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Versatile MXene Gels Assisted by Brief and Low‑Strength Centrifugation

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Nano-Micro Letters 2024年第5期16卷 231-247页

作者： Weiyan yu Yi Yang yunjing Wang Lulin Hu Jingcheng hao Lu Xu Weimin liu State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000People’s Republic of China Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai Yantai 264006People’s Republic of China Key Laboratory of Colloid and Interface Chemistry and Key Laboratory of Special Aggregated Materials Shandong UniversityJinan 250100People’s Republic of China

Due to the mutual repulsion between their hydrophilic surface terminations and the high surface energy facilitating their ran-dom restacking,2D MXene nanosheets usually cannot self-assemble into 3D macroscopic gels with various applications in the absence of proper linking *** this work,a rapid spontaneous gelation of Ti3C2Tx MXene with a very low dispersion concentration of 0.5 mg mL^(-1) into multifunctional architectures under moderate centrifugation is *** as-prepared MXene gels exhibit reconfigurable internal structures and tunable rheological,tribological,electrochemical,infrared-emissive and photothermal-conversion properties based on the pH-induced changes in the surface chemistry of Ti_(3)C_(2)T_(x) *** adopting a gel with optimized pH value,high lubrication,exceptional specific capacitances(~635 and~408 F g^(-1) at 5 and 100 mV s^(-1),respectively),long-term capacitance retention(~96.7%after 10,000 cycles)and high-precision screen-or extrusion-printing into different high-resolution anticounterfeiting patterns can be achieved,thus displaying extensive potential applications in the fields of semi-solid lubrication,control-lable devices,supercapacitors,information encryption and infrared camouflaging.

关键词： MXene Centrifugation-assisted rapid gelation Lubrication Supercapacitor Anti-counterfeiting applications

Intelligent Dynamic Heterogeneous Redundancy Architecture for IoT Systems

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China Communications 2024年第7期21卷 291-306页

作者： Zhang Han Wang yu liu hao Lin Hongyu Chen Liquan School of Cyber Science and Engineering Southeast UniversityNanjing 211102China Purple Mountain Laboratories Nanjing 211111China ZTE Corporation Nanjing 210012China Carbon Peaking&Carbon Neutrality Application Technology R&D Institute Nanjing University of Posts and TelecommunicationsNanjing 210002China

The conventional dynamic heterogeneous redundancy(DHR)architecture suffers from the security threats caused by the stability differences and similar vulnerabilities among the *** overcome these challenges,we propose an intelligent DHR architecture,which is more feasible by intelligently combining the random distribution based dynamic scheduling algorithm(RD-DS)and information weight and heterogeneity based arbitrament(IWHA)*** the proposed architecture,the random distribution function and information weight are employed to achieve the optimal selection of executors in the process of RD-DS,which avoids the case that some executors fail to be selected due to their stability difference in the conventional DHR ***,through introducing the heterogeneity to restrict the information weights in the procedure of the IWHA,the proposed architecture solves the common mode escape issue caused by the existence of multiple identical error output results of similar *** experimental results characterize that the proposed architecture outperforms in heterogeneity,scheduling times,security,and stability over the conventional DHR architecture under the same conditions.

关键词： dynamic heterogeneous redundancy heterogeneity IoT security security defense

Comparative proteomics reveals the response and adaptation mechanisms of white Hypsizygus marmoreus against the biological stress caused by Penicillium

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Food Science and Human Wellness 2024年第3期13卷 1645-1661页

作者： Xiuqing Yang Sizhu Li Xiaohang Li Chenxiao Zhang Meijie liu Lizhong Guo Lin liu hao yu Shandong Provincial Key Laboratory of Applied Mycology School of Life SciencesQingdao Agricultural UniversityQingdao 266109China

White Hypsizygus marmoreus is a popular edible *** mycelium is easy to be contaminated by Penicillium,which leads to a decrease in its quality and *** could compete for limited space and nutrients through rapid growth and produce a variety of harmful gases,such as benzene,aldehydes,phenols,etc.,to inhibit the growth of *** mycelium.A series of changes occurred in *** proteome after contamination when detected by the label-free tandem mass spectrometry(MS/MS)*** proteins with up-regulated expression worked together to participate in some processes,such as the non-toxic transformation of harmful gases,glutathione metabolism,histone modification,nucleotide excision repair,clearing misfolded proteins,and synthesizing glutamine,which were mainly used in response to biological *** proteins with down-regulated expression are mainly related to the processes of ribosome function,protein processing,spliceosome,carbon metabolism,glycolysis,and *** reduction in the function of these proteins affected the production of the cell components,which might be an adjustment to adapt to growth *** study further enhanced the understanding of the biological stress response and the growth restriction adaptation mechanisms in edible *** also provided a theoretical basis for protein function exploration and edible mushroom food safety research.

