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苯的微生物降解之谜稳定同位素分析法诠释苯的微生物降解

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实验与分析 2014年第2期 30-30,32页

作者： Carsten Voget Martin Taubert Sabine Kleinsteuber Martin Von Berger Jena Seifert hans-hermann richnow 海姆霍兹环保研究所

苯．是存在于自然界中最简单的芳香类化合物，也是一种致癌物质。被苯污染的地下水可能会带来多种风险．所以探明苯的生物降解过程对于风险的评估和控制是非常有意义的。

关键词：苯污染微生物降解同位素分析法诠释稳定芳香类化合物生物降解过程致癌物质

Reciprocity Relation between Alternative Gravity Formulas

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Journal of Applied Mathematics and Physics 2024年第4期12卷 1432-1440页

作者： hans hermann Otto Department of Materials Science and Crystallography Clausthal University of Technology Clausthal-Zellerfeld Germany

We compare Newton’s force law of universal gravitation with a corrected simple approach based on Bhandari’s recently presented work, where the gravitation constant G is maintained. A reciprocity relation exists between both alternative gravity formulas with respect to the distances between mass centers. We conclude a one-to-one mapping of the two gravitational formulas. We don’t need Einstein’s construct of spacetime bending by matter.

关键词： Gravity Formulas Reciprocity Distance Relation Newton Einstein Bhandari Higgs Field Dirac’s Large Number

Combined quantitative microscopy on the microstructure and phase evolution in Li1.3Al0.3Ti1.7(PO4)3 ceramics

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Journal of Advanced Ceramics 2020年第2期9卷 149-161页

作者： Deniz Cihan GUNDUZ Roland SCHIERHOLZ Shicheng YU hermann TEMPELa hans KUNGL Rudiger-AEICHEL Forschungszentrum Jülich Institute of Energy and Climate Research(IEK-9:Fundamental Electrochemistry)Julich D-52425Germany Forschungszentrum Julich Institute of Energy and Climate Research(IEK-12:Helmholtz-Institute Münster:Ionics in Energy Storage)Munster D-48149Germany RWTH Aachen University Institute of Physical ChemistryAachen D-52074Germany

Lithium aluminum titanium phosphate(LATP)is one of the materials under consideration as an electrolyte in future all-solid-state lithium-ion *** ceramic processing,the presence of secondary phases and porosity play an important *** a presence of more than one secondary phase and pores,image analysis must tackle the difficulties about distinguishing between these microstructural *** this study,we study the phase evolution of LATP ceramics sintered at temperatures between 950 and 1100℃by image segmentation based on energy-dispersive X-ray spectroscopy(EDS)elemental maps combined with quantitative analysis of LATP *** found aluminum phosphate(AlPO4)and another phosphate phase((Lix)PyOz).The amount of these phases changes with sintering ***,since the grains act as an aluminum source for AlPO4 formation,the aluminum content in the LATP grains ***,the amount of secondary phase changes from more(Lix)PyOz at 950℃to mainly AlPO4 at 1100℃sintering *** also used scanning electron microscopy(SEM)and confocal laser scanning microscopy(CLSM)to study the evolution of the LATP grains and AlPO4,and LATP grain size increases with sintering *** addition,transmission electron microscopy(TEM)was used for the determination of grain boundary width and to identify the amorphous structure of AlPO4.

