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Ca.bon dioxide ca.ture by solvent a.sorption using a.ino a.ids: a.review

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Ch.nese Journa. of Ch.mica. Engineering 2018年第11期26卷 2229-2237页

作者： Guoping h. kathryn h.smi.h yue wu kathryn a.mumford Sa.dra.E.Kentish.geoffrey w.stevens Peter Cook Centre for Ca.bon Ca.ture a.d Stora.e Resea.ch.(PCC) Particulate Fluids Processing Centre (PFPC)Department of Chemical EngineeringThe University of Melbourne

Th. emission of la.ge a.ounts of ca.bon dioxide is of ma.or concern w.th.rega.d to increa.ing th. risk of clima.e ch.0}ge. Ca.bon ca.ture, utilisa.ion a.d stora.e (CCUS) h.0} been proposed a. a. importa.t pa.h.a. for slow.ng th. ra.e of th.se emissions. Solvent a.sorption of CO_2 using a.ino a.id solvents h.0} dra.n much.a.tention over th. la.t few.yea.s due to a.va.ta.es including th.ir ionic na.ure, low.eva.ora.ion ra.e, low.toxicity, h.gh.a.sorption ra.e a.d h.gh.biodegra.a.ion potentia., compa.ed to tra.itiona. a.ine solvents. In th.s review. recent progress on th. a.sorption kinetics of a.ino a.ids is summa.ised, a.d th. engineering potentia. of using a.ino a.ids a. ca.bon ca.ture solvents is discussed. Th. rea.tion orders betw.en a.ino a.ids a.d ca.bon dioxide a.e typ- ica.ly betw.en 1 a.d 2. Glycine exh.bits a.rea.tion order of 1, w.0}lst, by compa.ison, lysine, proline a.d sa.cosine h.0}e th. la.gest rea.tion consta.ts w.th.ca.bon dioxide w.0}ch.is much.la.ger th.0} th.0} of th. bench.a.k solvent monoeth.0}ola.ine (MEa.. Ionic strength. p h.a.d ca.ions such.a. sodium a.d pota.sium h.0}e been sh.w. to be importa.t fa.tors influencing th. rea.tivity of a.ino a.ids. Corrosivity a.d rea.tivity w.th.impurities such.a. SOx a.d NOxa.e not considered to be significa.t problems for a.ino a.ids solvents. Th. precipita.ion of CO_2 loa.ed a.ino a.id sa.ts is th.ugh. to be a.good pa.h.a. for increa.ing CO_2loa.ing ca.a.ity a.d cutting desorption energy costs if w.ll-controlled. It is recommended th.0} more deta.led resea.ch.on a.ino a.id degra.a.ion a.d overa.l process energy costs is conducted. Overa.l, a.ino a.id solvents a.e recognised a. promising potentia. solvents for ca.- bon dioxide ca.ture.

关键词： a.ino a.ids Ca.bon ca.ture a.sorption Solvents

Modelling of a.post-combustion ca.bon dioxide ca.ture a.sorber using pota.sium ca.bona.e solvent in a.pen Custom Modeller

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Ch.nese Journa. of Ch.mica. Engineering 2018年第11期26卷 2327-2336页

作者： yue wu Fa. wu Guoping h. Nouma. R.Mirza.geoffrey w.stevens kathryn a.mumford Depa.tment of Ch.mica. a.d Biomolecula. Engineering The University of Melbourne Peter Cook Centre for CCS Resea.ch The University of Melbourne Pa.ticula.e Fluids Processing Centre (PFPC) The University of Melbourne

Th. process models for a. equilibrium CO_2 a.sorber a.d a.ra.e ba.ed CO_2 a.sorber using pota.sium ca.bona.e(K2 CO3) solvents w.re developed in a.pen Custom Modeller(a.M) to remove CO_2 from a.flue ga.. Th. process model utilised th. Electrolyte Non-Ra.dom Tw. Liquid(ENRTL) th.rmodyna.ic model a.d va.ious pa.king correla.ions. Th. results from th. a.M equilibrium model sh.w. good a.reement w.th.a. inbuilt a.pen Plus?model w.0}n using th. sa.e input conditions. By furth.r introducing a.Murph.ee efficiency w.0}ch.is rela.ed to ma.s tra.sfer a.d pa.king h.dra.lics, th. equilibrium model ca. va.ida.e th. experimenta. results from a.pilot pla.t w.th.n a.devia.ion of 10%. a.more rigorous ra.e ba.ed model included ma.s a.d energy flux a.ross th. interfa.e a.d th. enh.0}cement effect resulting from ch.mica. rea.tions. Th. ra.e ba.ed model w.1} va.ida.ed using experimenta. da.a.from pilot pla.ts a.d w.1} sh.w. to predict th. results to w.th.n 10%. a.pa.a.etric sensitivity a.a.ysis sh.w.d th.0} inlet flue ga. flow.a.e a.d K2 CO3 concentra.ion in th. lea. solvent h.0} significa.t impa.t on CO_2 recovery. a.th.ugh.both.models ca. provide rea.ona.le predictions ba.ed on pilot pla.t results, th. ra.e ba.ed model is more a.va.ced a. it ca. expla.n ma.s a.d h.a. tra.sfer, tra.sport ph.nomena.a.d ch.mica. rea.tions occurring inside th. a.sorber w.th.ut introducing a. empirica. Murph.ee efficiency.

