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One dimensional pea-shaped NiSe_(2) nanoparticles encapsulated in N-doped graphitic carbon fibers to boost redox reversibility in sodium-ion batteries

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Journal of Materials Science & Technology 2024年第1期168卷 215-226页

作者： Hyunjeong Gim Achmad Yanuar Maulana jiwon choi Jungwook Song Boram Yun Yuri Jeong Nahyun An Myeongkee Park Cybelle M.Futalan Jongsik Kim Department of Chemical Engineering(BK21 FOUR Graduate Program) Dong-A UniversityBusan 49315Korea(the Republic of) Department of Chemistry Dong-A UniversityBusan 49315Korea(the Republic of) Department of Chemistry Pukyong National UniversityBusan 48513Korea(the Republic of) Institute of Civil Engineering University of the PhilippinesDiliman 1127Philippines

In recent years,sodium-ion batteries(SIBs)have emerged as a promising technology for energy storage systems(ESSs)because of the abundance and affordability of ***,metal selenides have been studied as promising high-performance conversion-type anode materials in *** them,nickel se-lenide(NiSe_(2))has received considerable attention due to its high theoretical capacity of 495 mAh g^(-1)and ***,it still suffers from poor cycling stability because of the low electrochemical reactivity,large volume expansion,and structural instability during *** address these challenges,NiSe_(2)nanoparticles encapsulated in N-doped graphitic carbon fibers(NiSe_(2)@NGCF)were synthesized by using ZIF-8 as a ***_(2)@NGCF showed a high discharge capacity of 558.3 mAh g^(-1)with a fading rate of 0.14%per cycle after 200 cycles at 0.5 A g^(-1)in 0.01-3.0 *** a very high current density of 5 A g^(-1),the capacity still displayed excellent long-term cycle life with a discharge capacity of 406.1 mAh g^(-1)with a fading rate of 0.016%per cycle after 3000 *** mechanism of the excellent electrochem-ical performance of NiSe_(2)@NGCF was thoroughly investigated by ex-situ XRD,TEM,and SEM ***,NiSe_(2)@NGCF//Na_(3)V_(2)(PO_(4))_(3)full-cell also delivered an excellent reversible capacity of 378.7 mAh g^(−1)at 0.1 A g^(−1)after 50 cycles,demonstrating its potential for practical application in SIBs.

关键词： Sodium-ion batteries Anode materials Nickel selenide N-doped graphitic carbon fibers One-dimensional electrode

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Correlation between hydration properties and electrochemical performances on Ln cation size effect in layered perovskite for protonic ceramic fuel cells

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Journal of Energy Chemistry 2024年第1期88卷 1-9,I0001页

作者： Inhyeok Cho jiwon Yun Boseok Seong Junseok Kim Sun Hee choi Ho-Il Ji Sihyuk choi Department of Mechanical Engineering Kumoh National Institute of TechnologyGumi 39177GyeongbukRepublic of Korea Department of Aeronautics Mechanical and Electronic Convergence EngineeringKumoh National Institute of TechnologyGumi 39177GyeongbukRepublic of Korea Center for Energy Materials Research Korea Institute of Science and Technology(KIST)Seoul 02792Republic of Korea Center for Hydrogen and Fuel Cell Research Clean Technology Research DivisionKorea Institute of Science and Technology(KIST)Seoul 02792Republic of Korea Department of Energy and Environmental Engineering University of Science and TechnologySeoul 02792Republic of Korea Nanomaterials Science and Engineering Korea University of Science and Technology(UST)KIST CampusSeoul 02792Republic of Korea

