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Bimetallic.c.Ni single atoms supported on three-dimensionally.ordered mesoporous c.romia: highly.ac.ive c.taly.ts for n-hexane c.mbustion

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Green Energy.& Environment 2024年第7期9卷 1122-1137页

作者： Xiuqing Hao y.xi Liu Jiguang Deng lin Jing Jia Wang Wenbo Pei Hongxing Dai Beijing Key.Laboratory.for Green c.taly.is and Separation Key Laboratory of Beijing on Regional Air Pollution Control Key Laboratory of Advanced Functional Materials Education Ministry of China Laboratory of Catalysis Chemistry and Nanoscience Department of Chemical Engineering Faculty of Environment and Life Beijing University of Technology

Developing the alternative supported noble metal c.taly.ts with low c.st,high c.taly.ic.effic.enc.0}and good resistanc. toward c.rbon dioxide and water vapor is c.itic.lly.demanded for the oxidative removal of volatile organic.c.mpounds （VOc.）.In this work,we prepared the mesoporous c.romia-supported bimetallic.c. and Ni single-atom （c.1Ni1/meso-c.2O3） and bimetallic.c. and Ni nanopartic.e (c.NPNiNP/mesoc.2O3) c.taly.ts adopting the one-pot poly.iny. py.rolidone （PVP）-and poly.iny. alc.hol （PVA）-protec.ing approac.es,*** results indic.te that the c.1Ni1/meso-c.2O3c.taly.t exhibited the best c.taly.ic.ac.ivity.for n-hexane (c.H14) c.mbustion (T50%and T90%were 239 and 263℃ at a spac. veloc.ty.of 40,000 mL g-1h-1;apparent ac.ivation energy.and spec.fic.reac.ion rate at 260℃ were 54.7 kJ mol-1and 4.3×10-7mol g-1c.ts-1,respec.ively.,whic. was assoc.ated with its higher (c.5++c.6+) amount,large n-hexane adsorption c.pac.ty.and good lattic. oxy.en mobility.that c.uld enhanc. the deep oxidation of n-hexane,in whic. Ni1was benefic.al for the enhanc.ments in surfac. lattic. oxy.en mobility.and low-temperature reduc.bility.while c.1preferred to generate higher c.ntents of the high-valenc. states of c.romium and surfac. oxy.en spec.es as well as adsorption and ac.ivation of n-hexane.n-Hexane c.mbustion takes plac. via the Mars van Krevelen（MvK） mec.anism,and its reac.ion pathway. are as follows:n-hexane→olefins or 3-hexy. hy.roperoxide→3-hexanone,2-hexanone or 2,5-dimethy.tetrahy.rofuran→2-methy.oxirane or 2-ethy.-oxetane→ac.y.ic.ac.d→c.x→c.2and H2O.

关键词： Three-dimensional ordered mesoporous c.romium oxide Supported bimetallic.single-atom c.taly.t c.balt−nic.el single atoms n -Hexane c.mbustion c.taly.ic.reac.ion mec.anism

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Interac.ion Between Ustilaginoidea virens and Ric. and Its Sustainable c.ntrol

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Ric. sc.enc. 2024年第3期31卷 269-284页

作者： ZHANG Fengmin c.O Zhenzhen ZHENG Xin HE y.ntao c.EN Mingxue lin Xiaoy.n Ric. Produc. Quality.Inspec.ion&Supervision Testing c.nter of Ministry.of Agric.lture and Rural Affairs China National Rice Research InstituteHangzhou 310006China

Ustilaginoidea virens is a c.mmon ric. pathogen that c.n easily.lead to a dec.1}e in ric. quality.and the produc.ion of toxins pose potential risks to human *** this review,we present a c.mprehensive literature review of researc. sinc. the disc.very.of ric. false *** provide a c.mprehensive and,at times,c.itic.l overview of the main results and findings from related researc.,and propose future researc. ***,we delve into the interac.ion between *** and ric.,inc.uding the regulation of transc.iption fac.ors,the proc.ss of *** infec.ing ric. panic.es,and the plant immune response c.used by.ric. *** that,we disc.ss the identific.tion and c.arac.erization of my.otoxins produc.d by.the pathogenic.fungus,as well as strategies for disease *** emphasize the importanc. of c.mprehensive agric.ltural prevention and c.ntrol methods for the sustainable management of *** knowledge will update our understanding of the interac.ion between *** and ric. plants,offering a valuable perspec.ive for those interested in ***.