关键词： Hypsizygus marmoreus Penicillium Proteomics Biological stress response Adaptation

Publication-level analysis of Journal of Plant Ecology during 2018-2022

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Journal of Plant Ecology 2024年第4期17卷 197-201页

作者： yu Liao Pu Wang Lijuan liu Wen-hao Zhang National Science Library Chinese Academy of SciencesBeijing 100190China Center for Documentation and Information Institute of BotanyChinese Academy of SciencesBeijing 100093China State Key Laboratory of Vegetation and Environmental Change Institute of BotanyChinese Academy of SciencesBeijing 100093China

Journal of Plant Ecology(JPE)was established in 2008 and is sponsored by the Botanical Society of China and the Institute of Botany,Chinese Academy of *** by Oxford University Press,UK,JPE encompasses a wide range of article types within the expansive field of plant *** of July 2021,JPE has transitioned to fully Open Access,ensuring unrestricted access to the full text for both readers and *** shift enhances the journal’s role as a crucial platform for plant ecologists worldwide to disseminate their research findings.

关键词： Open Plant Access

Rate transient analysis methods for water-producing gas wells in tight reservoirs with mobile water

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Energy Geoscience 2024年第1期5卷 311-320页

作者： Qingyan yu Ying Jia Pengcheng liu Xiangyang Hu Shengye hao Research Institute of Petroleum Exploration and Development of SINOPEC Beijing100083China School of Energy Resources China University of GeosciencesBeijing100083China

Tight gas reservoirs with mobile water exhibit multi-phase flow and high stress *** analyzing the reservoir and well parameters using conventional single-phase rate transient analysis methods proves *** study introduces novel rate transient analysis methods incorporating evaluation processes based on the conventional flowing material balance method and the Blasingame type-curve method to examine fractured gas wells producing *** positing a gas-water two-phase equivalent homogenous phase that considers characteristics of mobile water,gas,and high stress sensitivity,the conventional single-phase rate transient analysis methods can be applied by integrating the phase's characteristics and defining the phase's normalized parameters and material balance *** rate transient analysis methods based on the equivalent homogenous phase can be used to quantitatively assess the parameters of wells and gas reservoirs,such as original gas-in-place,fracture half-length,reservoir permeability,and well drainage *** facilitates the analysis of production dynamics of fractured wells and well-controlled areas,subsequently aiding in locating residual gas and guiding the configuration of well *** specific evaluation processes are ***,a numerical simulation mechanism model was constructed to verify the reliability of the developed *** methods introduced have been successfully implemented in field water-producing gas wells within tight gas reservoirs containing mobile water.

关键词： Gas reservoirs with mobile water Gas-water two phase flow High stress sensitivity Equivalent homogenous phase Rate transient analysis

Fundamentals and photocatalytic hydrogen evolution applications of quaternary chalcogenide semiconductor:Cu_(2)ZnSnS_(4)

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Rare Metals 2022年第7期41卷 2153-2168页

作者： Xin-Long Zheng Ying-Jie Yang yu-hao liu Pei-Lin Deng Jing Li Wei-Feng liu Peng Rao Chun-Man Jia Wei Huang Yan-Lian Du Yi-Jun Shen Xin-Long Tian State Key Laboratory of Marine Resource Utilization in South China Sea Hainan Provincial Key Laboratory of Fine ChemistrySchool of ScienceHainan UniversityHaikou 570228China Mechanical and Electrical Engineering College Hainan UniversityHaikou 570228China

Inexpensive,safe,and efficient conversion of solar energy to hydrogen from water splitting requires the development of effective and durable ***_(2)ZnSnS_(4)(CZTS),the emerging quaternary chalcogenide material for solar energy conversion,possesses many advantages,such as narrow direct band gap(1.5 eV),nontoxic,earth-abundance,and low melting ***,CZTS-based photocatalysts have been extensively investigated for their application as an active photocatalyst in hydrogen evolution from water splitting,while the performance is still highly needed to be improved for the practical *** this review,first,the crystal and band structure properties of CZTS are briefly introduced,and afterward,the basic principle of photocatalytic hydrogen evolution from water splitting is ***,the performance and status of bare CZTS,the combination of CZTS and co-catalysts,and CZTSbased heterojunction photocatalysts for hydrogen evolution are reviewed and discussed in ***,the issues and challenges currently encountered in the application of CZTS and their possible solutions for developing advanced CZTS photocatalysts are provided.

