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Pressure-Induced Pre-lithiation Enables High-Performing Si Anodes in All-Solid-State Batteries

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ENERGY & ENVIRONMENTAL MATERIALS 2024年第6期7卷 1-3页

作者： hu, Weifei li, Yuanyuan liu, Jinping Wuhan Univ Technol Sch Chem Chem Engn & Life Sci Wuhan 430070 Peoples R China Wuhan Univ Technol State Key Lab Adv Technol Mat Synth & Proc Wuhan 430070 Peoples R China huazhong Univ Sci & Technol Sch Integrated Circuits Wuhan 430074 Peoples R China

A commentary on pressure-induced pre-lithiation towards Si anodes in all-solid-state li-ion batteries (ASSliBs) using sulfide electrolytes (SEs) is presented. First, feasible pre-lithiation technologies for Si anodes in SE-based ASSliBs especially the significant pressure-induced pre-lithiation strategies are briefly reviewed. Then, a recent achievement by Meng et al. in this field is elaborated in detail. Finally, the significance of Meng's work is discussed.

关键词： all-solid-state li-ion batteries pre-lithiation pressure Si anode sulfide electrolyte

Land use effects on the dynamics of soil C,N and microbes in the water-wind erosion crisscross region of the northern Loess Plateau,China

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Pedosphere 2024年第1期34卷 181-190页

作者： Yi WANG Chunyue li Shunjin hu State Key Laboratory of Loess and Quaternary Geology Institute of Earth EnvironmentChinese Academy of SciencesXi'an 710061China State Key Laboratory of Soil Erosion and Dryland Farming on the Loess Plateau Institute of Soil and Water ConservationNorthwest A&F UniversityYangling 712100China School of Geography and Tourism Shaanxi Normal UniversityXi'an 710119China Department of Entomology&Plant Pathology North Carolina State UniversityRaleigh 27695USA

The water-wind erosion crisscross region of the northern Loess Plateau in China is under constant pressure from severe erosion due to its windy and dry climate and intensive human activities. Identifying sustainable land use patterns is key to maintaining ecosystem sustainability in the area. Our aim was to appraise the impacts of different land use regimes on the dynamics of soil total organic C(TOC), total N(TN), and microbes in a typical watershed in the northern Loess Plateau to identify suitable land use types that can maintain soil fertility and sustainability. A field experiment was performed in liudaogou watershed in Shenmu City, Shaanxi Province, China, where the dynamics of soil TOC and TN, microbial biomass C and N, microbial respiration, and net N mineralization in six typical land use types, dam land, rainfed slope land, deciduous broadleaf forest, evergreen coniferous forest, shrubland, and grassland,were measured in three different growing seasons. Land use type and season significantly affected TOC, TN, and the dynamics of microbial biomass and activity. As the most anthropogenically disturbed land use pattern, dam land was an optimal land use pattern for TOC sequestration due to its higher TOC and TN, but lower microbial activity. Soil TOC, TN, and microbial properties demonstrated a decreasing trend after natural grassland was converted to shrubland,forest, and rainfed slope land. Shrubland with exotic N-fixing Korshinsk peashrub(Caragana korshinskii Kom.) can maintain TOC, TN, and microbial properties similar to those in grassland. Soil TOC, NH_(4+)^(-)N, TN, moisture, and extractable C were the principal indexes for soil microbial biomass and activity and explained 88.90% of the total variance. Thus, grassland was the optimal land use pattern in the water-wind erosion crisscross region of the northern Loess Plateau to maintain ecosystem stability and sustainability.

关键词： grassland microbial activity microbial biomass total organic C total N watershed

Fracture mechanism of inclusions in thick plate center under tensile loading

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Journal of Iron and Steel Research International 2024年第5期31卷 1196-1209页

作者： Lei hu li-qin Zhang Feng hu Guo-hong Zhang Kuan Zheng Collaborative Innovation Center for Advanced Steels Wuhan University of Science and TechnologyWuhan430081HubeiChina Department of Applied Physics Wuhan University of Science and TechnologyWuhan430081HubeiChina Analysis and Testing Center Wuhan University of Science and TechnologyWuhan430081HubeiChina

