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Structural and electrochemical stabilization enabling high-energy P3-type Cr-based layered oxide cathode for K-ion batteries

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Carbon Energy 2024年第5期6卷 81-93页

作者： Wonseok Ko Seokjin lee hyunyoung Park jungmin Kang jinho Ahn Yongseok lee Gwangeon Oh jung-Keun Yoo jang-Yeon hwang jongsoon Kim Department of Energy Science Sungkyunkwan UniversitySuwonRepublic of Korea SKKU Institute of Energy Science and Technology(SIEST) Sungkyunkwan UniversitySuwonRepublic of Korea Department of Energy Engineering Hanyang UniversitySeoulRepublic of Korea Carbon Composites Department Korea Institute of Materials Science(KIMS)ChangwonRepublic of Korea Department of Battery Engineering Hanyang UniversitySeoulRepublic of Korea

Layered-type transition metal(TM)oxides are considered as one of the most promising cathodes for K-ion batteries because of the large theoretical gravimetric capacity by low molar ***,they suffer from severe structural change by de/intercalation and diffusion of K^(+)ions with large ionic size,which results in not only much lower reversible capacity than the theoretical capacity but also poor power ***,it is important to enhance the structural stability of the layered-type TM oxides for outstanding electrochemical behaviors under the K-ion battery ***,it is investigated that the substitution of the appropriate Ti^(4+)contents enables a highly enlarged reversible capacity of P3-type KxCrO_(2) using combined studies of first-principles calculation and various *** the pristine P3-type KxCrO_(2) just exhibits the reversible capacity of∼120 mAh g^(−1) in the voltage range of 1.5-4.0 V(vs.K^(+)/K),the∼0.61 mol K^(+)corresponding to∼150 mAh g^(−1) can be reversible de/intercalated at the structure of P3-type K0.71[Cr_(0.75)Ti_(0.25)]O_(2) under the same ***,even at the high current density of 788 mA g^(−1),the specific capacity of P3-type K0.71[Cr_(0.75)Ti_(0.25)]O_(2) is∼120 mAh g^(−1),which is∼81 times larger than that of the pristine P3-type KxCrO_(2).It is believed that this research can provide an effective strategy to improve the electrochemical performances of the cathode materials suffered by severe structural change that occurred during charge/discharge under not only K-ion battery system but also other rechargeable battery systems.

关键词： cathodes first-principles calculations layered-type oxide materials potassium-ion batteries structural stabilization

Prenatal and postnatal factors associated with sudden infant death syndrome:an umbrella review of meta-analyses

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World journal of Pediatrics 2024年第5期20卷 451-460页

作者： Tae hyeon Kim hyeri lee Selin Woo hayeon lee jaeyu Park Guillaume Fond Laurent Boyer jong Woo hahn jiseung Kang Dong Keon Yon Department of Medicine Kyung Hee University College of MedicineSeoulSouth Korea Center for Digital health Medical Science Research InstituteKyung Hee University College of MedicineSeoulSouth Korea Department of Regulatory Science Kyung Hee UniversitySeoulSouth Korea Department of Biomedical Engineering Kyung Hee UniversityYonginSouth Korea CEReSS-health Service Research and Quality of Life Center Assistance Publique des Hôpitaux de MarseilleAix-Marseille UniversityMarseilleFrance Department of Pediatrics Seoul National University College of MedicineSeoulSouth Korea Department of Pediatrics Seoul National University Bundang HospitalSeongnamSouth Korea Department of Anesthesia Critical Care and Pain MedicineMassachusetts General Hospital14913th StreetRoom 4140CharlestownBostonMAUSA Division of Sleep Medicine Harvard Medical SchoolBostonMAUSA Department of Pediatrics Kyung Hee University Medical CenterKyung Hee University College of Medicine23 Kyungheedae-roDongdaemun-guSeoul02447South Korea Department of Precision Medicine Kyung Hee University College of MedicineSeoulSouth Korea

