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Upcycling end of lithium cobalt oxide batteries to electrocatalyst for oxygen reduction reaction in direct methanol fuel cell via sustainable approach

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Journal of Energy Chemistry 2023年第7期82卷 148-157,I0004页

作者： Keyru Serbara Bejigo Kousik Bhunia jungho kim Chaehyeon Lee Seoin Back Sang-Jae kim Nanomaterials&System Lab Major of Mechatronics EngineeringFaculty of Applied Energy SystemJeju National UniversityJeju 63243Republic of Korea Nanomaterials&System Lab Major of Mechanical System EngineeringCollege of EngineeringJeju National UniversityJeju 63243Republic of Korea Research Institute of New Energy Industry(RINEI) Jeju National UniversityJeju 63243Republic of Korea Department of Chemical and Biomolecular Engineering Institute of Emergent MaterialsSogang UniversitySeoul 04107Republic of Korea

Recycling spent lithium-ion batteries(SLIBs)has become essential to preserve the environment and reclaim vital resources for sustainable *** typical SLIBs recycling concentrated on separating valuable components had limitations,including high energy consumption and complicated separation *** work suggests a safe hydrometallurgical process to recover usable metallic cobalt from depleted LiCoO_(2)batteries by utilizing citric acid as leachant and hydrogen peroxide as an oxidizing agent,with ethanol as a selective precipitating *** anode graphite was also recovered and converted to graphene oxide(GO).The above components were directly resynthesized to cobaltintegrated nitrogen-doped graphene(Co@NG).The Co@NG showed a decent activity towards oxygen reduction reaction(ORR)with a half-wave potential of 0.880 V ***,almost similar to Pt/C(0.888 V ***)and with an onset potential of 0.92 V *** metal-nitrogen-carbon(Co-N-C)having the highest nitrogen content has decreased the barrier for ORR since the reaction was enhanced for Co@NG-800,as confirmed by density functional theory(DFT)*** Co@NG cathode catalyst coupled with commercial Pt-Ru/C as anode catalyst exhibits excellent performance for direct methanol fuel cell(DMFC)with a peak power density of 34.7 mW cm^(-2)at a discharge current density of120 m A cm^(-2)and decent stability,indicating the promising utilization of spent battery materials in DMFC ***,lithium was recovered from supernatant as lithium carbonate by coprecipitation *** work avoids sophisticated elemental separation by utilizing SLIBs for other renewable energy applications,lowering the environmental concerns associated with recycling.

关键词： Density functional theory(DFT) Direct methanol fuel cell Leaching Nitrogen doping Oxygen reduction reaction Recycling Spent lithium-ion batteries

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Rapid monitoring of indoor airborne influenza and coronavirus with high air flowrate electrostatic sampling and PCR analysis

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 73-85页

作者： Sanggwon An Sangsoo Choi Hyeong Rae kim jungho Hwang School of Mechanical Engineering Yonsei UniversitySeoul 02876Republic of Korea Gas Metrology Group Korea Research Institute of Standards and Science(KRISS)Daejeon 34113Republic of Korea

The World Health Organization has raised concerns about the possibility of airborne transmission in enclosed and poorly ventilated ***,rapid monitoring of airborne viruses is necessary in multi-use facilities with dense ***,an electrostatic air sampler(250 L/min)was developed in this work to obtain indoor viral aerosol samples for analysis via the Polymerase Chain Reaction(PCR).Aerosol tests with H1N1 and HCoV-229E were performed to evaluate the sample collection *** analysis,along with another aerosol test,was conducted to evaluate the recovery of the virus particles collected by the *** laboratory tests,our electrostatic sampler obtained viral samples that were detectable by PCR under the simulated viral pandemic scenario(3000 RNA copies per cubic meter of air)within 40 *** resulting cycle threshold(C)values were 35.07 and 37.1 for H1N1 and HCoV-229E,*** the performance evaluation in the laboratory,field tests were conducted in a university classroom from October 28 to December 2,*** A and HCoV-229E were detected in two air samples,and the corresponding C,values were 35.3 and *** PCR results are similar to those obtained from laboratory tests,considering the simulatedviralpandemic scenario.