Segregation of solute atoms in the center of thick plates of the tempered steel can cause an inhomogeneous structural transformation and generate micron-sized inclusions,which leads to lamellar tearing of thick plate and decreases the plasticity and *** formation and fragmentation mechanisms of micron-sized inclusions,like MnS and(Nb,Ti)C,in the center of thick plates were investigated by using thermodynamic calculations,finite element simulations,and electron backscatter diffraction characterization *** results show that micron-sized inclusions nucleate and grow in the liquid phase,and under tensile loading,they exhibit three fragmentation *** local stress during the fragmentation of inclusions is lower than the critical fracture stress of adjacent grains,and phase boundaries can effectively impede crack propagation into the *** existence of a low proportion of high-angle grain boundaries(58.1%)and high Kernel average misorientation value(0.534°)in the segregation band promotes inclusions fragmentation and crack *** difference in crack initiation and propagation direction caused by the morphology of inclusions and physical properties,as well as different matrix arrest abilities,is the main reasons for the diversity of inclusion fragmentation.

关键词： Thick plate Inclusion Finite element simulation Critical fracture stress Fracture mechanism

Semi-Varying Coefficient Panel Data Model with Technical Indicators Predicts Stock Returns in Financial Market

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Journal of Systems Science & Complexity 2024年第4期37卷 1638-1652页

作者： hu Xuemei PAN Ying li Xiang School of Mathematics and Statistics Chongqing Technology and Business UniversityChongqing 400067China Chongqing Key Laboratory of Social Economy and Applied Statistics Chongqing 400067China Research Center for Economy of Upper Reaches of the Yangtse River Chongqing Technology and Business UniversityChongqing 400067China

Accurately predicting stock returns is a conundrum in financial *** this conundrum can bring huge economic benefits for investors and also attract the attention of all circles of *** this paper the authors combine semi-varying coefficient model with technical analysis and statistical learning,and propose semi-varying coefficient panel data model with individual effects to explore the dynamic relations between the stock returns from five companies:CVX,DFS,EMN,LYB,and MET and five technical indicators:CCI,EMV,MOM,ln ATR,ln RSI as well as closing price(ln CP),combine semi-parametric fixed effects estimator,semi-parametric random effects estimator with the testing procedure to distinguish fixed effects(FE) from random effects(RE),and finally apply the estimated dynamic relations and the testing set to predict stock returns in December 2020 for the five *** proposed method can accommodate the varying relationship and the interactive relationship between the different technical indicators,and further enhance the prediction accuracy to stock returns.

关键词： Fixed effects random effects semi-varying coefficient panel data model stock returns technical indicators

One-step cell biomanufacturing platform:porous gelatin microcarrier beads promote human embryonic stem cell-derived midbrain dopaminergic progenitor cell differentiation in vitro and survival after transplantation in vivo

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Neural Regeneration Research 2024年第2期19卷 458-464页

作者： lin Feng Da li Yao Tian Chengshun Zhao Yun Sun Xiaolong Kou Jun Wu liu Wang Qi Gu Wei li jie Hao Baoyang hu Yukai Wang State Key Laboratory of Stem Cell and Reproductive Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Institute for Stem Cell and Regenerative Medicine Chinese Academy of SciencesBeijingChina National Stem Cell Resource Center Chinese Academy of SciencesBeijingChina Savaid Medical School University of Chinese Academy of SciencesBeijingChina Beijing Institute for Stem Cell and Regenerative Medicine BeijingChina State Key Laboratory of Membrane Biology Institute of ZoologyChinese Academy of SciencesBeijingChina

Numerous studies have shown that cell replacement therapy can replenish lost cells and rebuild neural circuitry in animal models of Parkinson’s *** of midbrain dopaminergic progenitor cells is a promising treatment for Parkinson’s ***,transplanted cells can be injured by mechanical damage during handling and by changes in the transplantation ***,we developed a one-step biomanufacturing platform that uses small-aperture gelatin microcarriers to produce beads carrying midbrain dopaminergic progenitor *** beads allow midbrain dopaminergic progenitor cell differentiation and cryopreservation without digestion,effectively maintaining axonal integrity in ***,midbrain dopaminergic progenitor cell bead grafts showed increased survival and only mild immunoreactivity in vivo compared with suspended midbrain dopaminergic progenitor cell ***,our findings show that these midbrain dopaminergic progenitor cell beads enhance the effectiveness of neuronal cell transplantation.

