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Gradient‑Layered MXene/Hollow Lignin Nanospheres Architecture Design for Flexible and Stretchable Supercapacitors

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Nano-Micro Letters 2025年第2期17卷 447-462页

作者： Haonan zhang Cheng Hao Tongtong Fu dian Yu Jane Howe Kaiwen Chen Ning Yan Hao Ren Huamin Zhai Jiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass Materials NanJing Forestry UniversityNanjing 210037People’s Republic of China Department of Chemical engineering and Applied Chemistry University of Toronto200 College StreetTorontoON M5S 3E5Canada Department of Materials Science and engineering University of Toronto184 College StreetTorontoON M5S 3E4Canada College of Materials Science and engineering Nanjing Forestry UniversityNanjing 210037People’s Republic of China

With the rapid development of flexible wearable electronics,the demand for stretchable energy storage devices has *** this work,a novel gradient-layered architecture was design based on single-pore hollow lignin nanospheres(HLNPs)-intercalated two-dimensional transition metal carbide(Ti_(3)C_(2)T_(x) MXene)for fabricating highly stretchable and durable *** depositing and inserting HLNPs in the MXene layers with a bottom-up decreasing gradient,a multilayered porous MXene structure with smooth ion channels was constructed by reducing the overstacking of MXene ***,the micro-chamber architecture of thin-walled lignin nanospheres effectively extended the contact area between lignin and MXene to improve ion and electron accessibility,thus better utilizing the pseudocapacitive property of *** these strategies effectively enhanced the capacitive performance of the *** addition,HLNPs,which acted as a protective phase for MXene layer,enhanced mechanical properties of the wrinkled stretchable electrodes by releasing stress through slip and deformation during the stretch-release cycling and greatly improved the structural integrity and capacitive stability of the *** electrodes and symmetric flexible all-solid-state supercapacitors capable of enduring 600%uniaxial tensile strain were developed with high specific capacitances of 1273 mF cm^(−2)(241 F g^(−1))and 514 mF cm^(−2)(95 F g^(−1)),***,their capacitances were well preserved after 1000 times of 600%stretch-release *** study showcased new possibilities of incorporating biobased lignin nanospheres in energy storage devices to fabricate stretchable devices leveraging synergies among various two-dimensional nanomaterials.

关键词： Hollow lignin nanospheres MXene Gradient-layered architecture Wrinkled electrodes Stretchable supercapacitors

碱激发高炉矿渣固化/稳定化Cr(VI)污染土试验研究

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岩土工程学报 2025年第1期47卷 57-64页

作者：张文杰金典郭兴璋李西斌台州学院建筑工程学院浙江台州318000 上海大学力学与工程科学学院上海200072 山东大学岩土与结构工程研究中心山东济南250061 浙江农林大学风景园林与建筑学院浙江杭州311300

碱激发高炉矿渣(GGBFS)替代水泥(PC)用于污染土固化处置,具有能耗低、碳排放少的特点,同时GGBFS中含的还原性硫可以将铬(Cr)从六价还原成三价,从而显著提高固化/稳定化效率。使用碱激发GGBFS固化/稳定化总Cr含量2000mg/kg(其中Cr(Ⅵ)121... 详细信息

碱激发高炉矿渣(GGBFS)替代水泥(PC)用于污染土固化处置,具有能耗低、碳排放少的特点,同时GGBFS中含的还原性硫可以将铬(Cr)从六价还原成三价,从而显著提高固化/稳定化效率。使用碱激发GGBFS固化/稳定化总Cr含量2000mg/kg(其中Cr(Ⅵ)1210mg/kg)的污染土,并与PC固化进行对比。通过浸出毒性、固定效率和无侧限抗压强度分析处理效果,借助pH、还原效率、化学形态、矿物成分和微观图像分析揭示了相关机理。结果表明,GGBFS固化污染土的Cr浸出浓度明显低于PC固化土,GGBFS掺量20%,养护龄期28 d时总Cr和Cr(Ⅵ)浸出浓度分别降至2.12,1.09 mg/L,满足填埋场进场浓度限值要求,且GGBFS固化污染土的强度明显高于PC固化土;还原效率分析表明,GGBFS中的S^(2-)可以有效地将Cr(Ⅵ)还原成Cr(Ⅲ),还原效率可达96.0%,从而很大程度上避免了Cr(Ⅵ)对水化过程的抑制作用,使用GGBFS固化/稳定化该含量的Cr(Ⅵ)污染土时不需额外添加还原剂;微观分析表明,与PC相比,GGBFS固化后更多不稳定态的Cr转化成稳定形态,Cr的迁移性显著降低,同时生成了更多水化凝胶,土颗粒胶结程度更高,因此具有更好的封固效果和更高强度。该研究为GGBFS固化/稳定化Cr(Ⅵ)污染土提供了科学依据。