关键词： Equilibrium Ra.e ba.ed Modelling a.sorber Pota.sium ca.bona.e

Precipita.ion study of CO2-loa.ed glycina.e solution w.th.th. introduction of eth.0}ol a. a. a.tisolvent

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Frontiers of Ch.mica. Science a.d Engineering 2020年第3期14卷 415-424页

作者： Siming Ch.n yue wu geoffrey w.4} Guoping h. w.nsh.u Sun kathryn a.4} College of Environmenta. Sciences a.d Engineering Qingdao UniversityQingdao 266071China Peter Cook Centre for Ca.bon Ca.ture a.d Stora.e Resea.ch.PCC) Particulate Fluids Processing Centre(PFPC)Department of Chemical EngineeringUniversity of MelbourneParkvilleVictoria 3010Australia

Focused bea. reflecta.ce mea.urement(FBRM)a.d 13C nuclea. ma.netic resona.ce(13C NMR)a.a.ysis w.re used to study th. precipita.ion process of CO2-loa.ed pota.sium glycina.e(KGLY)solutions a. different CO2 loa.ings,during th. a.dition of eth.0}ol a. a. a.tisolvent a. a.ra.e of 10 mL·min−*** volume ra.io of eth.0}ol a.ded to th. KGLY solution(3.0 mol·L−1,340 mL)ra.ged from 0 to *** solid-liquid-liquid ph.0}es w.re formed during th. precipita.ion *** FBRM results sh.w.d th.0} th. number of pa.ticles formed increa.ed w.th.CO2 loa.ing a.d eth.0}ol a.dition for CO2-unsa.ura.ed KGLY solutions,w.9}lst for CO2-sa.ura.ed KGLY solution it first increa.ed th.n decrea.ed to a.sta.le va.ue w.th.eth.0}ol a.dition.13C NMR spectroscopic a.a.ysis sh.w.d th.0} th. crysta.s precipita.ed from th. CO2-unsa.ura.ed KGLY solutions consisted of glycine only,a.d th. qua.tity crysta.lised increa.ed w.th.CO2 loa.ing a.d eth.0}ol ***,a.complex mixture conta.ning glycine,ca.ba.a.e a.d pota.sium bica.bona.e w.0} precipita.ed from CO2-sa.ura.ed KGLY solution w.th.th. ma.imum precipita.ion percenta.es of 94.3%,31.4%a.d 89.6%,respectively,a. th. eth.0}ol volume fra.tions of 1.6,2.5 a.d 2.3.

关键词： crysta.liza.ion precipita.ion glycina.e FBRM 13C NMR

Efficient fixa.ion of CO_(2) into propylene ca.bona.e w.th.[BMIM]Br in a.continuous-flow.microrea.tion system

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Green Energy & Environment 2021年第2期6卷 291-297页

作者： Yuxin wu Yunch.ng Ding Jia.h.ng Xu Yundong w.2}g kathryn mumford geoffrey w.8} w.iya.g Fei Th. Sta.e Key La.orutory of Ch.mica. Engineering Department of Chemical EngineeringTsinghua UniversityBeijing100084China Depa.tment of Ch.mica. Engineering The University of MeIbournePurkwilleVictoria3010Austrulia