关键词： Cu_(2)ZnSnS_(4) Quaternary chalcogenide Photocatalyst Hydrogen evolution

Pd Pt VO_(x)/CeO_(2)-ZrO_(2):Highly efficient catalysts with good sulfur dioxide-poisoning reversibility for the oxidative removal of ethylbenzene

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Journal of Environmental Sciences 2024年第4期138卷 153-166页

作者： Jia Wang yuxi liu Jiguang Deng Lin Jing Xiuqing hao Xing Zhang Xiaohui yu Hongxing Dai Beijing Key Laboratory for Green Catalysis and Separation Key Laboratory of Beijing on Regional Air Pollution ControlKey Laboratory of Advanced Functional MaterialsEducation Ministry of ChinaLaboratory of Catalysis Chemistry and NanoscienceDepartment of Chemical EngineeringFaculty of Environment and LifeBeijing University of TechnologyBeijing 100124China

The PdPtVO_(x)/CeO_(2)-ZrO_(2)(PdPtVO_(x)/CZO)catalysts were obtained by using different approaches,and their physical and chemical properties were determined by various *** activities of these materials in the presence of H_(2)O or SO_(2)were evaluated for the oxidation of ethylbenzene(EB).The PdPtVO_(x)/CZO sample exhibited high catalytic activity,good hydrothermal stability,and reversible sulfur dioxide-poisoning performance,over which the specific reaction rate at 160℃,turnover frequency at 160℃(TOF_(Pd or Pt)),and apparent activation energy were 72.6 mmol/(g_(Pt)·sec)or 124.2 mmol/(g_(Pd)·sec),14.2 sec^(-1)(TOF_(Pt))or 13.1 sec^(-1)(TOF_(Pd)),and 58 k J/mol,*** large EB adsorption capacity,good reducibility,and strong acidity contributed to the good catalytic performance of PdPtVO_(x)/*** activity of PdPtVO_(x)/CZO decreased when 50 ppm SO_(2)or(1.0 vol.%H_(2)O+50 ppm SO_(2))was added to the feedstock,but was gradually restored to its initial level after the SO_(2)was cut *** good reversible sulfur dioxide-resistant performance of PdPtVO_(x)/CZO was associated with the facts:(i)the introduction of SO_(2)leads to an increase in surface acidity;(ii)V can adsorb and activate SO_(2),thus accelerating formation of the SO_(x)^(2-)(x=3 or 4)species at the V and CZO sites,weakening the adsorption of sulfur species at the PdPt active sites,and hence protecting the PdPt active sites to be not poisoned by SO_(2).EB oxidation over PdPtVO_(x)/CZO might take place via the route of EB→styrene→phenyl methyl ketone→benzaldehyde→benzoic acid→maleic anhydride→CO_(2)and H_(2)O.

关键词： Ceria-zirconia Supported palladium-platinum-vanadium catalyst Volatile organic compound Ethylbenzene oxidation Sulfur dioxide resistance

Lattice Boltzmann simulation study of anode degradation in solid oxide fuel cells during the initial aging process

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International Journal of Minerals,Metallurgy and Materials 2024年第2期31卷 405-411页

作者： Shixue liu Zhijing liu Shuxing Zhang hao Wu Hydrogen Energy Industrial Technology Innovation Center China Nuclear Power Technology Research InstituteShenzhen 518031China Shenzhen Engineering Research Center for Hydrogen Safety Shenzhen 518031China

For present solid oxide fuel cells(SOFCs),rapid performance degradation is observed in the initial aging process,and the dis-cussion of the degradation mechanism necessitates quantitative ***,focused ion beam-scanning electron microscopy was em-ployed to characterize and reconstruct the ceramic microstructures of SOFC *** lattice Boltzmann method(LBM)simulation of multiphysical and electrochemical processes in the reconstructed models was *** samples collected from industrial-size cells were characterized,including a reduced reference cell and a cell with an initial aging *** parameters of the reconstructed microstructures revealed a significant decrease in the active triple-phase boundary and Ni connectivity in the aged cell compared with the reference *** LBM simulation revealed that activity degradation is dominant compared with microstructural degradation during the initial aging process,and the electrochemical reactions spread to the support layer in the aged *** microstructural and activity de-gradations are attributed to Ni migration and coarsening.

关键词： solid oxide fuel cell anode degradation focused ion beam-scanning electron microscopy lattice Boltzmann method

Is intestinal metaplasia the point of no return in the progression of gastric carcinogenesis?

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Chinese Medical Journal 2021年第24期134卷 2965-2967页

作者： Si-Ran Wu yu-hao liu Yong-Quan Shi State Key Laboratory of Cancer Biology National Clinical Research Center for Digestive DiseasesXijing HospitalAir Force Medical UniversityXi’anShaanxiChina Department of Gastroenterology Chinese Armed Police Force Fujian Armed Police Corps hospitalFuzhouFujianChina First Cadet Regiment School of Basic MedicineAir Force Medical UniversityXi’anShaanxiChina

Gastric cancer(GC)is one of the most common malignant tumors *** China,GC is the second most common malignant tumor,and it is the second leading cause of cancer mortality.[1]Correa model showed that the development of intestinal-type GC was a consecutive cancerous process including normal gastric mucosa,non-atrophic gastritis,atrophic gastritis(AG),intestinal metaplasia(IM),dysplasia and intestinal-type GC in sequence.[2]Epithelium-resembling intestinal morphology replaced gastric mucosa which was defined as IM.[3]Among these precancerous conditions,IM was demonstrated to be a vital risk factor for GC,especially incomplete IM and extensive IM.[4,5].

关键词： gastritis gastric metaplasia