atom doped metal oxide Aniline oxidation Selectivity New mechanism Active site

Effect of two-step solid solution on microstructure andδphase precipitation of Inconel 718 alloy

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International Journal of Minerals,Metallurgy and materials 2024年第10期31卷 2199-2207页

作者： Enyu Liu Qingshuang ma Xintong Li Aoxue Gao Jing Bai Liming Yu Qiuzhi Gao Huijun Li School of materials Science and Engineering Northeastern UniversityShenyang 110819China School of Resources and materials Northeastern University at QinhuangdaoQinhuangdao 066004China School of materials Science&Engineering Tianjin UniversityTianjin 300354China School of Mechanical Materials and Mechatronic EngineeringUniversity of WollongongWollongongNSW 2522Australia

Inconel 718 is the most popular nickel-based superalloy and is extensively used in aerospace,automotive,and energy indus-tries owing to its extraordinary thermomechanical *** effects of different two-step solid solution treatments on microstructure andδphase precipitation of Inconel 718 alloy were studied,and the transformation mechanism fromγ″metastable phase toδphase was *** precipitates were statistically analyzed by X-ray *** results show that theδphase content firstly increased,and then decreased with the temperature of the second-step solid *** changes in microstructure andδphase were studied by scanning electron microscopy and transmission electron *** intragranularδphase formed in Inconel 718 alloy at the second-[100]_(δ)[011]γ step solid solution temperature of 925℃,and its orientation relationship withγmatrix was determined as//and(010)_(δ)//(111)γ.Furthermore,the Vickers hardness of different heat treatment samples was measured,and the sample treated by second-step solid solution at 1010℃ reached the maximum hardness of HV 446.84.

关键词： Inconel 718 alloy two-step solid solution treatment δphase γ″-δtransformation

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船舶螺旋桨推力的在线高精度辨识方法

中国舰船研究 2024年第3期19卷 310-318页

作者：马相龙吴昊邹冬林薛林塔娜饶柱石上海船舶设备研究所上海200031 上海交通大学机械系统与振动全国重点实验室上海200240 上海交通大学振动、冲击、噪声研究所上海200240 高新船舶与深海开发装备协同创新中心上海200240

[目的]螺旋桨推力在轴系上产生的微弱形变信号易被干扰噪声所淹没,导致难以准确测量其推力,故提出一种在低信噪比下仍具有很高精度的螺旋桨推力测量方法。[方法]综合考虑测量数据误差的影响以及数据中潜藏的力学机制,基于Kalman滤波结... 详细信息

[目的]螺旋桨推力在轴系上产生的微弱形变信号易被干扰噪声所淹没,导致难以准确测量其推力,故提出一种在低信噪比下仍具有很高精度的螺旋桨推力测量方法。[方法]综合考虑测量数据误差的影响以及数据中潜藏的力学机制,基于Kalman滤波结合推力–位移状态方程建立轴系推力辨识模型,并以恒定转速、变转速及低频波动转速3种工况为例开展轴系推力测量研究,分析不同信噪比下该方法的推力辨识精度与鲁棒性。[结果]研究结果表明,当信噪比仅为20 dB时,推力辨识的最大相对误差仅为3.56%,验证了其在低信噪比下的高精度辨识能力与鲁棒性。[结论]研究成果可为实船环境下螺旋桨推力及轴系状态的在线实时高精度监测提供参考。

关键词： Kalman滤波推力辨识推进轴系位移测量在线监测

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A Deep Deterministic Policy Gradient-Based Method for Enforcing Service Fault-Tolerance in MEC

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Chinese Journal of Electronics 2024年第4期33卷 899-909页

作者： Tingyan LONG Peng CHEN Yunni XIA Yong ma Xiaoning SuN Jiale ZHAO Yifei LYu College of Computer Science Chongqing University School of Computer and Software Engineering Xihua University School of Computer and Information Engineering Jiangxi Normal University School of Computer and Information Science Chongqing Normal University

Mobile edge computing(MEC) provides edge services to users in a distributed and on-demand *** to the heterogeneity of edge applications, deploying latency and resource-intensive applications on resourceconstrained devices is a key challenge for service providers. This is especially true when underlying edge infrastructures are fault and error-prone. In this paper, we propose a fault tolerance approach named DFGP, for enforcing mobile service fault-tolerance in MEC. It synthesizes a generative optimization network(GON) model for predicting resource failure and a deep deterministic policy gradient(DDPG) model for yielding preemptive migration *** show through extensive simulation experiments that DFGP is more effective in fault detection and guaranteeing quality of service, in terms of fault detection accuracy, migration efficiency, task migration time, task scheduling time,and energy consumption than other existing methods.

