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Utilizing 3,4-ethylenedioxythiophene(EDOT)-bridged non-fullerene acceptors for efficient organic solar cells

Journal of Energy Chemistry 2022年第2期31卷 194-204页

作者： Sung Jae Jeon Young Hoon Kim Ie Na Kim Nam Gyu Yang Ji hee Yun Doo kyung Moon Nano and Information Materials(NIMs)Laboratory Department of Chemical EngineeringKonkuk University120 Neungdong-ro Gwangjin-guSeoul 05029South Korea Department of Academy of Applied Science and Technology Konkuk University120 Neungdong-ro Gwangjin-guSeoul 05029South Korea

A rational design of efficient low-band-gap non-fullerene acceptors(NFAs)for high-performance organic solar cells(OSCs)remains challenging;the main constraint being the decrease in the energy level of the lowest unoccupied molecular orbitals(LUMOs)as the bandgap of A-D-A-type NFAs ***,the short current density(J_(sc))and open-circuit voltage(V_(oc))result in a trade-off relationship,making it difficult to obtain efficient ***,three NFAs(IFL-ED-4 F,IDT-ED-4 F,and IDTT-ED-2 F)were synthesized to address the above-mentioned issue by introducing 3,4-ethylenedioxythiophene(EDOT)as aπ-*** NFAs exhibit relatively low bandgaps(1.67,1.42,and 1.49 eV,respectively)and upshifted LUMO levels(-3.88,-3.84,and-3.81 eV,respectively)compared with most reported low-band-gap ***,the photovoltaic devices based on IDT-ED-4 F blended with a PBDB-T donor polymer showed the best power conversion efficiency(PCE)of 10.4%with a high J_(sc) of 22.1 mA cm^(-2) and Voc of 0.884 V among the examined *** contrast,IDTT-ED-4 F,which was designed with an asymmetric structure of the D-p-A type,showed the lowest efficiency of 1.5%owing to the poor morphology and charge transport properties of the binary ***,when this was introduced as the third component of the PM6:BTP-BO-4 Cl,complementary absorption and cascade energy-level alignment between the two substances could be ***,the IDTT-ED-4 F-based ternary blend device not only improved the Jscand Voc,but also achieved a PCE of 15.2%,which is approximately 5.3%higher than that of the reference device with a minimized energy loss of 0.488 *** addition,the universality of IDTT-ED-2 F as a third component was effectively demonstrated in other photoactive systems,specifically,PM6:BTPe C9 and PTB7-Th:IEICO-4 *** work facilitates a better understanding of the structure–property relationship for utilizing efficient EDOT-bridged NFAs in high-performance OSC applications.

关键词： Non-fullerene acceptor 3,4-ethylenedioxythiophene Organic solar cell π-bridge π-spacer

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ALBERT with Knowledge Graph Encoder Utilizing Semantic Similarity for Commonsense Question Answering

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Intelligent Automation & Soft Computing 2023年第4期36卷 71-82页

作者： Byeongmin Choi YongHyun lee Yeunwoong kyung Eunchan Kim Department of Computer Science and Engineering Seoul National UniversitySeoul08826Korea School of Computer Engineering Hanshin UniversityOsan18101Korea Department of Intelligence and Information Seoul National UniversitySeoul08826Korea

Recently,pre-trained language representation models such as bidirec-tional encoder representations from transformers(BERT)have been performing well in commonsense question answering(CSQA).However,there is a problem that the models do not directly use explicit information of knowledge sources existing *** augment this,additional methods such as knowledge-aware graph network(KagNet)and multi-hop graph relation network(MHGRN)have been *** this study,we propose to use the latest pre-trained language model a lite bidirectional encoder representations from transformers(ALBERT)with knowledge graph information extraction *** also propose to applying the novel method,schema graph expansion to recent language ***,we analyze the effect of applying knowledge graph-based knowledge extraction techniques to recent pre-trained language models and conﬁrm that schema graph expansion is effective in some ***,we show that our proposed model can achieve better performance than existing KagNet and MHGRN models in CommonsenseQA dataset.

