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Molecular packing tuning via chlorinated end group enables efficient binary organic solar cells over 18.5%

Carbon Energy 2024年第3期6卷 196-203页

作者： Yafeng Li Zhenyu Chen Xingzheng Yan ziyi Ge Zhejiang Business Technology Institute NingboZhejiangChina Zhejiang Engineering Research Center for Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingboZhejiangChina Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijingChina

Designing novel nonfullerene acceptors(NFAs)is of vital importance for the development of organic solar cells(OSC).Modification on the side chain and end group are two powerful tools to construct efficient ***,based on the high-performance L8BO,we selected 3-ethylheptyl to substitute the inner chain of 2-ethylhexyl,obtaining the backbone of *** we introduced different halogen atoms of fluorine and chlorine on 2-(3-oxo-2,3-dihydro-1Hinden-1-ylidene)malononitrile end group(EG)to construct efficient NFAs named BON3-F and BON3-Cl,*** donor D18 was chosen to combine with two novel NFAs to construct OSC ***,D18:BON3-Cl-based device shows a remarkable power conversion efficiency(PCE)of 18.57%,with a high open-circuit voltage(V_(OC))of 0.907 V and an excellent fill factor(FF)of 80.44%,which is one of the highest binary PCE of devices based on D18 as the ***,BON3-F-based device shows a relatively lower PCE of 17.79%with a decreased FF of 79.05%.The better photovoltaic performance is mainly attributed to the red-shifted absorption,higher electron and hole mobilities,reduced charge recombination,and enhanced molecular packing in the D18:BON3-Cl ***,we performed stability tests on two binary systems;the D18:BON3-Cl and D18:BON3-F devices maintain 88.1%and 85.5%of their initial efficiencies after 169 h of storage at 85°C in an N2-filled glove box,*** work demonstrates the importance of selecting halogen atoms on EG and provides an efficient binary system of D18:BON3-Cl for further improvement of PCE.

关键词： binary organic solar cell chlorinated end group molecular packing

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Doped holographic superconductors in the Gubser–Rocha model

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Communications in Theoretical Physics 2024年第4期76卷 80-92页

作者： ziyi Zhao Wenhe Cai Shuta Ishigaki Department of Physics Shanghai UniversityShanghai 200444China Shanghai Key Laboratory of High Temperature Superconductors Department of PhysicsShanghai UniversityShanghai 200444China

We construct a doped holographic superconductor in the Gubser–Rocha model,and realize a superconducting dome in the middle of the temperature-doping phase *** is worth noting that unlike in previous research,the profile of our dome shrinks inward near to zero *** the numerical observation for the coupling dependence of the phase diagram,we find that the coupling between the two gauge fields plays a crucial role in the formation of the *** also analytically calculate the DC conductivity of the normal phase of the system in the momentum dissipation and obtain resistivity which is proportional to the *** AC conductivity is calculated numerically.

关键词： AdS-CFT correspondence High-Tc superconductor AC/DC conductivities Gubser-Rocha geometry

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Cancer cachexia:Focus on cachexia factors and inter-organ communication

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Chinese Medical Journal 2024年第1期137卷 44-62页

作者： Yongfei Wang Zikai Dong ziyi an Weilin Jin The First Clinical Medical College of Lanzhou University LanzhouGansu 730000China Institute of Cancer Neuroscience Medical Frontier Innovation Research CenterThe First Hospital of Lanzhou UniversityThe First Clinical Medical College of Lanzhou UniversityLanzhouGansu 730000China

Cancer cachexia is a multi-organ syndrome and closely related to changes in signal communication between organs,which is mediated by cancer cachexia *** cachexia factors,being the general name of inflammatory factors,circulating proteins,metabolites,and microRNA secreted by tumor or host cells,play a role in secretory or other organs and mediate complex signal communication between organs during cancer *** cachexia factors are also a potential target for the diagnosis and *** pathogenesis of cachexia is unclear and no clear effective treatment is ***,the treatment of cancer cachexia from the perspective of the tumor ecosystem rather than from the perspective of a single molecule and a single organ is urgently *** the point of signal communication between organs mediated by cancer cachexia factors,finding a deeper understanding of the pathogenesis,diagnosis,and treatment of cancer cachexia is of great significance to improve the level of diagnosis and *** review begins with cancer cachexia factors released during the interaction between tumor and host cells,and provides a comprehensive summary of the pathogenesis,diagnosis,and treatment for cancer cachexia,along with a particular sight on multi-organ signal communication mediated by cancer cachexia *** summary aims to deepen medical community’s understanding of cancer cachexia and may conduce to the discovery of new diagnostic and therapeutic targets for cancer cachexia.

