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Effective removal of Sb(V)from aqueous solutions by micro-electrolysis with composite scrap iron-manganese as filler

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第6期25卷 516-524页

作者： Shangkun DING Saihua HUANG yiping zhang Yongchao ZHOU nstitute of Municipal Engineering Zhejiang UniversityHangzhou310058China Zhejiang University of Water Resources and Electric Power Hangzhou310018China

Micro-electrolysis(ME)technology is investigated for improving the efficiency of removal of pentavalent antimony(Sb(V))from the *** this study,an ME system composed of scrap iron filings,waste manganese fillings,and activated carbon(Fe-Mn-C ME)was used to efficiently remove Sb(V).The results proved that,compared with conventional iron-carbon micro-electrolysis(Fe-C ME),Fe-Mn-C ME significantly enhances the removal rate of Sb(V)when the hydraulic retention time is 10–24 *** Fe-Mn flocs produced by this system were analyzed using X-ray diffraction(XRD),energy-dispersive X-ray spectroscopy(EDS),X-ray photoelectron spectroscopy(XPS),and Brunauer-Emmett-Teller(BET)surface area analysis,which revealed that the flocs were mostly Mn-substituted FeOOH and had a relatively larger specific surface area,providing better adsorption ***,it was found that the removal rate of Sb(V)decreased as the iron-carbon mass ratio increased,while it first increased and then decreased as the manganese content *** reduction of Fe(III)was accelerated with an increase in the addition of manganese,leading to an increase in the concentration of Fe(II).The electron transfer and the formation of Fe(II)were facilitated by the potential difference between manganese and carbon,as well as by the formation of microcells between iron and manganese,which improved the reduction ability of Sb(V).From our thorough investigation and research,this is the first report that has proposed Fe-Mn-C ME for removing *** provides a novel approach and technological support for removing Sb(V)efficiently.

关键词： Antimony Iron Manganese Micro-electrolysis(ME) Electrochemistry Mechanism

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Association of psychological stress with wives’hypertension across over 10 million Chinese married female population aged 20-49 years

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Chinese Medical Journal 2024年第13期137卷 1583-1591页

作者： Zhenyan Zhao Jiajing Jia Xinyi Lyu Lihua zhang Yuanyuan Wang Yuan He Zuoqi Peng Ya zhang Hongguang zhang Qiaomei Wang Haiping Shen yiping zhang Donghai Yan Xu Ma Ying Yang State Key Laboratory of Cardiovascular Disease Department of CardiologyFuwai HospitalNational Center for Cardiovascular DiseaseChinese Academy of Medical Science and Peking Union Medical CollegeBeijing 100037China National Research Institute for Family Planning Beijing 100081China National Human Genetic Resources Center Beijing 102206China Graduate School of Peking Union Medical College Beijing 100730China Department of Maternal and Child Health National Health and Family Planning Commission of the PRCBeijing 100044China

Background:Psychological stress has been reported to be a potential risk factor for hypertension among females,but it remains unclear whether spousal chronic stress levels alter the risk of hypertension among *** examined the associations between stress within the family and hypertension among married ***:Reproductive-aged women who were planning for pregnancy and their husbands were recruited from the National Free Pre-pregnancy Checkup Projects(NFPCP)across 31 provinces in China in 2016 and *** stress of wives or husbands was measured with a 5-point Likert-type scale,and assessed from three domains:work/life-related stress,economic stress,and overall ***-adjusted logistic regression models were used to assess the associations between stress status and the prevalence of ***:Of 10,027,644 couples,261,098(2.60%)women had *** results showed that higher stress levels among themselves or their husbands were associated with a higher prevalence of hypertension in women(P_(for trend)<0.001).Compared with non-stressed participants,female participants with the highest stress themselves were at a greater risk of hypertension,with adjusted odds ratio(OR)of 1.31(95%confidence interval[CI]:1.25-1.37);and compared with participants whose husbands had no stress,those whose husbands had the highest stress level were at a higher risk of hypertension with adjusted OR of 1.24(95%CI:1.20-1.29).Moreover,compared with non-stressed status for both couples,only-wife-stressed,only-husband-stressed,and both-stressed couples were found to be significantly associated with increased risks of wives’hypertension,with adjusted ORs of 1.28(95%CI:1.25-1.31),1.19(95%CI:1.17-1.21),and 1.28(95%CI:1.26-1.31),***:Moderate to severe stress in both spouses might be associated with female hypertension prevalence,which highlights the importance of paying attention to the psychological stresses of couples within the f

