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Synthesis of Compact NaA Zeolite Membrane by Microwave Heating Method

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Chinese Chemical Letters 2003年第8期14卷 874-876页

作者： Zhi lin CHENG Zi Sheng CHAO hui lin wan State Key Laboratory for Physical Chemistry of Solid Surface Department of ChemistryXiamen UniversityXiamen 361005

A continuous and dense NaA zeolite membrane was synthesized by microwave heating method while employing a multi-step seeding LTA zeolite with the average size of 120 nm. The gas H2/N2 mixture separating results indicated that the mixture selectivity increased with increasing of synthesis times. In addition, selectivity of the three-step synthesis was higher than the value(3.74) expected from Kundsen diffusion.

关键词： Microwave heating NaA zeolite membrane gas separation.

Oxidative dehydrogenation of ethane to ethene over a superbase supported LiCl system

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Chinese Chemical Letters 2010年第11期21卷 1366-1369页

作者： Yu Bao Zhao Wen Wen Tan hui Li Xiao hui Jia hui lin wan School of Chemistry and Chemical Engineering University of South China Hengyang 421001 China State Key Laboratory for Physical Chemistry of Solid Surfaces Department of Chemistry and Institute of Physical Chemistry Xiamen University Xiamen 361005 China

LiCl-promoted superbase catalysts were found to be stable and highly selective to ethene for oxidative dehydrogenation of ethane,giving 84%ethane conversion and 74%ethene yield at 923 *** indicated that the stronger t... 详细信息

关键词： Oxidative dehydrogenation ODH Ethane Ethene Superbase LiCl

P-modified cobalt oxide: A novel and effective catalyst for oxidative dehydrogenation of propane

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Chinese Chemical Letters 2013年第9期24卷 789-792页

作者： Xiao-Zhang lin Guang-Chao Li Chuan-Jing Huang Wei-Zheng Weng hui-lin wan State Key Laboratory of Physical Chemistry of Solid Surfaces National Engineering Laboratory for Green Chemical Productions of Alcohols Ethers and Esters and Department of Chemistry College of Chemistry and Chemical Engineering Xiamen University

A series ofnanosized cobalt oxide catalysts modified with phosphorus have been synthesized by the solgel method and investigated in the oxidative dehydrogenation of propane to propene. With the addition of phosphorus, the crystallite size of the catalyst was largely decreased, while the P species in the catalyst were highly dispersed. Compared to pure cobalt oxide, the P-modified samples showed higher propane conversion and enhanced propene selectivity. Over the PCoO catalyst with a P/Co atomic ratio of 0.05, the maximal propene yields of 15.7% with a propane conversion of 28.3% were obtained at 520 ℃.

关键词： Propane Propene Oxidative dehydrogenation Nanosized PCoO catalyst

XRD & XPS Study on the BaF_2 Promoted Sm_2O_3-LaF_3 Catalysts

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Chinese Chemical Letters 1997年第1期8卷 83-86页

作者： Ji Zhong LUO and hui lin wan(Department of Chemistry & State Key Laboratory for Physical Chemistry of the Solid Surface, Xiamen UniversityXiamen 361005) XIAMEN UNIV DEPT CHEMXIAMEN 361005PEOPLES R CHINA XIAMEN UNIV STATE KEY LAB PHYS CHEMXIAMEN 361005PEOPLES R CHINA

Sm2O3-LaF3 and BaF2 promoted Sm2O3W3 catalysts shown good catalytic performance for the Oxidative Dehydrogenation of Ethane(ODE). XRD and XPS characterizations of the catalysts show the structure defects, which may be produced by the partial exchange of anions and cations,enhance the electron donating ability and increase the surface absorbed oxygen concentration thus should be favorable to improve the catalytic activity. However, the higher concentration of surface adsorbed oxygen is unfavorable for the ethene selectivity.

