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Immobilization of cross-linked In-doped Mo(O,S)2 on cellulose nanofiber for effective organic-compound degradation under visible light illumination

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Progress in Natural Science:Materials International 2021年第3期31卷 404-413页

作者： Hairus Abdullah Chi-Ning hsu Hardy Shuwanto Noto Susanto Gultom Worku Lakew Kebede Chang-Mou wu Chiu-Chun Lai Ri-Ichi Murakami Masayuki Hirota Antonio Norio Nakagaito Dong-Hau Kuo Department of Materials Science and Engineering National Taiwan University of Science and Technology Department of Textile Engineering Chinese Culture University New Material Research & Development Department Frontier Materials Laboratories Osaka Gas Chemicals Co. Ltd. Graduate School of Technology Industrial and Social Sciences Tokushima University

Relatively small amounts of In-doped Mo(O,S)2(IMS) catalysts(10%, 20%, and 30%) were deposited on cellulose nanofiber(CNF) by cross-linking them with functional groups of siloxane and epoxy to form CNF-IMS hybrid composites. The as-prepared hybrid composites were characterized and tested their performances toward the photo degradations of cationic(MB and Rh B) and anionic(MO) dyes. As indium was doped into Mo(O,S)2lattice to form solid-solution, the charge transfer and photocarrier separation during the catalytic reaction were simultaneously enhanced as probed with electrochemical impedance spectroscopy and photoluminescence measurements, respectively. To ensure the catalyst on CNF was well deposited and recyclable, the hybrid composite was evaluated with a reusability experiment to show the stability performance in degrading organic dyes. It was found the environmentally friendly CNF-IMS hybrid composite was relatively stable during the reusability experiment, indicating no catalyst powder was leached out during the photocatalytic reaction. The photoreaction mechanism was convinced by radical-scavenging experiments to show that hydroxyl and superoxide played essential roles for the organic dye degradations in visible-light illuminated conditions. The cross-linked organic/inorganic hybrid catalyst showed a prospective visible light active material not only to solve the environmental issue due to the leaching of nanoparticles but also to lower the post-treatment/recycling cost of photocatalyst in industrial application.

关键词： Cellulose nanofiber In-doped Mo(O,S) 2 Cross-linking In 2 (O,S) 3 Organic dye degradation

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Systematic Approaches of UWB Low-Power CMOS LNA with Body Biased Technique

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Wireless Engineering and Technology 2015年第3期6卷 61-77页

作者： Meng-Ting hsu Kun-Long wu Wen-Chen Chiu Department and Institute of Engineering National Yunlin University of Science and Technology Taiwan Microwave Communication and Radio Frequency Integrated Circuit Lab Department and Institute of Engineering National Yunlin University of Science and Technology Taiwan

This paper presents research on a low power CMOS UWB LNA based on a cascoded common source and current-reused topology. A systematic approach for the design procedure from narrow band to UWB is developed and discussed in detail. The power reduction can be achieved by using body biased technique and current-reused topology. The optimum width of the major transistor device M1 is determined by the power-constraint noise optimization with inner parasitic capacitance between the gate and source terminal. The derivation of the signal amplification S21 by high frequency small signal model is displayed in the paper. The optimum design of the complete circuit was studied in a step by step analysis. The measurements results show that the proposed circuit has superior S11, gain, noise figure, and power consumption. From the measured results, S11 is lower than -12 dB, S22 is lower than -10 dB and forward gain S21 has an average value with 12 dB. The noise figure is from 4 to 5.7 dB within the whole band. The total power consumption of the proposed circuit including the output buffer is 4.6 mW with a supply voltage of 1 V. This work is implemented in a standard TSMC 0.18 μm CMOS process technology.