PrBa_(0.5)Sr_(0.5)Co_(1.5)Fe_(0.5)O_(5+δ)(PrBSCF) has attracted much research interest as a potential triple ionic and electronic conductor(TIEC) electrode for protonic ceramic fuel cells(PCFCs). The chemical formula for Pr BSCF is AA'B_(2)O_(5+δ), with Pr(A-site) and Ba/Sr(A'-site) alternately stacked along the c-axis. Due to these structural features, the bulk oxygen ion diffusivity is significantly enhanced through the disorder-free channels in the PrO layer;thus, the A site cations(lanthanide ions) play a pivotal role in determining the overall electrochemical properties of layered perovskites. Consequently, previous research has predominantly focused on the electrical properties and oxygen bulk/surface kinetics of Ln cation effects,whereas the hydration properties for PCFC systems remain unidentified. Here, we thoroughly examined the proton uptake behavior and thermodynamic parameters for the hydration reaction to conclusively determine the changes in the electrochemical performances depending on LnBa_(0.5)Sr_(0.5)Co_(1.5)Fe_(0.5)O_(5+δ)(LnBSCF,Ln=Pr, Nd, and Gd) cathodes. At 500 ℃, the quantitative proton concentration of PrBSCF was 2.04 mol% and progressively decreased as the Ln cation size decreased. Similarly, the Gibbs free energy indicated that less energy was required for the formation of protonic defects in the order of Pr BSCF < Nd BSCF < Gd BSCF. To elucidate the close relationship between hydration properties and electrochemical performances in LnBSCF cathodes, PCFC single cell measurements and analysis of the distribution of relaxation time were further investigated.

关键词： Protonic ceramic fuel cell Cathode Triple ionic and electronic conductor Hydration property Proton uptake Gibbs free energy

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The Most Irrational Number that Shows up Everywhere: The Golden Ratio

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Journal of Applied Mathematics and Physics 2023年第4期11卷 1185-1193页

作者： jiwon choi Agegnehu Atena Wondimu Tekalign Department of Biology Savannah State University Savannah GA USA Department of Mathematics Savannah State University Savannah GA USA

Since the time of the ancient Greeks, humans have been aware of this mathematical idea. Golden ratio is an irrational number that is symbolized by the Greek numeral phi (φ). One can find this ratio everywhere. It is in nature, art, architecture, human body, etc. But this symbolism can result in a strong connection with mathematical nature. In this paper we will be discussing the connection between Fibonacci sequence (a series of numbers where every number is equal to the sum of two numbers before it) and Golden ratio. Secondly, how this mathematical idea shows up in a nature, such as sunflower and human DNA.

关键词： The Golden Ratio Fibonacci Sequence Nature

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Efficient Object Localization Scheme Based on Vanishing Line in Road Image for Autonomous Vehicles

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Journal of Computer and Communications 2021年第9期9卷 85-97页

作者： Bongkyo Moon jiwon choi Juehyun Lee Minyoung Lee Department of Computer Science and Engineering Dongguk University Seoul South Korea Graduate School of Information Security KAIST Daejeon South Korea Electronics and Telecommunications Research Institute (ERTI) Daejeon South Korea

This paper proposes an efficient object localization method based on a vanishing line. The proposed method can be much improved in time efficiency since it requires scanning only vanishing line area. It requires the time complexity of O(n) while the existing sliding window method requires the time complexity O(n2) for detecting all objects in the entire image. In addition, the range of detection area can be also remarkably reduced when compared with the sliding window method. As a result, the total range and times for searching in the proposed method can be significantly reduced by considering together the distance and position of the object. The experiment on the proposed method is performed with the virtual road data set known as SYNTHIA, and the competitive results are obtained.

关键词： Object Localization Image Preprocessing Sliding Window Vanishing Line Autonomous Vehicle

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Trifunctional robust electrocatalysts based on 3D Fe/N-doped carbon nanocubes encapsulating Co4N nanoparticles for efficient battery-powered water electrolyzers

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Carbon Energy 2024年第6期6卷 124-139页

作者： Hyung Wook choi Hongdae Lee Jun Lu Seok Bin Kwon Dong In Jeong Beum Jin Park jiwon Kim Bong Kyun Kang Gun Jang Dae Ho Yoon Ho Seok Park SKKU Advanced Institute of Nano Technology(SAINT) Sungkyunkwan UniversitySuwon-siGyeonggi-doRepublic of Korea School of Chemical Engineering Sungkyunkwan UniversitySuwon-siGyeonggi-doRepublic of Korea School of Advanced Materials Science and Engineering Sungkyunkwan UniversitySuwon-siGyeonggi-doRepublic of Korea Department of Electronic Materials Devicesand Equipment EngineeringSoonchunhyang UniversityAsan CityChungnamRepublic of Korea SKKU Institute of Energy Science and Technology(SIEST) Sungkyunkwan UniversitySuwon-siGyeonggi-doRepublic of Korea Department of Health Sciences and Technology Samsung Advanced Institute for Health Sciences and Technology(SAIHST)Sungkyunkwan UniversitySuwonRepublic of Korea