关键词： Fault tolerance Multi-access edge computing Processor scheduling Fault detection Image edge detection Fault tolerant systems Quality of service

Enhancing multifunctional photocatalysis with acetate-assisted cesium doping and unlocking the potential of Z-scheme solar water splitting

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Carbon Energy 2024年第3期6卷 178-195页

作者： Mengmeng ma Jingzhen Li Xiaogang Zhu Kong Liu Kaige Huang Guodong Yuan Shizhong Yue Zhijie Wang Shengchun Qu Key Laboratory of Semiconductor materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijingChina Center of materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijingChina Department of Physics College of Physical Science and TechnologyXiamen UniversityXiamenChina State Key Laboratory for Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijingChina

Graphitic carbon nitride(g-C_(3)N_(4))has been extensively doped with alkali metals to enlarge photocatalytic output,in which cesium(Cs)doping is predicted to be the most ***,the sluggish diffusion and doping kinetics of precursors with high melting points,along with imprecise regulation,have raised the debate on whether Cs doping could make *** this matter,we attempt to confirm the positive effects of Cs doping on multifunctional photocatalysis by first using cesium acetate with the character of easy *** optimized Csdoped g-C_(3)N_(4)(CCN)shows a 41.6-fold increase in visible-light-driven hydrogen evolution reaction(HER)compared to pure g-C_(3)N_(4) and impressive degradation capability,especially with 77%refractory tetracycline and almost 100%rhodamine B degradedwithin an *** penetration ofCs+is demonstrated to be a mode of interlayer doping,and Cs–N bonds(especially with sp^(2) pyridine N in C═N–C),along with robust chemical interaction and electron exchange,are *** atomic configuration triggers the broadened spectral response,the improved charge migration,and the activated photocatalytic ***,we evaluate the CCN/cadmium sulfide hybrid as a Z-scheme configuration,promoting the visible HER yield to 9.02 mmol g^(−1) h^(−1),which is the highest ever reported among all CCN *** work adds to the rapidly expanding field of manipulation strategies and supports further development of mediating served for photocatalysis.

关键词： acetate-assisted cesium doping multifunctional photocatalysis Z-scheme

Efficient Electromagnetic Wave Absorption and Thermal Infrared Stealth in PVTMS@MWCNT Nano‑Aerogel via Abundant Nano‑Sized Cavities and Attenuation Interfaces

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Nano-Micro Letters 2024年第1期16卷 370-383页

作者： Haoyu ma maryam Fashandi Zeineb Ben Rejeb Xin Ming Yingjun Liu Pengjian Gong Guangxian Li Chul B.Park College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan University24 Yihuan RoadNanyiduanChengdu 610065SichuanPeople’s Republic of China Microcellular Plastics manufacturing Laboratory Department of Mechanical and Industrial EngineeringUniversity of Toronto5 King’s College RoadTorontoON M5S 3G8Canada Jiangsu JITRI Advanced Polymer materials Research Institute Tengfei Building88 Jiangmiao RoadJiangbei New DistrictNanjing 211800JiangsuPeople’s Republic of China MOE Key Laboratory of macromolecular Synthesis and Functionalization Department of Polymer Science and EngineeringInternational Research Center for X PolymersZhejiang University38 Zheda RoadHangzhou 310027People’s Republic of China

Pre-polymerized vinyl trimethoxy silane(PVTMS)@MWCNT nano-aerogel system was constructed via radical polymerization,sol-gel transition and supercritical CO_(2)*** fabricated organic-inorganic hybrid PVTMS@MWCNT aerogel structure shows nano-pore size(30-40 nm),high specific surface area(559 m^(2)g^(−1)),high void fraction(91.7%)and enhanced mechanical property:(1)the nano-pore size is beneficial for efficiently blocking thermal conduction and thermal convection via Knudsen effect(beneficial for infrared(IR)stealth);(2)the heterogeneous interface was beneficial for IR reflection(beneficial for IR stealth)and MWCNT polarization loss(beneficial for electromagnetic wave(EMW)attenuation);(3)the high void fraction was beneficial for enhancing thermal insulation(beneficial for IR stealth)and EMW impedance match(beneficial for EMW attenuation).Guided by the above theoretical design strategy,PVTMS@MWCNT nano-aerogel shows superior EMW absorption property(cover all Ku-band)and thermal IR stealth property(ΔT reached 60.7℃).Followed by a facial combination of the above nano-aerogel with graphene film of high electrical conductivity,an extremely high electromagnetic interference shielding material(66.5 dB,2.06 mm thickness)with superior absorption performance of an average absorption-to-reflection(A/R)coefficient ratio of 25.4 and a low reflection bandwidth of 4.1 GHz(A/R ratio more than 10)was experimentally obtained in this work.

关键词： Nano-pore size Heterogeneous interface Electromagnetic wave absorption Thermal infrared stealth Nano-aerogel

推进轴系弯-纵耦合非线性效应对推力测量精度影响研究

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船舶力学 2024年第7期28卷 1063-1072页

作者：邹冬林马相龙吴昊薛林杨宇泽塔娜饶柱石上海交通大学振动、冲击、噪声研究所机械系统与振动国家重点实验室上海200240 上海船舶设备研究所上海200031 高新船舶与深海开发装备协同创新中心上海200240

高精度监测推进轴系推力对船舶快速性预报、船-机-桨优化匹配及轴系健康管理等具有重要意义。然而,对于超长推进轴系,由于其跨距大、细长比(轴系半径与长度之比)小、且承受推力大,此时轴系将产生严重弯-纵耦合非线性变形。这将对基于应... 详细信息