关键词： Body Bias Common Source Low Noise Amplifier (LNA) Low Power RFCMOS Ultra-Wideband (UWB)

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Expression of CD86 and increased infiltration of NK cells are associated with Helicobacter pylori-dependent state of early stage high-grade gastric MALT lymphoma

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World Journal of Gastroenterology 2005年第28期11卷 4357-4362页

作者： Sung-Hsin Kuo Li-Tzong Chen Chi-Long Chen Shin-Lian Doong Kun-Huei Yeh Hui-Chen hsu Ming-Shiang wu Jaw-Town Lin Hsiu-Po Wang Ann-Lii Cheng Departments of Oncology National Taiwan University Hospital Taipei Cancer Research Center and Graduate Institute of Clinical Medicine National Taiwan University College of Medicine Taipei Taiwan China Division of Cancer Research National Health Research Institutes Taipei Department of Internal Medicine Kaohsiung Medical University Hospital Kaohsiung Taipei Taiwan China Department of Pathologyl Taipei MedicalUniversity Taipei Taiwan China Graduate Institute of Microbiology National Taiwan University College of Medicine Taipei Taiwan China Departments of Oncology National Taiwan University Hospital Taipei Cancer Research Center National Taiwan University College of Medicine Taipei Taiwan China Department of Internal Mcclicine National Taiwan University Hospital Taipei Taiwan China Department of Emergency Medicine National Taiwan University Hospital Taipei Taiwan China Department of internal Medicine and Department of Oncology National Taiwan University Hospital Taipei Cancer Research Center National Taiwan University College of MedicineTaipei Division of Cancer Research National Health Research Institutes Taipei Taiwan China

AIM： A high percentage of early-stage high-grade gastric mucosa-associated lymphoid tissue （MALT） lymphomas remain Helicobacter pylori （ H pylori）-dependent. However,unlike their low-grade counterparts, high-grade gastric MALT lymphomas may progress rapidly if unresponsive to H pylori eradication. It is mandatory to identify markers that may predict the H pylori-dependent status of these tumors. Proliferation of MALT lymphoma cells depends on cognate help and cell-to-cell contact of H pylori- spedfic intratumoral T-cells. To examine whether the expression of co-stimulatory marker CD86 （B7.2） and the infiltration of CD56 （＋） natural killer （NK） cells can be useful markers to predict Hpylori-dependent status of high-grade gastric MALT iymphoma.METHODS： Lymphoma biopsies from 26 patients who had participated in a prospective study of Hpylori-eradication for stage IE high-grade gastric MALT lymphomas were evaluated. Tumors that resolved to Wotherspoon grade Ⅱ or less alter H pylori eradication were dassified as H pylori-dependent; others were dassified as H *** infiltration of NK cells and the expression of CD86 in pre-treatment paraffin-embedded lymphoma tissues were determined by immunohistochemistry. RESULTS： There were 16 H pylori-dependent and 10 H pylori-independent cases. CD86 expression was detected in 11 （68.8%） of 16 H pylori-dependent cases but in none of 10 H pylori-independent cases （P = 0.001）.H pylori-dependent high-grade gastric MALT lymphomas contained significantly higher numbers of CD56 （＋） NK cells than H pylori-independent cases （2.8±1.4% vs 1.1±0.8%, P = 0.003）. CD86 positive MALT lymphomas also showed significantly increased infiltration of CD56 （＋） NK cells compared to CD86-negative cases （2.9±1.1% vs 1.4±1.3%; P= 0.005）.CONCLUSION： These results suggest that the expression of co-stimulatory marker CD86 and the increased infiltration of NK cells are associated with Hpylori-dependent state of early-stage high-grade gastric M

关键词： MALT lymphoma Hpylori CD86 CD56

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Functional and molecular mechanism of intracellular pH regulation in human inducible pluripotent stem cells

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World Journal of Stem Cells 2018年第12期10卷 196-211页

