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Influences of chemical reactions on polysulfide reduction reaction process on promotor surface in Li-S batteries

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Nano Research 2024年第4期17卷 2712-2718页

作者： Yufeng Luo Zhenhan Fang Zixin hong Shaorong duan Haitao liu Hengcai wu Qunqing Li Yuegang zhang Shoushan Fan Wenhui duan Jiaping Wang tsinghua-Foxconn Nanotechnology Research Center Tsinghua UniversityBeijing 100084China Department of Physics Tsinghua UniversityBeijing 100084China laboratory of Computational Physics Institute of Applied Physics and Computational MathematicsBeijing 100088China Frontier science Center for Quantum information Tsinghua UniversityBeijing 100084China

Polar promotors have been proven effective in catalyzing the polysulfide(PS)reduction reaction(PSRR)process in lithium-sulfur(Li-S)***,the promotor surface tends to be poisoned due to the accumulation of insoluble discharging products of lithium disulfide(Li_(2)S_(2))and lithium sulfide(Li_(2)S)during Li-S battery ***,we investigate the detailed PSRR mechanism on the surface of manganese sulfides(MnS)as a representative promoter by performing in-situ Raman mapping *** catalytic ability of MnS enables thorough electrochemical reduction of PSs to Li_(2)S_(2) and Li_(2)S on the MnS *** generated Li_(2)S_(2) and Li_(2)S then adsorb the dissolved PSs via chemical reactions among sulfur species during the subsequent PSRR *** phenomenon mitigates promotor poisoning and continuously improves the reversible ***,the assembled Li-S cell demonstrates excellent electrochemical performance after introducing a conductive interlayer containing a thin piece of carbon nanotube film and MnS promotors.

关键词： promotors polysulfides chemical reactions catalytic ability in-situ Raman measurements

Regulating the conductance of tungsten diselenide by oxygen plasma and improving its electrical stability by encapsulation

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Nano Research 2024年第4期17卷 3253-3260页

作者： Zhaofang Cheng Shaodan He Shimin zhang Shijun duan Min Wang Ziyu liu Rong zhang Wenya Qiang Xudong zhang Minggang Xia MOE Key laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter School of PhysicsXi’an Jiaotong UniversityXi’an 710049China Department of Applied Physics School of PhysicsXi’an Jiaotong UniversityXi’an 710049China Shaanxi Province Key laboratory of Quantum information and Optoelectronic Quantum Devices School of PhysicsXi’an Jiaotong UniversityXi’an 710049China

Two-dimensional(2D)tungsten selenide(WSe_(2))is promising candidate material for future electronic applications,owing to its potential for ultimate device *** improving the electronic performance of WSe_(2)-based field-effect transistors(FETs),the modification of surface properties is *** this study,the seamless structural phase transition in WSe_(2) lattice is achieved by soft oxygen plasma,regulating the electrical conductance of WSe_(2)-based *** found that during the soft oxygen plasma treatment with optimal processing time,the generated oxygen ions can substitute some selenium atoms and thus locally modify the bond length,inducing 2H→1T phase transition in WSe_(2) with seamless *** mosaic structures have been proven to tailor the electronic structure and increase the hole carrier concentration inside WSe_(2),significantly increasing the channel conductance of WSe_(2) *** the further increase of the oxygen plasma treatment time,the creation of more selenium vacancy defects leads to the electronic doping,resulting in the reduction of *** from the hexagonal boron nitride(h-BN)encapsulation to interrupt the partial structural relaxation from 1T to 2H phase,our WSe_(2) FET exhibits high electronic stability with conductance of 6.8×10^(-4) S,which is about four orders of magnitude higher than 2H WSe_(2)(5.8×10^(-8) S).This study could further broaden the WSe_(2) FETs in applications for functionalization and integration in electronics.

关键词： tungsten selenide(WSe2) structural phase transition oxygen plasma conductance hexagonal boron nitride(h-BN)encapsulation

3D bioprinting of in vitro porous hepatoma models:establishment,evaluation,and anticancer drug testing

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Bio-Design and Manufacturing 2024年第2期7卷 137-152页

作者： Xiaoyuan Wang Zixian liu Qianqian duan Boye zhang Yanyan Cao Zhizhong Shen Meng Li Yanfeng Xi Jianming Wang Shengbo Sang Shanxi Key laboratory of Micro Nano Sensors and Artificial Intelligence Perception College of Electronic Information and Optical EngineeringTaiyuan University of TechnologyTaiyuan 030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan 030024China Shanxi Institute of 6D Artificial Intelligence Biomedical science Taiyuan 030031China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030024China Department of Pathology Shanxi Provincial Cancer HospitalTaiyuan 030024China General Hospital of Taiyuan Iron and Steel Company Taiyuan 030809China