关键词： lithium aluminum titanium phosphate(LATP) microstructure quantitative microscopy grain size confocal laser scanning microscopy(CLSM) NASICON

Individual stages of bacterial dichloromethane degradation mapped by carbon and chlorine stable isotope analysis

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Journal of Environmental Sciences 2019年第4期31卷 147-160页

作者： Maria L.Torgonskaya Anatoly M.Zyakun Yuri A.Trotsenko Kestutis S.Laurinavichius Steffen Kümmel Stéphane Vuilleumier hans H.richnow Laboratory of Radioactive Isotopes G.K.Skryabin Institute of Biochemistry and Physiology of MicroorganismsFRC Pushchino Center for Biological ResearchRussian Academy of Sciences Laboratory of Mass Spectrometry G.K.Skryabin Institute of Biochemistry and Physiology of MicroorganismsFRC Pushchino Center for Biological ResearchRussian Academy of Sciences Department of Isotope Biogeochemistry Helmholtz Centre for Environmental Research-UFZ Université de Strasbourg CNRS

The fractionation of carbon and chlorine stable isotopes of dichloromethane(CH_2Cl_2,DCM)upon dechlorination by cells of the aerobic methylotroph Methylobacterium extorquens DM4 and by purified DCM dehalogenases of the glutathione S-transferase family was *** effects for individual steps of the multi-stage DCM degradation process,including transfer across the cell wall from the aqueous medium to the cell cytoplasm,dehalogenase binding,and catalytic reaction,were *** observed carbon and chlorine isotope fractionation accompanying DCM consumption by cell supensions and enzymes was mainly determined by the breaking of C\Cl bonds,and not by inflow of DCM into *** isotope effects of DCM dehalogenation were initially masked in high density cultures,presumably due to inverse isotope effects of non-specific DCM oxidation under conditions of oxygen *** cofactor supply remarkably affected the correlation of variations of DCM carbon and chlorine stable isotopes(Δδ^(13)C/Δδ^(37)Cl),increasing corresponding ratio from 7.2–8.6 to 9.6–10.5 under conditions of glutathione *** suggests that enzymatic reaction of DCM with glutathione thiolate may involve stepwise breaking and making of bonds with the carbon atom of DCM,unlike the uncatalyzed reaction,which is a one-stage process,as shown by quantum-chemical modeling.

关键词： Dichloromethane(DCM) Microbial degradation Aerobic methylotrophic bacteria Dichloromethane dehalogenase Carbon and chlorine isotopic fractionation

Do patients with gastroesophageal reflux disease and somatoform tendencies benefit from antireflux surgery?

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World Journal of Gastroenterology 2019年第3期25卷 388-397页

作者： hans Friedrich Fuchs Benjamin Babic Karl-hermann Fuchs Wolfram Breithaupt Gabor Varga Frauke Musial Department of General Surgery University of Cologne Department of General Surgery University of Mainz Department of Surgery University of California San Diego Department of Surgery Goethe University Frankfurt National Research Center in Complementary and Alternative Medicine NAFKAM Department of Community Medicine UiT The Arctic University of Norway

BACKGROUND The clinical presentation of gastroesophageal reflux disease(GERD) shows a large symptom variation also in different intensities among patients. As several studies have shown, there is a large overlap in the symptomatic spectrum between proven GERD and other disorders such as dyspepsia, functional heartburn and/or somatoform *** To prospectively evaluate the GERD patients with and without somatoform disorders before and after laparoscopic antireflux *** In a tertiary referral center for foregut surgery over a period of 3 years patients with GERD, qualifying for the indication of laparoscopic antireflux surgery, were investigated prospectively regarding their symptomatic spectrum in order to identify GERD and associated somatoform disorders. Assessment of symptoms was performed by an instrument for the evaluation of somatoform disorders[Somatoform Symptom Index(SSI) > 17]. Quality of life was evaluated by Gastrointestinal Quality of Life Index(GIQLI).RESULTS In 123 patients an indication for laparoscopic antireflux surgery was established and in 43 patients further medical therapy was suggested. The portion of somatoform tendencies in the total patient population was 20.48%(34 patients).Patients with a positive SSI had a preoperative GIQLI of 77(32-111). Patients with a normal SSI had a GIQLI of 105(29-140)(P < 0.0001). In patients with GERD the quality of life could be normalized from preoperative reduced values of GIQLI102(47-140) to postoperative values of 117(44-144). In patients with GERD and somatoform disorders, the GIQLI was improved from preoperative GIQLI 75(47-111) to postoperative 95(44-122)(P < 0.0043).CONCLUSION Patients with GERD and associated somatoform disorders have significantly worse levels of quality of life. The latter patients can also benefit from laparoscopic fundoplication, however they will not reach a normal level.