关键词： Psychological stress Hypertension Occupational stress Life stress Financial stress

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Late Triassic Intracontinental Deformation of South Tianshan,Central Asia:Evidence from Syn-tectonic Sedimentation and Detrital Zircon Provenances of the Kuqa Depression

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Acta Geologica Sinica(English Edition) 2024年第3期98卷 548-568页

作者： QIN Xiang CHEN Xuanhua SHAO Zhaogang zhang yiping WANG Yongchao LI Bing SU He WANG Ye LIU Kui HAN Lele China Aero Geophysical Survey and Remote Sensing Center for Natural Resources Beijing 100083China Key Laboratory of Airborne Geophysics and Remote Sensing Geology MNRBeijing 100083China Chinese Academy of Geological Sciences Beijing 100037China School of Earth Sciences and Resources China University of Geosciences(Beijing)Beijing 100083China

The Tianshan range,a Paleozoic orogenic belt in Central Asia,has undergone multiple phases of tectonic activities characterized by the N-S compression after the early Mesozoic,including the far-field effects of the Cenozoic Indian-Asian ***,there are limited reports on the tectonic deformation and initiation of Triassic intracontinental deformation in the Tianshan *** this structural context is crucial for interpreting the early intracontinental deformation history of the Eurasian continent during the early *** strata and syn-tectonic sediments provide a rich source of information on tectonic activities and have been extensively used in the studies of orogenic *** on detail fieldwork conducted in this study,the middle-late Triassic Kelamayi Formation of the northern Kuqa Depression in the southern Tianshan fold-thrust belt has been identified as the typical syn-tectonic growth *** youngest detrital zircon component in two lithic sandstone samples from the bottom and top of the Kelamayi growth strata yielded U-Pb ages of 223.4±3.1 and 215.5±2.9 Ma,respectively,indicating that the maximum depositional age of the bottom and top of the Kelamayi growth strata is 226-220 and 218-212 *** geochronological distribution of detrital samples from the Early-Middle Triassic and Late Triassic revealed abrupt changes,suggesting a new source supply resulting from tectonic activation in the Tianshan *** coupling relationship between the syn-tectonic sedimentation of the Kelamayi Formation and the South Tianshan fold-thrust system provides robust evidence that the Triassic intracontinental deformation of the South Tianshan range began at approximately 226-220 Ma(during the Late Triassic)and ended at approximately 218-212 *** findings provide crucial constraints for understanding the intraplate deformation in the Tianshan range during the Triassic.

关键词： growth strata basin-mountain coupling Triassic Indosinian event Kuqa Depression South Tianshan

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Maternal Preconception Serum Alanine Aminotransferase Levels and Risk of Preterm Birth among Reproductive-Aged Women—China,2013-2017

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China CDC weekly 2024年第10期6卷 181-188,I0001页

作者： Chuanyu Zhao Jiajing Jia Hanbin Wu Qin Xu Xinyi Lyu Meiya Liu Xuan Hu Jueming Lei Yuzhi Deng Yuan He Yuanyuan Wang Zuoqi Peng Ya zhang Hongguang zhang Qiaomei Wang Haiping Shen yiping zhang Donghai Yan Ying Yang Xu Ma National Research Institute for Family Planning BeijingChina National Human Genetic Resources Center BeijingChina Graduate School of Peking Union Medical College BeijingChina Department of Epidemiology Fuwai HospitalNational Center for Cardiovascular DiseasesChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijingChina

Summary What is already known about this topic?The significance of maternal liver health concerning preterm birth(PTB)is well recognized;however,there is a gap in understanding the precise influence of preconception s... 详细信息