Background Comprehensive quantitative evidence on the risk and protective factors for sudden infant death syndrome(SIDS)effects is *** investigated the risk and protective factors related to *** We conducted an umbrella review of meta-analyses of observational and interventional studies assessing SIDS-related ***/MEDLINE,Embase,EBSCO,and Google Scholar were searched from inception until january 18,*** extraction,quality assessment,and certainty of evidence were assessed by using A Measurement Tool Assessment Systematic Reviews 2 following PRISMA *** to observational evidence,credibility was graded and classified by class and quality of evidence(CE;convincing,highly suggestive,suggestive,weak,or not significant).Our study protocol was registered with PROSPERO(CRD42023458696).The risk and protective factors related to SIDS are presented as equivalent odds ratios(eORs).Results We identified eight original meta-analyses,including 152 original articles,covering 12 unique risk and protective factors for SIDS across 21 countries/regions and five *** risk factors,including prenatal drug exposure[eOR=7.84(95%CI=4.81–12.79),CE=highly suggestive],prenatal opioid exposure[9.55(95%CI=4.87–18.72),CE=suggestive],prenatal methadone exposure[9.52(95%CI=3.34–27.10),CE=weak],prenatal cocaine exposure[4.38(95%CI=1.95–9.86),CE=weak],prenatal maternal smoking[2.25(95%CI=1.95–2.60),CE=highly suggestive],postnatal maternal smoking[1.97(95%CI=1.75–2.22),CE=weak],bed sharing[2.89(95%CI=1.81–4.60),CE=weak],and infants found with heads covered by bedclothes after last sleep[11.01(95%CI=5.40–22.45),CE=suggestive],were *** the other hand,three protective factors,namely,breastfeeding[0.57(95%CI=0.39–0.83),CE=non-significant],supine sleeping position[0.48(95%CI=0.37–0.63),CE=suggestive],and pacifier use[0.44(95%CI=0.30–0.65),CE=weak],were also *** Based on the evidence,we propose several risk and protecti

关键词： Infant Protective factor Risk factor Sudden infant death syndrome Umbrella review

Review on inorganic and polymeric materials-coordinated metal-organic-framework photocatalysts for green hydrogen evolution

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journal of Energy Chemistry 2024年第5期92卷 322-356页

作者： Dong-Eun lee Mohtaram Danish Umair Alam Wan-Kuen jo School of Architecture CivilEnvironmental and Energy Engineering Kyungpook National University80 Daehak-roBuk-guDaegu 41566Republic of Korea School of Chemical Engineering Yeungnam UniversityGyeongsanGyeongbuk 38541Republic of Korea

Metal-organic frameworks(MOFs)possess a distinct advantage over conventional heterogeneous photocatalysts because of their carefully defined architecture and particular pores,which facilitate the targeted incorporation of other efficient cocatalysts or semiconductor *** integration of MOFs with other materials has resulted in significant breakthroughs,as the coupled materials improve the performance due to the combined *** unique MOF structures allow them to host foreign materials,which results in harvesting the visible region of the solar spectrum and effectively mitigating charge recombination by promoting charge *** review presents an evaluation of the latest developments in the utilization of surface and/or pore chemistry of MOF-supported heterojunctions for photocatalytic green-hydrogen generation with a basic understanding of the mechanism *** review begins with the basic principles of photocatalysis,the significance of MOFs,their optical properties,the methods used for synthesizing MOFs,and their coordination with other inorganic and polymeric ***,methods to increase photocatalytic h2 evolution using MOF-supported heterojunction have been proposed as standard ***,to address environmental challenges,we highlight the future potential of MOF-supported heterojunctions for use in green-energy *** hope that this review provides guidance to researchers in the development of effective heterojunctions based on MOFs to address challenges in energy applications and catalytic processes.

关键词： Renewable energy Environmental challenge heterojunction Water splitting Photocatalysis

Characterization of a smog chamber for studying formation of gas-phase products and secondary organic aerosol

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journal of Environmental Sciences 2024年第2期136卷 570-582页

作者： Qi Yuan Zhuozhi Zhang Meng Wang Kin Fai ho Tao Wang Shuncheng lee Department of Civil and Environmental Engineering The Hong Kong Polytechnic UniversityKowloonHong KongChina School of Public health and Primary Care The Chinese University of Hong KongShatinHong KongChina

Smog chambers provide a potent approach to explore the secondary organic aerosol formation under varied *** study describes the construction and characterization of a new smog chamber facility for studying the formation mechanisms of gas-phase products and secondary organic aerosol from the photooxidation of volatile organic *** chamber is a 5.4 m^(3) Fluorinated Ethylene Propylene(FEP)Teflon reactor with the potential to perform photooxidation experiments at controlled temperature and relative *** characterizations were conducted for evaluation of stability of environmental parameters,mixing time,background contamination,light intensity,and wall losses of gases and *** photolysis rate of NO_(2)(j_(NO2))ranged from(1.02-3.32)×10^(-3)sec^(-1),comparable to the average j_(NO2)in ambient *** wall loss rates for NO,NO_(2),and O_(3)were 0.47×10^(-4),0.37×10^(-4),and 1.17×10^(-4)min^(-1),while wall loss of toluene was obsoletely found in a 6 hr *** particle number wall loss rates are(0.01-2.46)×10^(-3)min^(-1)for 40-350 nm with an average lifetime of more than one day.A series of toluene photooxidation experiments were carried out in absence of NO_xunder dry *** results of the simulation experiments demonstrated that the chamber is well designed to simulate photolysis progress in the atmosphere.