关键词： Airborne virus Electrostatic sampler Rapid monitoring Indoor environment Field test

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HF SAR image cross-correlation technique for high accuracy orbit positioning

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Science China(Physics,Mechanics & Astronomy) 2011年第5期54卷 978-985页

作者： KOBAYASHI Takao LEE SeungRyeol kim jungho ONO Takayuki Planetary Science Group Korea Institute of Geoscience and Mineral Resources Daejeon 305-350 Korea Shanghai Astronomical Observatory

A novel technique to determine the position of spacecraft orbits is proposed. The technique is based on the cross-correlation function of HF SAR images and is able to determine the relative position of orbits with an accuracy of - λ/4 or better, where 2 is the wavelength of the HF radar pulse at its center frequency. The performance of the proposed technique was confirmed by simulation which was carried out under the condition of design facts of the SELENE LRS mission. The highly accurate orbit positioning enables precise superposition of HF SAR images so that the inherent mirror image ambiguity problem of HF SAR imaging is resolved to obtain a quality SAR image of the HF band. In addition ambitious 2D-SAR processing would be possible when the above accuracy is available.

关键词： high accuracy orbit determination SAR LRS SELENE

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日本对华发展援助政策调整解读

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经济研究导刊 2013年第10期 187-188页

作者：金晶华 kim jungho 烟台大学经济管理学院山东烟台264005 韩国高丽大学校国际研究生院韩国首尔100101

在国际关系的理论研究和实际操作中,官方发展援助(Official Development Assistance)以其官方背景、政府行为、战略目的等一系列特点,一直是国外援助研究的重要对象。通过分析日本对华发展援助的特点以及冷战后其战略的几次调整,揭示日... 详细信息

在国际关系的理论研究和实际操作中,官方发展援助(Official Development Assistance)以其官方背景、政府行为、战略目的等一系列特点,一直是国外援助研究的重要对象。通过分析日本对华发展援助的特点以及冷战后其战略的几次调整,揭示日本对中国积极推行ODA政策的深层次原因和目的。当今世界格局下,中日关系对亚太地区的影响非常重大,因此,研究长期以来日本对外援助理念对于正确理解和处理中日关系有着重要的意义。

关键词：官方发展援助中日关系调整

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Light-Material Interactions Using Laser and Flash Sources for Energy Conversion and Storage Applications

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Nano-Micro Letters 2024年第12期16卷 468-514页

作者： Jung Hwan Park Srinivas Pattipaka Geon-Tae Hwang Minok Park Yu Mi Woo Young Bin kim Han Eol Lee Chang Kyu Jeong Tiandong Zhang Yuho Min Kwi-Il Park Keon Jae Lee jungho Ryu Department of Mechanical Engineering(Department of Aeronautics Mechanical and Electronic Convergence Engineering)Kumoh National Institute of Technology61Daehak-RoGumiGyeongbuk 39177Republic of Korea Department of Materials Science and Engineering Pukyong National University45Yongso-RoNam-GuBusan 48513Republic of Korea Energy Technologies Area Lawrence Berkeley National LaboratoryBerkeleyCA 94720USA Department of Materials Science and Engineering Korea Advanced Institute of Science and Technology(KAIST)291 Daehak-RoYuseong-GuDaejeon 34141Republic of Korea Division of Advanced Materials Engineering Jeonbuk National UniversityJeonju 54896JeonbukRepublic of Korea School of Electrical and Electronic Engineering Harbin University of Science and TechnologyHarbin 150080People’s Republic of China Key Laboratory of Engineering Dielectrics and Its Application Ministry of EducationHarbin University of Science and TechnologyHarbin 150080People’s Republic of China Department of Materials Science and Metallurgical Engineering Kyungpook National University80 Daehak-RoBuk-GuDaegu 41566Republic of Korea School of Materials Science and Engineering Yeungnam UniversityDaehak-RoGyeongsan-Si 38541Gyeongsangbuk-doRepublic of Korea

This review provides a comprehensive overview of the progress in light-material interactions(LMIs),focusing on lasers and flash lights for energy conversion and storage *** discuss intricate LMI parameters such as light sources,interaction time,and fluence to elucidate their importance in material *** addition,this study covers various light-induced photothermal and photochemical processes ranging from melting,crystallization,and ablation to doping and synthesis,which are essential for developing energy materials and ***,we present extensive energy conversion and storage applications demonstrated by LMI technologies,including energy harvesters,sensors,capacitors,and *** the several challenges associated with LMIs,such as complex mechanisms,and high-degrees of freedom,we believe that substantial contributions and potential for the commercialization of future energy systems can be achieved by advancing optical technologies through comprehensive academic research and multidisciplinary collaborations.