作者： Shih-Chi Chao Gwo-Jang wu Shu-Fu Huang Niann-Tzyy Dai hsu-Kai Huang Mei-Fang Chou Yi-Ting Tsai Shiao-Pieng Lee Shih-Hurng Loh Graduate Institute of Life Sciences National Defense Medical Center Department of Obstetrics and Gynecology TriService General Hospital National Defense Medical Center Department of Pharmacy Practice Tri-Service General Hospital National Defense Medical Center Division of Plastic and Reconstructive Surgery Department of Surgery Tri-Service General Hospital National Defense Medical Center Division of Chest Surgery Department of Surgery Tri-Service General Hospital National Defense Medical Center Graduate Institute of Medical Sciences National Defense Medical Center Division of Cardiovascular Surgery Department of Surgery Tri-Service General Hospital National Defense Medical Center Division of Oral and Maxillofacial Surgery Department of Dentistry School of Dentistry Tri-Service General Hospital and National Defense Medical Center Department of Pharmacology National Defense Medical Center

AIM To establish a functional and molecular model of the intracellular pH(pH_i) regulatory mechanism in human induced pluripotent stem cells(hiPSCs).METHODS hiP SCs(HPS0077) were kindly provided by Dr. Dai from the Tri-Service General Hospital(IRB No. B-106-09). Changes in the pH_i were detected either by microspectrofluorimetry or by a multimode reader with a pH-sensitive fluorescent probe, BCECF, and the fluorescent ratio was calibrated by the high K^+/nigericin method. NH_4Cl and Na-acetate prepulse techniques were used to induce rapid intracellular acidosis and alkalization, respectively. The buffering power(β) was calculated from the ΔpH_i induced by perfusing different concentrations of(NH_4)_2SO_4. Western blot techniques and immunocytochemistry staining were used to detect the protein expression of pH_i regulators and pluripotency *** In this study, our results indicated that(1) the steadystate pH_i value was found to be 7.5 ± 0.01(n = 20) and 7.68 ± 0.01(n =20) in HEPES and 5% CO_2/HCO_3^- buffered systems, respectively, which were much greater than that in normal adult cells(7.2);(2) in a CO_2/HCO_3^--buffered system, the values of total intracellular buffering power(β) can be described by the following equation: β_(tot) = 107.79(pH_i)~2-1522.2(pH_i) + 5396.9(correlation coefficient R^2 = 0.85), in the estimated pH_i range of 7.1- 8.0;(3) the Na^+/H^+ exchanger(NHE) and the Na^+/HCO_3^- cotransporter(NBC) were found to be functionally activated for acid extrusion for pHi values less than 7.5 and 7.68, respectively;(4) V-ATPase and some other unknown Na^+-independent acid extruder(s) could only be functionally detected for pHi values less than 7.1;(5) the Cl^-/OH^- exchanger(CHE) and the Cl^- /HCO_3 anion exchanger(AE) were found to be responsible for the weakening of intracellular proton loading;(6) besides the CHE and the AE, a Cl^--independent acid loading mechanism was functionally identified; and(7) in hiPSCs, a strong positive correlation

关键词： microspectrofluorimetry human induced pluripotent stem cells Na^+/H^+exchanger Na^+/HCO3^-cotransporter Cl^-/OH^-exchanger Cl^-/HCO3^-exchanger V-ATPase intracellular buffering power intracellular pH BCECF

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3D-printed microelectronics for integrated circuitry and passive wireless sensors

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Microsystems & Nanoengineering 2015年第1期1卷 119-127页

作者： Sung-Yueh wu Chen Yang Wensyang hsu Liwei Lin Department of Mechanical Engineering University of CaliforniaBerkeleyCA 94720USA Department of Mechanical Engineering National Chiao Tung UniversityHsinchu 30010 Berkeley Sensor and Actuator Center(BSAC) University of CaliforniaBerkeleyCA 94720USA

Three-dimensional(3D)additive manufacturing techniques have been utilized to make 3D electrical components,such as resistors,capacitors,and inductors,as well as circuits and passive wireless *** the fused deposition modeling technology and a multiple-nozzle system with a printing resolution of 30μm,3D structures with both supporting and sacrificial structures are *** removing the sacrificial materials,suspensions with silver particles are injected subsequently solidified to form metallic elements/*** prototype results show good characteristics of fabricated 3D microelectronics components,including an inductor–capacitor-resonant tank circuitry with a resonance frequency at 0.53 GHz.A 3D“smart cap”with an embedded inductor–capacitor tank as the wireless passive sensor was demonstrated to monitor the quality of liquid food(e.g.,milk and juice)*** result shows a 4.3%resonance frequency shift from milk stored in the room temperature environment for 36 *** work establishes an innovative approach to construct arbitrary 3D systems with embedded electrical structures as integrated circuitry for various applications,including the demonstrated passive wireless sensors.