Traditional tumor models do not tend to accurately simulate tumor growth in vitro or enable personalized treatment and are particularly unable to discover more beneficial targeted *** address this,this study describes the use of threedimensional(3D)bioprinting technology to construct a 3D model with human hepatocarcinoma SMMC-7721 cells(3DP-7721)by combining gelatin methacrylate(GelMA)and poly(ethylene oxide)(PEO)as two immiscible aqueous phases to form a bioink and innovatively applying fluorescent carbon quantum dots for long-term tracking of *** GelMA(10%,mass fraction)and PEO(1.6%,mass fraction)hydrogel with 3:1 volume ratio offered distinct pore-forming characteristics,satisfactorymechanical properties,and biocompatibility for the creation of the 3DP-7721 *** analysis and quantitative real-time fluorescence polymerase chain reaction(PCR)were used to evaluate the biological properties of the *** with the two-dimensional culture cell model(2D-7721)and the 3D mixed culture cell model(3DM-7721),3DP-7721 significantly improved the proliferation of cells and expression of tumor-related proteins and ***,we evaluated the differences between the three culture models and the effectiveness of antitumor drugs in the three models and discovered that the efficacy of antitumor drugs varied because of significant differences in resistance proteins and genes between the three *** addition,the comparison of tumor formation in the three models found that the cells cultured by the 3DP-7721 model had strong tumorigenicity in nude *** evaluation of the levels of biochemical indicators related to the formation of solid tumors showed that the 3DP-7721 model group exhibited pathological characteristics of malignant tumors,the generated solid tumors were similar to actual tumors,and the deterioration was *** research therefore acts as a foundation for the application of 3DP-7721 models in drug devel

关键词： 3D bioprinting Hepatoma tumor models Drug screening Antitumor drug development

Perpendicularly assembled oriented electrospinning nanofibers based piezoresistive pressure sensor with wide measurement range

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Nano Research 2024年第7期17卷 6493-6501页

作者： Xiaoxue Bi Zhigang duan Xiaojuan Hou Shuo Qian Mengjiao Yuan Jiajun Hu Jie zhang Yuchen Lu Yanli liu Jian He Zhiling Peng Xiujian Chou School of Mechanical and Electrical Engineering North University of ChinaTaiyuan 030051China science and technology on Electronic Test and Measurement laboratory North University of ChinaTaiyuan 030051China School of Software North University of ChinaTaiyuan 030051China School of information and Communication Engineering North University of ChinaTaiyuan 030051China

With the rapid development of wearable electronics,flexible pressure sensors have attracted wide attention in human–computer interaction and intelligent ***,it is a challenge to achieve a sensor with high sensitivity,wide measurement range,and wearing ***,we develop an oriented electrospinning thermoplastic polyurethane/polyacrylonitrile(TPU/PAN)nanofibers(OETPN)based piezoresistive pressure sensor(PONPS)in which the active layer and the electrode are assembled *** interdigital electrode is fabricated by spraying silver nanowires(AgNWs)on the OETPN through a mask *** active layer is composed of OETPN coated with MXene,encapsulated on the electrode by polyurethane(PU)*** porous structure of nanofibers membrane broadens the measurement range of the *** oriented nanofibers as active layer can improve the sensitivity in low pressure,because oriented nanofibers without interweaving nanofibers are more compressible than disordered *** prepared using the spraying method creates nanoscale microstructure and increases *** perpendicular assembly has greater response between the active layer and the electrode than the parallel assembly to improve the *** sensor exhibits high sensitivity(6.71 kPa^(−1),0.02–2 kPa)and wide measurement range(0.02–700 kPa).The sensor can detect weak signals such as radial artery.A pressure array constructed precisely represents the distribution of *** intelligent throat is created by combining machine learning algorithms with the *** can detect and recognize subtle throat vibrations while speaking,achieving recognition accuracy up to 100%using support vector machine(SVM)for five words with different *** fabricated sensor shows promising prospects in personal healthcare and intelligent robots.