Herein,we have designed a highly active and robust trifunctional electrocatalyst derived from Prussian blue analogs,where Co_(4)N nanoparticles are encapsulated by Fe embedded in N-doped carbon nanocubes to synthesize hierarchically structured Co_(4)N@Fe/N-C for rechargeable zinc-air batteries and overall water-splitting *** confirmed by theoretical and experimental results,the high intrinsic oxygen reduction reaction,oxygen evolution reaction,and hydrogen evolution reaction activities of Co_(4)N@Fe/N-C were attributed to the formation of the heterointerface and the modulated local electronic ***,Co_(4)N@Fe/N-C induced improvement in these trifunctional electrocatalytic activities owing to the hierarchical hollow nanocube structure,uniform distribution of Co_(4)N,and conductive encapsulation by Fe/***,the rechargeable zinc-air battery with Co_(4)N@Fe/N-C delivers a high specific capacity of 789.9 mAh g^(-1) and stable voltage profiles over 500 ***,the overall water electrolyzer with Co_(4)N@Fe/N-C achieved better durability and rate performance than that with the Pt/C and IrO2 catalysts,delivering a high Faradaic efficiency of 96.4%.Along with the great potential of the integrated water electrolyzer powered by a zinc-air battery for practical applications,therefore,the mechanistic understanding and active site identification provide valuable insights into the rational design of advanced multifunctional electrocatalysts for energy storage and conversion.

关键词： battery-powered electrolyzers hierarchical structure Prussian blue analog trifunctional electrocatalyst zinc-air battery

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崛起进行时——对话四国新锐设计师

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现代装饰（家居） 2013年第7期 121-129页

作者：陈函溪曾熙凯 Flavio Scalzo jiwon choi Ola Giertz 陈志芳 DiciannoveDieciDesign

"江山代有才人出,各领风骚数百年",纵观古今,放眼东西,各行各业的新星莫不如同雨后春笋般,在每一段历史时期竞相涌现。一直勇立潮头的设计界自是概莫能外。似乎转眼之间,又一批后起之秀崭露头角,立足前沿。他们有着一样年轻的面孔,但都... 详细信息

"江山代有才人出,各领风骚数百年",纵观古今,放眼东西,各行各业的新星莫不如同雨后春笋般,在每一段历史时期竞相涌现。一直勇立潮头的设计界自是概莫能外。似乎转眼之间,又一批后起之秀崭露头角,立足前沿。他们有着一样年轻的面孔,但都发挥着不一样的自身优势,他们有着一样强烈的好奇心,但都追寻着不一样的前进方向。在很多人眼中,他们更像一个不可忽视的群体,带着各种醒目的标签,比如勇于打破常规,挑战传统;比如精于求新求异,思维活跃。

关键词：家具设计设计过程历史时期产品设计才人实体图国际家具展灵感来源产品形态生活形态

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Congenital stapes suprastructure fixation presenting with fluctuating auditory symptoms:A case report

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World Journal of Clinical Cases 2023年第1期11卷 249-254页

作者： Sun choi Seok Hyun Park Ji Su Kim jiwon Chang Department of Otolaryngology-Head and Neck Surgery Kangnam Sacred Heart HospitalHallym University College of MedicineSeoul 07441South Korea

BACKGROUND Stapes ankylosis is a rare cause of conductive hearing loss,and stapes suprastructure fixation is extremely rare with fewer than 30 reported *** usually visit the clinic with non-progressive conductive hearing loss that typically began in the early years of *** SUMMARY Herein,we report a case of a 37-year-old female with an isolated stapedial suprastructure *** patient presented with unusual fluctuating auditory symptoms of tinnitus,ear fullness and mixed hearing ***-operative temporal bone computed tomography findings and operative findings revealed an isolated stapedial suprastructure fixation with monopod stapes caused by elongated pyramidal *** hearing threshold recovered completely,and fluctuating auditory symptoms disappeared after the *** This is the first report of stapedial suprastructure fixation with fluctuating auditory *** results are expected with surgical treatment.