关键词： additive manufacturing radio-frequency passive sensors 3D inductors and capacitors three-dimensional printing wireless sensing

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Selection of Renewable Energy Based on Life Cycle Assessment and Multi-Criteria Decision Making

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Open Journal of Energy Efficiency 2016年第1期5卷 1-11页

作者： Wen-Fang wu Yao hsu Ya-Ju Chang Ying-Chu Chen Department of Mechanical Engineering and Graduate Institute of Industrial Engineering National Taiwan University Taiwan Department of Business and Entrepreneurial Management Kainan University Taiwan Graduate Institute of Industrial Engineering National Taiwan University Taiwan Department of Environmental Technology Technische Universitat Berlin Berlin Germany Institute of Natural Resource Management National Taipei University Taiwan

The development of renewable energy has become an important issue nowadays owing to the growing concerns about global warming and shortage of fossil fuels. The present study proposes an approach that integrates life cycle assessment (LCA), 3E (Energy-Economics-Environment) indicators and multi-criteria analysis (MCA) to evaluate environmental impacts and find the best choice or better choices among various renewable energy development plans. Several alternatives of wind turbines and photovoltaic (PV) systems are considered in the case study since they are found to be more feasible in Taiwan in a preliminary study. By using the proposed approach, the result indicates that the major environmental impacts arising from the development of wind turbines and PV systems in Taiwan are the generation of respiratory inorganics and minerals as well as the consumption of fossil fuels. Based on experts’ opinions, the outcome of multi-criteria analysis suggests that wind turbines have more advantages than PV systems in Taiwan. In particular, among the studied systems, a 2500-kW offshore wind turbine system has the greatest integrated performance, and a 4500-kW onshore wind turbine system comes in second.

关键词： Renewable Energy Life Cycle Assessment Multi-Criteria Decision Making

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The taxonomy and molecular phylogeny of Candidia（teleostei:cyprinidae） from Taiwan,with description of a new species and comments on a new cyprinid genus

The taxonomy and molecular phylogeny of Candidia（teleostei:...

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中国鱼类学会2008年学术研讨会

作者： I-Shiung Chen Jui-Hsieng wu Chi-Hsin hsu Institute of Marine Biology National Taiwan Ocean UniversityKeelung 202TaiwanR.O.C Department of Marine Biotechnology and Resources National Sun Yat-sen UniversityKaohsiung 804TaiwanR.O.C.

＜正＞The cyprinid genus,Candidia Jordan ＆ Richardson,1909,is revised and the taxonomic status and the phylogenetic position of related cyprinids from Taiwanese waters are *** molecular phylogenetic analyses inferred...

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Long-term hepatic consequences of chemotherapy-related HBV reactivation in lymphoma patients

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World Journal of Gastroenterology 2005年第34期11卷 5283-5288页

