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Recent advances in metastable alloys for hydrogen storage:a review

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Rare Metals 2022年第6期41卷 1797-1817页

作者： huai-jun lin Yan-Shan Lu Liu-Ting Zhang Hai-Zhen Liu Kaveh Edalati Adám Révész Institute of Advanced Wear and Corrosion Resistance and Functional Materials Jinan UniversityGuangzhou 510632China Guangdong Provincial Key Laboratory of Advance Energy Storage Materials South China University of TechnologyGuangzhou 510640China School of Materials and Energy Guangdong University of TechnologyGuangzhou 510006China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003China Guangxi Colleges and Universities Key Laboratory of Novel Energy Materials and Related Technology School of Physical Science and TechnologyGuangxi UniversityNanning 530004China Guangxi Novel Battery Materials Research Center of Engineering Technology School of Physical Science and TechnologyGuangxi UniversityNanning 530004China Guangxi Key Laboratory of Processing for Non-Ferrous Metallic and Featured Materials Guangxi UniversityNanning 530004China International Institute for Carbon-Neutral Energy Research(WPI-I2CNER) Kyushu UniversityFukuoka 819-0395Japan Department of Materials Physics E?tv?s UniversityBudapest 1518Hungary

Development of new materials with high hydrogen storage capacity and reversible hydrogen sorp-tion performances under mild conditions has very high value in both fundamental and application *** the past years,some new systems with metastable structures,such as ultra-fine nanocrystalline alloys,amorphous alloys,nanoglass alloys,immiscible alloys,high-entropy alloys,have been abundantly studied as hydrogen storage *** new hydrogen storage properties either from the kinetics or thermodynamics aspects have been *** this review,recent advances of studies on metastable alloys for hydrogen storage applications have been comprehensively *** materials preparation methods to synthesize metastable hydrogen storage alloys are firstly ***,hydrogen storage prop-erties of the metastable alloys are summarized and dis-cussed,focusing on the unique kinetics and thermodynamics properties by forming of such unique metastable *** examples,superior hydrogena-tion kinetics and higher hydrogen storage capacity have been achieved in Mg-based amorphous and nanoglass *** thermodynamics properties can be obtained in the immiscible Mg-Mn and Mg-Zr *** addition to highlighting the recent achievements of metastable alloys in the field of hydrogen storage,the remaining challenges and trends of the emerging research are also discussed.

关键词： Hydrogen storage Metastable alloys Kinetics Thermodynamics

2022 roadmap on hydrogen energy from production to utilizations

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Rare Metals 2022年第10期41卷 3251-3267页

作者： Zheng-Xuan Yang Xiu-Gang Li Qi-Lu Yao Zhang-Hui Lu Ning Zhang jun Xia Kai Yang Yu-Qing Wang Kan Zhang Hai-Zhen Liu Liu-Ting Zhang huai-jun lin Qing-jun Zhou Fang Wang Zhi-Ming Yu Jian-Min Ma School of Physics and Electronics Hunan UniversityChangsha410082China College of Material and Chemical Engineering Tongren UniversityTongren554300China Key Laboratory of Functional Small Molecules for Ministry of Education College of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang330022China School of Materials Science and Engineering Central South UniversityChangsha410083China School of Chemistry and Chemical Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Materials Science and Engineering Nanjing University of Science and TechnologyNanjing210094China Guangxi Novel Battery Materials Research Center of Engineering Technology Guangxi Key Laboratory of Processing for Non-Ferrous Metallic and Featured MaterialsGuangxi Colleges and Universities Key Laboratory of Novel Energy Materials and Related TechnologySchool of Physical Science and TechnologyGuangxi UniversityNanning530004China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang212003China Institute of Advanced Wear and Corrosion Resistance and Functional Materials Jinan UniversityGuangzhou510632China College of Science University of Shanghai for Science and TechnologyShanghai200093China School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun130022China School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu611731China

Hydrogen has been always the hot topic,which drives a lot of researchers to study and explore hydrogenrelated projects and *** first subfield is hydrogen production with green and cost-effective *** methods have been intensively used for high-efficient hydrogen production,i.e.,catalytic chemical hydrogen generation,electrocatalytic hydrogen evolution,photocatalytic hydrogen evolution,photo-electrocatalytic hydrogen *** of them are driven by various ***,the hydrogen storage is also an important question,which is also a present research hot topic,although the history is long with several *** fuel cells have also obtained great attention due to the zero *** related research mainly focuses on the cell systems and electrocatalysts *** this background,we invite some excellent research groups to write this progress on hydrogen from production to ***,we believe that this roadmap on hydrogen can give some useful guidance in future research.