关键词：粒化高炉矿渣 Cr(Ⅵ)污染土固化/稳定化浸出浓度还原效率

Population-influenced spatiotemporal pattern of natural disaster and social crisis in China, AD1–1910

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Science China Earth Sciences 2019年第7期62卷 1138-1150页

作者： Shengda zhang David dian zhang Department of Geography The University of Hong Kong School of Geographical Sciences Guangzhou University

Researchers mostly ascribe contemporary natural disaster and the concomitant social crisis to anomalous climate change or global warming. However, whether such a relationship is still valid in long-term historical settings remains doubtful. In this study, data obtained from historical records about natural calamities(flood and drought) and their social impacts(famine,cannibalism, and war) at provincial and decadal scales during AD1–1910 are applied to mathematical statistics such as correlation and regression analysis as well as spatial visualization. Also, the role of population in the nexus of meteorological catastrophes and human miseries is investigated. Results show that at the provincial scale, generally there is high consistency among different variables and most of them are clustered in eastern part of China, especially in the north. More in-depth examinations indicate regional disparities that variables account for higher proportion in the south during the later imperial era,which may be attributed to the southward movement of population center. At the decadal scale, drought is the primary contributor to famine and cannibalism, while severe or even out-of-control famine i.e. cannibalism is more likely to incur war than ordinary famine per se. Besides, population growth rate exerts its positive effect on natural hazards and food crises, whereas more wars bring population loss and relieve population stress despite the weak negative association. These findings supplement previous views and confirm that the distributions of disasters in ancient China are affected by population rather than climatic variability, which only determines the occurrence of disaster.

关键词： Natural disaster Social crisis Population Spatiotemporal pattern Historical China

Effect of nanosized NbC precipitates on hydrogen-induced cracking of high-strength low-alloy steel

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International Journal of Minerals,Metallurgy and Materials 2021年第2期28卷 249-256页

作者： en-dian Fan Shi-qi zhang Dong-han Xie Qi-yue Zhao Xiao-gang Li Yun-hua Huang Institution for Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China Key Laboratory of Advanced Materials(MOE) School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China Ningbo Institute of Material Technology&engineering Chinese Academy of SciencesNingbo 315201China

We investigated the effect of nanosized NbC precipitates on hydrogen-induced cracking(HIC)of high-strength low-alloy steel by conducting slow-strain-rate tensile tests(SSRT)and performing continuous hydrogen charging and fracture *** results reveal that the HIC resistance of Nb-bearing steel is obviously superior to that of Nb-free steel,with the fractured Nb-bearing steel in the SSRT exhibiting a smaller ratio of elongation reduction(Iδ).However,as the hydrogen traps induced by NbC precipitates approach hydrogen saturation,the effect of the precipitates on the HIC resistance *** speculate that the highly dispersed nanosized NbC precipitates act as irreversible hydrogen traps that hinder the accumulation of hydrogen at potential crack nucleation *** addition,much like Nb-free steel,the Nb-bearing steel exhibits both H-solution strengthening and the resistance to HIC.

