检索结果-南通市图书馆

居家痴呆老年人愉悦性活动参与情况及影响因素研究

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

中华护理杂志 2017年第5期52卷 524-529页

作者：王轶王志稳郝薇李小卫武杰北京大学护理学院北京市100191 北京市中关村医院北京大学第三医院

目的调查居家痴呆老年人愉悦性活动参与情况及影响因素。方法采用痴呆患者愉悦性活动量表,选取北京、广州及天津266例居家痴呆老年人进行问卷调查。结果研究对象愉悦性活动量表总得分为(14.0±6.7)分,4个维度得分由高到低依次为:感官刺... 详细信息

目的调查居家痴呆老年人愉悦性活动参与情况及影响因素。方法采用痴呆患者愉悦性活动量表,选取北京、广州及天津266例居家痴呆老年人进行问卷调查。结果研究对象愉悦性活动量表总得分为(14.0±6.7)分,4个维度得分由高到低依次为:感官刺激活动(0.9±0.5)分、家庭性活动(0.8±0.5)分、情感刺激活动(0.8±0.4)分、自主性活动(0.6±0.5)分。多元线性回归显示,痴呆老年人疾病越重、不伴随慢性病、文化程度越低、照顾者文化程度越低,其愉悦性活动总分越低,能解释总变异的41.1%。结论居家痴呆老年人感官刺激活动参与较好,家庭性活动和情感刺激活动次之,自主性活动较差。应指导照顾者根据痴呆老年人疾病严重度选择适当的愉悦性活动,改善其生活质量。

关键词：老年人痴呆愉悦性活动影响因素分析

维普期刊数据库

Low‑Temperature Fabrication of Stable Black‑Phase CsPbI_(3)Perovskite Flexible Photodetectors Toward Wearable Health Monitoring

在线全文

学校读者我要写书评

暂无评论

Nano-Micro Letters 2025年第3期17卷 232-245页

作者： Yingjie Zhao Yicheng Sun Chaoxin Pei Xing Yin Xinyi li Yi hao Mengru Zhang Meng Yuan Jinglin Zhou Yu Chen Yanlin Song College of Chemistry and Pingyuan Laboratory Zhengzhou UniversityZhengzhou 450001People’s Republic of China Key Laboratory of Green Printing Institute of ChemistryChinese Academy of SciencesBeijing 100190People’s Republic of China Key Laboratory of Bio‑Inspired Materials and Interfacial Science Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190People’s Republic of China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049People’s Republic of China

Flexible wearable optoelectronic devices fabricated fromorganic–inorganic hybrid perovskites significantly accelerate the developmentof portable energy,biomedicine,and sensing fields,but their poor thermal stabilityhinders further ***,all-inorganic perovskites possessexcellent thermal stability,but black-phase all-inorganic perovskite filmusually requires high-temperature annealing steps,which increases energy consumptionand is not conducive to the fabrication of flexible wearable *** this work,an unprecedented low-temperature fabrication of stable blackphaseCsPbI3perovskite films is demonstrated by the in situ hydrolysis reactionof diphenylphosphinic chloride *** released diphenyl phosphateand chloride ions during the hydrolysis reaction significantly lower the phasetransition temperature and effectively passivate the defects in the perovskitefilms,yielding high-performance photodetectors with a responsivity of 42.1 AW−1 and a detectivity of 1.3×10^(14)***,high-fidelity imageand photoplethysmography sensors are demonstrated based on the fabricated flexible wearable *** work provides a newperspective for the low-temperature fabrication of large-area all-inorganic perovskite flexible optoelectronic devices.

关键词： In situ hydrolyzation Low-temperature processing All-inorganic perovskite Flexible photodetectors Health monitoring

维普期刊数据库

Physical Layer Security Scheme With AoI-Awareness for Industrial IoT Based on Covert Communications

在线全文

学校读者我要写书评

暂无评论

IEEE/CAA Journal of Automatica Sinica 2025年第1期 276-278页

作者： Yaping li zhi-Xin liu Jia-Wei Su Ya-Zhou Yuan the Key Laboratory of Industrial Computer Control Engineering of Hebei Province Yanshan University

Dear Editor,Industrial Internet of things(IIoT) is a typical application of cyberphysical system(CPS). In the IIoT, wireless communication is an inevitable trend to replace the deployment-limited wired transmission for cases with large-scale and mobile devices. However, wireless communication gives rise to critical issues related to physical security, such as malicious detections and attacks [1].

