检索结果-南通市图书馆

Progress in Natural Science:Materials International 2024年第2期34卷 338-344页

作者： Yuan li Pengfei Huang Chunyu Cui Xiaoyuan Ma li Chen Zekun li linhai li Yuhong Tian School of Biological and Chemical Engineering Guangxi University of Science and Technology School of College of Chemistry and Chemical Engineering Hunan University Isky Future Energy Institute

li metal batteries（LMBs） have attracted much attention due to the ultra-high theoretical capacity of the li metal anode（LMA）.However,the uncontrollable dendrites growth and low coulombic efficiency hinder their practical application.Here,we explore 3,5-difluoropyridine（2F-BD） as a novel electrolyte additive to enable highperformance LMBs.The 2F-BD additive participates in and modifies the solvation structure of li ions by reducing the coordinated number of PF6-at the electrode surface,leading to the formation of a liF and li3N-rich solid electrolyte interphase（SEI）.The liF component increases the robustness of SEI and suppresses the formation of li dendrites,while the li3N component facilitates the transportation and reaction kinetics of li ions.As a result,the li‖li symmetric cell presents a stable cycling performance of up to 500 h at a current density of 1 mA cm-2.After coupling with liFePO4cathode,the obtained full cell achieves high specific capacities of 106.06 mA h g-1and 84.98 mA h g-1at 2.55 mA cm-2and 5.10 mA cm-2,respectively,and maintains a high capacity retention of84.0% after 1000 cycles at 0.13 mA cm-2,with an average cycling CE of 99.58%.

关键词： Electrolyte additive li dendrites li metal batteries liF and li3N-Rich electrode-electrolyte interphase liFePO4 cathode

Highly selective growth of(6,5)single-walled carbon nanotubes from sigma phase alloy catalyst

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第3期17卷 1999-2003页

作者： liantao Xin Chen Ma Qianru Wu Shaokang liu linhai li Xiuyun Zhang liu Qian Maoshuai He Dong li Fangqian Han Shulan Hao lihu Feng Yahan li Huaping liu lili Zhang Chang liu Jin Zhang College of Chemistry and Molecular Engineering Qingdao University of Science and TechnologyQingdao 266042China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China College of Physics Science and Technology Yangzhou UniversityYangzhou 225002China Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular SciencesCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

The chirality structure of a single-walled carbon nanotube(SWNT)strongly depends on the composition of catalyst used in the chemical vapor deposition process.In this study,we develop a porous magnesia supported manganese-rhenium(MnRe/MgO)catalyst for chirality-selective synthesis of SWNTs.Detailed characterizations reveal that(6,5)tubes with a selectivity higher than 70%are grown from the Re-rich MnRe/MgO catalyst.By comparing the SWNT growth results with those of monometallic Mn or Re,the formation of sigma phase,an intermetallic compound occurring in transition-metal alloy systems,is revealed to be crucial for the dominant synthesis of(6,5)SWNTs.This work not only extends the application of sigma phase alloy for catalytic synthesis of SWNTs,but also sheds lights on the growth of SWNTs with a high chirality selectivity.

关键词： single-walled carbon nanotubes sigma phase manganese-rhenium catalyst selective growth transition-metal alloy

Al-driven analysis establishes the single base substitution signatures as personalized prognostic predictors for five-year survival of gastric cancer

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Genes & Diseases 2024年第4期11卷 73-76页

作者： Zhenzhang li lingqing Xu Wen Luo Shaoan Zhangg Chunyu Hou Xiaohong Xu ,Xubei Peng E.Shiju Janak L.Pathak Shizhen Zhang Jiawei liu linhai li Yang li School of Biomedical Engineering The Sixth Affiliated HospitalGuangzhou Medical UniversityGuangzhouGuangdong 511436China College of Mathematics and Systems Science Guangdong Polytechnic Normal UniversityGuangzhouGuangdong 510665China The Second Affiliated Hospital Guangzhou Medical UniversityGuangzhouGuangdong 510260China Center for Learning Sciences and Technologies The Chinese University of Hong KongShatinNew Territories 999077China Affiliated Stomatology Hospital of Guangzhou Medical University Guangzhou Medical UniversityGuangzhouGuangdong 510182China International School of Photonics Cochin University of Science and TechnologyKochiKerala 682022India

Al-driven genetic engineering,as a burgeoning diagnostic tool,can offer predictive information on the five-year survival rate(FYSR)in the setup of a prognostic therapeutic schedule.This approach provides the individuality and accuracy of prognosis for FYSR of gastric cancer(GC).Unlike traditional neoplasm staging criteria,our technique ensures accuracy and individuality without relying on statistical data and empirical study.