关键词： oriented nanofibers perpendicular assembly parallel assembly intelligent throat machine learning algorithms

Two-dimensional materials for future information technology: status and prospects

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science china(information sciences) 2024年第6期67卷 1-147页

作者： Hao QIU Zhihao YU Tiange ZHAO Qi zhang Mingsheng XU Peifeng LI Taotao LI Wenzhong BAO Yang CHAI Shula CHEN Yiqi CHEN Hui-Ming CHENG Daoxin DAI Zengfeng DI Zhuo DONG Xidong duan Yuhan FENG Yu FU Jingshu GUO Pengwen GUO Yue HAO Jun HE Xiao HE Jingyi HU Weida HU Zehua HU Xinyue HUANG Ziyang HUANG Ali IMRAN Ziqiang KONG Jia LI Qian LI Weisheng LI Lei LIAO Bilu liu Can liu Chunsen liu Guanyu liu Kaihui liu Liwei liu Sheng liu Yuan liu Donglin LU Likuan MA Feng MIAO Zhenhua NI Jing NING Anlian PAN Tian-Ling REN Haowen SHU Litao SUN Yue SUN Quanyang TAO Zi-Ao TIAN Dong WANG Hao WANG Haomin WANG Jialong WANG Junyong WANG Wenhui WANG Xingjun WANG Yeliang WANG Yuwei WANG Zhenyu WANG Yao WE... School of Electronic science and Engineering Nanjing University School of Integrated Circuits Interdisciplinary Research Center for Future Intelligent Chips (Chip-X)Nanjing University School of Integrated Circuit science and Engineering Nanjing University of Posts and Telecommunications State Key laboratory of Infrared Physics Shanghai Institute of Technical Physics Chinese Academy of Sciences School of Physics and Key Lab of Quantum Materials and Devices of the Ministry of Education School of Electronic Science & EngineeringSoutheast University College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University Suzhou laboratory State Key laboratory of Integrated Chips and Systems School of MicroelectronicsFudan University Shaoxin laboratory Department of Applied Physics The Hong Kong Polytechnic University Key laboratory for Micro-Nano Physics and technology of Hunan Province College of Materials Science and EngineeringHunan University College of Integrated Circuits Zhejiang University Shenzhen Geim Graphene Center Shenzhen Key Laboratory of Layered Materials for Value-Added ApplicationsTsinghua-Berkeley Shenzhen Institute & Institute of Materials ResearchTsinghua Shenzhen International Graduate SchoolTsinghua University State Key laboratory of Extreme Photonics and Instrumentation College of Optical Science and EngineeringInternational Research Center for Advanced PhotonicsZijingang CampusZhejiang University national Key laboratory of Materials for Integrated Circuits Shanghai Institute of Microsystem and Information TechnologyChinese Academy of Sciences CAS Key laboratory of Nanophotonic Materials and Devices & Key laboratory of Nanodevices and Applications i-LabSuzhou Institute of Nano-Tech and Nano-Bionics (SINANO)Chinese Academy of Sciences College of Chemistry and Chemical Engineering Hunan University Key laboratory of Quantum State Construction and Manipulation (Ministry of Education) Department of PhysicsRenmin University of China School

Over the past 70 years, the semiconductor industry has undergone transformative changes,largely driven by the miniaturization of devices and the integration of innovative structures and materials. Two-dimensional(2D) materials like transition metal dichalcogenides(TMDs) and graphene are pivotal in overcoming the limitations of silicon-based technologies, offering innovative approaches in transistor design and functionality, enabling atomic-thin channel transistors and monolithic 3D integration. We review the important progress in the application of 2D materials in future information technology, focusing in particular on microelectronics and optoelectronics. We comprehensively summarize the key advancements across material production, characterization metrology, electronic devices, optoelectronic devices, and heterogeneous integration on silicon. A strategic roadmap and key challenges for the transition of 2D materials from basic research to industrial development are outlined. To facilitate such a transition, key technologies and tools dedicated to 2D materials must be developed to meet industrial standards, and the employment of AI in material growth, characterizations, and circuit design will be essential. It is time for academia to actively engage with industry to drive the next 10 years of 2D material research.

关键词： two-dimensional (2D) materials information technology production technology standardization of characterization microelectronic devices optoelectronic devices multi-functional integration

The In-Flight Realtime Trigger and Localization Software of GECAM

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Research in Astronomy and Astrophysics 2024年第10期24卷 11-24页