关键词： Smog chamber Gas-phase oxidation Chamber characterization Chemical mechanism

Patterning of SnO2/SnTe binary mask structure for extreme ultra-violet lithography using inductively coupled h2/Ar plasmas

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Patterning of SnO2/SnTe binary mask structure for extreme ul...

两种不同气体中的高速爆燃波及其向爆轰的转变

第三届微电子及等离子体技术国际会议

作者： S.j.lee j.h.lee N.-E.lee S.j.Park C.K.hwangbo h.S.Seo S.S.Kim Department of Advanced Materials Science and Engineering Sungkyunkwan University SKKU Advanced Institute of Nanotechnology Sungkyunkwan University Department of Physics Inha University Photomask Team Memory DivisionSemiconductor BusinessSamsung Electronics Co.Ltd.

Currently,extreme ultra-violet lithography（EUVL） is the major candidate of next generation lithography for below 25 nm technology *** fabrication is quite different from the transmissive optics of conventional photolithography masks because of the use of new reflective optics due to absorption of UV light by the quartz *** investigated selective etching of SnTe（tin tellurium alloy） as a new absorber material having high EUV absorbance due to its large extinction *** additional SnO2（tin oxide） layer as an anti reflection coating（ARC） required to reduce the reflectance of the absorber layer was selectively ***,patterning process of the binary mask structure of SnO2（anti reflection coating）/SnTe（absorber layer）/Ru（capping/etch stop layer）/Mo-Si multilayer（reflective layer）/Si（substrate） was *** infinitely high selectivity of the SnTe layer to the Ru ESL is required due to the ultrathin nature of the Ru layer,the various etch parameters were varied in the inductively coupled h2/Ar plasmas in order to find the process window required for the infinitely high etch selectivity of the SnTe layer to Ru layer during one-step etching of SnO2/SnTe stacked *** results showed that the gas flow ratio and self-bias voltage Vdc played an important role in determining the process window for the ultra-high selective etching even with increasing overetch *** high EUV-absorbance SnTe layer,patternable by a dry process,would allow a smaller absorber thickness,which can mitigate the geometric shadowing effects observed during exposure of EUV by using high performance binary EUVL masks.

关键词： EUVL ESL(Etch Stop Layer) SnTe SnO2

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实验力学 2008年第2期23卷 110-117页

作者：朱雨建杨基明 j. h. S. lee 中国科学技术大学近代力学系合肥230027 Department of Mechanical Engineering McGill UniversityMontrealCA

对2C2h2+5O2及2C2h2+5O2+80%Ar两种可燃混合气体中的高速爆燃波及其向爆轰的转变过程进行实验研究。高速爆燃波由孔栅干涉爆轰波的方法直接生成,观测手段则以高速转鼓摄影获取孔栅近场流场x-t纹影图,以传感器追踪波面的后继发展。研究发... 详细信息

对2C2h2+5O2及2C2h2+5O2+80%Ar两种可燃混合气体中的高速爆燃波及其向爆轰的转变过程进行实验研究。高速爆燃波由孔栅干涉爆轰波的方法直接生成,观测手段则以高速转鼓摄影获取孔栅近场流场x-t纹影图,以传感器追踪波面的后继发展。研究发现,两种气体中的爆燃波具有迥异的特性。前者燃烧波面在较低初压条件下为层流结构,而较高初压下为湍流结构,向爆轰转变点可以延伸至下游较长距离;后者在不同初压条件下燃烧波面无明显差异,爆轰的再次形成只能在孔栅下游近场内建立。两种气体中高速爆燃波的维持和爆轰转变过程均非纯粹激波压缩所致,湍流输运在其中起着必不可少的作用。分析显示,激波压缩效应对纯氧炔气体的高速爆燃和DDT贡献较小,湍流输运占主导地位;而氩气稀释气体较为稳定,缺乏自行衍生剧烈湍流燃烧的能力,因而激波压缩和外界扰动对其高速爆燃传播和爆轰转变起十分重要的作用。

关键词：高速爆燃爆燃转爆轰孔栅纹影迹线

Genome of a thermophilic bacterium Geobacillus sp. TFV3 from Deception Island, Antarctica

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Advances in Polar Science 2020年第2期31卷 146-152页