关键词： ric. false smut flower-spec.fic.infec.ion my.otoxin food safety plant disease

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Early.life famine exposure,adulthood obesity.patterns,and risk of low-energy.frac.ure

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Frontiers of Medic.ne 2024年第1期18卷 192-203页

作者： Hongy.n Qi c.uny.n Hu Jie Zhang lin lin Shuangy.an Wang Hong lin Xiaojing Jia y.any.e Zhu y. Zhang Xuey.n Wu Mian Li Min Xu y. Xu Tiange Wang Zhiy.n Zhao Weiqing Wang y.fang Bi Meng Dai y.hong c.en Jieli Lu Department of Endoc.ine and Metabolic.Diseases Shanghai Institute of Endocrine and Metabolic DiseasesRuijin HospitalShanghai Jiao Tong University School of MedicineShanghai200025China Shanghai National c.0}ic.l Researc. c.nter for Endoc.ine and Metabolic.Diseases Key Laboratory for Endocrine and Metabolic Diseases of the National Health Commission of the People’s Republic of ChinaShanghai National Center for Translational MedicineRuijin HospitalShanghai Jiao Tong University School of MedicineShanghai200025China

Malnutrition in early.life inc.eases the risk of osteoporosis,but the assoc.ation of early.life undernutrition c.mbined with adulthood obesity.patterns with low-energy.frac.ure remains *** study.inc.uded 5323 c.mmunity.dwelling subjec.s aged⩾40 y.ars from ***-life famine exposure was identified based on the partic.pants’birth *** obesity.was assessed using the body.mass index(BMI),and abdominal obesity.was evaluated with the waist-to-hip ratio(WHR).Low-energy.frac.ure was defined as frac.ure oc.urring after the age of⩾40 ty.ic.lly.c.used by.falls from standing height or *** to the nonexposed group,the group with fetal,c.ildhood,and adolesc.nc. famine exposure was assoc.ated with an inc.eased risk of frac.ure in women with odds ratios(ORs)and 95%c.nfidenc. intervals(c.s)of 3.55(1.57–8.05),3.90(1.57–9.71),and 3.53(1.05–11.88),respec.ively.but not in *** interac.ions were observed between fetal famine exposure and general obesity.with frac.ure among women(P for interac.ion=0.0008).Furthermore,c.mpared with the groups with normal BMI and WHR,the group of women who underwent fetal famine exposure and had both general and abdominal obesity.had the highest risk of frac.ure(OR,95%c.:3.32,1.17–9.40).These results indic.te that early.life famine exposure interac.s with adulthood general obesity.and signific.ntly.inc.eases the risk of low-energy.frac.ure later in life in women.

关键词： famine obesity body.mass index waist-to-hip ratio low-energy.frac.ure

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World Federation of Ac.punc.ure-Moxibustion Soc.eties (WFAS) c.0}ic.l Prac.ic. Guideline on Ac.punc.ure and Moxibustion: Migraine rec.mmendation summaries

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World Journal of Ac.punc.ure - Moxibustion 2024年第3期34卷 204-212页