关键词： Serum precise concerning

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IMpower210:A phase Ⅲ study of second-line atezolizumab vs. docetaxel in East Asian patients with non-small cell lung cancer

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Chinese Journal of Cancer Research 2024年第2期36卷 103-113页

作者： Yi-Long Wu Shun Lu Gongyan Chen Jianxing He Jifeng Feng yiping zhang Liyan Jiang Hongming Pan Jianhua Chang Jian Fang Amy Cai Lilian Bu Jane Shi Jinjing Xia Guangdong Lung Cancer Institute Guangdong Provincial Key Laboratory of Translational Medicine in Lung CancerGuangdong Provincial People's Hospital&Guangdong Academy of Medical SciencesSouthern Medical UniversityGuangzhou 510080China Shanghai Lung Cancer Center Shanghai Chest HospitalSchool of MedicineShanghai Jiao Tong UniversityShanghai 200025China Department of Respiration Harbin Cancer HospitalHarbin Medical UniversityHarbin 150081China Department of Thoracic Oncology and Surgery the First Affliated Hospital of Guangzhou Medical UniversityGuangzhou 510120China Department of Medical Oncology Jiangsu Cancer HospitalNanjing 210009China Department of Medical Oncology Zhejiang Cancer HospitalHangzhou 330022China Department of Pulmonary Medicine Shanghai Chest HospitalShanghai Jiao Tong UniversityShanghai 200030China Department of Medical Oncology Sir Run Run Shaw HospitalZhejiang University School of MedicineHangzhou 310016China Department of Medical Oncology Shenzhen HospitalCancer Hospital of Chinese Academy of Medical SciencesShenzhen 518116China Department of Thoracic Oncology Beijing Cancer HospitalBeijing 100142China Product Development Shanghai Roche Pharmaceutical LtdShanghai 201203China

Objective: IMpower210(NCT02813785) explored the efficacy and safety of single-agent atezolizumab *** as second-line treatment for advanced non-small cell lung cancer(NSCLC) in East Asian ***: Key eligibility criteria for this phase Ⅲ, open-label, randomized study included age ≥18 years;histologically documented advanced NSCLC per the Union for International Cancer Control/American Joint Committee on Cancer staging system(7th edition);Eastern Cooperative Oncology Group performance status of 0 or 1;and disease progression following platinum-based chemotherapy for advanced or metastatic NSCLC. Patients were randomized 2:1 to receive either atezolizumab(1,200 mg) or docetaxel(75 mg/m^(2)). The primary study endpoint was overall survival(OS) in the intention-to-treat(ITT) population with wild-type epidermal growth factor receptor expression(ITT EGFR-WT) and in the overall ITT ***: Median OS in the ITT EGFR-WT population(n=467) was 12.3 [95% confidence interval(95% CI),10.3-13.8] months in the atezolizumab arm(n=312) and 9.9(95% CI, 7.8-13.9) months in the docetaxel arm[n=155;stratified hazard ratio(HR), 0.82;95% CI, 0.66-1.03]. Median OS in the overall ITT population was 12.5(95% CI, 10.8-13.8) months with atezolizumab treatment and 11.1(95% CI, 8.4-14.2) months(n=377) with docetaxel treatment(n=188;stratified HR, 0.87;95% CI, 0.71-1.08). Grade 3/4 treatment-related adverse events(TRAEs) occurred in 18.4% of patients in the atezolizumab arm and 50.0% of patients in the docetaxel ***: IMpower210 did not meet its primary efficacy endpoint of OS in the ITT EGFR-WT or overall ITT populations. Atezolizumab was comparatively more tolerable than docetaxel, with a lower incidence of grade3/4 TRAEs.