关键词： Gastroesophageal reflux disease Antireflux surgery Laparoscopic fundoplication Somatization Gastroesophageal reflux disease symptoms

Galactic Route to the Strong Coupling Constant α_s(m_z) and Its Implication on the Mass Constituents of the Universe

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Journal of Applied Mathematics and Physics 2022年第12期10卷 3572-3585页

作者： hans hermann Otto Materials Science and Crystallography Clausthal University of Technology Clausthal-Zellerfeld Germany

Some fundamental physical quantities need an alternative description. We derive the word average value of interaction coupling constant αs(mz) from the observed maximum galactic rotation velocity by the simple relation , where is the velocity, at which the difference between galactic rotation velocity and Thomas precession is equal, and α is Sommerfeld’s constant. The result is in excellent agreement with the value of αs = 0.1170 ± 0.0019, recently measured and verified via QCE analysis by CERN researchers. One can formulate a reciprocity relation, connecting αs with the circle constant: . It is the merit of Preston Guynn to derive the Milky Way maximum value of the galactic rotation velocity βg, pointing to its “extremely important role in all physics”. The mass (energy) constituents of the Universe follow a golden mean hierarchy and can simply be related to the maximum of Guynn’s difference velocity respectively to αs(mz), therewith excellently confirming Bouchet’s WMAP data analysis. We conclude once more that the golden mean concept is the leading one of nature.

关键词： Strong Coupling Constant Sommerfeld’ Constant Gravitational Coupling Constant Galactic Velocity Structure-Matter Theory Reciprocity Relation Goldem Mean Hierarchy Mass and Energy Constituents of the Universe Superconductivity Matter-Antimatter Asymmetry Unification of Science

Golden Quartic Polynomial and Moebius-Ball Electron

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Journal of Applied Mathematics and Physics 2022年第5期10卷 1785-1812页

作者： hans hermann Otto Materials Science and Crystallography Clausthal University of Technology Clausthal-Zellerfeld Germany

A symmetrical quartic polynomial, named golden one, can be connected to coefficients of the icosahedron equation as well as to the gyromagnetic correction of the electron and to number 137. This number is not a mystic one, but is connected with the inverse of Sommerfeld’s fine-structure constant and this way again connected with the electron. From number-theoretical realities, including the reciprocity relation of the golden ratio as effective pre-calculator of nature’s creativeness, a proposed closeness to the icosahedron may point towards the structure of the electron, thought off as a single-strand compacted helically self-confined charged elemantary particle of less spherical but assumed blunted icosahedral shape generated from a high energy double-helix photon. We constructed a chiral Moebius “ball” from a 13 times 180˚twisted double helix strand, where the turning points of 12 generated slings were arranged towards the vertices of a regular icosahedron, belonging to the non-centrosymmetric rotation group I532. Mathematically put, we convert the helical motion of an energy quantum into a stationary motion on a Moebius stripe structure. The radius of the ball is about the Compton radius. This chiral closed circuit Moebius ball motion profile can be tentatively thought off as the dominant quantum vortex structure of the electron, and the model may be named CEWMB (Charged Electromagnetic Wave Moebius Ball). Also the gyromagnetic factor of the electron (ge = 2.002319) can be traced back to this special structure. However, nature’s energy infinity principle would suggest a superposition with additional less dominant (secondary) structures, governed also by the golden mean. A suggestion about the possible structure of delocalized hole carriers in the superconducting state is given.