作者： Chi-Chung Wen Chao A.Hsiung Ih-Jen Su Ann-Lii Cheng Ming-Chih Chang Chao-Jung Tsao Woei-Yao Kao wu-Ching Uen Chiun hsu Chih-Hung hsu Yen-Shen Lu Hwei-Fan Tien Tsu-Yi Chao Li-Tzong Chen Jacqueline Whang-Peng Pei-Jer Chen Division of Biostatics and Bioinformatics National Health Research Institutes Taipei Taiwan China Division of Clinical Research National Health Research Institutes Taipei Taiwan China Department of Oncology National Taiwan University Hospital Taipei Taiwan China Department of Internal Medicine National Taiwan University Hospital Taipei Taiwan China Department of Internal Medicine Mackay Memorial Hospital Taipei Taiwan China Department of Internal Medicine Chi-Mei Hospital Tainan Taiwan China Department of Internal Medicine Tri-Service General Hospital Taipei Taiwan China Department of Internal Medicine Shin Kong Memorial Hospital Taipei Taiwan China Department of Oncology National Taiwan University Hospital Taipei Taiwan China Department of Internal Medicine National Taiwan University Hospital Taipei Taiwan China Division of Cancer Research National Health Research Institutes Taipei Taiwan China

AIM: To investigate the long-term consequences of chemotherapy-related HBV reactivation in patients with ***: This study was based on the database of published prospective study evaluating HBV reactivation in HBV lymphoma patients during *** liver reserve (DLR) was defined as development of either one of the following conditions during follow-up: (1) newly onset parenchyma liver disease, splenomegaly or ascites without evidence of lymphoma involvement; (2) decrease of the ratio (albumin/globulin ratio) to less than 0.8 or increase of the ratio of INR of prothrombin time to larger than 1.2 without evidence of malnutrition or infection. Liver cirrhosis was diagnosed by imaging ***: A total of 49 patients were included. The median follow-up was 6.2 years (range, 3.9-8.1 years).There were 31 patients with and 18 patients without HBV reactivation. Although there was no difference of overall survival (OS) and chemotherapy response rate between the two groups, DLR developed more frequently in patients with HBV reactivation (48.4% vs 16.7%; P= 0.0342). Among the HBV reactivators, HBV genotype C was associated with a higher risk of developing DLR (P = 0.0768) and liver cirrhosis (P = 0.003). Four of five patients with sustained high titer of HBV DNA and two of three patients with multiple HBV reactivation developed DLR. Further, patients with a sustained high titer of HBV DNA had the shortest OS among the HBV reactivators (P= 0.0000). No patients in the non-HBV reactivation group developed hepatic failure or liver ***: Chemotherapy-related HBV reactivation is associated with the long-term effect of deterioration of hepatic function.

关键词： HBV reactivation Liver function Non-HodgkJn'slymphoma, Chemotherapy

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Novel methylation gene panel in adjacent normal tissues predicts poor prognosis of colorectal cancer in Taiwan

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World Journal of Gastroenterology 2020年第2期26卷 154-167页

作者： Chih-Hsiung hsu Cheng-Wen Hsiao Chien-An Sun Wen-Chih wu Tsan Yang Je-Ming Hu Chi-Hua Huang Yu-Chan Liao Chao-Yang Chen Fu-Huang Lin Yu-Ching Chou Graduate Institute of Medical Sciences National Defense Medical CenterTaipei 114Taiwan Teaching Office Tri-Service General HospitalNational Defense Medical CenterTaipei 114Taiwan Division of Colorectal Surgery Department of SurgeryTri-Service General HospitalNational Defense Medical CenterTaipei 114Taiwan Department of Public Health College of MedicineFu-Jen Catholic UniversityNew Taipei City 242Taiwan Big Data Research Center College of MedicineFu-Jen Catholic UniversityNew Taipei City 242Taiwan School of Public Health National Defense Medical CenterTaipei 114Taiwan Department of Surgery Suao and Yuanshan Branches of Taipei Veterans General HospitalYilan County 264Taiwan Department of Health Business Administration Meiho UniversityPingtung County 912Taiwan Adjunct Instructor School of MedicineNational Defense Medical CenterTaipei 114Taiwan

