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Plasmonic tandem heterojunctions enable high-efficiency charge transfer for broad spectrum photocatalytic hydrogen production

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Journal of Energy Chemistry 2025年第1期100卷 710-720页

作者： Wenxuan Chen Xiu-Qing Qiao Guo Hui Bojing Sun dongfang Hou Meidi Wang Xueqian Wu Tao Wu dong-Sheng Li College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials China Three Gorges University Hubei Three Gorges Laboratory College of Chemistry and Materials Science and Guangdong Provincial Key Laboratory of Supramolecular Coordination Chemistry Jinan University

Rational engineering of semiconductor photocatalysts for efficient hydrogen production is of great significance but still challenging,primarily due to the limitations in charge transfer ***,a fascinating plasmonic tandem heterojunction with the hc-CdS/Mo2C@C heterostructure is aimfully prepared for effectively promoting the charge separation kinetics of the CdS photocatalyst via the synergistic strategy of phase junction,Schottky junction,and photothermal *** difference in atomic configuration between cubic-CdS （c-CdS） and hexagonal-CdS （h-CdS） leads to effective charge separation through a typical Ⅱ charge transfer mechanism,and plasmonic Schottky junction further extracts the electrons in the hc-CdS phase junction to realize gradient charge ***,the photothermal effect of Mo2C@C helps to expand the light absorption,accelerate charge transfer kinetics,and reduce the hydrogen evolution energy *** carbon layer provides a fast channel for charge transfer and protects the photocatalyst from *** a result,the optimized hc-CMC photocatalyst exhibits a significantly high photocatalytic H2production activity of 28.63 mmol/g/h and apparent quantum efficiency of 61.8%,surpassing most of the reported *** study provides a feasible strategy to enhance the charge transfer kinetics and photocatalytic activity of CdS by constructing plasmonic tandem heterogeneous junctions.

关键词： Heterojunctions LSPR Photocatalyst Phase junction Schottky junction Photothermal effect

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Organic/inorganic nanocomposite polymer electrolyte

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Chinese Chemical Letters 2007年第2期18卷 185-188页

作者： Li Qi shao Jun dong State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied Chemistry Chinese Academy of Sciences Changchun 130022 China

The organic/inorganic nanocomposites polymer electrolytes were designed and synthesized. The organic/inorganic nanocomposites membrane materials and their lithium salt complexes have been found thermally stable below 200 °C. The conductivity of the organic/inorganic nanocomposites polymer electrolytes prepared at room temperature was at magnitude range of 10(?6) S/cm.

关键词： Organic/inorganic nanocomposites Polymer electrolyte Polymer lithium battery Conductivity Characterization Thermal stability

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NON C^0 NONCONFORMING ELEMENTS FOR ELLIPTIC FOURTH ORDER SINGULAR PERTURBATION PROBLEM

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Journal of Computational Mathematics 2005年第2期23卷 185-198页

作者： shao-chunChen Yong-chengZhao dong-yangShi DepartmentofMathematics ZhengzhouUniversityZhengzhou450052China

In this paper we give a convergence theorem for non C^0 nonconforming finite element to solve the elliptic fourth order singular perturbation problem. Two such kind of elements, a nine parameter triangular element and a twelve parameter rectangular element both with double set parameters, are presented. The convergence and numerical results of the two elements are given.

关键词： singular perturbation problem nonconforming element double set parametermethod

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Predictive Zone Control of Pressure Management for Water Supply Network Systems

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International Journal of Automation and computing 2016年第6期13卷 607-614页

作者： dong-Ming Liu shao-Yuan Li Department of Automation Shanghai Jiao Tong University Shanghai 200240 China Key Laboratory of System Control and Information Processing Ministry of Education Shanghai 200240 China Changzhou Institute of Light Industry Technology Jiangsu 213164 China

In this paper we address the problem of pressure management in water supply system （WSS） network. The model-based predictive control （MPC） strategies have some important features to deal with WSS. By hydraulic analysis of WSS, the predictive model is derived from the dynamic model and static model of WSS. Through WSS, the consumers＇ demands are required to be met at all times according to some operational constraints that must be satisfied. The constraints of flow through actuators, the water level of reservoirs and the consumer areas＇ pressure demand are determined by a specific system. In this work, we develop a constrained MPC controller that considers the zone control of the pressure outputs and incorporates steady state economic targets in the control cost function. The designed management strategies are applied to a case study and simulation results, covering different aspects, are provided. The output nodal pressure can be controlled in the desired zone by optimal scheduling the actuators of the WSS. If the variation range of reservoir＇s water level is broader, the rate of flow through the actuators is gentle, and vice versa.