关键词： Sm La XRD XPS Study on the BaF2 Promoted Sm2O3-LaF3 Catalysts

Metabolomic Analysis in Saliva and Different Brain Regions of Older Mice with Postoperative Delirium Behaviors

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Biomedical and Environmental Sciences 2024年第2期37卷 133-145页

作者： LIU Xiao CAO Ying lin Xiao wan GAO Dan Yang MIAO hui hui LI Tian Zuo Department of Anesthesiology Beijing Shijitan HospitalCapital Medical UniversityBeijing 100038China

Objective Postoperative delirium(POD)has become a critical challenge with severe consequences and increased incidences as the global population ***,the underlying mechanism is yet *** study aimed to explore the changes in metabolites in three specific brain regions and saliva of older mice with postoperative delirium behavior and to identify potential non-invasive *** Eighteen-month-old male C57/BL6 mice were randomly assigned to the anesthesia/surgery or control *** tests were conducted 24 h before surgery and 6,9,and 24 h after *** C3(C3)and S100 calcium-binding protein B protein(S100beta)levels were measured in the hippocampus,and a metabolomics analysis was performed on saliva,hippocampus,cortex,and amygdala *** In total,43,33,38,and 14 differential metabolites were detected in the saliva,hippocampus,cortex,and amygdala,respectively.“Pyruvate”“alpha-linolenic acid”and“2-oleoyl-1-palmitoy-snglycero-3-phosphocholine”are enriched in one common pathway and may be potential non-invasive biomarkers for *** changes were observed in the three brain regions,with the upregulation of 1-methylhistidine and downregulation of *** Dysfunctions in energy metabolism,oxidative stress,and neurotransmitter dysregulation are implicated in the development of *** identification of changes in the level of salivary metabolite biomarkers could aid in the development of noninvasive diagnostic methods for POD.

关键词： Metabolomic Postoperative delirium(POD) Mechanism Biological marker

A New Catalyst for Hydrogen Transfer Hydrogenation of Acetophenone

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Chinese Chemical Letters 1997年第3期8卷 255-258页

作者： Pian Pian XU Rong hui ZHENG Jing Xing GAO Pei Qing HUANG hui lin wan （Department of Chemistry and Stste Key Laboratory of Physical Chemistry of Solid Surface Xiamen University, Xiamen 361005 ） XIAMEN UNIV DEPT CHEMXIAMEN 361005PEOPLES R CHINA XIAMEN UNIV STATE KEY LAB PHYS CHEM & SOLID SURFACEXIAMEN 361005PEOPLES R CHINA

A new C-2-symmetric diamine/diphosphine Ruthenium (II) complex, RuCl2P2N2H4, was used as an excellent catalyst to carry out the catalytic hydrogen transfer reduction of acetophenone. The conversion of acetophenone to 2-phenylethanol was up to 99% under the following reaction conditions: substrate:Ru:(CH3)(2)CHOK = 200:1:12; reaction temperature of 65 degrees C; reaction time of 2 h; normal pressure. A hydride transfer mechanism was also discussed.

关键词： A New Catalyst for Hydrogen Transfer Hydrogenation of Acetophenone Pro Chen wang

Microstructure evolution and mechanical properties of brazing joint for ultra-thin-walled Inconel 718 considering grain size effect and brazing temperature

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Chinese Journal of Aeronautics 2024年第2期37卷 541-556页

作者： Rui ZHAO Yueshuai SONG hui KANG Min wan School of Mechanical Engineering and Automation Beihang UniversityBeijing 100191China Jiangxi Research Institute of Beihang University Jiangxi 330000China