关键词： cancer gastric prognosis

A review on the transformation of birnessite in the environment:Implication for the stabilization of heavy metals

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2024年第5期139卷 496-515页

作者： Miao Shi Qingzhu li Qingwei Wang Xuelei Yan Bensheng li linhai Feng Chao Wu Rongrong Qiu Hongkai Zhang Zhihui Yang Weichun Yang Qi liao liyuan Chai School of Metallurgy and Environment Central South UniversityChangsha 410083China National Engineering Research Centre for Control and Treatment ofHeavy Metal Pollution Central South UniversityChangsha 410083China Water Pollution Control Technology Key Lab of Hunan Province Changsha 410083China

Birnessite is ubiquitous in the natural environment where heavy metals are retained and easily transformed.The surface properties and structure of birnessite change with the changes in external environmental conditions,which also affects the fate of heavy metals.Clarifying the effect and mechanism of the birnessite phase transition process on heavy metals is the key to taking effective measures to prevent and control heavy metal pollution.Therefore,the four transformation pathways of birnessite are summarized first in this review.Second,the relationship between transformation pathways and environmental conditions is proposed.These relevant environmental conditions include abiotic(e.g.,co-existing ions,pH,oxygen pressure,temperature,electric field,light,aging,pressure)and biotic factors(e.g.,microorganisms,biomolecules).The phase transformation is achieved by the key intermediate of Mn(Ⅲ)through interlayer-condensation,folding,neutralizationdisproportionation,and dissolution-recrystallization mechanisms.The AOS(average oxidation state)of Mn and interlayer spacing are closely correlated with the phase transformation of birnessite.Last but not least,the mechanisms of heavy metals immobilization in the transformation process of birnessite are summed up.They involve isomorphous substitution,redox,complexation,hydration/dehydration,etc.The transformation of birnessite and its implication on heavy metals will be helpful for understanding and predicting the behavior of heavy metals and the crucial phase of manganese oxides/hydroxides in natural and engineered environments.

关键词： Birnessite Transformation Heavy metals Pathways Mechanism

维普期刊数据库

Chirality-dependent concentration boundaries of single-wall carbon nanotubes for photoluminescence characterization and applications

在线全文

学校读者我要写书评

暂无评论

Nano Research 2023年第2期16卷 1820-1825页

作者： Shilong li linhai li Xiaojun Wei Weiya Zhou Sishen Xie Huaping liu Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China Department of Physical Science and Center of Materials Science and Optoelectronics EngineeringUniversity of Chinese Academy of SciencesBeijing 100049China Beijing Key Laboratory for Advanced Functional Materials and Structure Research Beijing 100190China Songshan Lake Materials Laboratory Dongguan 523808China

Increasing the concentration of single-wall carbon nanotubes(SWCNTs)is an effective method for enhancing their luminescence intensity.However,an increase in the concentration of SWCNTs would inevitably increase their reabsorption effect,degrading their luminescence efficiency.Herein,we systematically investigated variations in the photoluminescence(PL)intensity of(6,5)single-chirality SWCNTs while increasing their concentration.The results show that the PL intensity first increased to a maximum and then decreased with increasing concentration.Numerical analysis indicates that the concentration boundary corresponding to the maximum PL intensity was strongly dependent on the ratio of the optical absorbances of the SWCNTs at their excitation and emission wavelengths.According to this,statistical analysis by experimentally measuring the optical absorption spectra of 18 kinds of single-chirality SWCNTs shows that the concentration boundaries of SWCNTs were dependent upon their Types and diameters.The concentration boundary of Type I SWCNTs was higher than that of Type II SWCNTs,and the concentration boundaries of both Types increased with increasing diameter.These results provide important guidance for spectral characterization and applications in bioimaging and photoelectronic devices.

关键词： single-wall carbon nanotube photoluminescence concentration boundary reabsorption

Metagenomic Analysis of Mangshan Pit Viper (Protobothrops mangshanensis) Gut Microbiota Reveals Differences among Wild and Captive Individuals linked to Hibernating Behaviors

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Asian Herpetological Research 2022年第4期13卷 251-268页

作者： Bing ZHANG Xiangyun DING Jianping JIANG linhai li Daode YANG Institute of Wildlife Conservation Central South University of Forestry and TechnologyChangsha 410004HunanChina Qilu Normal University Jinan 250200ShandongChina Chengdu Institute of Biology Chinese Academy of SciencesChengdu 610041SichuanChina Department for Wildlife and Forest Plants Protetion National Forestry and Grassland AdministrationBeijing 100714China