关键词： Light Light-material interaction Nanomaterials Energy conversion and storage devices

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PIR-based data integrity verification method in sensor network

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Journal of Central South University 2014年第10期21卷 3883-3888页

作者： Yong-Ki kim Kwangnam Choi Jaesoo kim jungho Seok Korea Institute of Science and Technology Information 245 DaehangnoYuseong Daejeon 305-806 Korea

Since a sensor node handles wireless communication in data transmission and reception and is installed in poor environment, it is easily exposed to certain attacks such as data transformation and sniffing. Therefore, it is necessary to verify data integrity to properly respond to an adversary's ill-intentioned data modification. In sensor network environment, the data integrity verification method verifies the final data only, requesting multiple communications. An energy-efficient private information retrieval(PIR)-based data integrity verification method is proposed. Because the proposed method verifies the integrity of data between parent and child nodes, it is more efficient than the existing method which verifies data integrity after receiving data from the entire network or in a cluster. Since the number of messages for verification is reduced, in addition, energy could be used more efficiently. Lastly, the excellence of the proposed method is verified through performance evaluation.

关键词： data integrity verification private information retrieval sensor network

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Capillary-force-induced collapse lithography for controlled plasmonic nanogap structures

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Microsystems & Nanoengineering 2020年第1期6卷 404-412页

作者： Inki kim jungho Mun Wooseup Hwang Younghwan Yang Junsuk Rho Department of Mechanical Engineering Pohang University of Science and Technology(POSTECH)Pohang 37673Republic of Korea Department of Chemical Engineering Pohang University of Science and Technology(POSTECH)Pohang 37673Republic of Korea Department of Chemistry Pohang University of Science and Technology(POSTECH)Pohang 37673Republic of Korea National Institute of Nanomaterials and Technology(NINT) Pohang 37673Republic of Korea

The capillary force effect is one of the most important fabrication parameters that must be considered at the micro/nanoscale because it is strong enough to deform micro/***,the deformation of micro/nanostructures due to such capillary forces(e.g.,stiction and collapse)has been regarded as an undesirable and uncontrollable obstacle to be avoided during ***,we present a capillary-force-induced collapse lithography(CCL)technique,which exploits the capillary force to precisely control the collapse of micro/*** uses electron-beam lithography,so nanopillars with various shapes can be fabricated by precisely controlling the capillary-force-dominant cohesion process and the nanopillar-geometry-dominant collapse process by adjusting the fabrication parameters such as the development time,electron dose,and shape of the *** aims to achieve sub-10-nm plasmonic nanogap structures that promote extremely strong focusing of *** is a simple and straightforward method to realize such nanogap structures that are needed for further research such as on plasmonic nanosensors.

关键词： capillary structures collapse

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Electromagnetic chirality:from fundamentals to nontraditional chiroptical phenomena

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Light(Science & Applications) 2020年第1期9卷 550-567页

作者： jungho Mun Minkyung kim Younghwan Yang Trevon Badloe Jincheng Ni Yang Chen Cheng-Wei Qiu Junsuk Rho Department of Chemical Engineering Pohang University of Science and TechnologyPohang 37673Korea Department of Mechanical Engineering Pohang University of Science and TechnologyPohang 37673Korea Department of Electrical and Computer Engineering National University of SingaporeSingapore 117583Singapore

Chirality arises universally across many different *** advancements in artificial nanomaterials have demonstrated chiroptical responses that far exceed those found in natural *** phenomena are complicated processes that involve transitions between states with opposite parities,and solid interpretations of these observations are yet to be clearly *** this review,we present a comprehensive overview of the theoretical aspects of chirality in light,nanostructures,and nanosystems and their chiroptical *** of observed chiroptical phenomena based on these fundamentals are intensively *** start with the strong intrinsic and extrinsic chirality in plasmonic nanoparticle systems,followed by enantioselective sensing and optical manipulation,and then conclude with orbital angular momentum-dependent *** review will be helpful for understanding the mechanisms behind chiroptical phenomena based on underlying chiral properties and useful for interpreting chiroptical systems for further studies.