关键词： Commonsense reasoning question answering knowledge graph language representation model

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Rumex acetosella Inhibits Platelet Function via Impaired MAPK and Phosphoinositide 3-Kinase Signaling

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Chinese Journal of Integrative Medicine 2022年第9期28卷 802-808页

作者： Bo-Ra Jeon Muhammad Irfan Seung Eun lee Jeong Hoon lee Man hee Rhee Laboratory of Physiology and Cell Signaling College of Veterinary MedicineKyungpook National UniversityDaegu41566Republic of Korea Department of Herbal Crop Research National Institute of Horticultural and Herbal Science(NIHHS)Eumseong27709Republic of Korea

Objective:To examine the antiplatelet and antithrombotic activity of Rumex acetosella ***:Standard light aggregometry was used for platelet aggregation,intracellular calcium mobilization assessed using Fura-2/AM,granule secretion(ATP release)by luminometer,and fibrinogen binding to integrin α_(Ⅱb)β_(3) detected using flow *** blotting is carried out to determine the phosphorylation of mitogen-activated protein kinase(MAPK)and phosphoinositide 3-kinase(PI3K)/Akt ***:Rumex acetosella displayed the ability to inhibit platelet aggregation,calcium mobilization,granule secretion,and fibrinogen binding to integrin α_(Ⅱb)β_(3).Rumex acetosella has also down-regulated MAPK and PI3K/Akt phosphorylation(all P<0.01).Conclusion:Rumex acetosella extract exhibits antiplatelet activity via modulating GPVI signaling,and it may protect against the development of platelet-related cardiovascular diseases.

关键词： antiplatelet ethnomedicine integrinα_(Ⅱb)β_(3) mitogen-activated protein kinase Rumex acetosella L.

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Structurally engineered colloidal quantum dot phosphor using TiO_(2) photonic crystal backbone

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Light(Science & Applications) 2022年第11期11卷 2782-2789页

作者： Hansol lee Tae-Yun lee Yeonsang Park kyung-Sang Cho Young-Geun Rho Hyuck Choo Heonsu Jeon Department of Physics and Astronomy Seoul National UniversitySeoul 08826Republic of Korea Inter-university Semiconductor Research Center Seoul National UniversitySeoul 08826Republic of Korea Department of Physics Chungnam National UniversityDaejeon 34134Republic of Korea Institute of Quantum Systems Chungnam National UniversityDaejeon 34134Republic of Korea Samsung Advanced Institute of Technology Suwon 16678Republic of Korea Institute of Applied Physics Seoul National UniversitySeoul 08826Republic of Korea

Photonic crystal(PhC)phosphor,in which the phosphor material is periodically modulated for an enhancement in color-conversion efficiency via resonant absorption of excitation photons,is a paradigm-shifting structural phosphor ***-dimensional(2D)square-lattice PhC phosphor is currently considered the most advanced platform because of not only its high efficiency,but also its immunity to excitation *** the present study,two major modifications are made to further improve the performance of the 2D PhC phosphor:increasing the refractive index contrast and planarizing the *** index contrast is improved by replacing the PhC backbone material with TiO_(2)whereas the surface planarization is achieved by removing excessive colloidal quantum dots from the *** comparison with the reference phosphor,the upgraded PhC phosphor exhibits~59 times enhanced absorption(in simulations)and~7 times enhanced emission(in experiments),both of which are unprecedentedly *** results not only brighten the viability and applicability of the PhC phosphor but also spur the phosphor development through structural engineering of phosphor materials.