关键词： Water supply system (WSS) network mathematical modelling zone control pressure control model predictive control(MPC).

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Cheeger's cut, maxcut and the spectral theory of1-Laplacian on graphs

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Science China Mathematics 2017年第11期60卷 1963-1980页

作者： CHANG KungChing shao SiHong ZHANG dong LMAM and School of Mathematical Sciences Peking University

This is primarily an expository paper surveying up-to-date known results on the spectral theory of1-Laplacian on graphs and its applications to the Cheeger cut, maxcut and multi-cut problems. The structure of eigenspa... 详细信息

关键词： spectral graph theory Laplacian graph cut optimization critical point theory

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A low redox potential and long life organic anode material for sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 557-564页

作者： Zhi Li Yang Wei Kang Zhou Xin Huang Xing Zhou Jie Xu Taoyi Kong Junwei Lucas Bao Xiaoli dong Yonggang Wang Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials Institute of New Energy Collaborative Innovation Center of Chemistry for Energy Materials (iChEM) Fudan University Department of Chemistry Boston College School of Materials Science and Engineering Anhui University of Technology

Sodium-ion batteries （SIBs） with organic electrodes are an emerging research direction due to the sustainability of organic materials based on elements like C,H,O,and sodium ***,organic electrode materials for SIBs are mainly used as cathodes because of their relatively high redox potentials（>1 V）.Organic electrodes with low redox potential that can be used as anode are ***,a novel organic anode material （tetrasodium 1,4,5,8-naphthalenetetracarboxylate,Na4TDC） has been developed with low redox potential （<0.7 V） and excellent cyclic *** three-sodium storage mechanism was demonstrated with various in-situ/ex-situ spectroscopy and theoretical calculations,showing a high capacity of 208 mAh/g and an average decay rate of merely 0.022%per ***,the Na4TDC-hard carbon composite can further acquire improved capacity and cycling stability for 1200 cycles even with a high mass loading of up to 20 mg *** pairing with a thick Na3V2（PO4）3cathode (20.6 mg cm-2),the as-fabricated full cell exhibited high operating voltage （2.8 V）,excellent rate performance and cycling stability with a high capacity retention of 88.7% after 200 cycles,well highlighting the Na4TDC anode material for SIBs.

关键词： Organic anode material Low redox potential Composite anode Sodium-ion batteries

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基于双目视觉和改进YOLOv8n的火灾检测及测距方法

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陕西科技大学学报 2025年第1期43卷 152-160页

作者：刘振董绍江罗家元孙世政潘学娇重庆交通大学机电与车辆工程学院重庆400074

针对火灾检测出现的漏检误检、模型参数量大及定位困难的问题,基于双目视觉和改进YOLOv8n提出了一种轻量化火灾检测及测距方法.通过双目相机拍摄图片,使用改进的检测算法YOLOv8n-AEM和现有的测距算法SGBM进行检测和测距.首先,在主干网... 详细信息

针对火灾检测出现的漏检误检、模型参数量大及定位困难的问题,基于双目视觉和改进YOLOv8n提出了一种轻量化火灾检测及测距方法.通过双目相机拍摄图片,使用改进的检测算法YOLOv8n-AEM和现有的测距算法SGBM进行检测和测距.首先,在主干网络中引入可变核卷积AKConv和EMA注意力机制,通过构建不规则卷积核有效提取火灾的特征;然后,在颈部网络中构建C2f-SCConv模块,通过特征重组降低模型参数,提高检测速度;其次,基于最小点距离改进损失函数,解决火源与光源重叠导致的漏检与误检问题;最后,增加小目标检测头,提高对小火苗的检测能力.实验结果表明,改进后的检测算法P、R、mAP分别为83.6%、76.4%、83.6%,分别提高了2.5%、3.6%、4.8%;参数量和模型大小分别为2.54 M和5.1 MB,分别降低了15.3%和15%;测距精度误差不超过2.5%,证明改进的方法能准确完成火灾的检测及测距.