关键词： Isolated stapes ankylosis Stapes suprastructure fixation Elongated pyramidal eminence Stapes monopod Fluctuating auditory symptoms Exploratory tympanotomy Case report

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Effect of expanding nanocellulose sponge on nasal mucosal defects in an animal model

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Regenerative Biomaterials 2020年第1期7卷 47-52页

作者： jiwon Kim Kyungbae Woo Jeong Mi Kim Mi Eun choi Young-Mo Kim Su-Geun Yang Bong Sup Shim Jeong-Seok choi Department of Otorhinolaryngology Inha UniversityCollege of Medicine27 Inhang-roJung-guIncheon 22332Republic of Korea Department of Chemical Engineering Inha University100 InharoMichuholguIncheon 22212Republic of Korea Department of New Drug Development Inha UniversityCollege of MedicineB-308Chungsuk Bldg.366Seohae-DaeroJung-GuIncheon 22332Republic of Korea

Nanocellulose has emerged for a wide range of applications in biomedical engineering because of its water absorption capacity,appropriate *** investigated the hemostatic and regenerative abilities of an expanding polyvinyl alcohol(PVA)-nanocellulose sponge on nasal mucosal defects.A 3 mm-diameter nasal defect was made in experimental *** were divided into four groups with control,vaseline,PVA and PVA-nanocellulose packing *** the defect was created,bleeding times and amounts were *** materials were removed on experimental day(ED)*** ED 3,7 and 14,histological analysis and immunohistochemical study for neutrophils were *** cells were counted and epithelial thicknesses were *** amounts and times in the vaseline packing group were smaller than in the PVA ***-nanocellulose group showed less neutrophils than in the other groups on ED *** epithelium thickness in the PVA-nanocellulose group was significantly smaller than in the control group at ED 7,but at ED 14,there was no significant intergroup *** group had a significant lower inflammatory cell count than the control group on ED ***-nanocellulose sponge applied to nasal mucosal defects can significantly enhance mucosal regeneration during early wound healing.

关键词： polyvinyl alcohol nasal mucosa nanocellulose

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Manifolding active sites and in situ/operando electrochemical-Raman spectroscopic studies of single-metal nanoparticle-decorated CuO nanorods in furfural biomass valorization to H_(2) and 2-furoic acid

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能源化学:英文版 2023年第9期84卷 50-61页

作者： jiwon Kim Talshyn Begildayeva Jayaraman Theerthagiri Cheol Joo Moon Ahreum Min Seung Jun Lee Gyeong-Ah Kim Myong Yong choi Department of Chemistry(BK21 FOUR) Research Institute of Natural SciencesGyeongsang National UniversityJinju 52828Republic of Korea Core-Facility Center for Photochemistry&Nanomaterials Gyeongsang National UniversityJinju 52828Republic of Korea Department of IT-Energy Convergence(BK21 FOUR) Korea National University of TransportationChungju 27469Republic of Korea

Here,CuO nanorods fabricated via pulsed laser ablation in liquids were decorated with Ir,Pd,and Ru NPs(loading~7 wt%) through pulsed laser irradiation in the liquids *** resulting NPs-decorated CuO nanorods were characterized spectroscopically and employed as multifunctional electrocatalysts in OER,HER,and the furfural oxidation reactions(FOR).Ir-CuO nanorods afford the lowest overpotential of~345 mV(HER) and 414 mV(OER) at 10 mA cm^(-2),provide the highest 2-furoic acid yield(~10.85 mM) with 64.9% selectivity,and the best Faradaic efficiency~72.7% in 2 h of FOR at 1.58 V(***).In situ electrochemical-Raman analysis of the Ir-CuO detects the formation of the crucial intermediates,such as Cu(Ⅲ)-oxide,Cu(OH)_(2),and Ir_x(OH)_y,on the electrode-electrolyte surface,which act as a promoter for HER and *** Ir-CuO ‖ Ir-CuO in a coupled HER and FOR-electrolyzer operates at~200 mV lower voltage,compared with the conventional electrolyzer and embodies the dual advantage of energy-saving H_(2) and 2-furoic acid production.

关键词： Single-metal nanoparticle-decorated CuO nanorods Pulsed laser ablation and irradiation in liquids Furfural oxidation reaction Hydrogen evolution reaction Energy-saving H_(2)production 2-Furoic acid

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