关键词： immunity phosphor backbone

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Characterization of focal hypermetabolic thyroid incidentaloma: An analysis with F-18 fluorodeoxyglucose positron emission tomography/computed tomography parameters

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World Journal of Clinical Cases 2022年第1期10卷 155-165页

作者： Haejun lee Yoo Seung Chung Joon-Hyop lee Ki-Young lee kyung-Hoon Hwang Department of Nuclear Medicine Gachon University College of MedicineGil Medical CenterIncheon 21565South Korea Department of Endocrine Surgery Gachon University College of MedicineGil Medical CenterIncheon 21565South Korea Department of Endocrinology and Metabolism Gachon University College of MedicineGil Medical CenterIncheon 21565South Korea

BACKGROUND Incidentally found thyroid tumor(thyroid incidentaloma,TI)on F-18 fluorodeoxyglucose(FDG)positron emission tomography-computed tomography(PETCT)is reported in 2.5%-5%of patients being investigated for non-thyroid *** to 50%of these cases have been diagnosed to be malignant by cytological/histological ***(US)and fine-needle aspiration cytology are recommended for thyroid nodules with high FDG uptake(hypermetabolism)that are 1 cm or greater in *** is important to accurately determine whether a suspicious hypermetabolic TI is malignant or *** To distinguish malignant hypermetabolic TIs from benign disease by analyzing F-18 FDG PET-CT parameters and to identify a cut-off *** Totally,12761 images of patients who underwent F-18 FDG PET-CT for nonthyroid purposes at our hospital between January 2016 and December 2020 were retrospectively reviewed,and 339 patients[185 men(mean age:68±11.2)and 154 women(mean age:63±15.0)]were found to have abnormal,either focal or diffuse,thyroid FDG *** a thorough review of their medical records,US,and cytological/histological reports,46 eligible patients with focal hypermetabolic TI were included in this *** TIs were categorized as malignant and benign according to the cytological/histological reports,and four PET parameters[standardized uptake value(SUV)max,SUV_(peak),SUV_(mean),and metabolic tumor volume(MTV)]were measured on FDG *** lesion glycolysis(TLG)was calculated by multiplying the SUV_(mean) by *** parametric and non-parametric methods were used to compare the five parameters between malignant and benign *** operating characteristic(ROC)curve analysis was performed to identify a cut-off *** Each of the 46 patients[12 men(26.1%;mean age:62±13.1 years)and 34 women(73.9%;mean age:60±12.0 years)]with focal hypermetabolic TIs had one focal hypermetabolic *** them,26(56.5%)were malignant and 20(43.5%)were ***_(max

关键词： Thyroid incidentaloma Malignancy Fluorodeoxyglucose positron emission tomography/computed tomography Standardized uptake value Cut-off

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A unique and well-designed 2D graphitic carbon nitride with sponge-like architecture for enhanced visible-light photocatalytic activity

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Journal of Materials Science & Technology 2023年第28期159卷 99-111页

作者： Mahdieh Razi Asrami Milad Jourshabani Min hee Park Daiha Shin Byeong-Kyu lee Department of Civil and Environment Engineering University of UlsanDaehakro 93NamguUlsan 680-749Republic of Korea Western Seoul Center Korea Basic Science InstituteSeoul 03759Republic of Korea

A unique and well-designed 2D graphitic carbon nitride(g-CN)with sponge-like architecture has been successfully synthesized by engineering supramolecular self-assembly and well-organized SiO 2 *** resulting material showed great optical and textural characteristics with plenty of open and uni-form pores,which are very helpful whether for multiple light scattering or mass *** formation of boosted delocalizedπ-conjugated electrons at the molecular level and condensed heptazine building blocks result in enhanced carrier density and charge transfer *** emission spectroscopy and time-resolved fluorescence lifetime(TRPL)strongly confirmed the enhancement of light harvesting and prolonged charge carrier *** optimized sample exhibited a degradation performance of 95%of bisphenol A(BPA,10 mg L-1)after 60 min under visible-light irradiation at pH=*** the scavenging experiments,probing experiments as well as electron paramagnetic resonance(EPR)confirm that•O 2-is the dominant reactive species that fragments bisphenol ***,density functional theory(DFT)calculations unveil that the BPA interaction with a modified g-CN containing porous structure is energeti-cally more favorable than non-porous pure ***,the toxicity assessment showed that the final degradation products were placed in the non-harmful category based on acute and chronic *** study presents a promising strategy to modify the g-CN properties and provides an efficient technique for boosting its visible-light photocatalytic activity.