关键词： Atezolizumab East Asia non-small cell lung cancer programmed death-ligand 1 inhibitors monoclonal antibody

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基于分割环阵的CFRP分层缺陷超声全聚焦成像

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仪器仪表学报 2024年第1期45卷 200-210页

作者：杨宁陆铭慧张萍朱颖张毅萍南昌航空大学无损检测技术教育部重点实验室南昌330063 上海飞机制造有限公司上海201324

碳纤维复合材料在钻孔加工时易产生分层缺陷,分层缺陷严重影响了构件的力学性能,存在严重的安全隐患。针对碳纤维复合材料孔边分层缺陷的检测,提出一种基于分割环形阵列的1/4矩阵全聚焦成像方法。设计了R4×S8、R3×S12、R3×S16和R4×... 详细信息

碳纤维复合材料在钻孔加工时易产生分层缺陷,分层缺陷严重影响了构件的力学性能,存在严重的安全隐患。针对碳纤维复合材料孔边分层缺陷的检测,提出一种基于分割环形阵列的1/4矩阵全聚焦成像方法。设计了R4×S8、R3×S12、R3×S16和R4×S12四种分割环形阵列结构,通过数值仿真对比分析了各阵列的聚焦声场特点,最终确定分割环阵探头为5 MHz的R4×S12探头。使用该探头对碳纤维复合材料孔边分层试块的上层、中层、下层缺陷进行全矩阵采集,利用VTK工具包分别进行全矩阵三维成像和1/4矩阵三维成像。结果表明,1/4矩阵方法比全矩阵方法三维成像的缺陷对比度更高,1/4矩阵方法的缺陷尺寸表征误差更小,误差不超过6%。与全矩阵成像相比,1/4矩阵成像信噪比提升范围为3.43~7.61 dB,有效提升了图像质量。

关键词：分层缺陷全聚焦分割环形阵列 1/4矩阵三维成像

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脉冲激光改性碳纤维复合材料及其金属化研究

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表面技术 2024年第11期53卷 228-238页

作者：刘镜波张义萍邓超李龙义王楠樊勋中国电子科技集团公司第二十九研究所成都610036 中国空间技术研究院北京卫星制造厂有限公司北京100094

目的选择性地实现碳纤维复合材料(Carbon fiber reinforced plastic,CFRP)表面良好的导电性,满足它在共形天线上的应用。方法采用波长为1064 nm的纳秒脉冲激光器对惰性极高的CFRP表面进行表面改性处理,并结合化学镀铜技术,制备激光改性... 详细信息

目的选择性地实现碳纤维复合材料(Carbon fiber reinforced plastic,CFRP)表面良好的导电性,满足它在共形天线上的应用。方法采用波长为1064 nm的纳秒脉冲激光器对惰性极高的CFRP表面进行表面改性处理,并结合化学镀铜技术,制备激光改性碳纤维复合材料表面金属层。利用扫描电镜、X射线光电子能谱仪对改性后的材料表面进行表征,利用焊点拉脱方法表征金属层结合力。结果研究表明,激光能量密度越高,则CFRP基材表面树脂被去除得越多;激光搭接率越大,则碳纤维束表面越粗糙;在适当的激光能量密度(60 J/cm^(2))和横/纵向搭接率(50%)下,会产生大量的极性化学基团。当激光能量密度为10~100 J/cm^(2)、激光搭接率为0%时,CFRP表面镀铜层的结合强度为0.57~3.16 MPa,且激光能量密度与镀层结合强度呈正相关。当激光能量密度为60 J/cm^(2)、激光搭接率为−100%~90%时,CFRP表面镀铜层的结合强度为0.19~3.24 MPa,且激光搭接率与镀层结合强度呈正相关。结论脉冲红外纳秒激光在一定能量密度和搭接率的条件下,可改变碳纤维表面形貌、化学成分,实现金属层的制备。

关键词：脉冲激光红外纳秒表面改性碳纤维复合材料化学成分金属化

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信号重构中l_(1)-l_(2)极小化的等价模型理论研究

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重庆理工大学学报（自然科学） 2024年第5期38卷 210-215页

作者：谢挺刘昊张艺萍张望哲重庆理工大学理学院重庆400054

非凸l_(1)-l_(2)极小化方法是信号重构中最有效、最重要的模型之一,为研究信号恢复中极小化l_(1)-l_(2)重构的条件,从极小化l_(1)-l_(2)的定义出发,结合零空间的性质,基于对原优化模型中的目标函数进行松弛并利用相干性函数,推导出与原... 详细信息