作者： Xiao-Yun Zhao Shao-Lin Xiong Xiang-Yang Wen Xin-Qiao Li Ce Cai Shuo Xiao Qi Luo Wen-Xi Peng Dong-Ya Guo Zheng-Hua An Ke Gong Jin-Yuan Liao Yan-Qiu zhang Yue Huang Lu Li Xing Wen Fei zhang Jing duan Chen-Wei Wang Dong-Li Shi Peng zhang Qi-Bin Yi Chao-Yang Li Yan-Bing Xu Xiao-Hua Liang Ya-Qing liu Da-Li zhang Xi-Lei Sun Fan zhang Gang Chen Huan-Yu Wang Sheng Yang Xiao-Jing liu Min Gao Mao-Shun Li Jin-Zhou Wang Xing Zhou Yi Zhao Wang-Chen Xue Chao Zheng Jia-Cong liu Xing-Bo Han Jin-Ling Qi Jia Huang Ke-Ke zhang Can Chen Xiong-Tao Yang Dong-Jie Hou Yu-Sa Wang Rui Qiao Xiang Ma Xiao-Bo Li Ping Wang Xin-Ying Song Li-Ming Song Shi-Jie Zheng Bing Li hong-Mei zhang Yue Zhu Wei Chen Jian-Jian He Zhen zhang Jin Hou hong-Jun Wang Yan-Chao Hao Xiang-Yu Wang Zong-Yuan Yang Zhi-Long Wen Zhi Chang Yuan-Yuan Du Rui Gao Xiao-Fei Lan Yan-Guo Li Gang Li Xu-Fang Li Fang-Jun Lu hong Lu Bin Meng Feng Shi Hui Wang Hui-Zhen Wang Yu-Peng Xu Jia-Wei Yang Xue-Juan Yang Shuang-Nan zhang Chao-Yue zhang Cheng-Mo zhang Zhi-Cheng Tang Cheng Cheng Key laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China university of Chinese Academy of sciences Chinese Academy of SciencesBeijing 100049China School of information science and technology Southwest Jiaotong UniversityChengdu 611756China Key laboratory of Stellar and Interstellar Physics and Department of Physics Xiangtan UniversityXiangtan 411105China Physics and Space science College China West Normal UniversityNanchong 637002China Department of Astronomy Beijing Normal UniversityBeijing 100875China Innovation Academy for Microsatellites of CAS Shanghai 201203China Changchun university of science and technology Changchun 130022China Chinese Academy of sciences South America Center for Astronomy National Astronomical ObservatoriesCASBeijing 100101China

Realtime trigger and localization of bursts are the key functions of GECAM,an all-sky gamma-ray monitor launched on 2020 December *** developed a multifunctional trigger and localization software operating in the CPU of the GECAM Electronic *** onboard software has the following features:high trigger efficiency for real celestial bursts with a suppression of false triggers caused by charged particle bursts and background fluctuation,dedicated localization algorithm optimized for both short and long bursts,and low time latency of the trigger information which is downlinked through the Global Short Message Communication service of the global BeiDou navigation *** paper provides a detailed description of the design and development of the trigger and localization software system for *** covers the general design,workflow,the main functions,and the algorithms used in the *** paper also includes on-ground trigger tests using simulated gamma-ray bursts generated by a dedicated X-ray tube,as well as an overview of the performance for real celestial bursts during its in-orbit operation.

关键词： telescopes instrumentation:detectors methods:observational

CAS FGOALS-f3-L Large-ensemble Simulations for the CMIP6 Polar Amplification Model Intercomparison Project

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Advances in Atmospheric sciences 2021年第6期38卷 1028-1049页

作者： Bian HE Xiaoqi zhang Anmin duan Qing BAO Yimin liu Wenting HU Jinxiao LI Guoxiong wu State Key laboratory of Numerical Modeling for Atmospheric sciences and Geophysical Fluid Dynamics(LASG) Institute of Atmospheric Physics(IAP)Chinese Academy of SciencesBeijing100029China university of Chinese Academy of sciences Beijing 100029China School of Atmospheric sciences Nanjing University of Information Science and TechnologyNanjing 210044China

Large-ensemble simulations of the atmosphere-only time-slice experiments for the Polar Amplification Model Intercomparison Project(PAMIP)were carried out by the model group of the Chinese Academy of sciences(CAS)Flexible Global Ocean-Atmosphere-Land System(FGOALS-f3-L).Eight groups of experiments forced by different combinations of the sea surface temperature(SST)and sea ice concentration(SIC)for pre-industrial,present-day,and future conditions were performed and *** time-lag method was used to generate the 100 ensemble members,with each member integrating from 1 April 2000 to 30 June 2001 and the first two months as the spin-up *** basic model responses of the surface air temperature(SAT)and precipitation were *** results indicate that Arctic amplification is mainly caused by Arctic SIC forcing *** SAT responses to the Arctic SIC decrease alone show an obvious increase over high latitudes,which is similar to the results from the combined forcing of SST and ***,the change in global precipitation is dominated by the changes in the global SST rather than SIC,partly because tropical precipitation is mainly driven by local SST *** uncertainty of the model responses was also investigated through the analysis of the large-ensemble *** relative roles of SST and SIC,together with their combined influence on Arctic amplification,are also *** of these model datasets will contribute to PAMIP multi-model analysis and improve the understanding of polar amplification.