关键词： Hydrogen Hydrogen production Hydrogen generation Hydrogen evolution Hydrogen storage Fuel cells

Impact of severe plastic deformation on kinetics and thermodynamics of hydrogen storage in magnesium and its alloys

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Journal of Materials Science & Technology 2023年第15期146卷 221-239页

作者： Kaveh Edalati Etsuo Akiba Walter J.Botta Yuri Estrin Ricardo Floriano Daniel Fruchart Thierry Grosdidier Zenji Horita Jacques Huot Hai-Wen Li huai-jun lin Ádám Révész Michael J.Zehetbauer WPI International Institute for Carbon-Neutral Energy Research(WPI-I2CNER)Kyushu UniversityFukuokaJapan International Research Center for Hydrogen Energy Kyushu UniversityFukuokaJapan Departamento de Engenharia de Materiais Universidade Federal de São CarlosSao Carlos-SPBrazil Department of Materials Science and Engineering Monash UniversityClaytonVIC 3800Australia Department of Mechanical Engineering the University of Western AustraliaCrawleyWA 6009Australia School of Applied Sciences University of Campinas(UNICAMP)LimeiraSão PauloBrazil Institut Néel CNRS&UGA38042 GrenobleFrance JOMI-LEMAN SA 74890 FessyFrance Universitéde Lorraine Laboratory of Excellence on Design of Alloy Metals for low-mass Structures(DAMAS)MetzF-57070France Universitéde Lorraine Laboratoire d’Etude des Microstructures et de Mécanique des Matériaux(LEM3 UMR 7239)MetzF-57070France Graduate School of Engineering Kyushu Institute of TechnologyKitakyushuJapan Magnesium Research Center Kumamoto UniversityKumamotoJapan Synchrotron Light Application Center Saga UniversitySagaJapan Hydrogen Research Institute Universitédu QuébecàTrois-Rivières3351 des ForgesTrois-RivièresQC G9A 5H7Canada Hefei General Machinery Research Institute Hefei 230031China Institute of Advanced Wear&Corrosion Resistance and Functional Materials Jinan UniversityGuangzhou 510632China Department of Materials Physics Eötvös UniversityBudapestH-1518P.O.B.32BudapestHungary Faculty of Physics University of ViennaBoltzmanngasse 5A-1090 WienAustria

Magnesium and its alloys are the most investigated materials for solid-state hydrogen storage in the form of metal hydrides,but there are still unresolved problems with the kinetics and thermodynamics of hydrogenation and dehydrogenation of this group of *** plastic deformation(SPD)methods,such as equal-channel angular pressing(ECAP),high-pressure torsion(HPT),intensive rolling,and fast forging,have been widely used to enhance the activation,air resistance,and hydrogenation/dehydrogenation kinetics of Mg-based hydrogen storage materials by introducing ultrafine/nanoscale grains and crystal lattice *** severely deformed materials,particularly in the presence of alloying additives or second-phase nanoparticles,can show not only fast hydrogen absorption/desorption kinetics but also good cycling *** was shown that some materials that are apparently inert to hydrogen can absorb hydrogen after SPD ***,the SPD methods were effectively used for hydrogen binding-energy engineering and synthesizing new magnesium alloys with low thermodynamic stability for reversible low/room-temperature hydrogen storage,such as nanoglasses,high-entropy alloys,and metastable phases including the high-pressureγ-MgH2 *** work reviews recent advances in the development of Mg-based hydrogen storage materials by SPD processing and discusses their potential in future applications.