关键词： Cancer cachexia Cancer cachexia factors Inter-organ communication Tumor ecosystem Tumor microenvironment

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Multi-UAV cooperative maneuver decision-making for pursuitevasion using improved MADRL

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Defence Technology（防务技术） 2024年第5期35卷 187-197页

作者： Delin Luo Zihao Fan ziyi Yang Yang Xu School of Aerospace Engineering Xiamen UniversityXiamen 361102China School of Civil Aviation Northwestern Polytechnical UniversityXi'an 710072China

Aiming at the problem of multi-UAV pursuit-evasion confrontation, a UAV cooperative maneuver method based on an improved multi-agent deep reinforcement learning(MADRL) is proposed. In this method, an improved Comm Net network based on a communication mechanism is introduced into a deep reinforcement learning algorithm to solve the multi-agent problem. A layer of gated recurrent unit(GRU) is added to the actor-network structure to remember historical environmental states. Subsequently,another GRU is designed as a communication channel in the Comm Net core network layer to refine communication information between UAVs. Finally, the simulation results of the algorithm in two sets of scenarios are given, and the results show that the method has good effectiveness and applicability.

关键词： Reinforcement learning UAV Maneuver decision GRU Cooperative control

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CO_(2)-switched porous metal-organic framework magnets

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Chinese Journal of Structural Chemistry 2024年第2期43卷 4-5页

作者： ziyi Zhu Yang Cao Jun Zhang College of Chemistry and Molecular Sciences Wuhan UniversityWuhan430072China School of Microelectronics Hubei UniversityWuhan430062China

Magnetic materials play a crucial role in modem industrial and technological *** to traditional magnets,metal-organic framework magnets offer greater adjustability and the design ability at molecular *** these,the porous magnet with suffi-cient building blocks may combine porosity and magnetic ordering,thus garnering numerous interests for their ability to change their physical properties in response to external stimuli(such as electric field,light,temperature and molecular guests like solvents and gas molecules).Using such gas molecules as a means to regulate the magnetic properties of porous magnet is particularly promising due to their fast response speed and reversible adsorption/desorption *** pore structure and surface chemistry of porous magnet can be tailored to achieve selective responses to different gases(Fig.1).

关键词： porous magnets switched

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Coherence analysis of noise-like pulses generated by an erbium-doped fiber mode-locked laser

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Optoelectronics Letters 2024年第4期20卷 205-210页

作者： ZHANG ziyi WANG Chuncan LI Jing WANG Peng Key Laboratory of All Optical Network and Advanced Telecommunication Network Ministry of EducationInstitute of Lightwave TechnologyBeijing Jiaotong University Beijing 100044China

The noise-like pulses(NLPs)with tunable fraction of the pedestal height in the whole intensity autocorrelation(AC)trace are numerically demonstrated in the designed erbium-doped fiber(EDF)mode-locked laser,which contains the saturable absorber(SA)with nonlinear polarization rotation(NPR),sinusoidal-shaped or Gaussian-shaped filter,two segments of EDFs,and two pieces of single-mode fibers(SMFs)with normal dispersion and anomalous dispersion,*** pedestal ratio of the intensity AC trace can be tuned by changing the gain saturation energies of *** results show that when the net cavity dispersion is 1.06 ps^(2),the tuning range of the pedestal ratio for the NLPs can reach its maximum values,which are 0.51—0.89 and 0.58—0.88 for the sinusoidal-shaped and Gaussian-shaped filters,*** addition,an appropriate choice of filter bandwidth is also conducive to obtain a wide range of the tuning pedestal ratio for the intensity AC trace.

关键词： fiber tuning polarization

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A Knowledge-enhanced Two-stage Generative Framework for Medical Dialogue Information Extraction

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Machine Intelligence Research 2024年第1期21卷 153-168页

作者： Zefa Hu ziyi Ni Jing Shi Shuang Xu Bo Xu School of Artificial Intelligence University of Chinese Academy of SciencesBeijing 100049China Institute of Automation Chinese Academy of SciencesBeijing 100190China

This paper focuses on term-status pair extraction from medical dialogues(MD-TSPE),which is essential in diagnosis dia-logue systems and the automatic scribe of electronic medical records(EMRs).In the past few years,works on MD-TSPE have attracted increasing research attention,especially after the remarkable progress made by generative ***,these generative methods output a whole sequence consisting of term-status pairs in one stage and ignore integrating prior knowledge,which demands a deeper un-derstanding to model the relationship between terms and infer the status of each *** paper presents a knowledge-enhanced two-stage generative framework(KTGF)to address the above *** task-specific prompts,we employ a single model to com-plete the MD-TSPE through two phases in a unified generative form:We generate all terms the first and then generate the status of each generated *** this way,the relationship between terms can be learned more effectively from the sequence containing only terms in the first phase,and our designed knowledge-enhanced prompt in the second phase can leverage the category and status candidates of the generated term for status ***,our proposed special status"not mentioned"makes more terms available and en-riches the training data in the second phase,which is critical in the low-resource *** experiments on the Chunyu and CMDD datasets show that the proposed method achieves superior results compared to the state-of-the-art models in the full training and low-re-sourcesettings.