关键词： nanosized NbC precipitates high-strength low-alloy steel hydrogen-induced cracking slow-strain-rate tensile,hydrogen charging

Gapless Genome Assembly of ZH8015 and Preliminary Multi-Omics Analysis to Investigate ZH8015's Responses Against Brown Planthopper Infestation

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Rice science 2024年第3期31卷 317-327,I0042-I0045页

作者： LI dian DUAN Wenjing LIU Qun’en WU Weixun ZHAN Xiaodeng SUN Lianping zhang Yingxin CHenG Shihua State Key Laboratory of Rice Biology and Breeding China National Rice Research InstituteHangzhou 310006China

Accurate genomic information is essential for advancing genetic breeding research in specific rice *** study presented a gapless genome assembly of the indica rice cultivar Zhonghui 8015(ZH8015)using Pac Bio HiFi,Hi-C,and ONT(Oxford Nanopore Technologies)ultra-long sequencing technologies,annotating 43037 gene ***,utilizing this genome along with transcriptomic and metabolomic techniques,we explored ZH8015's response to brown planthopper(BPH)*** transcriptomic sampling indicated significant changes in gene expression levels around 48 h after BPH *** analysis revealed particularly significant alterations in genes related to reactive oxygen species scavenging and cell wall *** results demonstrated marked increases in levels of several monosaccharides,which are components of the cell wall and dramatic changes in flavonoid *** association analysis identified differentially expressed genes associated with key metabolites,shedding light on ZH8015's response to BPH *** summary,this study constructed a reliable genome sequence resource for ZH8015,and the preliminary multi-omics results will guide future insect-resistant breeding research.

关键词： brown planthopper gapless genome genome assembly multi-omics Nilaparvata lugens rice

Algorithm Design and Application of Laminar Cooling Feedback Control in Hot Strip Mill

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Journal of Iron and Steel Research International 2012年第4期19卷 39-42页

作者： LIU en-yang zhang dian-hua SUN Jie PenG Liang-gui GAO Bai-hong SU Li-tao State Key Laboratory of Rolling and Automation Northeastern University Shenyang 110819 LiaoningChina Shenyang Machine Tool Co Ltd Shenyang 110004 Liaoning China Sales Company ofShougang Group Beijing 100043 China

Feedback control is one of the most important ways to improve coiling temperature control precision during laminar cooling *** cooling equipments of a hot strip mill and structure of the control system were *** control algorithm based on PI controller and that based on Smith predictor were designed and tested in a hot strip mill *** application shows that the feedback control system based on PI controller plays a limited role in improving coiling temperature control *** feedback control system based on Smith predictor runs stable and *** the measured coiling temperature deviates from the target value,it can be adjusted to the required range quickly and steadily by Smith predictor feedback control,which improves the coiling temperature control precision greatly,and qualities of hot rolled strips are improved significantly

关键词： hot strip mill laminar cooling feedback control Smith predictor PI controller

Global Stability of a Viral Infection Model with Defectively Infected Cells and Latent Age

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Chinese Annals of Mathematics,Series B 2024年第4期45卷 555-572页

作者： Jianquan LI Yuming CHen Peijun zhang dian zhang School of Computer Science Xijing UniversityXi’an 710123China Department of Mathematics Wilfrid Laurier UniversityWaterlooON N2L 3C5Canada Corresponding author.Xi’an Key Laboratory of Human-Machine Integration and Control Technology for Intelligent Rehabilitation Xijing UniversityXi’an 710123China Equal contributor.Department of Immunology Xi’an Medical UniversityXi’an 710021China

The authors propose and analyze a viral infection model with defectively infected cells and age of the latently infected *** existence of steady states is determined by the basic reproduction number of *** the Lyapunov's direct method,they establish a threshold dynamics of the model with the basic reproduction number of virus as the threshold *** achieve it,a novel procedure is *** novelties are *** one hand,the coefficients involved in the specific forms of the used Lyapunov functionals for the two feasible steady states are determined by the same set of *** the other hand,for the infection steady state,a new approach is proposed to check whether the derivative of the Lyapunov functional candidate along solutions is negative(semi-)definite or *** procedure not only simplifies the analysis but also exhibits the relationship between the two Lyapunov functionals for the two feasible steady ***,the procedure is expected to be applicable for other similar models.

