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Liquid metal compartmented by polyphenol-mediated nanointerfaces enables high-performance thermal management on electronic devices

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InfoMat 2024年第1期6卷 83-95页

作者： Chaoj.n zhang Yang Tang Tianyu Guo Yizhou Sang Ding Li Xiaoling Wang Orlando j.Roj.s j.nling Guo BMI Center for Biomass Materials and Nanointerfaces College of Biomass Science and EngineeringSichuan UniversityChengduSichuanthe People's Republic of China Bioproducts Institute Departments of Chemical and Biological EngineeringThe University of British ColumbiaVancouverBritish ColumbiaCanada Institute of Development Studies Southwestern University of Finance and EconomicsChengduSichuanthe People's Republic of China National Engineering Laboratory for Clean Technology of Leather Manufacture Sichuan UniversityChengduSichuanthe People's Republic of China State Key Laboratory of Polymer Materials Engineering Sichuan UniversityChengduSichuanthe People's Republic of China

The exponentially increasing heat generation in electronic devices,induced by high power density and miniaturization,has become a dominant issue that affects carbon footprint,cost,performance,reliability,and *** metals(LMs)with high thermal conductivity are promising candidates for effective thermal management yet are facing pump-out and surface-spreading *** in the form of metallic particles can address these problems,but apparent alloying processes elevate the LM melting point,leading to severely deteriorated ***,we propose a facile and sustainable approach to address these challenges by using a biogenic supramolecular network as an effective diffusion barrier at copper particle-LM(EGaIn/Cu@TA)interfaces to achieve superior thermal *** supramolecular network promotes LM stability by reducing unfavorable alloying and fluidity *** EGaIn/Cu@TA exhibits a record-high metallic-mediated thermal conductivity(66.1 W m^(-1) K^(-1))and fluidic ***,mechanistic studies suggest the enhanced heat flow path after the incorporation of copper particles,generating heat dissipation suitable for computer central processing units,exceeding that of commercial *** results highlight the prospects of renewable macromolecules isolated from biomass for the rational design of nanointerfaces based on metallic particles and LM,paving a new and sustainable avenue for high-performance thermal management.

关键词： Electronic devices High thermal conductivity Liquid metals Natural polyphenols Thermal management

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Wide temperature range,air stable,transparent,and self-powered photodetectors enabled by a hybrid film of graphene and singlewalled carbon nanotubes

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Nano Research 2024年第7期17卷 6582-6593页

作者： Ying Yue Di zhang Pengyu Wang Xin Wu Yuej.an zhang Yanchun Wang Xiao zhang Xiaoj.n Wei Huaping Liu Weiya Zhou Beij.ng National Laboratory for Condensed Matter Physics and Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences and College of Materials Science and Optoelectronic Technology University of Chinese Academy of SciencesBeijing 100049China Songshan Lake Materials Laboratory Dongguan 523808China Beij.ng Key Laboratory for Advanced Functional Materials and Structure Research Beijing 100190China

Transparent photovoltaic devices(TPVDs)have attracted increasing attention in emerging electronic *** the application scenarios extend,there raise higher requirements regarding the stability and operating temperature range of *** this work,a unique preparation strategy is proposed for air stable TPVD with a wide operating temperature range,i.e.,a nanoscale architecture termed as H-TPVD is constructed that integrates a free-standing and highly transparent conductive hybrid film of graphene and single-walled carbon nanotubes(G-SWNT TCF for short)with a metal oxide NiO/TiO_(2)*** preparation approach is suitable for scaling *** to the excellent transparent conductivity of the freestanding G-SWNT hybrid film and the ultrathin NiO/TiO_(2)heteroj.nction(100 nm),H-TPVD selectively absorbs the ultraviolet(UV)band of sunlight and has a transparency of up to 71%in the visible *** integrated nanoscale architecture manifests the significant holecollecting capability of the G-SWNT hybrid film and the efficient carrier generation and separation within the ultrathin NiO/TiO_(2)heteroj.nction,resulting in excellent performance of the H-TPVD with a specific detectivity of 2.7×10^(10) ***,the freestanding G-SWNT TCF is a super stable and non-porous two-dimensional film that can insulate gas molecules,thereby protecting the surface properties of NiO/TiO_(2)heteroj.nctions and enhancing the stability of *** subj.cted to 20,000 cycles and storage in air for three months,the performance parameters such as photo-response signal,output power,and specific detectivity show no noticeable *** particular,the as-fabricated self-powered H-TPVD can operate over a wide temperature range from −180 to 300℃,and can carry out solar-blind UV optical communication in this *** addition,the 4×4 array H-TPVD demonstrates clear optical *** results make it possible for H-TPVD to expand its potential application scenarios.