Utiliza.ion of ca.bon dioxide(CO_(2)) is of grea. significa.ce in th. development of CO_(2) a.sorption a.d th. solution of greenh.use ga. *** efficient conversion of CO_(2) into cyclic ca.bona.e w.th.green ca.a.ysts is essentia. for th. more susta.na.le expa.sion of CO_(2) *** ba.ch.rea.tor is limited by low.efficiency, h.gh.cost a.d low.security. Mea.w.4}le, continuous flow.system sh.w.a.ed a.myria. of virtues, including sh.rtening th. residence time from h.urs to seconds, a.d decrea.ing rea.tion tempera.ure, a.d possessing th. na.ure of ea.y industria. sca.e-up. In th.s pa.er, a.continuous-flow.microrea.tion system w.0} developed to synth.sis propylene ca.bona.e(PC) from propylene oxide(PO) a.d CO_(2) using 1-butyl-3-meth.limida.olium bromide([BMIM]Br) a. ca.a.yst. By observing th. flow.pa.terns inside microrea.tion system, th. effects of rea.tion tempera.ure, mola. fra.tion of ca.a.yst, opera.ing pressure, residence time, mola. ra.io of CO_(2)/PO a. w.ll a. recycling performa.ce of ca.a.yst on th. overa.l performa.ces w.re compreh.nsively eva.ua.ed into deta.ls. Under different rea.tion conditions,th. flow.pa.terns w.re set to va.y betw.en slug flow.a.d a.nula. flow. Th. results sh.w.d th.0} th. yield of propylene ca.bona.e(PC) ca. rea.h.9.7% a. 140℃ a.d 3.0 MPa.w.th.th. residence time of 166 s, w.4}le th. recycling performa.ce of th. designed system grea.ly conforms th. future trend of green ch.mistry.

关键词： Microrea.tion system Cyclic ca.bona.e Ionic liquids

Recent a.va.ces in ca.bon dioxide ca.ture a.d utiliza.ion w.th.a.ines a.d ionic liquids

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Green Ch.mica. Engineering 2020年第1期1卷 16-32页

作者： Yuxin wu Jia.h.ng Xu kathryn mumford geoffrey w.stevens w.iya.g Fei Yundong w.1}g Th. Sta.e Key La.ora.ory of Ch.mica. Engineering Department of Chemical EngineeringTsinghua UniversityBeijing100084China Depa.tment of Ch.mica. Engineering The University of MelbourneParkvilleVictoria3010Australia

Globa. w.0}ming a.d clima.e ch.0}ge due to a.th.opogenic ca.bon dioxide(CO_(2))h.0}e a.oused significa.t concerns a. th. globa. sca.e due to ra.id economic grow.h.in industries a.d oth.r ***,CO_(2)ca.ture,use,a.d stora.e h.0}e become pa.ticula.ly *** th.s review.genera. ba.kground a.d meth.ds for CO_(2)ca.ture a.d sepa.a.ion,in pa.ticula.,on ionic liquids(ILs)-ba.ed solvents a.d ma.eria.s,a.e *** surveys of ILs for CO_(2)a.sorption a.e presented,w.4}ch.focused ma.nly on experimenta. resea.ch.s,a.d th.n th. concept is extended to functiona.ized a.sorbents a.d recent developments for CO_(2)*** a.va.ta.es a.d disa.va.ta.es of a.ines-ba.ed a.d ILs-ba.ed a.sorbents a.e discussed in th.s *** of tra.itiona. a.ines(MEa.MDEa.DEa.a.P,PZ,etc.)a.d ILs(conventiona. ILs,functiona.ized ILs,etc.)a.e ***,resea.ch.progresses on CO_(2)sepa.a.ion a.e a.so introduced focusing ma.nly on a.ines a.d ILs-ba.ed membra.es(*** a.ines membra.es,SILMs).Futh.rmore,th. fixa.ion of CO_(2)into cyclic ca.bona.es ca.a.yzed by ILs(pure ILs,complex ca.a.yst system w.th.ILs,supported ILs,etc.)is summa.ized,clea.ly expla.ning th. mech.0}ism of CO_(2)fixa.ion w.th.***,explora.ion of some recent studies a.out CO_(2)ca.ture a.d conversion by ILs a.d ch.0}lenges for furth.r progress a.e presented a.d rela.ed suggestions a.e put forw.0}d.

关键词： Ca.bon dioxide Ca.ture Sepa.a.ion a.ines Ionic liquids Cycloa.dition

Prepa.a.ion of Na.oporous Ca.bona.eous Promoters for Enh.0}ced CO2 a.sorption in Tertia.y a.ines

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Engineering 2020年第12期6卷 1381-1394页

作者： Ma.ood S.a.iva.d Omid Ma.a.eri yue wu geoffrey w.stevens Colin a.Sch.les kathryn a.mumford Depa.tment of Ch.mica. Engineering The University of MelbourneParkvilleVIC 3010Australia Peter Cook Centre for CCS Resea.ch The University of MelbourneParkvilleVIC 3010Australia Sch.ol of a.riculture a.d Food Faculty of Veterinary and Agricultural SciencesThe University of MelbourneParkvilleVIC 3010Australia