非凸l_(1)-l_(2)极小化方法是信号重构中最有效、最重要的模型之一,为研究信号恢复中极小化l_(1)-l_(2)重构的条件,从极小化l_(1)-l_(2)的定义出发,结合零空间的性质,基于对原优化模型中的目标函数进行松弛并利用相干性函数,推导出与原优化问题等价的新目标函数。结合信号重构中限制等距性的充分性条件,得到了极小化l_(1)-l_(2)完全重构的充分性条件,并证明了在噪声情形下两类条件的等价性。

关键词：压缩感知信号重构零空间

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负风压作用下隐框玻璃幕墙承载行为和脱胶损伤实验研究

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上海交通大学学报 2024年第7期58卷 1130-1138页

作者：周练张凯徐涵王斐亮章一萍唐丽娜杨健四川省建筑设计研究院有限公司成都610000 四川省建筑工业化工程技术研究中心成都610000 上海交通大学海洋工程国家重点实验室上海200240 上海交通大学城市公共建筑与基础设施数字化运维重点实验室上海200240

隐框玻璃幕墙连接用的硅酮结构胶发生损伤导致玻璃面板坠落是当前幕墙服役过程中的常见问题.现有研究大多采用动力学方法对幕墙的脱胶损伤进行检测和评估,该方法通常需要额外施加荷载激励,且测量的动力响应数据易受环境影响,难以实现幕... 详细信息

隐框玻璃幕墙连接用的硅酮结构胶发生损伤导致玻璃面板坠落是当前幕墙服役过程中的常见问题.现有研究大多采用动力学方法对幕墙的脱胶损伤进行检测和评估,该方法通常需要额外施加荷载激励,且测量的动力响应数据易受环境影响,难以实现幕墙安全状态的可靠评估.为解决上述问题,提出在负风压作用下利用玻璃面板的挠度和转角对玻璃面板的脱胶损伤进行检测和评估的方法.首先,设计一系列隐框玻璃幕墙脱胶损伤实验,验证了在风荷载作用下利用挠度和转角对玻璃面板的安全状态进行检测的可行性;之后,基于实验结果构建了隐框玻璃幕墙安全风险监测评估系统,实现玻璃面板脱胶位置和数量的实时监测和快速识别.

关键词：隐框玻璃幕墙负风压挠度转角损伤监测

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海洋多糖基益生菌微胶囊的制备及应用研究进展

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食品工业科技 2024年第11期45卷 351-360页

作者：周烨琳郭洪辉洪专陈晖谢全灵张怡评张铭恩福州大学先进制造学院福建泉州362200 自然资源部第三海洋研究所海洋生物资源开发利用工程技术创新中心福建厦门361005 厦门海洋职业技术学院海洋生物学院福建厦门361100

益生菌具有多种益生功效,但其在加工、贮存或消化等过程中易受外界不利环境的影响而降低活性,利用微胶囊技术可以对益生菌起到良好的保护作用,减少或避免不利环境的影响。海洋多糖作为益生菌微胶囊壁材不仅能够提高益生菌的抗胁迫能力... 详细信息

益生菌具有多种益生功效,但其在加工、贮存或消化等过程中易受外界不利环境的影响而降低活性,利用微胶囊技术可以对益生菌起到良好的保护作用,减少或避免不利环境的影响。海洋多糖作为益生菌微胶囊壁材不仅能够提高益生菌的抗胁迫能力和稳定性,改善益生菌产品的感官特性,还能与益生菌产生协同作用增强治疗效果。本文分析了不同来源海洋多糖的种类和特性,并概述了海洋多糖基益生菌微胶囊的制备方法,同时阐述了海洋多糖基益生菌微胶囊在食品工业、生物医药、养殖饲料等领域的应用,以期为益生菌微胶囊的未来研究方向和海洋资源高值化利用提供一些参考。

关键词：海藻多糖海洋动物多糖海洋微生物多糖微胶囊益生菌

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