关键词： axonal integrity cell cryopreservation cellular environment cellular niche cell replacement therapy dopaminergic progenitors human pluripotent stem cell mechanical damage neuronal cell delivery Parkinson’s disease small-aperture gelatin microcarriers

Mn-modified nitrogen-doped Pt-based electrocatalyst for efficient oxygen reduction in aluminum-air batteries

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Nano Research 2024年第8期17卷 7126-7135页

作者： li Gao Yang Song Xuebing Xu Chang li Chaoquan hu State Key Laboratory of Mesoscience and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Zhongke Nanjing Institute of Green Manufacturing Industry Nanjing 211135China

In this study,a Mn-modified Pt-based catalyst loaded on nitrogen-doped Ketjen black(Mn-Pt/NKB)is prepared using a simple ethylene glycol reduction *** size of Pt nanoparticles(NPs)is effectively controlled by doping with Mn and *** the smallest average particle size of 1.7 nm,Mn-Pt/NKB demonstrates half-wave potentials of 0.890 and 0.688 V in the alkaline and neutral electrolytes,respectively,which are superior to those of commercial platinum on activated carbon(Pt/C).When applied as an air cathode in aluminum-air battery,it exhibits ultra-high power densities of 190(alkaline)and 26.2 mW·cm^(−2)(neutral).Moreover,the voltage remains stable after 5 h of *** practical application performance of the Mn-Pt/NKB catalyst in an aluminum-air battery is better than that of commercial Pt/***,the oxygen reduction reaction(ORR)mechanism on surfaces with different particle sizes is analyzed using density functional *** cracking is the major pathway on the surface of the small particles with lower energy consumption of 0.5 eV,while water molecule cleavage is the major pathway on the surface of the large particles with higher energy consumption of 0.97 *** lower energy consumption of the oxygen cracking pathway further confirms the ORR mechanism for higher activity on small-sized *** study provides a direction for the rational design of Pt-based catalysts for ORR and sheds light on the commercial development of aluminum-air batteries.

关键词： oxygen reduction reaction precious metal catalysts aluminum-air battery density functional theory(DFT)calculations reaction pathway

Fault diagnosis of a marine power-generation diesel engine based on the Gramian angular field and a convolutional neural network

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第6期25卷 470-482页

作者： Congyue li Yihuai hu Jiawei JIANG Dexin CUI Merchant Marine College Shanghai Maritime UniversityShanghai 201306China School of Mechanical and Energy Engineering Shanghai Technical Institute of Electronics&InformationShanghai 201411China

Marine power-generation diesel engines operate in harsh *** vibration signals are highly complex and the feature information exhibits a non-linear *** is difficult to extract effective feature information from the network model,resulting in low fault-diagnosis *** address this problem,we propose a fault-diagnosis method that combines the Gramian angular field(GAF)with a convolutional neural network(CNN).Firstly,the vibration signals are transformed into 2D images by taking advantage of the GAF,which preserves the temporal *** raw signals can be mapped to 2D image features such as texture and *** integrate the feature information,the images of the Gramian angular summation field(GASF)and Gramian angular difference field(GADF)are fused by the weighted average fusion ***,the channel attention mechanism and temporal attention mechanism are introduced in the CNN model to optimize the CNN learning *** the concept of residuals in the attention mechanism improves the feasibility of ***,the weighted average fused images are fed into the CNN for feature extraction and fault *** validity of the proposed method is verified by experiments with abnormal valve *** average diagnostic accuracy is 98.40%.When−20 dB≤signal-to-noise ratio(SNR)≤20 dB,the diagnostic accuracy of the proposed method is higher than 94.00%.The proposed method has superior diagnostic ***,it has a certain anti-noise capability and variable-load adaptive capability.