作者： Xin jie ChING Chui Peng TEOh Dexter j.h.lee Marcelo GONZáLEZ-ARAVENA Nazalan NAjIMUDIN Yoke Kqueen ChEAh Paris LAVIN Clemente Michael Vui Ling WONG Biotechnology Research Institute Universiti Malaysia SabahJalan UMS88400 Kota KinabaluSabahMalaysia Instituto Antártico Chileno Plaza Munoz Gamero 1055Punta ArenasChile School of Biological Science Universiti Sains MalaysiaPersiaran Bukit Jambul 11900 Bayan LepasPenangMalaysia Department of Biomedical Science Faculty of Medicine and Health SciencesUniversiti Putra Malaysia43400 UPM SerdangSelangor Darul EhsanMalaysia Universidad de Antofagasta Facultad de Ciencias del Mary Recursos BiologicosDepartamento de BiotecnologiaLaboratorio de Complejidad Microbianay Ecología FuncionalInstituto AntofagastaChile National Antarctic Research Centre University of Malaya50603 Kuala LumpurMalaysia

Thermophilic microorganisms have always been an important part of the ecosystem,particularly in a hot environment,as they play a key role in nutrient recycling at high temperatures where most microorganisms cannot *** most of the thermophiles are archaea,thermophiles can also be found among some species of *** bacteria are very useful in the fundamental study of heat adaptation,and they are also important as potential sources of thermostable enzymes and ***,we have isolated a Gram-positive thermophilic bacterium,Geobacillus ***3 from a volcanic soil sample from Deception Island,*** project was undertaken to analyze the genes of this thermophilic Antarctic bacterium and to determine the presence of thermal-stress adaptation proteins in its *** genome of Geobacillus ***3 was first purified,sequenced,assembled,and *** complete genome was found to harbor genes encoding for useful thermal-stress adaptation *** majority of these proteins were categorized under the family of molecular chaperone and heat shock *** genomic information could eventually provide insights on how the bacterium adapts itself towards high growth temperatures.

关键词： temperature 16SrDNA genomes Geobacillus Deception Island

holographic dark energy in non-conserved gravity theory

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Communications in Theoretical Physics 2024年第4期76卷 126-133页

作者： h R Fazlollahi Institute of Gravitation and Cosmology Peoples Friendship University of Russia(RUDN University)6 Miklukho-Maklaya StMoscow117198Russia

Recently, reconsidering the Rastall idea T_(μ;νν)^(v)=α_(,μ) through relativistic thermodynamics gives a new form for the scalar field α which led us to construct modern modified theory of gravity debugged ‘non-conserved gravity theory’ Fazlollahi 2023 Euro. Phys. j. C 83 923. This theory unlike other modified theories of gravity cannot directly explain the current acceleration expansion in the absence of the cosmological constant and or existence of other forms of dark energy. hence, in this study we have reinvestigated holographic dark energy Ρ_(X)~h^(2) in the non-conserved theory of gravity. In this context, the density and pressure of dark energy depend on the non-conserved term and density of the dust matter field. As shown, due to non-conservation effects on large-scale structures, unlike the original holographic model, our model onsets an acceleration epoch for the current Universe satisfies observations. Moreover, the interaction and viscous scenarios are studied for this model.

关键词： non-conserved gravity covariant form of thermodynamics holographic dark energy

Anticipating the lifespan: Predicting the durability of an anode-supported solid oxide fuel cell short stack over 50,000 h

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Progress in Natural Science:Materials International 2024年第3期34卷 606-613页

作者： Muhammad Zubair Khan Amjad hussain Seung-Bok lee Tak-hyoung Lim Rak-hyun Song Department of Materials Science & Engineering Pak-Austria Fachhochschule: Institute of Applied Sciences and Technology hydrogen Energy Research Division Korea Institute of Energy Research Department of Advanced Energy and System Engineering Korea University of Science and Technology (UST)

In the present study, the operational lifetime of a solid oxide fuel(SOFC) short stack is predicted by investigating the performance degradation of both the short stack and its cells throughout 1000 h at 800°C. The short stack and integral cell voltages are continuously measured during the long-term test, with electrochemical impedance spectroscopy(EIS) conducted every 200 h. The short stack voltage decreased rapidly for the initial 200–300 h and afterwards, it decreased at a slow rate due to the increase in the Ohmic and polarization resistances in the same manner. Scanning electron microscopy results show that there is no delamination or cracking among constituent layers of the short-stack cells. The single degradation effects of the Ni coarsening in the anode, cation migration and surface segregation in cathode and oxide scale growth in metallic interconnect mesh are successfully integrated into a comprehensive lifetime prediction model. The experimentally measured voltage degradation data of the short stack fits well with the developed mathematical model and allows the successful prediction of the lifetime up to 50,000 h.

关键词： Degradation Impedance Lifetime SOFC Stack