关键词： transparent photovoltaic devices hybrid films of graphene and single-walled carbon nanotubes metal oxides stability wide temperature range

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Excellent energy storage properties in non-stoichiometric Bi_(0.5)Na_(0.5)TiO_(3)-based relaxor ferroelectric ceramics

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Chinese Chemical Letters 2024年第7期35卷 470-472页

作者： Shunshun j.ang j. zhang j.ng Wang Shan-Tao zhang School of Materials Science and Engineering Nanjing University of Science&TechnologyNanjing 210094China State Key Laboratory of Mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China National Laboratory of Solid State Microstructures Department of Materials Science and EngineeringCollege of Engineering and Applied Science&Jiangsu Key Laboratory of Artificial Functional Materials&Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China

The rapid development of high-power and pulsed-power techniques inspires extensive investigates on high-performance ceramic-based ***,the low recoverable energy density(Wrec)hampers their wider ***,the non-stoichiometric Bi_(0.5)Na_(0.5)TiO_(3)-based ceramics were designed and *** proper introduction of oxygen vacancies facilitated activating defect dipole,giving rise to reduced remanent ***,the optimal composition exhibited an exceptional high Wrec of 8.3 j.cm^(3),a high efficiency of 85%,and excellent anti-fatigue and thermal *** work provides an efficient approach to explore ceramic capacitors with high capacitive energy storage performances.

关键词： Non-stoichiometric Bi_(0.5)Na_(0.5)TiO_(3) Ceramic capacitor Energy density Thermal stability

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Influence of the Acoustic Liner in Large Eddy Simulation of Longitudinal Thermoacoustic Instability in a Model Annular Combustor

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j.urnal of Thermal Science 2024年第2期33卷 710-724页

作者： MENG Sheng zhang Man GAO Yi AECC Commercial Aircraft Engine Co. Ltd.Shanghai200241China School of Aeronautics and Astronautics Shanghai Jiao Tong UniversityShanghai200240China

Although extensive efforts have been made to dampen the thermoacoustic instability,successfully controlling the pressure oscillations in modern gas turbines or aeroengines remains *** influence of the acoustic liner on the longitudinal thermoacoustic mode in a model annular combustor is investigated by Large Eddy Simulation(LES) in this *** result of the self-excited longitudinal thermoacoustic instability without the liner agrees well with the frequency and acoustic analysis of the pressure mode based on experimental *** different bias flow velocities of the liner located downstream of the combustor are then *** results reveal that the existence of the liner influences not only the acoustic field but also the flow *** the bias velocity is large,it leads to intense turbulence-induced fluctuations,and the pressure oscillation is modulated *** shows that the weak coupling between flow and pressure oscillations plays a significant role in the onset of the intermittency of a thermoacoustic *** on the dynamic analysis of the thermoacoustic system with the acoustic liner,this intermittency is caused by the influence of the flow field on the flame-acoustic ***,a low-order modeling method based on Van der Pol(VdP) oscillator with additive stochastic forcing is conducted to reproduce the evolving dynamics of the thermoacoustic *** the numerical cases demonstrated in this work are relatively simpler than those in a practical combustion system,the results are helpful for us to understand the effect of the acoustic liner and show the attractive potential to apply this device to suppress thermoacoustic instability.