Gut microbiota play important roles in the immunity,digestion,and energy meta bolism of their reptile hosts.Mangshan pit viper(Protobothrops mangshanensis)is a critically endangered snake species that is a Class I national protected species in China.little is known regarding the relationship between P.mangshanensis and their gut microbial communities.In this study,the gut microbiota of wild P.mangshanensis individuals,artificially hiberna ting captive individuals,and non-hibernating captive individuals were compared across nine samples.Comparative shotgun metagenomic analysis was used to investigate the taxonomic composition,diversity,and function of P.mangshanensis gut microbial communities and assess whether their gut microbiomes were affected by their living environments and captivity conditions.The dominant phyla within P.mangshanensis gut microbial communities were Proteobacteria(65.55%),Bacteroidetes(15.97%),and Firmicutes(8.11%).Enriched functional pathways within the gut microbiota included meta bolism(54.9%),environmental information processing(9.67%),and genetic information processing(9.37%).Wild snake gut communities exhibited higher microbial diversity than the other two groups.The gut microbiomes of wild and hibernating captive snakes may be more reflective of healthy intestinal homeostasis than that in nonhibernating snakes.Specifically,non-hibernating snakes exhibited increased levelsof potentially pathogenic populations and functional specialization within gut microbial communities.Thus,different livingenvironments and captivitymethodsmay correspond to major shifts in microbiota composition,diversity,and function within P.mangshanensis.This study provides important insights to help guide the conservation of P.mangshanensis,while also carrying broad implications for our understanding of the effects of living environments and non-hibernating captivity conditions on the gut microbiota of snakes.

关键词： composition and diversity gene functions and pathways gutmicrobiota metagenomics Protobothrops mangshanensis

维普期刊数据库

Diameter-dependent photoelectric performances of semiconducting carbon nanotubes/perovskite heterojunctions

在线全文

学校读者我要写书评

暂无评论

Nano Research 2023年第11期16卷 12662-12669页

作者： Yayang Yu Wenke Wang Xiao li linhai li Shilong li Xiaojun Wei Weiya Zhou Jing lin Yang Huang Huaping liu School of Materials Science and Engineering Hebei Key Laboratory of Boron Nitride Micro and Nano MaterialsHebei University of TechnologyTianjin 300130China Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering School of Physical SciencesUniversity of Chinese Academy of SciencesBeijing 100049China Beijing Key Laboratory for Advanced Functional Materials and Structure Research Beijing 100190China Songshan Lake Materials Laboratory Dongguan 523808China

The heterojunction of single-wall carbon nanotubes(SWCNTs)and perovskite quantum dots(QDs)shows excellent photodetection performances due to the combination of the advantages of high carrier mobility of SWCNTs and high absorption coefficient of perovskite QDs.However,the band structure of a SWCNT is determined by its atomic arrangement structure.How the structure of SWCNTs affects the photoelectric performance of the composite film remains elusive.Here,we systematically explored the diameter effect of SWCNTs with different bandgaps on the photodetection performances of SWCNTs/perovskite QDs heterojunction films by integrating semiconducting SWCNTs(s-SWCNTs)with different diameters with CsPbBr3 QDs.The results show that with an increase in diameter of s-SWCNTs,the heterojunction exhibits increasing responsivity(R),detectivity(D*),and faster response time.The great improvement in the optoelectronic performances of devices should be attributed to the higher carrier mobility of larger-diameter SWCNT films and the increasing built-in electric field at the heterojunction interfaces between larger-diameter SWCNTs and CsPbBr3 QDs,which enhances the separation of the photogenerated excitons and the transport of the resulted carriers in SWCNT films.

关键词： carbon nanotubes perovskite quantum dots diameter effect responsivity detectivity

Ring finger protein 157 is a prognostic biomarker and is associated with immune infiltrates in human breast cancer

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

BIOCELL 2023年第10期47卷 2265-2281页

作者： XIN ZHU BIN XIAO WENWU ZHANG XIAOYU SONG WEI GONG linhai li XINPING CHEN School of life Sciences Hainan UniversityHaikou570228China Department of Medical Laboratory Hainan Cancer HospitalAffiliated Cancer Hospital of Hainan Medical UniversityHainan Tropical Cancer Research InstituteHaikou570312China Department of Laboratory Medicine The Sixth Affiliated Hospital of Guangzhou Medical UniversityQingyuan People’s HospitalQingyuan511518China Graduate School Guangzhou University of Chinese MedicineGuangzhou510006China School of Pharmaceutical Sciences Hainan UniversityHaikou570228China