关键词： Golden Qartic Polynomial Number Theory Icosahedron Equation Golden Mean Fifth Power of the Golden Mean Moebius Ball Electron Structure Chirality Fine-Structure Constant Fibonacci Number 13 Lucas Numbers Superconductivity

Nuclear Fusion Research and Development Need New Relativistic Mass and Energy Corrections Given by the Information Relativity Theory

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Journal of Applied Mathematics and Physics 2022年第5期10卷 1813-1836页

作者： hans hermann Otto Materials Science and Crystallography Clausthal University of Technology Clausthal-Zellerfeld Germany

Hundred years after the conjecture of the British astronomer Eddington that the sun is powered by nuclear fusion of hydrogen, new physics theory may help make energy harvesting by nuclear fusion soon a reality. Researchers as well as investors funding fusion megaprojects are asked to deal with new relativistic corrections for mass and energy proposed by Suleiman in his Information Relativity Theory (IRT). These corrections were calculated in this contribution. It will help to decide whether a venture will be successful and to save big investments when in doubt. The assumed optimal kinetic energy for controlled nuclear fusion must be corrected to a somewhat higher level. At very high kinetic energy in the upper GeV range, it remains not enough baryonic mass to be transformed in energy. The fusion probability faded out to zero already at the golden limit of the recession speed of between target nucleon and projectile nucleon. Cold nuclear fusion, if ever possible, is recommended for protons rather than deuterons at highest experimental possible temperatures around 1000 (K) and needs fine-tuned kinetic nucleon energy. It would be also of interest whether a golden ratio based nuclear fuel confinement chamber could be beneficial. In this connection, also cold nuclear fusion setups should be discussed. Nature is governed by the golden ratio and criticality of physical systems influenced by it, and nuclear physics is not an exception. Computer simulations of the underlying controlled nuclear fusion processes should gain profit from IRT corrected starting information and may tackle anew possible low energy nuclear transmutations considering the wave-like dark components of matter and energy.

关键词： Controlled Thermonuclear Fusion IRT Theory Relativistic Mass Correction Low Energy Nuclear Reaction Golden Ratio Golden Limit of Nuclear Fusion

Fibonacci Stoichiometry and Superb Performance of Nb₁₆W₅O₅₅ and Related Super-Battery Materials

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Journal of Applied Mathematics and Physics 2022年第6期10卷 1936-1950页

作者： hans hermann Otto Materialwissenschaftliche Kristallographie Clausthal University of Technology Clausthal-Zellerfeld Lower Saxony Germany

In this contribution, two important crystallographic concepts for the formation of a series of block structures associated with channeling have been compared: chemical twinning and crystallographic shear. Twin planes respectively shear planes besides formed channels serve as a sink for charge carriers or, when the oxidation state of metal ions can be reduced, as a reservoir for intercalated lithium. In this way, Wadsley-Roth shear phases such as niobium tungsten oxide exhibit channels for ultra-fast lithium-ion diffusion. They are in focus as anode material for super-batteries, superb in terms of energy respectively power density, charging time, cycle life and safety. It should be noted that the transition metal to oxygen ratio TM/O = 21/55 of the title compound is a Fibonacci number quotient. Also, the crystal lattice can be traced back to Fibonacci geometry. When replacing only 0.0213 tungsten atoms in the formula with less expensive titanium, a TM/O ratio of 0.381966 =ϕ2 can be adapted besides an average valence electron concentration of 2⋅ϕ-2, where represents the most irrational number of the golden mean. The additional disorder caused by even such small titanium replacement and accompanied oxygen vacancies could fasten up the already high lithium diffusion further. Ultrasonic treatment may be applied besides thermal cycling to prepare phase-pure of the highest electrochemical performance. A replacement of oxygen by some fluorine atoms is an obvious synthesis possibility, but the higher binding energy expected between lithium and fluorine in contrast to oxygen may rather hinder than promote lithium diffusion.

关键词： Super Battery Niobium Tungsten Oxide Crystallographic Shear Chemical Twinning Fibonacci Stoichiometry Ti Substitution