关键词： thermoacoustic instability acoustic liner Large Eddy Simulation low-order modeling

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Processing,microstructure,and properties of porous ceramic composites with directional channels

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j.urnal of Materials Science & Technology 2024年第1期168卷 1-15页

作者： Bo zhang Yang Yang Xueling Fan Key Laboratory of Service Performance and Protection Technology in Extreme Environments Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory for Strength and Vibration of Mechanical Structures School of Aerospace EngineeringXi’an Jiaotong UniversityXi’an 710049China

Porous ceramic composites with directional microchannels from micrometer to dozens of micrometer levels have attracted more and more attention in various fields including aerospace,biomedicines,and thermal insulation due to their excellent fluid permeability,mechanical properties,*** this article,we summarize the recent directional porous ceramics developments including their main processing routes and respective ***,the properties get from different processing routes have been com-pared and analyzed in terms of microstructures,mechanical properties,and *** has been given to the deeper understanding which can allow one to control the microstructural features of these porous ceramic composites to obtain the desired *** work can provide a useful reference for the development and application of porous ceramic composites with directional microchan-nels.

关键词： Porous ceramic composites Directional microchannels Processing routes Permeability

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Design method of multivariable PI controller for turboprop engine based on equivalent transfer function

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Chinese j.urnal of Aeronautics 2024年第9期37卷 237-260页

作者： Shancheng LI Yong WANG Haibo zhang j.angsu Province Key Laboratory of Aerospace Power System College of Energy and Power EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China

Traditional centralized Proportional Integral(PI)controller design methods based on Equivalent Transfer Functions(ETFs)have poor decoupling effect in turboprop *** this paper,a centralized PI design method based on dynamic imaginary matrix and equivalent transfer function is ***,a method for solving equivalent transfer functions based on the dynamic imaginary matrix is proposed,which adopts dynamic imaginary matrix to describe the dynamic characteristics of the system,and obtains the equivalent transfer function based on the dynamic imaginary matrix ***,for the equivalent transfer function,a central-ized PI control gain is designed using the Taylor expansion ***,this paper further proves that the centralized PI design method proposed in this paper has integral ***-ering the impact of altitude and Mach number on turboprop engines,a linear feedforward control method based on the transfer function matrix is further proposed based on the centralized PI con-troller,and the stability of the entire comprehensive control method is ***,to ensure the safe and effective operation of the turboprop engine,a temperature and torque limiting protection controller is designed for the turboprop *** results show that the centralized PI con-troller design method and linear feedforward control method proposed can effectively improve the control quality of turboprop engine control systems.

关键词： Multivariable control sys-tems Equivalent transfer function Disturbance compensation control Control parameter design Turboprop engine control

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Effect of applied bias potential on the photocatalytic oxidation of nitrite over Cr-doped TiO2 under visible light

Effect of applied bias potential on the photocatalytic oxida...

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第三届全国环境化学学术大会

作者： j. Y. Shi, W. H. Leng, j. Q. zhang Department of Chemistry, Yuquan Campus, Zhej.ang University, Hangzhou, 310027, PR China Department of Chemistry, Quanzhou Normal College, Quanzhou, 362000, PR China

＜正＞1. Introduction Nitrite is a common inorganic pollutant in the environment. Up to now, the removal of nitrite by photocatalytic oxidation （PCO） was carried out mostly under UV-light [1-10], rarely under solar ... 详细信息

关键词： Nitrite ion Applied bias potential Photocatalytic oxidation Cr-doped TiO2 visible light

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Experimental and theoretical analysis of loading characteristics of electret filter media for charged particles

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Particuology 2024年第10期93卷 87-98页