关键词： Sponge-like Carbon nitride Photocatalysis Visible-light

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Single-cell RNA sequencing of mitoticarrested prospermatogonia with DAZL::GFP chickens and revealing unique epigenetic reprogramming of chickens

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Journal of Animal Science and Biotechnology 2022年第5期13卷 1305-1325页

作者： Hyeon Jeong Choi kyung Min Jung Deivendran Rengaraj kyung Youn lee Eunhui Yoo Tae Hyun Kim Jae Yong Han Department of Agricultural Biotechnology and Research Institute of Agriculture and Life Sciences Seoul National UniversitySeoul 08826South Korea Department of Animal Science Pennsylvania State UniversityState CollegePA 16801USA

Background:Germ cell mitotic arrest is conserved in many vertebrates,including birds,although the time of entry or exit into quiescence phase *** arrest is essential for the normal differentiation of male germ cells into spermatogonia and accompanies epigenetic reprogramming and meiosis inhibition from embryonic development to ***,mitotic arrest was not well studied in chickens because of the difficulty in obtaining pure germ cells from relevant developmental ***:We performed single-cell RNA sequencing to investigate transcriptional dynamics of male germ cells during mitotic arrest in DAZL::GFP *** differentially expressed gene analysis and K-means clustering to analyze cells at different developmental stages(E12,E16,and hatch),we found that metabolic and signaling pathways were regulated,and that the epigenome was reprogrammed during mitotic *** particular,we found that histone H3K9 and H3K14 acetylation(by HDAC2)and DNA demethylation(by DNMT3B and HELLS)led to a transcriptionally permissive chromatin ***,we found that global DNA demethylation occurred gradually after the onset of mitotic arrest,indicating that the epigenetic-reprogramming schedule of the chicken genome differs from that of the mammalian *** hypomethylation persisted after hatching,and methylation was slowly re-established 3 weeks ***:We found a unique epigenetic-reprogramming schedule of mitotic-arrested chicken prospermatogonia and prolonged hypomethylation after *** will provide a foundation for understanding the process of germ-cell epigenetic regulation in several species for which this process is not clearly *** findings on the biological processes related to sex-specific differentiation of prospermatogonia could help studying germline development in vitro more elaborately.

关键词： DAZL::GFP chickens DNA methylation Epigenetic reprogramming Histone acetylation Male germ cell Mitotic arrest Prospermatogonia Single-cell RNA sequencing

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Case mistaken for leukemia after mRNA COVID-19 vaccine administration:A case report

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World Journal of Clinical Cases 2022年第33期10卷 12268-12277页

作者： Seul Bi lee Chi Young Park Sang-Gon Park hee Jeong lee Department of Internal Medicine Hemato-oncologyChosun University HospitalGwangju 501-717South Korea

BACKGROUND Following the global outbreak of coronavirus disease 2019(COVID-19),unlike other vaccines,COVID-19 vaccines were developed and commercialized in a relatively short period of *** large-scale administration of this vaccine in a short time-period led to various unexpected side effects,including severe cytopenia and thrombosis with thrombocytopenia *** many reports on adverse reactions,vaccination was necessary to prevent the spread of COVID-19;thus,it is essential to understand and discuss various cases of adverse reactions after *** SUMMARY A 77-year-old woman was administered the second dose of Pfizer mRNA COVID-19 *** vaccination she experienced fever,myalgia,and *** were subsequently administered for several days,but there was no improvement in the *** patient showed severe thrombocytopenia and *** and abdominopelvic computed tomography showed no infection related findings,but splenomegaly and cirrhotic liver features were observed.A large number of immature cells were observed in the peripheral blood smear;thus,bone marrow examination was performed for acute ***,there were no *** patient recovered after administration of hepatotoxins and transfusion treatment for cytopenia and was diagnosed with an adverse reaction to COVID-19 *** Adverse reactions of vaccination could be mistaken for hematologic malignancies including *** report a patient with leukocytosis following COVID-19 vaccination.