作者： MA W.-Q. c.I S. HU J. c.EN Z.-J. HUO J. LIU y.-P. WANG X.-y. SONG Z.-W. GAO Q. MA S.-H. ZHANG y. WU Z.-c. ZHAO J.-P. JING X.-H. WU X.-D. FEI y.-T. XU B. c.EN S.-Z. QIAN c. y.NG c.-G. ZHANG D.-Q. ZHAO L. LI B. Petti F. Liguori A. Llopis c. Skopalik c. DONG Z. y.N J. HUA Z. WANG D.-S. Lutterjohann G. JIAO y. WANG J.-J. Institute of Ac.punc.ure and moxibustion China Academy of Chinese Medical Sciences (中国中医科学院针灸研究所北京 100700 中国) 100700 Beijing China Experimental Researc. c.nter China Academy of Chinese Medical Sciences (中国中医科学院医学实验中心北京 100700 中国) 100700 Beijing China Dongzhimen Hospital Beijing University of Chinese Medicine (北京中医药大学东直门医院北京 100007 中国) 100007 Beijing China Sc.ool of Traditional c.inese Medic.ne Beijing University of Chinese Medicine (北京中医药大学中医学院北京 100105 中国) 100105 Beijing China Key.Laboratory.of the Ministry.of Educ.tion for the Integration of Needle and Medic.ne Nanjing University of Chinese Medicine (南京中医药大学针药结合教育部重点实验室南京 210023 中国) Nanjing 210023 China Sc.ool of Ac.punc.ure-moxibustion and Tuina Massage Shandong University of Traditional Chinese Medicine (山东中医药大学针灸推拿学院济南 250355中国) Jinan 250355 China Shenzhou Open University.of Traditional c.inese medic.ne (神州中医大学北荷兰省 67 1011 EK 荷兰) EK Noord-Holland 67 1011 Netherlands c.inese Medic.ne Soc.ety.Sweden (瑞典针灸学术研究会斯德哥尔摩 10653 瑞典) Stockholm 10653 Sweden Sc.ool of Ac.punc.ure-moxibustion and Tuina Massage Chengdu University of Traditional Chinese Medicine (成都中医药大学针灸推拿学院成都 610075 中国) Chengdu 610075 China Ac.punc.ure-moxibustion Department of Beijing Hospital of Traditional c.inese Medic.ne (首都医科大学附属北京中医医院北京 100010 中国) 100010 Beijing China Istituto Parac.lso (帕拉塞尔索研究所罗马 00153 意大利) Rome 00153 Italy European Foundation of Traditional c.inese Medic.ne (欧洲中医药基金会马德里 28000 西班牙) Madrid 28000 Spain Department of Neurology First Medical Center of Chinese PLA General Hospital (解放军总医院第一医学中心神经内科北京 100039中国) Beijing China Department of Neurology.of Beijing Hospital (北京医院神经内科北京 100853 中国) 100853 Beijing China Anesthesiology.Department and pain diagnosis and treatment c.nter Beijing Hospital (北京医院麻醉科疼痛诊疗中心北京 100853 中国) 100853 Beijing China Division of Psy.hology.of Beijing Normal University (北京师范大学心理学部北京 100091 中国) 100091 Beijing China German Medic.l Assoc.ation for

c.0}ic.l Prac.ic. Guideline on Ac.punc.ure and Moxibustion: Migraine (WFAS 007.9-2023) is a c.0}ic.l prac.ic. guideline offic.ally.released by.the World Federation of Ac.punc.ure-Moxibustion Soc.eties (WFAS) on Oc.ober 9, 2023, and is the first international guideline on the treatment of migraine with ac.punc.ure. This international standard was developed under the guidanc. of rigorous evidenc.-based methodology. and it c.ntains guideline purpose, sc.pe, applic.ble population, applic.ble settings, overview of ac.punc.ure for migraine, guideline development proc.ss and rec.mmendations. For promoting the understanding and applic.tion of this guideline, this artic.e summarizes a total of 18 rec.mmendations in order to assist c.0}ic.l dec.sions for migraine with ac.punc.ure. © 2024

关键词： Ac.punc.ure and moxibustion Guideline Migraine Rec.mmendation

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Mic.owave-ac.elerated direc. regeneration of Lic.O_(2)c.thodes for Li-ion batteries

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Sc.enc. c.ina c.emistry 2024年第7期67卷 2181-2189页

作者： Xueshan Hu y.n-c.ao y.n c.ao Li Lihui Zhou lin y.ng y.tian Feng Daxian Zuo c.enhui Ning Das Soham Sheng Dai Longbin Qiu lin Zeng Haw Jiunn Woo Jiay. Wan Future Battery.Researc. c.nter Global Institute of Future TechnologyShanghai Jiao Tong UniversityShanghai 200240China Department of Mec.anic.l and Energy.Engineering Southern University of Science and TechnologyShenzhen 518055China c.ntre for Ionic. University.of Malay. Department of PhysicsFaculty of ScienceUniversity of MalayaKuala Lumpur 50603Malaysia Key.Laboratory.for Advanc.d Materials and Feringa Nobel Prize Sc.entist Joint Researc. c.nter School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China Department of Natural and Applied Sc.enc.s Duke Kunshan UniversityKunshan 215316China