关键词：

Effect of order–disorder transition on thermodynamic and electronic properties of σ and χ phases in W–Re alloy: the first-principles calculation

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Tungsten 2025年第1期7卷 195-213页

作者： zhi-Peng Zhu Dian Jia William Yi Wang Jun-Lei Yin Xing-Yu Gao Shu-Feng Yang Hai-Feng Song Jin-Shan li State Key Laboratory of Solidification Processing Northwestern Polytechnical University Laboratory of Computational Physics Institute of Applied Physics and Computational Mathematics School of Metallurgical and Ecological Engineering University of Science and Technology Beijing

The Tungsten-Rhenium(W-Re) alloys,celebrated for their high melting point,strength at elevated temperatures,electrical resistivity,and radiation resistance,have been widely utilized in high-temperature components,aerospace,electronics,and nuclear *** constituents of the topologically close-packed(TCP) phases,the sigma phase(σ) and chi phase(χ) formed within W-Re alloys wield considerable influence on the mechanical properties and the stability of the *** calculations were utilized in the present work to explore the structural,thermodynamic,and electronic properties of both ordered and disordered configurations within the σ and χ phases,culminating in a systematic elucidation of the higher phase stability exhibited by the ordered *** is found that the bulk modulus of these two phases is directly proportional to the concentration of Re in the alloy,while the equilibrium volume is inversely *** thermodynamic parameters of the σ and χ phases are calculated via the mean-field potential *** similar trends observed in the isobaric heat capacity,enthalpy increment,and entropy change curves for these two phases suggest they possess comparable thermodynamic *** is noteworthy that the contribution of ionic vibrations predominantly affects the isobaric heat capacity,while the contribution of thermal electronic excitations increases linearly with *** the structure and thermodynamic properties of TCP phases in W-Re alloys at low temperatures has profound significance for optimizing material performance,microstructures features,establishing theoretical foundations,and predicting material behavior.

关键词： First-principles calculations Phase stability TCP phases Thermodynamic properties W–Re alloy

Small modifications of endo-functionalized cavities lead to large changes in molecular interaction in water

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Science China Chemistry 2025年第1期68卷 369-376页

作者： Song-Meng Wang hao Nian Yan-Fang Wang li-Shuo Zheng Yu-Tao Zheng Yi-Wei Dong liping Huang Xiaoping Wang Wei Jiang liu-Pan Yang Department of Chemistry Southern University of Science and Technology School of Chemistry and Pharmaceutical Sciences State Key Laboratory for Chemistry and Molecular Engineering of Medicinal ResourcesGuangxi Normal University School of Pharmaceutical Science Hengyang Medical School University of South China

Studying molecular recognition in aqueous environments is crucial for understanding biological processes. Herein, we present a series of N-doped endo-functionalized anthracene-based cavities by introducing inward-directed pyridine units. The subtle modifications can significantly affect the binding properties of these receptors, which is similar to the mutations in biological systems. Combining theoretical calculations and molecular recognition experiments demonstrated that these “mutations” have an impact on the hydrophobicity and charge distribution of the hosts, consequently significantly influencing molecular *** is crucial for understanding the intricate mechanisms of molecular-level interactions in biological receptors.

关键词： host-guest interaction hydrophobic effect endo-functionalized cavity mutation pyridine

Deciphering the role of ultra-low-loaded rhodium in NiFe-MIL-53 for superior oxygen evolution reaction

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2025年第1期100卷 77-86页

作者： Jinzhi Jia Jinhua Zhang Kailu Guo Lanyue Zhang Gening Du hao You Junfeng Huang Mudong Tu Hua li Yong Peng Wei Dou Cailing Xu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical Engineering School of Materials and Energy Lanzhou University College of Chemistry and Chemical Engineering Luoyang Normal University

Designing highly active and stable electrocatalysts of oxygen evolution reaction （OER） is one of the crucial *** this study,a novel OER electrocatalyst,NiFe-MIL-53 modified with ultra-low rhodium（Rh@NiFe-MIL-53）,is successfully prepared via the hydrothermal ***-situ Raman spectroscopy and electrochemical impedance spectroscopy reveal that the doped Rh accelerates the phase transformation of NiFe-MIL-53 and the in-situ formed Rh@NiFeOOH is the actual active *** importantly,the enhanced reversibility of electrochemical reconstruction between NiFeOOH and NiFe（OH）2after doping Rh is beneficial for improving the electrochemical stability of the catalyst.X-ray photoelectron spectroscopy spectra show the strong electronic interaction between single-atom Rh and Ni/Fe in Rh@***,theoretical calculations confirm that the integration of single-atom Rh into the NiFeOOH successfully reduces the band gap,regulates the d-band center （εd）,accelerates the charge transfer,and optimizes the adsorption behavior of oxygen-containing intermediates,thereby lowering the energy barrier of rate-determining ***,the optimized Rh@NiFe-MIL-53 exhibits excellent OER activity （240 mV） with a small Tafel slope of 48.2 mV dec-1and long-term durability (over1270 h at 10 m A cm-2and 110 h at 200 mA cm-2).This work presents a new perspective on designing highly efficient OER electrocatalysts.