关键词：火灾检测双目视觉测距 YOLOv8n 轻量化

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Deubiquitinases as pivotal regulators of T cell functions

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Frontiers of Medicine 2018年第4期12卷 451-462页

作者： Xiao-dong Yang shao-Cong Sun Shanghai Institute of Immunology Shanghai Jiao Tong University School of Medicine Shanghai 200025 China Department of Immunology The University of Texas MD Anderson Cancer Center 7455 Fannin Street Box 902 Houston TX 77030 USA The University of Texas Graduate School of Biomedical Sciences at Houston Houston TX 77030 USA

T cells efficiently respond to foreign antigens to mediate immune responses against infections but are tolerant to self-tissues. Defect in T cell activation is associated with severe immune deficiencies, whereas aberrant T cell activation contributes to the pathogenesis of diverse autoimmune and inflammatory diseases. An emerging mechanism that regulates T cell activation and tolerance is ubiquitination, a reversible process of protein modification that is counter-regulated by ubiquitinating enzymes and deubiquitinases （DUBs）. DUBs are isopeptidases that cleave polyubiquitin chains and remove ubiquitin from target proteins, thereby controlling the magnitude and duration of ubiquitin signaling. It is now well recognized that DUBs are crucial regulators of T cell responses and serve as potential therapeutic targets for manipulating immune responses in the treatment of immunological disorders and cancer. This review will discuss the recent progresses regarding the functions of DUBs in T cells.

关键词： deubiquitinase ubiquitination T cell activation T cell differentiation T cell tolerance

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Experimental study of non-uniform bubbles in a plume

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Journal of Hydrodynamics 2022年第1期34卷 116-124页

作者： Xin-wei Ye Hao-jie Zhou dong-dong shao Xiao-jing Niu State Key Laboratory of Hydroscience and Engineering Department of Hydraulic EngineeringTsinghua UniversityBeijing100084China State Key Laboratory of Water Environment Simulation School of EnvironmentBeijing Normal UniversityBeijing100875China

The bubble plume is an important flow phenomenon, ubiquitous in many fields. The non-uniform bubbles in a plume are often simply considered as uniform and moving with a same slip velocity in an integral model. This study aims to have a better understanding of the behavior of the non-uniform bubbles in a plume. A set of experiments are conducted in a transparent water tank, in which the air plumes are generated through different injectors to vary the spectrum of the bubble size. The shadow images of the bubbles are simultaneously recorded with the illumination of a plane backlight. The algorithm used in the image analysis for tracing the bubbles is a newly developed multi-frame method based on the predictor-corrector method, with a good accuracy in estimating the size and the velocity of the overlapped bubbles based on the bubble shadow images. The bubbles are divided into several groups by their equivalent diameters with an interval of 0.5 mm. The spectrums of the bubble size and the void fraction are measured. It is found that the bubbles of different sizes show different dynamics features, resulting in a difference in the radial distribution. It is shown that the large bubbles gather in the center of the plume, while the medium bubbles spread the widest and even wider than the small bubbles. The difference can be explained by the effects of the transverse lift force and the amplitude of the bubble oscillation.

关键词： Bubble plume experiment image analysis bubble size transverse lift force

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Corrosion inhibition of stainless steel by a sulfate-reducing bacteria biofilm in seawater

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International Journal of Minerals,Metallurgy and Materials 2012年第8期19卷 717-725页

作者： Fu-shao Li Mao-zhong An dong-xia Duan School of Chemistry and Chemical Engineering Qujing Normal University Qujing 655011 China State Key Laboratory for Marine Corrosion and Protection Qingdao 266071 China Chemical Engineering School Harbin Institute of Technology Harbin 150001 China

Corrosion inhibition of stainless steel due to a sulfate-reducing bacteria （SRB） biofilm in seawater was studied. By atomic force microscopy, a layer of fish-scale-like biofilm was found to form as stainless steel coupons were exposed to the culture media with SRB, and this biofilm grew more and more compact. As a result, coupons＇ surface under the biofilm turned irregular less slowly than that exposed to the sterilized culture media. Then, physicoelectric characteristics of the electrode/biofilrn/solution interface were investigated by electro- chemical impedance spectroscopy （EIS）, and the coverage of the biofilm as well as the relative irregularity of coupons＇ surface was also re- corded by EIS spectra.. Finally, anodic cyclic polarization results further demonstrated the protective property of the biofilm. Therefore, in es- timation of SRB-implicated corrosion of stainless steel, not only the detrimental SRB metabolites but also the protective SRB biofilm as well should be taken into account.

关键词： stainless steel corrosion prevention microbiology microorganisms biofilms electrochemistry

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