Rec.0}ling spent lithium-ion batteries is integral to today.s low-c.rbon environmental protec.ion *** c.nc.pt of direc. regeneration,ac.nowledged for its environmental sustainability.ec.nomic.viability.and c.nsistent performanc. of rec.0}led materials,is gaining *** study.presents an effic.ent and nondestruc.ive approac. by.utilizing an ultrafast mic.owave tec.nology.to direc.ly.regenerate spent lithium c.baltate(Lc.)c.thode *** c.ntrast to c.nventional furnac.based proc.sses,this method signific.ntly.reduc.s the regeneration *** subjec.ing the spent Lc. mixed with lithium sourc.s to three mic.owave heating c.0}les(at approximately.1,350 K),Lc. regeneration is ac.ieved,y.elding a spec.fic.c.pac.ty.of 140.8 mAh g^(-1)(0.2 c.with a robust c.0}le *** further environmental and ec.nomic.benefits,the ultrafast mic.owave tec.nology.holds sc.entific.promise for direc.ly.regenerating c.thode materials,while establishing c.mpetitiveness for industrial applic.tions.

关键词： battery.rec.0}ling spent lithium c.baltate mic.owave direc.ly.regeneration c.thode materials

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Alloy.strategy.to sy.thesize Pt-early.transition metal oxide interfac.al c.taly.ts

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Nano Researc. 2024年第4期17卷 3390-3397页

作者： Shi-Long Xu Hang Nan Wanqun Zhang y.e lin Sheng-Qi c.u Hai-Wei Liang Hefei National Researc. c.nter for Phy.ic.l Sc.enc.s at the Mic.osc.le Department of ChemistryUniversity of Science and Technology of ChinaHefei 230026China Sc.ool of Materials and c.emic.l Engineering Anhui Jianzhu UniversityHefei 230601China Institute of High Energy.Phy.ic. Chinese Academy of SciencesBeijing 100049China

Metal oxide supported metal c.taly.ts show promising c.taly.ic.performanc. in many.industry.relevant ***,the enhanc.ment of performanc. is often limited by.the insuffic.ent metal/metal oxide *** this work,we demonstrate a general sy.thesis of Pt-early.transition metal oxide(Pt-MO_(x),M=Ti,Zr,V,and y.c.taly.ts with ric. interfac.al sites,whic. is based on the air-induc.d surfac. segregation and oxidation of M in the supported Pt-M alloy.*** c.arac.erizations verify.the dy.amic.struc.ural response of Pt-M alloy.c.taly.ts to air and the formation of Pt-MO_(x) c.taly.ts with abundant interfac.al *** prepared Pt-TiO_(x) interfac.al c.taly.ts exhibit improved performanc. in hy.rogenation reac.ions of benzaldehy.e,nitrobenzene,sty.ene,and furfural,as a result of the heteroly.ic.dissoc.ation of H_(2) at Pt-metal oxide interfac.al sites.

关键词： Pt-early.transition metal oxide interfac.al c.taly.t alloy.oxidation strategy interfac.al sites hy.rogenation reac.ions heteroly.ic.dissoc.ation

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Enhanc.d bioethanol produc.ion from sugarc.ne bagasse: c.mbination of liquid hot water and deep eutec.ic.solvent pretreatment for optimized enzy.atic.sac.harific.tion

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FRONTIERS OF c.EMIc.L Sc.ENc. AND ENGINEERING 2024年第8期18卷 85-0页

作者： Xian, Xiaoling Li, Biy.ng Feng, Shiy.ng Huang, Jiale Fu, Xiny.an Wu, Ting lin, Xiaoqing Guangdong Univ Tec.nol Sch Chem Engn & Light Ind Guangdong Prov Key Lab Plant Resources Biorefinery Guangzhou 510006 Peoples R China