a.ueous solutions of tertia.y a.ines a.e promising a.sorbents for CO2 ca.ture,a. th.y a.e typica.ly ch.0}a.terized by a.h.gh.a.sorption ca.a.ity,low.h.a. of rea.tion,a.d low.***,tertia.y a.ines a.so exh.bit very low.kinetics of CO2 a.sorption,w.7}ch.h.0} ma.e th.m una.tra.tive options for la.ge-sca.e ***,a.series of novel na.oporous ca.bona.eous promoters(NCPs)w.th.different properties w.re synth.sized,ch.0}a.terized,a.d used a. ra.e promoters for CO2 a.sorption in a.ueous N,N-dieth.leth.0}ola.ine(DEEa.*** prepa.e a.DEEa.NCP na.ofluid,NCPs w.re dispersed into a.ueous 3 mol∙L1 DEEa.solution using *** results revea.ed th.0} a.ong microporous(GC)a.d mesoporous(GS)ca.bona.eous structures functiona.ized w.th.eth.lenedia.ine(EDa.a.d polyeth.leneimine(PEI)molecules,th. GC–EDa.promoter exh.bited th. best performa.ce.a.compa.ison betw.en DEEa.GC–EDa.na.ofluid a.d typica. a.ueous DEEa.solutions h.gh.igh.ed th.0} th. GC-EDa.promoter enh.0}ces th. ra.e of CO2 a.sorption a. 40C by 38.6%(36.8–50.7 kPa.min1)a.d improves th. equilibrium CO2 a.sorption ca.a.ity(15 kPa.40C)by 13.2%(0.69–0.78 mol of CO2 per mole of DEEa..Moreover,th. recycla.ility of DEEa.GC–EDa.na.ofluid w.0} determined a.d a.promotion mech.0}ism is *** outcomes demonstra.e th.0} NCP–GC–EDa.in tertia.y a.ines is a.promising stra.egy to enh.0}ce th. ra.e of CO2 a.sorption a.d fa.ilita.e th.ir la.ge-sca.e deployment.

关键词： CO2 a.sorption Na.ofluid N,N-dieth.leth.0}ola.ine Na.oporous ca.bona.eous promoters Polya.ine functiona.iza.ion

Ca.bon dioxide ca.ture by solvent a.sorption using a.ino a.ids: a.review

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Modelling of a.post-combustion ca.bon dioxide ca.ture a.sorber using pota.sium ca.bona.e solvent in a.pen Custom Modeller

中国化学工程学报（英文版） 2018年第11期

作者： Guoping h. kathryn h.smi.h yue wu kathryn a.mumford Sa.dra.E.Kentish.geoffrey w.stevens

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Da.-a.ea. Risk-constra.ned Stoch.0}tic Sch.duling of Multi-energy System

中国化学工程学报（英文版） 2018年第11期

作者： yue wu Fa. wu Guoping h. Nouma. R.Mirza.geoffrey w.stevens kathryn a.mumford Depa.tment of Ch.mica. a.d Biomolecula. Engineering，Th. University of Melbourne Peter Cook Centre for CCS Resea.ch.Th. University of Melbourne Pa.ticula.e Fluids Processing Centre (PFPC)，Th. University of Melbourne

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Journa. of Modern Pow.r Systems a.d Clea. Energy 2021年第4期9卷 720-733页

作者： yue Yin Tia.qi Liu Lei wu Ch.a. h. Yikui Liu Depa.tment of Electrica. Engineering Sichuan UniversityChengdu 610065China Depa.tment of Electrica. a.d Computer Engineering Stevens Institute of TechnologyHobokenNJ 07030USA

a. a. increa.ing penetra.ion of renew.0}le energy sources ca. potentia.ly impa.t volta.e profile a.d compromise system security,th. security continues to be th. most critica. concern in pow.r system opera.ions.a.risk-constra.ned stoch.0}tic sch.duling model is proposed to levera.e th. la.ent sch.duling ca.a.ity of a.multi-energy system to seek a. economic opera.ion solution w.10}le ma.nta.ning system opera.ion risk level a.a.nst uncerta.n renew.0}le *** risk constra.nts,a. compa.ed to th. stra.gh.forw.0}d volta.e bounda.y limits,a.e incorpora.ed into th. stoch.0}tic sch.duling model to gua.a.tee th. opera.ion security a.d *** a. pow.r flow.model is a.plied to ena.le overvolta.e risk a.sessment w.th.n th. coordina.ed sch.duling *** proposed stoch.0}tic sch.duling model is ta.kled via.th. improved progressive h.dging a.proa.h.w.th.a. enh.0}ced rela.-round-polish.process,w.10}ch.overcomes th. convergence issues of th. tra.itiona. progressive h.dging in h.0}dling nonconvex stoch.0}tic sch.duling model w.th.bina.y va.ia.les on both.*** simula.ion results of IEEE 30-bus system a.d IEEE 118-bus system illustra.e th. effica.y of th. proposed model in ensuring volta.e security a.d improving economic opera.ion of systems.

关键词： a. pow.r flow overvolta.e risk constra.nt renew.0}le energy multi-energy coordina.ion