作者： Yiqi Cai Rongrong Cai Lizhi zhang Key Laboratory of Enhanced Heat Transfer and Energy Conservation of Education Ministry School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou510640China State Key Laboratory of Subtropical Building Science South China University of TechnologyGuangzhou510640China

The degradation of filtration performance in electret filter media during usage poses a significant challenge. Pre-charging of aerosols has been identified as an effective method to mitigate this issue. However, the effects of particle charging characteristics on the loading characteristics of electret filters still need a comprehensive understanding. In this study, a needle-cylinder corona charger was employed to pre-charge aerosols, and the particle charge state was determined by multiphysics simulation. The effects of particle charge polarity and charge quantity on the loading performance of the electret filter were quantitatively investigated. The results showed that the particle charge polarity had a negligible impact on the loading performance under the condition of the equivalent particle charge quantity. In addition, the charged particles effectively improved the efficiency degradation during the loading process of electret media, with higher charge quantities resulting in more pronounced improvements. The electrostatic attenuation factor showed a negative exponential correlation with the particle charge quantity. This was attributed to the uneven particle deposition on fiber surface due to the attraction of charged particles by the opposite charges on the electret fibers, which alleviated the effect of electrostatic shielding.

关键词： Electret filter Charged particles Loadingcharacteristic Corona charging Electrostatic screening

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Deflagration and detonation induced by shock wave focusing at different Mach numbers

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Chinese j.urnal of Aeronautics 2024年第2期37卷 249-258页

作者： Zezhong YANG j.n CHENG Bo zhang School of Aeronautics and Astronautics Shanghai Jiao Tong UniversityShanghai 200240China

Shock wave focusing is an effective way to create a hot spot or a high-pressure and hightemperature region at a certain place,showing its unique usage in detonation initiation,which is beneficial for the development of detonation-based *** flame propagation behavior after the autoignition induced by shock wave focusing is crucial to the formation and self-sustaining of the detonation *** this study,wedge reflectors with two different angles(60°and 90°)and a planar reflector are employed,and the Mach number of incident shock waves ranging from 2.0 to 2.8 is utilized to trigger different flame propagation *** pressure transducers and the high-speed schlieren imaging system are both employed to investigate the shock-shock collision and ignition *** results reveal a total of four flame propagation modes:deflagration,DDT(Deflagration-to-Detonation Transition),unsteady detonation,and direct *** detonation wave formed in the DDT and unsteady detonation mode is only approximately 75%-85%of the Chapman-j.uguet(C-j.speed;meanwhile,the directly induced detonation wave speed is close to the C-j.*** waves,which are strong evidence for the existence of detonation waves,are discovered in *** usage of wedge reflectors significantly reduces the initial pressure difference ratio needed for direct detonation *** also provide a practical method for differentiating between detonation and deflagration modes,which involves contrasting the speed of the reflected shock wave with the speed of the theoretically nonreactive reflected shock *** findings should serve as a reference for the detonation initiation technique in advanced detonation propulsion engines.

关键词： Deflagration Detonation Hydrogen Ignition Shock wave focusing

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Preparation of mesoporous ZnO and its application in dye-sensitized solar cells

Preparation of mesoporous ZnO and its application in dye-sen...

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第18届国际真空大会

作者： G. Z. Wu Y. Shen * M. M. Wu F. Gu j. C. zhang L. j. Wang School of Materials Science and Engineering Shanghai University Shanghai 200072 China

Dye-sensitized solar cells （DSSCs） have been regarded as the most promising alternative to conventional silicon-based photovoltaic devices because they are relatively cost-effective and easy to manufacture. Commonly, nanocrystalline TiO2 has been used as photoanode material in DSSCs since the first demonstration by O’Regan and Grtzel. Compared to mesoporous TiO2, mesoporous ZnO nano-material is considered another important functional material in photovoltaic devices or solar batteries due to its unique electro-optical properties.

关键词： mesoporous ZnO solar cell

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