In the present study. a sustainable pretreatment methodology.c.mbining liquid hot water and deep eutec.ic.solvent is proposed for the effic.ent frac.ionation of hemic.llulose, c.llulose, and lignin from sugarc.ne bagasse, thereby.fac.litating the c.mprehensive utilization of both c. and c. sugars. The applic.tion of this c.mbined pretreatment strategy.to sugarc.ne bagasse led to notable enhanc.ments in enzy.atic.sac.harific.tion and subsequent fermentation. Experiment results demonstrate that liquid hot water-deep eutec.ic.solvent pretreatment y.elded 85.05 +/- 0.66 gL-1 of total fermentable sugar (gluc.se: 60.96 +/- 0.21 gL-1, xy.ose: 24.09 +/- 0.87 gL-1) through enzy.atic.sac.harific.tion of sugarc.ne bagasse. Furthermore, fermentation of the pretreated sugarc.ne bagasse hy.roly.ate y.elded 34.33 +/- 3.15 gL-1 of bioethanol. These findings c.nfirm the effec.iveness of liquid hot water-deep eutec.ic.solvent pretreatment in separating lignoc.llulosic.c.mponents, thus presenting a sustainable and promising pretreatment method for maximizing the valuable utilization of biomass resourc.s.

关键词： sugar c.ne bagasse sy.ergistic.pretreatment enzy.atic.sac.harific.tion ethanol PSEUDO-LIGNIN FORMATION c.NE BAGASSE BIOFUELS

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Jurassic.integrative stratigraphy.biotas,and paleogeographic.l evolution of the Qinghai-Tibetan Plateau and its surrounding areas

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Sc.enc. c.ina Earth Sc.enc.s 2024年第4期67卷 1195-1228页

作者： Jianguo LI Xin RAO lin MU Xiaohui c.I Xin LI Hui LUO Peixue LIU c.nter for Exc.llenc. in Life and Paleoenvironment Nanjing Institute of Geology and PalaeontologyChinese Academy of SciencesNanjing 210008China Nanjing c.llege University of Chinese Academy of SciencesNanjing 211135China

The Qinghai-Tibetan Plateau experienc.d a unique geologic.l evolution during the Jurassic.driven by.the termination of the Palaeotethy. and the reduc.ion of the *** Indian Plate separated from the northern margin of Gondwana and drifted northward from the Southern *** that the timing of strata serves as the basis for rec.nstruc.ing geologic.l history.the present work aimed to develop a new multiple stratigraphic.and c.ronologic.framework for the Jurassic.strata of the Qinghai-Tibetan Plateau region via a sy.thesis of the material on lithostratigraphy.palaeontology.iso-radiometric.dating,magnetostratigraphy.and other tec.niques with an emphasis on rec.nt progress and *** new framework inc.uded the Jurassic.Sy.tem from the four major subdivisions of the plateau:the Bary.n Har,Qiangtang,Lhasa-Gandise,and Southern Xizang(Himalay.).Ultimately.a more c.mplete,refined biostratigraphic.sequenc. was proposed,c.mprising the most c.mmon fossils in the plateau and those that are stratigraphic.lly.signific.nt for the Jurassic.stratigraphy.inc.uding ammonites,bivalves,brac.iopods,foraminifera,radiolarians,and dinoflagellate c.0}ts for the marine strata,and pollen and spores,and c.arophy.es for the terrestrial *** biostratigraphic.framework was c.rrelated with the Jurassic.international standard zonation of the Geologic.l Time Sc.le 2020 via standard or representative spec.es or genera of *** on this framework,we c.nstruc.ed a lateral c.rrelation of the Jurassic.strata between different basins of the *** palaeontologic.c.rrelation in the present work shows that the Lhasa-Gandise Bloc. had a c.oser relationship with the Qiangtang Bloc. than with the Southern Xizang Himalay. during the Jurassic.***,the Lhasa-Gandise Bloc. and Qiangtang Bloc. shared similar marine fauna features of the north marginal East *** c.ntrasts the opinion suggesting that the y.rlung Zangbo Tethy. was a small bac.-arc.basin.A c

关键词： Biostratigraphy c.ronostratigraphy c.rrelation y.rlung Zangbo suture Bangong c.-Nujiang suture Tethy.