关键词： Viral infection model Basic reproduction number Equilibrium Global stability Lyapunov direct method Age structure

B_(111),B_(112),_(B113),and B_(114):The most stable core-shell borospherenes with an icosahedral B_(12) core at the center exhibiting superatomic behaviors

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Nano Research 2021年第12期14卷 4719-4724页

作者： Min zhang Hai-Gang Lu Si-dian Li Institute of Molecular Science Shanxi UniversityTaiyuan030006China

Boron allotropes are known to be predominately constructed by icosahedral B_(12) cages,while icosahedral-B_(12) stuffing proves to effectively improve the stability of fullerene-like boron nanoclusters in the size range between B_(98)–B_(102).However,the thermodynamically most stable core-shell borospherenes with a B_(12) icosahedron at the center still remains *** on the structural motif of D5h C_(70) and extensive first-principles theory calculations,we predict herein the high-symmetry C5v B111+(3)which satisfies the Wade’s n+1 and n+2 skeletal electron counting rules exactly and the approximately electron sufficient Cs B_(111)(4),Cs B_(112)(5),Cs B_(113)(6),and Cs B_(114)(7)which are the most stable neutral core-shell borospherenes with a B_(12) icosahedron at the center reported to date in the size range between B_(68)–B_(130),with Cs B112(5)being the thermodynamically most favorite species in the *** orbital and bonding analyses indicate that these spherically aromatic species all contain a negatively charged icosahedral B_(122)−core at the center which exhibits typical superatomic behaviors in the electronic configuration of 1S21P61D101F8,with its dangling valences saturated by twelve radial B-B 2c-2eσbonds between the B_(12) inner core and the B_(70) outer *** infrared(IR)and Raman spectra of the concerned species are computationally simulated to facilitate their future characterizations.

关键词： first-principles theory borospherenes structures bonding superatomic behaviors spherical aromaticity

A Radio-Telemetry System for Navigation and Recording Neuronal Activity in Free-Roaming Rats

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Journal of Bionic engineering 2012年第4期9卷 402-410页

作者： dian zhang Yanling Dong Megan Li Houjun Wang School of Automation engineering University of Electronic Science and Technology of China Chengdu 611731 P. R. China School of Medicine Qingdao University Qingdao 266071 P R. China Shandong Eye Institute Qingdao 266071 P. R. China Zanvyl Krieger School of Arts and Sciences The Johns Hopkins University Baltimore 21218 USA

A radio-telemetry recording system is presented which is applied to stimulate specific brain areas and record neuronal ac- tivity in a free-roaming rat. The system consists of two major parts： stationary section and mobile section. The stationary section contains a laptop, a Micro Control Unit （MCU）, an FM transmitter and a receiver. The mobile section is composed of the headstage and the backpack （which includes the mainboard, FM transmitter, and receiver）, which can generate biphasic mi- crocurrent pulses and simultaneously acquire neuronal activity. Prior to performing experiments, electrodes are implanted in the Ventral Posterolateral （VPL） thalamic nucleus, primary motor area （M1） and Medial Forebrain Bundle （MFB） of the rat. The stationary section modulates commands from the laptop for stimulation and demodulates signals for neuronal activity recording. The backpack is strapped on the back of the rat and executes commands from the stationary section, acquires neuronal activity, and transmits the neuronal activity singles of the waking rat to the stationary section. All components in the proposed system are commercially available and are fabricated from Surface Mount Devices （SMD） in order to reduce the size （25 mm×15 mm ×2 mm） and weight （10 g with battery）. During actual experiments, the backpack, which is powered by a rechargeable Lithium battery （4 g）, can generate biphasic microcurrent pulse stimuli and can also record neuronal activity via the FM link with a maximum transmission rate of 1 kbps for more than one hour within a 200 m range in an open field or in a neighboring chamber. The test results show that the system is able to remotely navigate and control the rat without any prior training, and acquire neuronal activity with desirable features such as small size, low power consumption and high precision when compared with a commercial 4-channel bio-signal acquisition and processing system.

关键词： bio-robot radio-telemetry microcurrent stimulation navigation neuronal activity recording