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Transfer of Heavy Metals from Soils to Vegetables and Associated Human Health Risks at Selected Sites in Pakistan

Pedosphere 2018年第4期28卷 666-679页

作者： zahir ur rehman Sardar KHAN Mohammad Tahir SHAH Mark L.BRUSSEAU Said Akbar KHAN Jon MAINHAGU Department of Environmental Sciences University of Peshawar School of Earth and Environmental Sciences University of Arizona National Centre of Excellence in Geology University of Peshawar

Contamination of the food chain with heavy metals is considered as one of the major environmental pathways of human exposure to metals leading to potential health risks. This study aimed to investigate the concentrations of heavy metals such as copper （Cu）, zinc （Zn）, chromium （Cr）, nickel （Ni）, and manganese （Mn） in agricultural soils and food crops （fruit, leaf, and root vegetables）, and their associated health risks to the local population in selected southern districts of Khyber Pakhtunkhwa Province, Pakistan. The concentrations of the selected metals in soil varied over a wide range, in the following decreasing order： Mn 〉 Zn 〉 Cr 〉 Ni 〉 Cu. The bioaccunmlation of metals in vegetables was within the permissible risk limits, except for Cr which showed higher contamination in all the tested food crops. The trend of metal transfer factors for different vegetables was in the order of Cu 〉 Ni 〉 Cr 〉 Mn 〉 Zn, while the calculated daily intake of metals （DIM） in adults and children through consumption of food crops was in the decreasing order of Mn 〉 Zn 〉 Ni 〉 Cr 〉 Cu. The health risk index （HRI） values for the heavy metals for both adults and children were less than 1. Therefore, no significant health risk is anticipated for the local consumers through ingestion of these food crops.

关键词： contamination daily intake food crops metal accumulation metal pollution metal transfer factor risk index

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Hydrothermal synthesis of triangular CeCO3OH particles and photoluminescence properties

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Chinese Chemical Letters 2017年第3期28卷 663-669页

作者： Md.Hasan zahir Shamseldin A.Mohamed Mohammad Mizanur Rahman Ateeq ur rehman Center of Research Excellence in Renewable Energy Research Institute King Eahd University of Petroleum and Minerals Dhahran 31261 Saudi Arabia Center of Research Excellence in Nanotechnology King Fahd University of Petroleum and Minerals Dhahran 31261 Saudi Arabia Center of Research Excellence in Corrosion King Fahd University of Petroleum and Minerals Dhahran 31261 Saudi Arabia Center for Engineering Research King Fahd University of Petroleum and Minerals Dhahran 31261 Saudi Arabia

Ru/CeO_2[RC] and Ru/CeO_2/ethylene glycol（EG） [RCE] nanoparticles were produced by performing a simple hydrothermal reaction at 200℃ for 24 h and found to have two distinct morphologies. The RC nanoparticles are phase pureCeO_2; triangular highly crystallineCeCO_3OH nanoparticles are formed from the solution containing EG under the same hydrothermal reaction conditions at p H 8.5. EG plays an important role in the formation of the triangularCeCO_3OH nanoparticles. The polycrystallineCeCO_3OH nanoparticles retain their triangular structure even after calcination at 600℃in air but are transformed into a pureCeO_2 phase. The room temperature photoluminescence of the RC and RCE nanoparticles and of RCE calcined at 600℃[RCE-600] was also investigated. It was found that the high crystallinity triangular RCE-600 sample exhibits the highest photoluminescence intensity.

关键词： CeCO_3OH particles Ru/CeO_2 Ethylene glycol Hydrothermal process Luminescence

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Prospects and challenges of graphene based fuel cells

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Journal of Energy Chemistry 2019年第12期28卷 217-234页

作者： Muhammad zahir Iqbal Assad-ur rehman Saman Siddique Nanotechnology Research Laboratory Faculty of Engineering Sciences GIK Institute of Engineering Sciences and Technology

Novel characteristics of graphene have captured great attention of researchers for energy technology *** of graphene related hybrid and composite materials have demonstrated high performance and durability for fuel cell energy conversion *** article overviews graphene based materials for fuel cell technology applications such as electrodes additives,bipolar plates and proton conducting electrolyte *** graphene dispersion over electrodes has revealed enhanced exposure of electrochemically active surface area for improved electro-catalytic activity towards fuel oxidation and oxidant reduction *** issue of device stack durability and degraded performance due to corrosion of bipolar plates is discussed by incorporating graphene based *** proton exchange membrane devices,graphene as an electrolyte has shown an excellent performance towards high ionic conductivity and power *** graphene incorporation in fuel cell devices has exhibited commendable performance and has bright future for commercial applications.

关键词： Graphene Fuel cell Electro-catalyst Power density Durability

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Electron doping induced semiconductor to metal transitions in ZrSe2 layers via copper atomic intercalation

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Nano Research 2018年第9期11卷 4914-4922页

作者： zahir Muhammad Kejun Mu Haifeng Lv Chuanqiang Wu Zia ur rehman Muhammad Habib Zhe Sun Xiaojun Wu Li Song National Synchrotron Radiation Laboratory CAS Center for Excellence in Nanoscience CAS Key Laboratory of Strongly-coupled Quantum Matter Physics University of Science and Technology of China Hefei 230029 China CAS Key Laboratory of Materials for Energy Conservation Synergetic Innovation Centre of Quantum Information & Quantum Physics CAS Center for Excellence in Nanoscience and Department of Material Science and Engineering University of Science and Technology of China Hefei 230026 China

Atomic intercalation in two-dimensional （2D） layered materials can be used to engineer the electronic structure at the atomic scale and generate tuneable physical and chemical properties which are quite distinct in comparison with the pristine material. Among them, electron-doped engineering induced by intercalation is an efficient route to modulate electronic states in 2D layers. Herein, we demonstrate a semiconducting to metallic phase transition in zirconium diselenide （ZrSe2） single crystals via controllable incorporation of copper （Cu） atoms. Our angle resolved photoemission spectroscopy （ARPES） measurements and first-principles density functional theory （DFT） calculations dearly revealed the emergence of conduction band dispersion at the M/L point of the Brillouin zone due to Cu-induced electron doping in ZrSe2 interlayers. Moreover, electrical measurements in ZrSe2 revealed semiconducting behavior, while the Cu-intercalated ZrSe2 exhibited a linear current-voltage curve with metallic character. The atomic intercalation approach may have high potential for realizing transparent electron-doping systems for many specific 2D-based nanoelectronic applications.

关键词： layered materials phase transition angle resolved photoemission spectroscopy electron doping

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