关键词： X ray photoelectron spectroscopy

Controllably elevating the initial Coulombic efficiency of li3VO4 anode via a facile electrode pre-lithiation technique for lithium-ion batteries

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Science China Chemistry 2025年

作者： haoyue liang Xingguo Zhong Guxin Huang Wenpan liu Yao liu Shuhao Wang Deyu Wang hao liu hao Wang Tianyou Zhai Huiqiao li State Key Laboratory of Materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Shenzhen Research Institute of Huazhong University of Science and Technology Key Laboratory of Optoelectronic Chemical Materials and Devices (Ministry of Education) School of Optoelectronic Materials &Technology Jianghan University Centre for Clean Energy Technology Faculty of Science University of Technology Sydney Yichang Brunp Recycling Technology Co. Ltd.

li3VO4has been a promising insertion anode material for li-ion batteries,which has high theoretical capacity (up to～600 mAh g-1) and safe li insertion voltage （0.5–1 V ***/li+）.However,the low initial Coulombic efficiency （ICE） has always been the bottleneck limiting its ***,we propose a facile pre-lithiation method to controllably elevate the ICE by the post-treatment of the prepared li3VO4composite electrode based on an immersion *** this process,the whole electrode was immersed in the liquid li source,via which the ICE of the li3VO4electrode can be controllably elevated from 80%to over 100%within 5 min of *** than the traditional powder treatment for pre-lithiation,this process we proposed minimizes the impact of pre-lithiation on the battery assembly ***,we further investigated the effect of this pre-lithiation process on the functional components in the *** the first time the ICE of li3VO4electrode was elevated to 100%.As a result,the initial reversible capacity of liFePO4||li3VO4full cell was improved from 44.0 to146.3 m Ah g-1,demonstrating the feasibility and great potential of the process.

关键词：

Unveiling the relationship between Fabry-Perot laser structures and optical field distribution via symbolic regression

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Optoelectronics Letters 2025年第3期21卷 149-154页

作者： li Wenqiang WU Min li Weijun hao Meilan YU lina Ann Lab Institute of Semiconductors Chinese Academy of Sciences School of Electronic Electrical and Communication Engineering & School of Integrated Circuits University of Chinese Academy of Sciences Beijing Key Laboratory of Semiconductor Neural Network Intelligent Sensing and Computing Technology

In recent years, machine learning (ML) techniques have been shown to be effective in accelerating the development process of optoelectronic devices. However, as"black box"models, they have limited theoretical interpretability. In this work, we leverage symbolic regression (SR) technique for discovering the explicit symbolic relationship between the structure of the optoelectronic Fabry-Perot (FP) laser and its optical field distribution, which greatly improves model transparency compared to ML. We demonstrated that the expressions explored through SR exhibit lower errors on the test set compared to ML models, which suggests that the expressions have better fitting and generalization capabilities.

关键词：

Positive effect of Mo on mechanical properties of a Ni-42W-10Co-x Mo medium heavy alloy

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

China Foundry 2025年

作者： Guo-xin Cao Jian-xin Dong Yong-sheng He He Jiang Fang hao zhi-hua Nie Teng-fei Ma Bao-quan Fu School of Materials Science and Engineering University of Science and Technology Beijing Xi'an Superalloy Technology Co. Ltd. School of Materials Science and Engineering Beijing Institute of Technology Key Laboratory of Air-driven Equipment Technology of Zhejiang Province Quzhou University

In this study,a novel Ni-W-Co-Mo medium heavy alloy (MHA) was designed to improve its mechanical strength via Mo *** the Ni-42W-10Co-xM o alloy series,where x represents the weight percent of Mo and varies between 0,1,2,5,and 10,the microstructure transitions from a dendritic structure to a hypoeutectic structure as the Mo content increases from 0 to 5wt.%.Moreover,as the Mo content increases from 0to 10wt.%,the distribution of theμ-phase shifts from being individually dispersed to forming aggregates,and its volume fraction rises from 0.5%to 7.9%.Notably,theμ-phase evolves into an eutectic microstructure,which helps in minimizing the segregation of *** change is accompanied by a substantial enhancement in mechanical properties;specifically,the compressive yield strength at room temperature increases from 350 MPa to 646 MPa,indicating a significant 85%***,the microhardness increases from 230 HV to 304 *** dynamics simulations further reveal that the strengthening mechanism of Ni-42W-10Co-xM o alloys is Mo-induced solid solution strengthening and precipitation strengthening.

关键词：