关键词： Severe plastic deformation(SPD) Nanostructured materials Ultrafine-grained(UFG)materials Magnesium hydride(MgH_(2)) Magnesium-based alloys Hydrogen absorption Hydrogenation kinetics Hydrogen storage thermodynamics

Effect of cholesterol metabolism on hepatolithiasis

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World Journal of Gastroenterology 2025年第1期31卷 157-162页

作者： lin Zheng Zi-Yu Ye jun-Ji Ma Department of Gastroenterology The Second Hospital of Hebei Medical UniversityHebei Key Laboratory of GastroenterologyHebei Institute of GastroenterologyHebei Clinical Research Center for Digestive DiseasesNo.215 Heping West RoadShijiazhuang 050000Hebei ProvinceChina

Surgical intervention is currently the primary treatment for hepatolithiasis;how-ever,some patients still experience residual stones and high recurrence rates after *** metabolism seems to play an important role in hepatoli-thiasis pathogenesis.A high cholesterol diet is one of the significant reasons for the increasing incidence of ***,regular diet and appropriate medical intervention are crucial measures to prevent hepatolithiasis and reduce recurrence rate after *** dietary cholesterol and drugs that increase cholesterol stone solubility are key therapeutic approaches in treating *** article discusses the cholesterol metabolic pathways related to the pathogenesis of hepatolithiasis,as well as food intake and targeted therapeutic drugs.

关键词： Hepatolithiasis Cholesterol metabolism High-fat diet 3-hydroxy-3-methylglutaryl-coenzyme A reductase Interlobular bile duct

Multi-model ensemble learning for battery state-of-health estimation:Recent advances and perspectives

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Journal of Energy Chemistry 2025年第1期100卷 739-759页

作者： Chuanping lin jun Xu Delong Jiang Jiayang Hou Ying Liang Zhongyue Zou Xuesong Mei State Key Laboratory for Manufacturing Systems Engineering Xi'an Jiaotong University Shaanxi Key Laboratory of Intelligent Robots School of Mechanical Engineering Xi'an Jiaotong University Department of Electrical Engineering and Automation Luoyang Institute of Science and Technology School of Mechanical Engineering Hangzhou Dianzi University

The burgeoning market for lithium-ion batteries has stimulated a growing need for more reliable battery performance monitoring. Accurate state-of-health(SOH) estimation is critical for ensuring battery operational performance. Despite numerous data-driven methods reported in existing research for battery SOH estimation, these methods often exhibit inconsistent performance across different application scenarios. To address this issue and overcome the performance limitations of individual data-driven models,integrating multiple models for SOH estimation has received considerable attention. Ensemble learning(EL) typically leverages the strengths of multiple base models to achieve more robust and accurate outputs. However, the lack of a clear review of current research hinders the further development of ensemble methods in SOH estimation. Therefore, this paper comprehensively reviews multi-model ensemble learning methods for battery SOH estimation. First, existing ensemble methods are systematically categorized into 6 classes based on their combination strategies. Different realizations and underlying connections are meticulously analyzed for each category of EL methods, highlighting distinctions, innovations, and typical applications. Subsequently, these ensemble methods are comprehensively compared in terms of base models, combination strategies, and publication trends. Evaluations across 6 dimensions underscore the outstanding performance of stacking-based ensemble methods. Following this, these ensemble methods are further inspected from the perspectives of weighted ensemble and diversity, aiming to inspire potential approaches for enhancing ensemble performance. Moreover, addressing challenges such as base model selection, measuring model robustness and uncertainty, and interpretability of ensemble models in practical applications is emphasized. Finally, future research prospects are outlined, specifically noting that deep learning ensemble is poised to advance ens

关键词： Lithium-ion battery State-of-health estimation Data-driven Machine learning Ensemble learning Ensemble diversity

Revolutionizing breast cancer detection:Advances in fluorescent probe technology

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Nano Research 2025年第1期18卷 653-674页