关键词： COVID-19 Vaccine mRNA Leukocytosis Adverse reaction Case report

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Speed vernalization to accelerate generation advance in winter cereal crops

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Molecular Plant 2022年第8期15卷 1300-1309页

作者： Jin-kyung Cha Kathryn O'Connor Samir Alahmad Jong-hee lee Eric Dinglasan Hyeonjin Park So-Myeong lee Dominique Hirsz Soon-Wook Kwon Youngho Kwon Kyeong-Min Kim Jong-Min Ko lee T.Hickey Dongjin Shin Laura E.Dixon National Institute of Crop Science RDAMiryang 50424Korea School of Biology Faculty of Biological SciencesUniversity of LeedsLeeds LS29JTUK Queensland Alliance for Agriculture and Food Innovation The University of QueenslandSt.LuciaQLDAustralia Department of Plant Bioscience Pusan National UniversityMiryang 60463Korea

There are many challenges facing the development of high-yielding,nutritious crops for future *** limiting factor is generation time,which prolongs research and plant breeding *** advances in speed breeding protocols have dramatically reduced generation time for many short-day and long-day species by optimizing lightand temperature conditions during plant ***,winter crops with a vernalization requirement stillrequire upto 6-10weeks in low-temperature conditions before thetransition to ***,we tested a suite of environmental conditions and protocols to investigate whether the vernalization process can be *** identified a vernalization method consisting of exposing seeds at the soil surface to an extended photoperiod of 22 h day:2 h night at 10°C with transfer to speed breeding conditions that dramatically reduces generation time in both winter wheat(Triticum aestivum)and winter barley(Hordeum vulgare).Implementation of the speedvernalization protocolfollowed byspeedbreedingallowed the completion ofuptofivegenerations per yearforwinter wheat or barley,whereas only two generations can be typically completed under standard vernalization and plant growth *** speed vernalization protocol developed in this study has great potential to accelerate biological research and breeding outcomes for winter crops.

关键词： speed breeding photoperiod temperature wheat barley breeding

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Graphene Bridge Heterostructure Devices for Negative Differential Transconductance Circuit Applications

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Nano-Micro Letters 2023年第2期15卷 161-171页

作者： Minjong lee Tae Wook Kim Chang Yong Park Kimoon lee Takashi Taniguchi Kenji Watanabe Min‑gu Kim Do kyung Hwang Young Tack lee Department of Electrical and Computer Engineering Inha UniversityIncheon 22212Republic of Korea Department of Materials Science and Engineering The University of Texas at DallasRichardsonTX 75080USA Center for Opto‑Electronic Materials and Devices Post‑Silicon Semiconductor InstituteKorea Institute of Science and Technology(KIST)Seoul 02792Republic of Korea Department of Physics Kunsan National UniversityGunsan 54150Republic of Korea Advanced Materials Laboratory National Institute for Materials ScienceTsukuba 305‑0044Japan Department of Information and Communication Engineering Inha UniversityIncheon 22212Republic of Korea Division of Nanoscience and Technology KIST SchoolUniversity of Science and Technology(UST)Seoul 02792Republic of Korea Department of Electronic Engineering Inha UniversityIncheon 22212Republic of Korea

Two-dimensional van der Waals(2D vdW)material-based heterostructure devices have been widely studied for high-end electronic applications owing to their heterojunction *** this study,we demonstrate graphene(Gr)-bridge heterostructure devices consisting of laterally series-connected ambipolar semiconductor/Gr-bridge/n-type molybdenum disulfide as a channel material for field-effect transistors(FET).Unlike conventional FET operation,our Gr-bridge devices exhibit nonclassical transfer characteristics(humped transfer curve),thus possessing a negative differential *** phenomena are interpreted as the operating behavior in two series-connected FETs,and they result from the gate-tunable contact capacity of the Gr-bridge ***-value logic inverters and frequency tripler circuits are successfully demonstrated using ambipolar semiconductors with narrow-and wide-bandgap materials as more advanced circuit applications based on non-classical transfer ***,we believe that our innovative and straightforward device structure engineering will be a promising technique for future multi-functional circuit applications of 2D nanoelectronics.

关键词： Graphene bridge Heterostructure device Non-classical transfer characteristics Multi-value logic inverter Frequency tripler

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