The systematic investigation of the mechanical properties and microstructure evolution process of ultra-thin-walled Inconel 718 capillary brazing joints is of great significance because of the exceptionally high demands on its *** achieve this objective,this study investigates the impact of three distinct brazing temperatures and five typical grain sizes on the brazed joints’mechanical properties and microstructure evolution *** evolution analysis was conducted based on Electron Back Scatter Diffraction(EBSD),Scanning Electron Microscopy(SEM),X-Ray Diffraction(XRD),High-Resolution Transmission Electron Microscopy(HRTEM),and Focused Ion Beam(FIB).Besides,the mechanical properties and fracture behavior were studied based on the uniaxial tension tests and in-situ tension *** findings reveal that the brazing joint’s strength is higher for the fine-grain capillary than the coarse-grain one,primarily due to the formation of a dense branch structure composed of G-phase in the brazing *** effects of grain size,such as pinning and splitting,are amplified at higher brazing ***,micro-cracks initiate around brittle intermetallic compounds and propagate through the eutectic zone,leading to a cleavage fracture *** fracture stress of fine-grain specimens is higher than that of coarse-grain due to the complex micro-crack ***,this study contributes significantly to the literature by highlighting the crucial impact of grain size on the brazing properties of ultra-thin-walled Inconel 718 structures.

关键词： EYWORDS Ultra-thin-walled structure Brazing Inconel 718 Grain size effect Brazing temperature

RIOK1 synergizes with TRIP13 by regulating the E2F-Rb signaling pathway to promote the proliferation of esophageal cancer cells

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Genes & Diseases 2024年第3期11卷 55-58页

作者： Chengyu Li Deyuan Pan wan lin Danxia Deng Yingxin Zhou hui Zhao Feng Pan Liyan Xu Enmin Li lin Long The Key Laboratory of Molecular Biology for High Cancer Incidence Coastal Chaoshan Area Department of Biochemistry and Molecular BiologyShantou University Medical CollegeShantouGuangdong 515041China Guangdong Provincial Key Laboratory of Infectious Diseases and Molecular Immunopathology Institute of Oncologic PathologyShantou University Medical CollegeShantouGuangdong 515041China Institute of Basic Medical Science Cancer Research CenterShantou University Medical CollegeShantouGuangdong 515041China Clinical Research Center Shantou Central HospitalShantouGuangdong 515041China

Esophageal cancer is one of the leading causes of cancer death in the world,with approximately half of the new cases occurring in China every year.^(1)Esophageal squamous cell carcinoma(ESCC)is the main subtype,accounting for more than 90%,and the five-year survival rate is less than 10%.Using large-scale genome analysis,many driver mutations and key pathways associated with ESCC have been ***,these genomic signatures have not improved the clinical management of EscC patients,or established effective targeted therapy.^(2)Esophageal cancer still lacks representative molecular markers.

关键词： cancer esophageal Esophageal

Dynamics modeling and optimal control for multi-information diffusion in Social Internet of Things

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Digital Communications and Networks 2024年第3期10卷 655-665页

作者： Yaguang lin Xiaoming wang Liang wang Pengfei wan School of Computer Science Shaanxi Normal UniversityXi'an710119China

As an ingenious convergence between the Internet of Things and social networks,the Social Internet of Things(SIoT)can provide effective and intelligent information services and has become one of the main platforms for people to spread and share ***,SIoT is characterized by high openness and autonomy,multiple kinds of information can spread rapidly,freely and cooperatively in SIoT,which makes it challenging to accurately reveal the characteristics of the information diffusion process and effectively control its *** this end,with the aim of exploring multi-information cooperative diffusion processes in SIoT,we first develop a dynamics model for multi-information cooperative diffusion based on the system dynamics theory in this ***,the characteristics and laws of the dynamical evolution process of multi-information cooperative diffusion are theoretically investigated,and the diffusion trend is *** this basis,to further control the multi-information cooperative diffusion process efficiently,we propose two control strategies for information diffusion with control objectives,develop an optimal control system for the multi-information cooperative diffusion process,and propose the corresponding optimal control *** optimal solution distribution of the control strategy satisfying the control system constraints and the control budget constraints is solved using the optimal control ***,extensive simulation experiments based on real dataset from Twitter validate the correctness and effectiveness of the proposed model,strategy and method.

关键词： Social Internet of Things Information diffusion Dynamics modeling Trend prediction Optimal control