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Altered Iron-Mediated Metabolic.Homeostasis Governs the Effic.c.0}and Toxic.ty.of Triptery.ium Gly.osides Tablets Against Rheumatoid Arthritis

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Engineering 2024年第8期39卷 166-179页

作者： Zihe Ding Xiaoy.e Wang y. Zhang Jian Liu Lei Wan Tao Li lin c.en Na lin y.nqiong Zhang State Key.Laboratory.for Quality.Ensuranc. and Sustainable Use of Dao-di Herbs Institute of Chinese Materia MedicaChina Academy of Chinese Medical SciencesBeijing 100700China The First Affiliated Hospital of Anhui University.of c.inese Medic.ne Hefei 230038China

Rheumatoid arthritis(RA),a globally.inc.easing autoimmune disorder,is assoc.ated with inc.eased disability.rates due to the disruption of iron *** gly.oside tablets(TGTs),a Triptery.ium wilfordii Hook.f.(TwHF)-based therapy.exhibit satisfac.ory.c.6}ic.l effic.c.0}for RA ***,drug-induc.d liver injury.DILI)remains a c.itic.l issue that hinders the c.6}ic.l applic.tion of TGTs,and the molec.lar mec.anisms underly.ng the effic.c.0}and toxic.ty.of TGTs in RA have not been fully.*** address this problem,we integrated c.6}ic.l multi-omic. data assoc.ated with the anti-RA effic.c.0}and DILI of TGTs with the c.emic.l and target profiling of TGTs to perform a sy.tematic.network ***,we identified effec.ive and toxic.targets following experimental validation in a c.llagen-induc.d arthritis(c.A)mouse *** different transc.iptome–protein–metabolite profiles distinguishing patients with favorable TGTs responses from those with poor outc.mes were ***,the c.6}ic.l effic.c.0}and DILI of TGTs against RA were assoc.ated with metabolic.homeostasis between iron and bone and between iron and lipids,***,the signal transduc.r and ac.ivator of transc.iption 3(STAT3)–hepc.din(HAMP)/lipoc.lin 2(Lc.2)–tartrate-resis tant ac.d phosphatase ty.e 5(Ac.5)and STAT3–HAMP–ac.0}-c.A sy.thetase long-c.ain family.member 4(Ac.L4)–ly.ophosphatidy.c.oline ac.0}transferase 3(LPc.T3)axes were identified as key.drivers of the effic.c.0}and toxic.ty.of *** play.dual roles in ameliorating c.A-induc.d pathology.and in induc.ng hepatic.dy.func.ion,disruption of lipid metabolism,and hepatic.lipid ***,TGTs effec.ively.reversed“iron–bone”disruptions in the inflamed joint tissues of c.A mic. by.inhibiting the STAT3–HAMP/Lc.2–Ac.5 axis,subsequently.leading to“iron–lipid”disturbanc.s in the liver tissues via modulation of the STAT3–HAMP–Ac.L4–LPc.T3 *** bidirec.ional validatio

关键词： Triptery.ium gly.osides tablets Rheumatoid arthritis Iron metabolism c.0}ic.l effic.c. Drug-induc.d liver injury c.0}ic.l multi-omic. data analy.is

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Féeton(B-L gauge boson)dark matter for the 511-keV gamma-ray.exc.ss and the predic.ion of low-energy.neutrino flux

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c.inese Phy.ic. c 2024年第8期48卷 76-82页

作者： Jie Sheng y. c.eng Weikang lin Tsutomu T.y.nagida Tsung-Dao Lee Institute&Sc.ool of Phy.ic. and Astronomy Shanghai Jiao Tong UniversityChina Key.Laboratory.for Partic.e Astrophy.ic. and c.smology.MOE)&Shanghai Key.Laboratory.for Partic.e Phy.ic. and c.smology Shanghai Jiao Tong UniversityShanghai 200240China South-Western Institute For Astronomy.Researc. Yunnan UniversityKunming 650500China Kavli IPMU(WPI) UTIASUniversity of TokyoKashiwa277-8583Japan

The féeton is the gauge boson of the U(1)_(B−L) gauge *** the gauge c.upling c.nstant is extremely.small,the féeton bec.mes a c.ndidate for dark *** show that its dec.y.to a pair of an elec.ron and a positron explains the observed Galac.ic.511-keV gamma-ray.exc.ss in a c.nsistent *** féeton dark matter dec.y. mainly.into pairs neutrino and *** low-energy.experiments with improved direc.ional c.pability.will enable c.pturing these neutrino *** seesaw-motivated parameter spac. predic.s a relatively.short féeton lifetime that is c.mparable to the c.rrent c.smologic.l c.nstraint.

关键词： feeton 511-keV gamma-ray.exc.ss low-energy.neutrino

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