作者： Qian Gao lin Tang jun Zhan Yiyuan Xue Feng Luo State Key Laboratory of Oral Diseases&National Center for Stomatology&National Clinical Research Center for Oral Diseases West China Hospital of StomatologySichuan UniversityChengdu 610041China Emergency Obstetrics and Gynecology West China Second University HospitalSichuan UniversityChengdu 610041China Department of Obstetrics and Gynecology West China Second University HospitalSichuan UniversityChengdu 610041China Department of Prosthodontics West China School of StomatologySichuan UniversityChengdu 610041China

With the increasing incidence of breast cancer globally,there is an urgent demand for enhanced diagnostic and therapeutic *** comprehensive review explores advancements in fluorescent probe technology for breast cancer imaging and early *** probes offer unparalleled sensitivity and specificity in detecting cancer biomarkers,enabling early diagnosis and delineation of tumor margins during *** categorize these probes into molecular,nano,ratiometric,the second near-infrared window(NIR-II),and multifunctional varieties,each with unique capabilities for targeting specific cancer *** review highlights recent innovations in probe design,emphasizing their applications in pathogenesis studies,drug development,precision medicine,and fluorescence-guided *** their promising clinical potential,challenges such as safety,biomarker targeting accuracy,system compatibility,and clinical translation *** these hurdles is crucial for the integration of fluorescent probes into standard cancer care,aiming to improve treatment outcomes and patient quality of life.

关键词： breast cancer fluorescent probes imaging early diagnosis biomarker

Engineering of Fe d-band center in Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles via orbital coupling for high-efficiency oxygen reduction electrocatalysis

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Nano Research 2025年第1期18卷 129-139页

作者： Jiayi Liu Jingwen Yin Yingzi lin Mingxin Pang Huan Pang Songtao Zhang lin Xu jun Yang Yawen Tang Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Center of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023Chin a 2 State Key Laboratory of Multiphase Complex Systems Center of MesoscienceInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009China Testing Center Yangzhou UniversityYangzhou 225009China

The deliberate engineering of the d-band center of metal site represents an effective strategy to boost the intrinsic electrocatalytic performance toward the oxygen reduction reaction(ORR).Herein,following a heterointerfaceinduced orbital coupling rationale,we report a judicious design of an efficient ORR electrocatalyst consisting of Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles in-situ encased into N-doped carbon nanofibers(abbreviated as Fe_(3)O_(4)/CeO_(2)@N-CNFs hereafter).The theoretic calculations uncover that the Fe_(3)O_(4)/CeO_(2)heterointerface-triggered orbital coupling can cause the down shift of the d-band center positions of Fe sites,which leads to the weakened chemisorption of oxygenated groups and lowered energy barrier for the potential-determining step,ultimately dramatically boosting the ORR intrinsic *** a consequence,the well-designed Fe_(3)O_(4)/CeO_(2)@N-CNFs display admirable ORR activity with a half-wave potential of 0.84 V and outstanding structural/electrochemical stability in an alkaline electrolyte,surpassing the commercial Pt/C benchmark and a majority of recently reported Fe_(3)O_(4)-based *** encouragingly,the Fe_(3)O_(4)/CeO_(2)@N-CNFsincorporated Zn-air battery outperforms the Pt/C-assembled counterpart with higher power density,larger energy density,and excellent cycling stability,serving as a competent candidate for ORR-involved renewable energy *** study offers an innovative approach for the rational manipulation of the d-band center and interfacial electron behavior of active sites toward the optimization of electrocatalytic performance.

关键词： hetero-nanoparticles electrospinning interfacial engineering orbital coupling oxygen reduction reaction

变形和能量注入协同作用制备可控非晶纳米晶结构超高饱和磁化强度FeCoB粉末

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Science China Materials 2024年第6期67卷 1985-1993页

作者：李枧邵里良白荣晟周靖童星林怀俊张猛柯海波汪卫华 Institute of Advanced Wear&Corrosion Resistance and Functional Materials Jinan UniversityGuangzhou 510632China Songshan Lake Materials Laboratory Dongguan 523808China Institute of Physics Chinese Academy of SciencesBeijing 100190China