Background: The protein encoded by ring finger protein 157 (RNF157) is known to function as an E3 ubiquitinligase. However, whether the level of RNF157 expression in breast cancer correlates with prognosis and immune cellinfiltration among breast cancer patients remains to be further explored. Methods: In this study, publicly availabledatasets were used for evaluating RNF157 expression in different tumors compared with normal samples. Severalindependent datasets were screened for investigating the relationship between RNF157 and breast cancer survival,different mutation profiles, and tumor immune cell infiltration. We conducted a pathway enrichment analysis toidentify signaling pathways associated with RNF157. Results: Analysis of public and online databases revealed thatRNF157 expression markedly decreased in breast cancer tissue samples compared to non-carcinoma counterparts.Consistently, immunohistochemistry assays also demonstrated this RNF157 down-regulation in breast cancer samples.RNF157 up-regulation could predict the improved survival of breast cancer cases. Further, different RNF157expression level groups exhibited different mutational profiles. Pathway enrichment profiling of RNF157-related genessuggested its possible involvement in regulating breast cancer via the mitogen-activated protein kinase (MAPK)pathway. RNA sequencing (RNA-seq) data and genomic enrichment analysis showed that RNF157 downregulatedseveral genes positively associated with the MAPK signaling pathway. We also explored RNF157 expression andimmune cell infiltration in breast cancer and found that RNF157 mRNA levels were negatively related to non-Timmune cell infiltration. Conclusion: According to our work, RNF157 may be a promising diagnostic biomarker andtherapeutic target for breast cancer.

关键词： RNF157 Prognosis Immune infiltrate MAPK signal pathway Breast cancer

Prognostic impact of gene copy number instability and tumor mutation burden in patients with resectable gastric cancer

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Cancer Communications 2020年第1期40卷 63-66页

作者： lisheng Cai linhai li Dandan Ren Xue Song Beibei Mao Bo Han Henghui Zhang Department of General Surgery Zhangzhou Afiliated Hospital of Fujian Medical UniversityZhangzhouFujian363000P.R.China Department of General Surgery The First People's Hospital of Yunnan ProvinceThe Affliated Hospital of Kunming University of Science and TechnologyKunmingYunan650032P.R.China Genecast Precision Medicine Technology Institute Beijing100191P.R.China The Second Ward of Oncology Department The First Affiliated Hospital of Harbin Medical UniversityHarbinHeilongiang150086P.R.China Institute of Infectious Diseases Bejing Ditan HospitalCapital Medical UniversityBeijing100015P.R.China

Dear Editor,Gastric cancer(GC)is a leading cause of cancer-related deaths worldwide,especially in China and other East Asian countries[1,2].Although considerable achievements have been made in its treatment[3]and predictive biomarkers[4]in past decades,the prognosis of GC remains poor[5].Therefore,more effective prognostic markers are needed to improve the prognosis prediction of GCs.Small panels based on next-generation sequencing,such as FoundationOne CDx and MSK-IMPACT,are widely used for selecting appropriate treatment approaches(such as targeted therapies,immunotherapies,and chemotherapies)with the advantages of a higher sequencing depth and more cost-effectiveness than whole-exome sequencing(WES).Previous studies have demonstrated that molecular characteristics based on the designed cancer-related gene panel were consistent with those determined by WES and could be prognostic markers for various cancer types[6-8].As such,we analyzed the molecular features with the designed panel to investigate probable prognostic biomarkers for Chinese patients with GC.

关键词： patients Gastric treatment

The Structure Entropy of Social Networks

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Systems Science & Complexity 2024年第3期37卷 1147-1162页

作者： li Zhenpeng YAN Zhihua YANG Jian TANG Xijin School of Electronics and Information Engineering Taizhou UniversityLinhai 317000China Academy of Mathematics and Systems Science Chinese Academy of SciencesBeijing 100190China Yunnan Key Laboratory of Smart City in Cyberspace Security Yuxi Normal UniversityYuci 653100China University of Chinese Academy of Sciences Beijing 100039China

Micro triadic structure is an important motif and serves the building block of complex networks.In this paper,the authors define structure entropy for a social network and explain this concept by using the coded triads proposed by Davis and Leinhardt in 1972.The proposed structure entropy serves as a new macro-evolution index to measure the network’s stability at a given timestamp.Empirical analysis of real-world network structure entropy discloses rich information on the mechanism that yields given triadic motifs frequency distribution.This paper illustrates the intrinsic link between the micro dyadic/triadic motifs and network structure entropy.Importantly,the authors find that the high proportion of reciprocity and transitivity results in the emergence of hierarchy,order,and cooperation of online social networks.

关键词： Dyadic and triadic motifs network structure entropy reciprocity and transitivity

维普期刊数据库