BACKGROUND It is evident that current clinical criteria are suboptimal to accurately estimate patient *** have identified epigenetic aberrant changes as novel prognostic factors for colorectal cancer(CRC).AIM To estimate whether a methylation gene panel in different clinical stages can reflect a different *** We enrolled 120 CRC patients from Tri-Service General Hospital in Taiwan and used the candidate gene approach to select six genes involved in carcinogenesis *** were divided into two groups based on the methylation status of the six evaluated genes,namely,the<3 aberrancy group and≥3 aberrancy *** tumor stages were divided into two subgroups(local and advanced stages)on the basis of the pathological type of the following tissues:Tumor and adjacent normal tissues(matched normal).We assessed DNA methylation in tumors and adjacent normal tissues from CRC patients and analyzed the association between DNA methylation with different cancer stages and the prognostic outcome including time to progression(TTP)and overall *** We observed a significantly increasing trend of hazard ratio as the number of hypermethylated genes increased both in normal tissue and tumor *** 5-year TTP survival curves showed a significant difference between the≥3 aberrancy group and the<3 aberrancy *** with the<3 aberrancy group,a significantly shorter TTP was observed in the≥3 aberrancy *** further analyzed the interaction between CRC prognosis and different cancer stages(local and advanced)according to the methylation status of the selected genes in both types of *** was a significantly shorter 5-year TTP for tumors at advanced stages with the promoter methylation status of selected genes than for those with local *** found an interaction between cancer stages and the promoter methylation status of selected genes in both types of *** Our data provide a significant association

关键词： DNA methylation Panel genes Clinical stage Prognosis outcome Adjacent normal tissues Colorectal cancer

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Subgrouping time-dependent prescribing patterns of first-onset major depressive episodes by psychotropics dissection

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World Journal of Psychiatry 2021年第11期11卷 1116-1128页

作者： Hsi-Chung Chen Hui-hsuan hsu Mong-Liang Lu Ming-Chyi Huang Chun-Hsin Chen Tzu-Hua wu Wei-Chung Mao Chuhsing K Hsiao Po-Hsiu Kuo Department of Psychiatry&Center of Sleep Disorders National Taiwan University HospitalTaipei 100Taiwan Center of Statistical Consultation and Research National Taiwan University HospitalTaipei 100Taiwan Department of Psychiatry Wan-Fang Hospital&School of MedicineCollege of MedicineTaipei Medical UniversityTaipei 100Taiwan Department of Psychiatry Taipei City HospitalSongde BranchTaipei 100Taiwan Department of Clinical Pharmacy School of PharmacyCollege of PharmacyTaipei Medical UniversityTaipei 110Taiwan Department of Psychiatry Cheng-Hsin General HospitalTaipei 100Taiwan Graduate Institute of Epidemiology and Preventive Medicine College of Public HealthNational Taiwan UniversityTaipei 100Taiwan

BACKGROUND Subgrouping patients with major depressive disorder is a promising solution for the issue of ***,the link between available subtypes and distinct pathological mechanisms is weak and yields disappointing results in clinical *** To develop a novel approach for classification of patients with time-dependent prescription patterns at first onset in real-world *** Drug-naive patients experiencing their first major depressive episode(n=105)participated in this *** agents prescribed in the first 24 mo following disease onset were recorded monthly and categorized as antidepressants,augmentation agents,and *** cumulative doses of agents in each category were converted into relevant *** parameters were used to summarize the time-dependent prescription patterns for each psychotropic load:Stability,amount,frequency,and the time trend of monthly prescriptions.A K-means cluster analysis was used to derive subgroups of participants based on these input parameters of psychotropic agents across 24 *** validity of the resulting data-driven clusters was compared using relevant severity *** Four distinct clusters were derived from K-means analysis,which matches experts’consent:"Short-term antidepressants use","long-term antidepressants use","long-term antidepressants and sedatives use",and"long-term antidepressants,sedatives,and augmentation use".At the first 2 years of disease course,the four clusters differed on the number of antidepressants used at adequate dosage and duration,frequency of outpatient service use,and number of psychiatric *** the first 2 years following disease onset,depression severity was differed in the four *** Our findings suggested a new approach to optimize the subgrouping of patients with major depressive disorder,which may assist future etiological and treatment response studies.

关键词： First episode Depression Classification Psychopharmacology Depression treatment

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