非晶纳米晶磁粉芯(ANMPCs)是电子元器件在高频应用的关键软磁材料.但其相对较低的饱和磁化强度无法满足器件的小型化要求.强Fe-Co交换耦合非晶纳米晶粉是制备高磁化强度ANMPCs的潜在材料.本文采用机械球磨法制备了一系列(Fe_(0.8)Co_(0.... 详细信息

非晶纳米晶磁粉芯(ANMPCs)是电子元器件在高频应用的关键软磁材料.但其相对较低的饱和磁化强度无法满足器件的小型化要求.强Fe-Co交换耦合非晶纳米晶粉是制备高磁化强度ANMPCs的潜在材料.本文采用机械球磨法制备了一系列(Fe_(0.8)Co_(0.2))_(87)B_(13)软磁粉末,这些粉末的非晶相、纳米晶相含量和粒径可调.在球磨过程中,出现了合金化、玻璃化和纳米化三个阶段以及粉末形貌和尺寸的非线性变化,进而导致ANMPCs软磁性能的非单调变化.磁粉具有超高饱和磁化强度达239 emu g^(-1),有效磁导率为33.球磨150 h后,FeCoB粉末非晶-纳米晶双相结构达到动态平衡,同时粒径达亚微米尺度,从而提高了粉末高频稳定性且降低了磁芯损耗.在变形和能量注入的协同作用下,机械球磨实现了含极高铁磁元素的非晶-纳米晶双相粉末可控制备、提高了高磁化强度ANMPCs综合软磁性能.

关键词： amorphous-nanocrystalline magnetic powder core mechanical ball milling ultrahigh ferromagnetic element sa-turation magnetization high-frequency properties

Hypoxia-preconditioned bone marrow-derived mesenchymal stem cells protect neurons from cardiac arrest-induced pyroptosis

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Neural Regeneration Research 2025年第4期20卷 1103-1123页

作者： Xiahong Tang Nan Zheng Qingming lin Yan You Zheng Gong Yangping Zhuang Jiali Wu Yu Wang Hanlin Huang jun Ke Feng Chen Shengli Clinical Medical College of Fujian Medical University Fujian Medical UniversityFuzhouFujian ProvinceChina Department of Emergency Fujian Provincial HospitalFuzhouFujian ProvinceChina Fujian Provincial Key Laboratory of Emergency Medicine FuzhouFujian ProvinceChina The Second Department of Intensive Care Unit Fujian Provincial Hospital South BranchFuzhouFujian ProvinceChina

Cardiac arrest can lead to severe neurological impairment as a result of inflammation,mitochondrial dysfunction,and post-cardiopulmonary resuscitation neurological *** preconditioning has been shown to improve migration and survival of bone marrow–derived mesenchymal stem cells and reduce pyroptosis after cardiac arrest,but the specific mechanisms by which hypoxia-preconditioned bone marrow–derived mesenchymal stem cells protect against brain injury after cardiac arrest are *** this end,we established an in vitro co-culture model of bone marrow–derived mesenchymal stem cells and oxygen–glucose deprived primary neurons and found that hypoxic preconditioning enhanced the protective effect of bone marrow stromal stem cells against neuronal pyroptosis,possibly through inhibition of the MAPK and nuclear factor κB ***,we transplanted hypoxia-preconditioned bone marrow–derived mesenchymal stem cells into the lateral ventricle after the return of spontaneous circulation in an 8-minute cardiac arrest rat model induced by *** results showed that hypoxia-preconditioned bone marrow–derived mesenchymal stem cells significantly reduced cardiac arrest–induced neuronal pyroptosis,oxidative stress,and mitochondrial damage,whereas knockdown of the liver isoform of phosphofructokinase in bone marrow–derived mesenchymal stem cells inhibited these *** conclude,hypoxia-preconditioned bone marrow–derived mesenchymal stem cells offer a promising therapeutic approach for neuronal injury following cardiac arrest,and their beneficial effects are potentially associated with increased expression of the liver isoform of phosphofructokinase following hypoxic preconditioning.

关键词： bone marrow–derived mesenchymal stem cells cardiac arrest cardiac resuscitation hypoxic preconditioning liver isoform of phosphofructokinase mitochondria neuroinflammation oxidative stress pyroptosis reactive oxygen species