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Vasarely painting at the nanoscale on sapphire crystals

Nano Research 2020年第9期13卷 2512-2516页

作者： Caroline Matringe Elsa Thune Rémy Cavalotti Ahmad Fakih Stephan Amaud Nils Blanc Nathalie Boudet Alessandro Coati yves garreau David Babonneau René Guinebretière IRCER UMR CNRS 7315Centre Europeen de la CeramiqueUniversite de Limoges12 rue Atlantis87068 LimogesFrance Institut Neel UPR CNRS 2940 CRG D2AM BeamlineESRFUniversite Grenoble Alpes38042 GrenobleFrance SixS Beamline Synchrotron SOLEILBP4891192 Gifsur YvetteFrance Laboratoire Materiaux et Phenomenes Quantiques UMR CNRS 7162Universite de Paris75013 ParisFrance Institut Pprime Departement Physique et Mecanique des Materiauxf UPR CNRS 3346Universite de PoitiersSP2MITSA 4112386073 Poitiers Cedex 9France

We demonstrate that convenient thermal treatment of a specific sapphire vicinal surface can induce the formation of a fully two-dimensional(2D)ordered surface made of a periodic assembly of(006)*** simiarity between the resuting surface topography and pattemns represented in the hexagon series"of paintings by Vasarely is really striking!We thus propose to call these surfaces as"nanoscaled Vasarely surfaces".We also show that the self-organization process,which is driven by the minimization of the free energy of a closed system,results in a quasi-linear isothermal growth of the facets'surface area over time.

关键词： nanoscaled Vasarely surfaces two-dimensional(2D)-self-organization sapphire vicinal surfaces

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Huge metastable axial strain in ultrathin heteroepitaxial vertically aligned nanowires

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Nano Research 2015年第6期8卷 1964-1974页

作者： Vivien Schuler Francisco Javier Bonilia Dominique Demaille Alessandro Coati Alina Vlad yves garreau Michele Sauvage-Simkin Anastasiia Novikova Emiliano Fonda Sarah Hidki Victor Etgens Franck Vidal Yunlin Zheng Sorbonne Universites UPMC Institut des NonoSciences de Paris 4 place Jussieu Paris 75005 France CNRS UMR7588 Institut des NanoSciences de Paris 4 place Jussieu Paris 75005 France Synchrotron Soleil L'Orme des Merisiers Saint-Aubin BP 48 91192 Gif-sur-Yvette Cedex France Universite Paris Diderot Sorbonne Paris Cite MPO UMR 7162 CNRS Batiment Condorcet Case courrier 7021 75205 Paris Cedex 13 France Universite de Versailles Saint-Quentin en Yvelines 55 Av. de Paris Versailles 78035 France

Strain engineering is a powerful tool to tailor the physical properties of materials coherently stacked in an epitaxial heterostructure. Such an approach, applied to the mature field of planar heteroepitaxy, has yielded a variety of new phenomena and devices. Recently, heteroepitaxial vertically aligned nanocomposites have emerged as alternatives to planar structures. Owing to the peculiar geometry of such nanoarchitectures, efficient strain control can be achieved, opening the way to novel functionalities. In this paper, we report a very large tensile axial strain in epitaxial transition metal nanowires embedded in an oxide matrix. We show that axial strains in excess of 1.5% can be sustained over a large thickness （a few hundred nanometers） in epitaxial nanowires having ultrasmall diameters （-3-6 nm）. The axial strain depends on the diameter of the nanowires, reflecting its epitaxial nature and the balance of interface and elastic energies. Furthermore, it is experimentally shown that such strain is metastable, in agreement with the calculations performed in the framework of the Frenkel-Kontorova model. The diameter dependence and metastability provide effective ways to control the strain, an appealing feature for the design of functional nanoarchitectures.

关键词： self-assembly heteroepitaxy nanowires strain

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