关键词： Multi-attention mechanisms(MAM) Convolutional neural network(CNN) Gramian angular field(GAF) Image fusion Marine power-generation diesel engine Fault diagnosis

Crustal structure in the Anyuan Coal Mine and its adjacent areas of Jiangxi Province by P-wave receiver functions

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Earthquake Research Advances 2024年第1期4卷 47-58页

作者： Xingmian Zhang Meng Gong Jian Lü Hongxing li jie hu Junwen He Jianhua Peng Bingyue liu State Key Laboratory of Nuclear Resources and Environment East China University of TechnologyNanchang330013China Nanchang Key Laboratory of Intelligent Sensing Technology and Instruments for Geological Hazards East China University of TechnologyNanchang330013China Jiangxi Earthquake Agency Nanchang330026China East China University of Technology School of Geophysics and Measurement-Control TechnologyNanchang330013China hunan Earthquake Agency Changsha410004China

We collected high-quality teleseismic events recorded by 12 broadband seismographs deployed in the Anyuan Coal Mine and its adjacent areas in Pingxiang City,Jiangxi Province for nearly two *** H-κ-c stacking method was employed to obtain the crustal thickness and Poisson's ratio distribution,then the characteristics of crustal structure below the stations were obtained by using the time-domain linear inversion *** crustal thickness in the Anyuan Coal Mine and its adjacent areas ranges from approximately 32~35 km,with an average thickness of 33 km,which is consistent with the crustal thickness results in South China from previous studies using the receiver function *** average Poisson's ratio of the crustal bulk composition in the study area varies between 0.22 and 0.25,which is lower than the global value with a 0.27 average,indicating a predominantly intermediate-acidic or felsic crustal *** is a weak negative correlation between Poisson's ratio and crustal thickness estimates in the Anyuan Coal Mine and its adjacent areas,suggesting that the absence of mafic-ultramafic materials in the lower crust is associated with the process of crustal *** velocity inversion results indicate that the crustal structure including three velocity discontinuity interfaces,with the first at a depth of approximately 1.5 km,the second at about 10~15 km,and the third being the *** study also indicates that the results obtained by the H-κ-c stacking method are significantly better than those obtained by the H-κmethod,effectively reducing the standard deviation and dispersion of crustal thickness and vP/vSratio.

关键词： Anyuan Coal Mine Receiver function H-κ-c stacking Crustal thickness Poisson's ratio

Natural vibration and critical velocity of translating Timoshenko beam with non-homogeneous boundaries

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Applied Mathematics and Mechanics(English Edition) 2024年第9期45卷 1523-1538页

作者： Yanan li jieyu DING hu DING liqun CHEN Shanghai Institute of Applied Mathematics and Mechanics Shanghai Key Laboratory of Mechanics in Energy EngineeringShanghai Frontier Science Center of MechanoinformaticsSchool of Mechanics and Engineering ScienceShanghai UniversityShanghai 200072China School of Mathematics and Statistics Qingdao UniversityQingdao 266071Shandong ProvinceChina

In most practical engineering applications,the translating belt wraps around two fixed *** boundary conditions of the dynamic model are typically specified as simply supported or fixed *** this paper,non-homogeneous boundaries are introduced by the support *** the translating belt as the mechanical prototype,the vibration characteristics of translating Timoshenko beam models with nonhomogeneous boundaries are investigated for the first *** governing equations of Timoshenko beam are deduced by employing the generalized Hamilton's *** effects of parameters such as the radius of wheel and the length of belt on vibration characteristics including the equilibrium deformations,critical velocities,natural frequencies,and modes,are numerically calculated and *** numerical results indicate that the beam experiences deformation characterized by varying curvatures near the *** radii of the wheels play a pivotal role in determining the change in trend of the relative difference between two beam *** the results unearths that the relative difference in equilibrium deformations between the two beam models is more pronounced with smaller-sized *** the two wheels are of equal size,the critical velocities of both beam models reach their respective *** addition,the relative difference in natural frequencies between the two beam models exhibits nonlinear variation and can easily exceed 50%.Furthermore,as the axial velocities increase,the impact of non-homogeneous boundaries on modal shape of translating beam becomes more *** dealing with non-homogeneous boundaries is challenging,beam models with non-homogeneous boundaries are more sensitive to parameters,and the differences between the two types of beams undergo some interesting variations under the influence of non-homogeneous boundaries.

关键词： translating beam Timoshenko beam non-homogeneous boundary natural frequency critical velocity