高精度监测推进轴系推力对船舶快速性预报、船-机-桨优化匹配及轴系健康管理等具有重要意义。然而,对于超长推进轴系,由于其跨距大、细长比(轴系半径与长度之比)小、且承受推力大,此时轴系将产生严重弯-纵耦合非线性变形。这将对基于应变或变形位移等形变信息来测量推力的方法产生重要影响。因此,本文研究推进轴系弯-纵耦合非线性效应对推力测量精度的影响。考虑Von Karman非线性位移-应变关系,利用Hamilton变分原理结合有限元方法建立推进轴系非线性力学模型,研究弯-纵耦合效应对轴系变形位移和应变的影响规律,以及由此引起的推力测量误差。研究结果表明:在低转速时,轴系弯-纵耦合效应较弱,对推力测量影响很小;高转速时,忽略轴系弯-纵耦合效应将引起较大测量误差(240 r/min时,误差可达13.95%);测点越靠近螺旋桨,弯-纵耦合效应越强,推力测量误差越大,因此将测点布置在轴系前端推力轴承附近可有效减少轴系弯-纵耦合效应引起的测量误差。研究结果对跨度大、细长比小的超长轴系推力测量有指导意义。

关键词：推进轴系推力测量非线性弯-纵耦合有限元法

Salicylic acid positively regulates maize defenses against lepidopteran insects

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Plant Diversity 2024年第4期46卷 519-529页

作者： Yohannes Besufekad Setotaw Jing Li Jinfeng Qi Canrong ma Mou Zhang Cuilian Huang Lei Wang Jianqiang Wu Department of Economic Plants and Biotechnology Yunnan Key Laboratory for Wild Plant ResourcesKunming Institute of BotanyChinese Academy of SciencesKunming 650201China CAS Center for Excellence in Biotic Interactions University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Plant Diversity and Specialty Crops Beijing 100093China

In response to insect attack,plants use intricate signaling pathways,including phytohormones,such as jasmonate(JA),ethylene(ET),and salicylic acid(SA),to activate ***(Zea mays)is one of the most important staple food crops around the *** studies have shown that the JA and ET signaling play important roles in maize defense against insects,but little is known about whether and how SA regulates maize resistance to insect *** this study,we ectopically expressed the NahG(salicylate hydroxylase)gene in maize plants(NahG maize)to block the accumulation of *** was found that compared with the wild-type(WT)maize,the NahG-maize exhibited decreased resistance to the generalist insects Spodoptera litura and Spodoptera frugiperda and the specialist Mythimna separata.a.d the compromised resistance in the NahG maize was associated with decreased levels of defensive metabolites benzoxazinoids(Bxs)and chlorogenic acid(CA).Quantification of simulated *** feedinginduced JA,JA-isoleucine conjugate(JA-Ile),and ET in the WT and NahG maize indicated that SA does not regulate JA or JA-Ile,but positively controls *** provide evidence suggesting that the SA pathway does not crosstalk with the JA or the ET signaling in regulating the accumulation of Bxs and *** analysis revealed that the bHLH,ERF,and WRKY transcription factors might be involved in SAregulated *** study uncovers a novel and important phytohormone pathway in maize defense against lepidopterous larvae.

关键词： Benzoxazinoids Salicylic acid Herbivory maize Transcriptome

Evolution of chemistry and selection technology for DNA-encoded library

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Acta Pharmaceutica Sinica B 2024年第2期14卷 492-516页

作者： Peixiang ma Shuning Zhang Qianping Huang Yuang Gu Zhi Zhou Wei Hou Wei Yi Hongtao Xu Shanghai Key Laboratory of Orthopedic Implants Department of OrthopedicsShanghai Ninth People’s HospitalShanghai Jiao Tong UniversitySchool of MedicineShanghai 200025China Shanghai Institute for Advanced Immunochemical Studies ShanghaiTech UniversityShanghai 201210China Guangzhou Municipal and Guangdong Provincial Key Laboratory of Molecular target&Clinical Pharmacology The NMPA and State Key Laboratory of Respiratory DiseaseGuangzhou Medical UniversityGuangzhou 511436China College of Pharmaceutical Science and Institute of Drug Development&Chemical Biology Zhejiang University of TechnologyHangzhou 310014China

DNA-encoded chemical library(DEL)links the power of amplifiable genetics and the nonself-replicating chemical phenotypes,generating a diverse chemical *** analogy with the biological world,the DEL world can evolve by using a chemical central dogma,wherein DNA replicates using the PCR reactions to amplify the genetic codes,DNA sequencing transcripts the genetic information,and DNA-compatible synthesis translates into chemical ***,DNA-compatible synthesis is the key to expanding the DEL chemical ***,the evolution-driven selection system pushes the chemicals to evolve under the selective pressure,i.e.,desired selection *** this perspective,we summarized recent advances in expanding DEL synthetic toolbox and panning strategies,which will shed light on the drug discovery harnessing in vitro evolution of chemicals via DEL.

关键词： DNA-encoded library Drug discovery High-throughput selection DNA-compatible synthesis In vitro evolution Chemical central dogma