关键词： materials interpreting momentum

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Artificial Nanoscale Erythrocytes from Clinically Relevant Compounds for Enhancing Cancer Immunotherapy

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Nano-Micro Letters 2020年第7期12卷 156-174页

作者： Wenquan Ou Kang Sik Nam Dae Hoon Park jungho Hwang Sae Kwang Ku Chul Soon Yong Jong Oh kim Jeong Hoon Byeon College of Pharmacy Yeungnam UniversityGyeongsan 38541Republic of Korea School of Mechanical Engineering Yonsei UniversitySeoul 03722Republic of Korea College of Korean Medicine Daegu Haany UniversityGyeongsan 38610Republic of Korea School of Mechanical Engineering Yeungnam UniversityGyeongsan 38541Republic of Korea

Because of enhanced e cacy and lower side e ects,cancer immunotherapies have recently been extensively investigated in clinical trials to overcome the limitations of conventional cancer *** engineering attempts have been made to build nanosystems even including stimulus nanomaterials for the e cient delivery of antigens,adjuvants,or anticancer drugs to improve immunogenic cancer cell death,this requires huge R&D e orts and investment for clinically relevant findings to be approved for translation of the *** this end,in this study,an air–liquid two-phase electrospray was developed for stable bubble pressing under a balance between mechanical and electrical parameters of the spray to continuously produce biomimetic nanosystems consisting of only clinically relevant compounds[paclitaxel-loaded fake blood cell Eudragit particle(Eu-FBCP/PTX)]to provide a conceptual leap for the timely development of translatable chemo-immunotherapeutic *** was pursued as the e cacy of systems for delivering anticancer agents that has been mainly influenced by nanosystem shape because of its relevance to transporting behavior to organs,blood circulation,and cell–membrane *** resulting Eu-FBCP/PTX nanosystems exhibiting phagocytic and micropinocytic uptake behaviors can confer better e cacy in chemo-immunotherapeutics in the absence and presence of anti-PD-L1 antibodies than similar sized PTX-loaded spherical Eu particles(Eu-s/PTX).

关键词： Cancer immunotherapies Air–liquid two-phase electrospray Paclitaxel-loaded fake blood cell Eudragit particle Translatable chemo-immunotherapeutic nanosystems Anti-PD-L1 antibodies

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Elucidating the photoluminescence-enhancement mechanism in a push-pull conjugated polymer induced by hot-electron injection from gold nanoparticles

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Photonics Research 2021年第2期9卷 131-141页

作者： DONGKI LEE SE GYO HAN jungho MUN KIHYUK YANG SUNG HYUK kim JUNSUK RHO KILWON CHO DONGYEOP X.OH MUN SEOK JEONG Department of Energy Science Sungkyunkwan UniversitySuwon 16419Republic of Korea Department of Chemical Engineering Pohang University of Science and TechnologyPohang 37673Republic of Korea Department of Mechanical Engineering Pohang University of Science and TechnologyPohang 37673Republic of Korea Research Center for Bio-based Chemistry Korea Research Institute of Chemical Technology(KRICT)Ulsan 44429Republic of Korea

Understanding the photophysical interactions between the components in organic-inorganic nanocomposites is a key factor for their efficient application in optoelectronic devices. In particular, the photophysical study of nanocomposites based on organic conjugated polymers is rare. We investigated the effect of surface plasmon resonance(SPR) of gold nanoparticles(Au NPs) on the photoluminescence(PL) property of a push-pull conjugated polymer(PBDB-T). We prepared the hybrid system by incorporating poly(3-hexylthiophene)-stabilized Au NPs(P3 HT-Au NPs) into PBDB-T. The enhanced and blueshifted PL was observed in the hybrid system compared to PL in a neat PBDB-T system, indicating that the P3 HT chains attached to the Au NPs suppressed charge-transfer from PBDB-T to the Au NPs and relayed the hot electrons to PBDB-T(the band-filling effect).This photophysical phenomenon limited the auto-dissociation of PBDB-T excitons. Thus, the radiative recombination of the excitons occurred more in our hybrid system than in the neat system.

关键词： conjugated system polymer

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