关键词： polar amplification PAMIP large-ensemble simulation sea ice FGOALS-f3-L CMIP6

A preliminary analysis of the surface chemistry of atmospheric aerosol particles in a typical urban area of beijing

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Journal of Environmental sciences 2016年第9期28卷 71-81页

作者： Zhengzheng zhang hong Li hongyan liu Runxiang Ni Jinjuan Li Liqun Deng Defeng Lu Xueli Cheng Pengli duan Wenjun Li College of Resource and Enuironmental Engineering Guizhou Uniuersity Guiyang 550025 China State Key laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental Sciences Beijing 110012China Collaborative Innovation Center on Atmospheric Environment and Equipment technology Nanfing University of Information Science andTechnology Nanjing 210044 China Institute of Geographic sciences and Natural Resources Research CAS Beijing lO0101 China Core Tech Integrated (beijing) Pry. Ltd. Beijing 100086 China Sichuan Academy of Environmental sciences Sichuan 610042 China SAE technology Development (Don99uan) Co. Ltd. Guanfdong 523087 China Institute of Environment science Shaanxi University Shaanxi 030006 China

Atmospheric aerosol particle samples were collected using an Ambient Eight Stage（Non-Viable） Cascade Impactor Sampler in a typical urban area of beijing from 27 th *** 5th Oct.,*** surface chemistry of these aerosol particles was analyzed using Static Time of Flight-Secondary Ion Mass Spectrometry（Static TOF-SIMS）.The factors influencing surface compositions were evaluated in conjunction with the air pollution levels,meteorological factors,and air mass transport for the sampling *** results show that a variety of organic ion groups and inorganic ions/ion groups were accumulated on the surfaces of aerosol particles in urban areas of beijing;and hydrophobic organic compounds with short-or middle-chain alkyl as well as hydrophilic secondary inorganic compounds were *** these compounds have the potential to affect the atmospheric behavior of urban aerosol ***1.1–2.1and PM3.3–4.7had similar elements on their surfaces,but some molecules and ionic groups demonstrated differences in Time of Flight-Secondary Ion Mass Spectrometry *** suggests that the quantities of elements varied between PM1.1–2.1and PM3.3–*** particular,more intense research efforts into fluoride pollution are required,because the fluorides on aerosol surfaces have the potential to harm human *** levels of air pollution had the most significant influence on the surface compositions of aerosol particles in our ***,heavier air pollution was associated with more complex surface compositions on aerosol *** addition,wind,rainfall,and air masses from the south also greatly influenced the surface compositions of these urban aerosol particles.

关键词： Atmospheric aerosol Surface chemistry Influential factors TOF-SIMS beijing

Ultrafast optical spectroscopy evidence of pseudogap and electronphonon coupling in an iron-based superconductor KCa_(2)Fe_(4)As_(4)F_(2)

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science china(Physics,Mechanics & Astronomy) 2022年第3期65卷 92-98页

作者： Chen zhang Qi-Yi wu Wen-Shan hong Hao liu Shuang-Xing Zhu Jiao-Jiao Song Yin-Zou Zhao Fan-Ying wu Zi-Teng liu Shu-Yu liu Ya-Hua Yuan Han Huang Jun He Shiliang Li Hai-Yun liu Yu-Xia duan Hui-Qian Luo Jian-Qiao Meng School of Physics and Electronics Central South UniversityChangsha 410083China beijing national laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical sciences University of Chinese Academy of SciencesBeijing 100049China Songshan Lake Materials laboratory Dongguan 523808China beijing Academy of Quantum information sciences Beijing 100193China

We use ultrafast optical spectroscopy to study the nonequilibrium quasiparticle relaxation dynamics of the iron-based superconductor KCa_(2)Fe_(4)A_(s4)F_(2)with T_(c)= 33.5 K. Our results reveal a possible pseudogap(△_(PG)=(2.4 ± 0.1) me V) below T*≈ 50 K but prior to the opening of a superconducting gap(△SC(0) ≈(4.3 ± 0.1) me V). Measurements under high pump fluence reveal two distinct, coherent phonon oscillations with 1.95 and 5.51 THz frequencies, respectively. The high-frequency A1 g(2) mode corresponds to the c-axis polarized vibrations of Fe As planes with a nominal electron-phonon coupling constant λA1 g(2)= 0.194 ± *** findings suggest that the pseudogap is likely a precursor of superconductivity, and the electron-phonon coupling may play an essential role in the superconducting pairing in KCa_(2)Fe_(4)A_(s4)F_(2).

关键词： KCa_(2)Fe_(4)A_(s4)F_(2) ultrafast spectroscopy electron-phonon coupling superconductivity