关键词： Medical dialogue understanding information extraction text generation knowledge-enhanced prompt low-resource setting dataaugmentation

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Interdecadal change and projection of the relationship between spring Arctic Oscillation and summer precipitation in the Yangtze River valley in CMIP6 models

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Atmospheric and Oceanic Science Letters 2024年第4期17卷 15-22页

作者： Weikai Jia Botao Zhou ziyi Song Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters/Key Laboratory of Meteorological Disaster Ministry of Education/Joint International Research Laboratory of Climate and Environment ChangeNanjing University of Information Science and TechnologyNanjingChina

评估了20个CMIP6模式对春季北极涛动(AO)与长江流域夏季降水(YRP)关系的模拟能力.结果表明, 4个模式(ACCESS-ESM1-5, CMC-CM2-SR5, MRI-ESM2-0, NorESM2-LM))能合理模拟出1990年代后期AO-YRP关系的减弱. 1980-1998年,当春季AO位于正位相时,夏季东亚急流北移,长江流域为异常下沉运动,同时西太平洋副热带高压减弱,减少向长江流域的水汽输送,结果导致降水减少. 1999-2014年,上述大气环流与春季AO的联系不显著,从而减弱AO-YRP的关系.利用这四个模式进一步预估了RCP4.5情景下2015-2100年期间AO-YRP的关系.两者在2015-2040年为显著负相关关系,随后再次减弱.

关键词：北极涛动降水长江流域年代际变化 CMIP6

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A Non-Parametric Scheme for Identifying Data Characteristic Based on Curve Similarity Matching

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IEEE/CAA Journal of Automatica Sinica 2024年第6期11卷 1424-1437页

作者： Quanbo Ge Yang Cheng Hong Li ziyi Ye Yi Zhu Gang Yao School of Automation Nanjing University of Information Science&TechnologyJiangsu Provincial University Key Laboratory of Big Data Analysis and Intelligent SystemsNanjing University of Information Science&Technologyand the Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET)Nanjing University of Information Science&TechnologyNanjing 210044China School of Department of Logistics Engineering Shanghai Maritime UniversityShanghai 201306China China Classification Society Nantong Office Nantong 226006China Chinese Flight Test Establishment Xi’an 710089China School of Mathematics Tsinghua UniversityBeijing 100084China School of Automation Nanjing University of Information Science&TechnologyNanjing 210044China Department of Logistics Engineering Shanghai Maritime UniversityShanghai 201306China IEEE

For accurately identifying the distribution charac-teristic of Gaussian-like noises in unmanned aerial vehicle(UAV)state estimation,this paper proposes a non-parametric scheme based on curve similarity *** the framework of the pro-posed scheme,a Parzen window(kernel density estimation,KDE)method on sliding window technology is applied for roughly esti-mating the sample probability density,a precise data probability density function(PDF)model is constructed with the least square method on K-fold cross validation,and the testing result based on evaluation method is obtained based on some data characteristic analyses of curve shape,abruptness and *** com-parison simulations with classical methods and UAV flight exper-iment shows that the proposed scheme has higher recognition accuracy than classical methods for some kinds of Gaussian-like data,which provides better reference for the design of Kalman filter(KF)in complex water environment.

关键词： Curve similarity matching Gaussian-like noise non-parametric scheme parzen window.

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A self-centering and stiffness-controlled MEMS accelerometer

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Microsystems & Nanoengineering 2024年第1期10卷 27-40页

作者： Yiming Jin Zhipeng Ma ziyi Ye Mingkang Li Xudong Zheng Zhonghe Jin School of Aeronautics and Astronautics Zhejiang UniversityHangzhou 310013China Key Laboratory of Micro/Nano-Satellite Research of Zhejiang Province Hangzhou 310007PR China

This paper presents a high-performance MEMS accelerometer with a DC/AC electrostatic stiffness tuning capability based on double-sided parallel plates(DSPPs).DC and AC electrostatic tuning enable the adjustment of the effective stiffness and the calibration of the geometric offset of the proof mass,respectively.A dynamical model of the proposed accelerometer was developed considering both DC/AC electrostatic tuning and the temperature *** on the dynamical model,a self-centering closed loop is proposed for pulling the reference position of the forceto-rebalance(FTR)to the geometric center of *** self-centering accelerometer operates at the optimal reference position by eliminating the temperature drift of the readout circuit and nulling the net electrostatic tuning *** stiffness closed-loop is also incorporated to prevent the pull-in instability of the tuned low-stiffness accelerometer under a dramatic temperature ***-time adjustments of the reference position and the DC tuning voltage are utilized to compensate for the residue temperature drift of the proposed *** a result,a novel controlling approach composed of a self-centering closed loop,stiffness-closed loop,and temperature drift compensation is achieved for the accelerometer,realizing a temperature drift coefficient(TDC)of approximately 7μg/℃ and an Allan bias instability of less than 1μg.

关键词： stiffness electrostatic centering

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